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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Long-term measurements of ice nucleating particles at Atmospheric Radiation Measurement (ARM) sites worldwide

Ice nucleating particles (INPs) play a critical role in cloud microphysics and precipitation formation, yet long-term, spatially extensive observational datasets remain limited. Here, we present one of the most comprehensive publicly available datasets of immersion-mode INP concentrations using a single analytical method, generated through the U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) user facility. INP filter samples have been collected across a broad range of environments – including agricultural plains, Arctic coastlines, high-elevation mountain sites, marine regions, and urban areas – via fixed observatories, mobile facility deployments, and vertically-resolved tethered balloon system operations. We describe the standardized processing and quality assurance pipeline, from filter collection and processing using the Ice Nucleation Spectrometer to final data products archived on the ARM Data Discovery portal. The dataset includes both total INP concentrations and selectively treated samples, allowing for classification of biological, organic, and inorganic INP types. It features a continuous 5-year record of INP measurements from a central U.S. site, with data collection still ongoing. Seasonal and site-specific differences in INP concentrations are illustrated through intercomparisons at −10 and −20 °C, revealing distinct regional sources and atmospheric drivers. We also outline mechanisms for researchers to access existing data, request additional sample analyses, and propose future field campaigns involving ARM INP measurements. This dataset supports a wide range of scientific applications, from observational and mechanistic studies to model development, and provides critical constraints on aerosol-cloud interactions across diverse atmospheric regimes (Creamean et al., 2024, 2020b; https://doi.org/10.5439/1770816).

Creamean, Jessie M. [Colorado State Univ., Fort Co↗
DOE OSTI2025

Over three decades, and counting, of near-surface turbulent flux measurements from the Atmospheric Radiation Measurement (ARM) user facility

Processes mediating the coupling of terrestrial, aquatic, biospheric, and atmospheric systems influence weather, climate, and ecosystem dynamics via transfer of energy, momentum, water, and carbon (or other species). These exchange processes are quantified by measurements of near-surface turbulent fluxes. Understanding processes at these interfaces provides insight toward understanding and predicting current and future states within the Earth system. The Atmospheric Radiation Measurement (ARM) user facility has been conducting measurements of near-surface turbulent fluxes since the early 1990s at long-term fixed locations and shorter-term mobile deployments across the Earth. ARM has utilized two established methods for conducting these measurements: energy balance Bowen ratio (EBBR) and eddy covariance (EC). Primary measurements from the former include sensible and latent heat flux, while the latter also measures fluxes of momentum and carbon (primarily carbon dioxide, with methane fluxes measured at two locations to date). The EBBR systems have been deployed at 22 locations, and, to date, the EC systems have been deployed at over 50 sites, with plans for additional novel site locations in the future. Herein, the history, evolution, and key aspects of these instrument systems are documented, along with information on data quality assurance and post-processing, as well as best use practices. Additionally, three data validation experiments were recently conducted, and their key findings are summarized. Finally, ancillary datasets acquired by ARM, which can contextualize and aid interpretation of the near-surface turbulent flux measurements, are discussed. The datasets described herein include the eddy correlation flux measurement system: 30ECOR (https://doi.org/10.5439/1879993, Sullivan et al., 1997), 30QCECOR (https://doi.org/10.5439/1097546, Gaustad, 2003), ECORSF (https://doi.org/10.5439/1494128, Sullivan et al., 2019a), and associated AmeriFlux and Methane Value-Added Product, AMCMETHANE (https://doi.org/10.5439/1508268, Billesbach, 2011); the energy balance Bowen ratio system: 30EBBR (https://doi.org/10.5439/1023895, Sullivan et al., 1993) and 30BAEBBR (https://doi.org/10.5439/1027268, Gaustad and Xie, 1993); and the carbon dioxide flux measurement system: CO2FLX (https://doi.org/10.5439/1287574, https://doi.org/10.5439/1287575, https://doi.org/10.5439/1287576, Koontz et al., 2015a, b, c; https://doi.org/10.5439/1989774, https://doi.org/10.5439/1989776, https://doi.org/10.5439/1992202, Biraud and Chan, 2002a, b, c). These data can be found by searching the above data stream names at https://adc.arm.gov/discovery/#/results/ (last access: 8 September 2025).

