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DOE OSTI2020

Carbon Dioxide Fluxes to the Atmosphere From Waters Within Flooded Forests in the Amazon Basin

Aquatic habitats in the lowland Amazon emit large quantities of carbon dioxide (CO 2 ). However, information on CO 2 fluxes from seasonally flooded forests that constitute 80% of the surface area of aquatic environments in the lowland Amazon basin is sparse. We provide the first multi-year measurements of CO 2 exchanges within flooded forests of the central Amazon basin. Our approach combines measurement of dissolved CO 2 concentrations and fluxes between the water and atmosphere and ecological data. Although the rates of CO 2 emission by flooded forests are lower than other aquatic habitats, such as open waters in rivers and lakes, the combination of high CO 2 concentrations and a large area results in an appreciable regional out gassing of carbon dioxide from flooded forests. These fluxes can represent about half of the net primary production of flooded forests in the central Amazon basin.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2007

Distribution of Aboveground Live Biomass in the Amazon Basin

The amount and spatial distribution of forest biomass in the Amazon basin is a major source of uncertainty in estimating the flux of carbon released from land-cover and land-use change. Direct measurements of aboveground live biomass (AGLB) are limited to small areas of forest inventory plots and site-specific allometric equations that cannot be readily generalized for the entire basin. Furthermore, there is no spaceborne remote sensing instrument that can measure tropical forest biomass directly. To determine the spatial distribution of forest biomass of the Amazon basin, we report a method based on remote sensing metrics representing various forest structural parameters and environmental variables, and more than 500 plot measurements of forest biomass distributed over the basin. A decision tree approach was used to develop the spatial distribution of AGLB for seven distinct biomass classes of lowland old-growth forests with more than 80% accuracy. AGLB for other vegetation types, such as the woody and herbaceous savanna and secondary forests, was directly estimated with a regression based on satellite data. Results show that AGLB is highest in Central Amazonia and in regions to the east and north, including the Guyanas. Biomass is generally above 300Mgha(sup 1) here except in areas of intense logging or open floodplains. In Western Amazonia, from the lowlands of Peru, Ecuador, and Colombia to the Andean mountains, biomass ranges from 150 to 300Mgha(sup 1). Most transitional and seasonal forests at the southern and northwestern edges of the basin have biomass ranging from 100 to 200Mgha(sup 1). The AGLB distribution has a significant correlation with the length of the dry season. We estimate that the total carbon in forest biomass of the Amazon basin, including the dead and below ground biomass, is 86 PgC with +/- 20% uncertainty.

rainforest↗

NASA NTRS2020

Basin-Scale River Runoff Estimation from GRACE Gravity Satellites, Climate Models and In Situ Observations: a Case Study in the Amazon Basin

River runoff is estimated as a water budget residual using Gravity Recovery and Climate Experiment (GRACE) terrestrial water storage time series, ERA5 reanalysis data, and precipitation observations for January 2003 through December 2015 for the Obidos upstream drainage basin and for the entire Amazon basin. Estimated runoff based on the water budget agrees remarkably well with in situgauge observations at Obidos, especially at seasonal time scales, with nearly perfect phase agreementbut slightly larger seasonal amplitude. The discrepancy in the seasonal amplitude maybe attributed to underestimation of river gauge runoff during the wet season when water overflows the riverbanks. The ERA5 model appears to overestimate long-term mean evapotranspiration in the Amazon by ~2 cm/monthb ased on comparisons with precipitation and runoff observations. Using precipitation data based on satellites and gauge observations relative to gauge observations alone improved agreement between water budget runoff estimates and in situ runoff observations. Seasonal variations in ERA5 simulated runoff are about twice as large as those from in situobservations and show a large phase lag as well. Water budget based runoff for the entire Amazon (~ 7,200 km3averaged 29over the 13 yr period) is significantly larger than observed runoff (~5,700 km3) at notably larger than previous estimates for the entire Amazon. These differences may be partly related to submarine runoff from the Amazon basin that cannot be captured by surface gauges.

Jianli Chen↗

NASA NTRS1992

Saharan dust in the Amazon Basin

It is shown that Saharan dust enters the Central Amazon Basin in bursts that accompany major wet season rain systems. Low-level horizontal convergence feeding these rain systems draws dust from plumes that have crossed the tropical Atlantic under the large-scale circulation fields. Mass exchange of air between the surface and four kilometers over the eastern Amazon basin is calculated utilizing rawinsonde data collected during storm events. Mean concentrations of dust observed by aircraft over the western tropical Atlantic are employed to calculate the amount of dust injected into the basin.

Swap, R.↗

DOE OSTI2020

Mixing states of Amazon basin aerosol particles transported over long distances using transmission electron microscopy

The Amazon basin is important for understanding the global climate because of its carbon cycle and as a laboratory for obtaining basic knowledge of the continental background atmosphere. Aerosol particles play an important role in the climate and weather, and knowledge of their compositions and mixing states is necessary to understand their influence on the climate. For this study, we collected aerosol particles from the Amazon basin during the Green Ocean Amazon (GoAmazon2014/5) campaign (February to March 2014) at the T3 site, which is located about 70 km from Manaus, and analyzed them using transmission electron microscopy (TEM). TEM has better spatial resolution than other instruments, which enables us to analyze the occurrences of components that attach to or are embedded within other particles. Based on the TEM results of more than 10 000