Sullivan, Ryan C. [Argonne National Laboratory (AN↗
DOE OSTI2024

2024 Atmospheric Radiation Measurement (ARM) Annual Report

This report provides an overview of the Atmospheric Radiation Measurement (ARM) user facility and a sample of achievements for fiscal year 2024 (FY2024). Strong collaborations between nine DOE national laboratories enable ARM to successfully operate in remote locations around the world. This unique partnership supports the DOE mission to provide for the energy security of the nation. Without the support of the following laboratories, ARM would not be the state-of-the-art facility that it is today. ARM is a multi-laboratory, U.S. Department of Energy (DOE) Office of Science user facility and a key contributor to national and international atmospheric and climate research efforts. ARM offers scientists cutting-edge, ground-based observatories, aerial observation capabilities, and high-performance computing. ARM’s capabilities have enabled more than 30 years of continuous measurements of cloud and aerosol properties and their effects on Earth’s energy balance.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Why Does Atmospheric Radiative Heating Weaken Midlatitude Cyclones?

Abstract Recent work has indicated that atmospheric radiative heating reduces the kinetic energy of large‐scale eddies in the midlatitudes. However, a physical mechanism that connects radiation to the midlatitude eddy kinetic energy is still uncertain. Using a high‐resolution general circulation model we perform an experiment in which the radiative cooling profile at each model time step is overwritten with the climatological mean, computed from a control simulation. This approach separates the mean and transient effects of radiative heating on the extratropical circulation. We find that, when radiative heating is fixed, the globally‐averaged eddy kinetic energy is enhanced by ∼6%. We show that thermal radiation dampens temperature anomalies near the surface and tropopause in low‐pressure systems, destroying eddy available potential energy and eddy kinetic energy. We identify this as a possible mechanism by which atmospheric radiative heating weakens midlatitude cyclones.

Mischell, Eric↗
DOE OSTI2026

Performance and Reliability Assessment of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Data Advisor (ADA)

The Atmospheric Radiation Measurement (ARM) User Facility provides one of the world's largest openly accessible repositories of atmospheric observations through the ARM Data Discovery platform. Although the repository contains more than three decades of measurements collected from permanent observatories, mobile facilities, aircraft campaigns, and field experiments, identifying appropriate datasets can be challenging, particularly for new users unfamiliar with ARM instrumentation and datastream organization. To improve data accessibility, the ARM Data Center developed the ARM Data Advisor (ADA), an artificial intelligence-powered assistant designed to facilitate scientific data discovery, dataset interpretation, and user guidance. This report evaluates ADA's performance as a domain-specific scientific assistant using realistic atmospheric science workflows. The evaluation examines five key capabilities: data retrieval and curation efficiency, hallucination resistance, scientific reasoning, response to ambiguous queries, and content retention and session continuity. Representative prompts were developed to simulate typical interactions between researchers and the ARM Data Discovery platform, and ADA's responses were assessed for retrieval completeness, scientific accuracy, consistency, and practical usefulness. In these representative tests, ADA reduced the complexity of discovering and accessing ARM datasets by recommending appropriate datastreams, explaining instrumentation, interpreting metadata, and assisting with data processing workflows. ADA also exhibits strong domain knowledge of atmospheric science terminology and generally resists hallucination by acknowledging unavailable datasets and requesting clarification when appropriate. Overall, the results indicate that ADA represents a promising advancement in scientific data discovery within the ARM User Facility and has considerable potential to improve researcher productivity, particularly for new users and interdisciplinary scientists seeking efficient access to ARM observations.

Salvador, Christian [ORNL] (ORCID:0000000283287777↗
DOE OSTI2025

2025 Atmospheric Radiation Measurement (ARM) Annual Report

ARM is a multi-laboratory, U.S. Department of Energy (DOE) Office of Science user facility and a key contributor to atmospheric research efforts. For more than 30 years, ARM has supported the DOE and Office of Science missions by providing atmospheric observations to enable scientific discovery, transform our understanding of the atmosphere, and evaluate and improve the accuracy of atmospheric models. ARM’s cutting-edge capabilities for scientists include continuously operating ground-based observatories, aerial observation platforms, and high performance computing.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Evaluation of the hyperspectral radiometer (HSR1) at the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site

Abstract. The Peak Design Ltd hyperspectral radiometer (HSR1) was tested at the Atmospheric Radiation Measurement (ARM) user facility Southern Great Plains (SGP) site in Lamont, Oklahoma, for 2 months from May to July 2022. The HSR1 is a prototype instrument that measures total (Ftotal) and diffuse (Fdiffuse) spectral irradiance from 360 to 1100 nm with a spectral resolution of 3 nm. The HSR1 spectral irradiance measurements are compared to nearby collocated spectral radiometers, including two multifilter rotating shadowband radiometers (MFRSRs) and the Shortwave Array Spectroradiometer–Hemispheric (SASHe) radiometer. The Ftotal at 500 nm for the HSR1 compared to the MFRSRs has a mean (relative) difference of 0.01 W m−2 nm−1 (1 %–2 %). The HSR1 mean Fdiffuse at 500 nm is smaller than the MFRSRs' by 0.03–0.04 (10 %) W m−2 nm−1. The HSR1 clear-sky aerosol optical depth (AOD) is also retrieved by considering Langley regressions and compared to collocated instruments such as the Cimel sunphotometer (CSPHOT), MFRSRs, and SASHe. The mean HSR1 AOD at 500 nm is larger than the CSPHOT's by 0.010 (8 %) and larger than the MFRSRs' by 0.007–0.017 (6 %–18 %). In general, good agreement between the HSR1 and other instruments is found in terms of the Ftotal, Fdiffuse, and AODs at 500 nm. The HSR1 quantities are also compared at other wavelengths to the collocated instruments. The comparisons are within ∼ 10 % for the Ftotal and Fdiffuse, except for 940 nm, where there is relatively larger disagreement. The AOD comparisons are within ∼ 10 % at 415 and 440 nm; however, a relatively larger disagreement in the AOD comparison is found for higher wavelengths.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Atmospheric Radiation Measurement (ARM) airborne field campaign data products between 2013 and 2018

Airborne measurements are pivotal for providing detailed, spatiotemporally resolved information about atmospheric parameters and aerosol and cloud properties, thereby enhancing our understanding of dynamic atmospheric processes. For 30 years, the US Department of Energy (DOE) Office of Science supported an instrumented Gulfstream 1 (G-1) aircraft for atmospheric field campaigns. Data from the final decade of G-1 operations were archived by the Atmospheric Radiation Measurement (ARM) Data Center and made publicly available at no cost to all registered users. To ensure a consistent data format and to improve the accessibility of the ARM airborne data, an integrated dataset was recently developed covering the final 6 years of G-1 operations (2013 to 2018, https://doi.org/10.5439/1999133; Mei and Gaustad, 2024). The integrated dataset includes data collected from 236 flights (766.4 h), which covered the Arctic, the US Southern Great Plains (SGP), the US West Coast, the eastern North Atlantic (ENA), the Amazon Basin in Brazil, and the Sierras de Córdoba range in Argentina. These comprehensive data streams provide much-needed insight into spatiotemporal variability in the thermodynamic quantities and aerosol and cloud properties for addressing essential science questions in Earth system process studies. This paper describes the DOE ARM merged G-1 datasets, including information on the acquisition, data collection challenges and future potentials, and quality control processes. It further illustrates the usage of this merged dataset to evaluate the Energy Exascale Earth System Model (E3SM) with the Earth System Model Aerosol–Cloud Diagnostics (ESMAC Diags) package.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Source Attribution of Methane Enhancements at the Southern Great Plains Atmospheric Radiation Measurement Site Field Campaign Report

Tower data from 2017 to 2020 revealed that the U.S. Department of Energy’s Southern Great Plains (SGP) Atmospheric Radiation Measurements (ARM) observatory in Oklahoma exhibited significant CH 4 enhancements compared to other U.S. tower sites. On average, near-surface CH 4 at the ARM site was higher, had larger diurnal and seasonal variations, and had sharper near-surface increases at night compared to other tower sites in the U.S. A field campaign was conducted in June 2024 to identify and quantify the surrounding CH 4 emission sources by two researchers from the University of Oklahoma. During the campaign, a mobile measurement was conducted using a LI-COR 7810 tracer gas analyzer mounted on a vehicle during June 23-26, 2024 near the SGP site (within 7 km distance). We sampled CH 4 along predefined routes surrounding a suspected source, i.e., a large animal feeding operation (AFO) farm 5.8 km northwest of the SGP ARM site. Measurements were collected between 04:30 and 09:00 local time when the planetary boundary layer (PBL) was shallow, increasing sensitivity to surface emissions. Driving speed was kept below 5 mph to minimize pressure-related artifacts. CH 4 concentrations downwind of the AFO exceeded 6000 ppb on the early morning of June 26, corresponding to an emission rate of ~95 kg⋅hr -1 estimated using the mass balance method. Additional sources identified during the campaign include nearby open-range cattle and leaks from a nearby natural gas pipeline.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

The Efficiency of Water Vapor on Top‐of‐Atmosphere Radiation

Earth's climate sensitivity is greatly affected by the compensation between temperature feedback and water vapor (WV) feedback. Using abrupt 4xCO 2 experiments, we show that the global-mean WV feedback is nearly a linear function of the temperature feedback, the slope of which is explained by the longwave radiative efficiency of WV (ϵ). Although ϵ remains constant across models in the global mean, it exhibits substantial spatial variations and is particularly weak in Antarctica, where near-surface inversions decouple the surface from the free troposphere. We introduce a surface–free troposphere temperature difference (SFTD) metric, showing that positive SFTD (e.g., high lifting condensation level) amplifies ϵ, while negative SFTD (e.g., strong surface inversion) suppresses it. These findings provide a clear explanation of how local climate conditions modulate the radiative compensation between temperature and WV feedbacks.

climate feedback↗
DOE OSTI2026

Surface Observations From Atmospheric Radiation Measurement Sites Constrain the Anthropogenic Contribution to Cloud Droplet Number

Uncertainty in anthropogenic forcing driven by aerosol-cloud interactions (aci) limits our ability to infer the sensitivity of the Earth system to forcing from historical records. The driver of aci is the change in cloud droplet number concentration (N d ) due to changes in aerosol serving as cloud condensation nuclei (CCN). Here, we combine a perturbed parameter ensemble run in a global Earth system model with observations of CCN and single-layer-cloud N d at surface sites in the Azores, the Southern Great Plains, and Ascension Island to provide a constraint on the anthropogenic contribution to present-day N d . These observational lines of evidence constrain the preindustrial to present-day change in N d to be between 11 and 43 cm −3 . This is consistent with the upper end of some previous estimates but has a higher minimum perturbation, pointing to a stronger historical aerosol cooling.

ARM↗
DOE OSTI2025

Refining the representations of high-latitude surface-atmosphere radiative coupling in the E3SM (Final project report)

Over the course of this project, we have successfully carried out proposed studies and reported our findings in leading peer-reviewed journals and national/international conferences. So far, we have published 7 peer-reviewed articles reporting these findings and contributed to 1 additional peer-reviewed article. One additional manuscript resulting from this project is currently under review. We have made 22 presentations at national and international conferences about the results from this project. We have also given 3 presentations at the E3SM all-hands or PI meetings to update the E3SM community on our results.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Distinctive Pattern of Global Warming in Ocean Heat Content

Abstract Huge heat anomalies in the atmosphere and ocean in recent years are not yet explained. Strong characteristic patterns in temperatures for upper layers of the ocean occurred from 2000 to 2023 in the presence of global warming from increasing atmospheric greenhouse gases. Here, we show that the deep tropics are warming, although sharply modulated by El Niño–Southern Oscillation events, with strong heating in the extratropics near 40°N and 40°–45°S but little heating near 20°N and 25°–30°S. The heating is most clearly manifested in zonal-mean ocean heat content and is evident in sea surface temperatures. The strongest heating is in the Southern Hemisphere, where aerosol effects are small. Estimates are made of the contributions to heating of top-of-atmosphere (TOA) radiation, atmospheric energy transports, surface fluxes of energy, and redistribution of energy by surface winds and ocean currents. The patterns of change are not directly related to TOA radiation but are evident in net surface energy fluxes and inferred ocean heat transports, underscoring their coupled origin. Changes in the atmospheric circulation through a poleward shift in ocean jet streams and storm tracks are reflected in surface wind-driven ocean Ekman transports. As well as human-induced climate change, internal natural variability is likely in play. Hence, the atmosphere and ocean currents are systematically redistributing heat from global warming, profoundly affecting local climates. Significance Statement As the climate changes, it has been difficult to discern meaningful patterns. Distinctive patterns of change have occurred in the ocean when examined as zonal averages around latitude bands. Most excess heat from global warming resides in the ocean and, since 2005, has become focused into bands near 40°N and 40°S, with little net warming in the subtropics. The strongest warming is in the Southern Hemisphere, although sea surface temperatures have increased more in the Northern Hemisphere. Changes in the atmospheric circulation through a poleward shift in the jet stream and storm tracks are primarily responsible along with corresponding changes in ocean currents. These changes are linked through surface exchanges of energy via heat, moisture, and wind stress.

Trenberth, Kevin E. [National Center for Atmospher↗
DOE OSTI2026

Southern Hemisphere Polar Infrared Radiation Experiment (SHIRE) Field Campaign Report

An extended-range atmospheric emitted radiance interferometer (AERI) instrument to be deployed to Scott Base (78 S, 166 E) in McMurdo Sound, Antarctica for the purpose of synergizing with the National Aeronautics and Space Administration (NASA) Polar Radiant Energy in the Far-InfraRed Experiment (PREFIRE) satellite mission (https://prefire.ssec.wisc.edu/), examining the closure of atmospheric thermal emission, and providing validation for PREFIRE. The PREFIRE mission is the first satellite mission to map Earth’s spectrally resolved thermal emission, from 5 to 50 microns, over seasonal to annual timescales. These new observations represent the beginning of an intensive examination of the nature of thermal emission from Earth (emission from both the surface and atmosphere). A primary requirement of the PREFIRE mission is to provide validation of the retrieved variables. Numerous field sites in the Arctic (such as the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) North Slope of Alaska observatory and Summit Station, Greenland) have existing instrumentation to facilitate validation, leaving an observational gap in Antarctica. Through SHIRE, we propose to establish a temporary, intensive measurement site in Antarctica to ensure that both poles are suitably represented, and benefit from this state-of-the art science. This will also allow Arctic and Antarctic atmospheric radiative states to be compared and contrasted. For SHIRE specifically, we also propose further objectives to examine the spectrally resolved thermal radiative closure of the polar atmosphere and the historical changes in Antarctic radiative forcing, using previous Antarctic field campaigns, such as the ARM West Antarctic Radiation Experiment (AWARE).

54 ENVIRONMENTAL SCIENCES↗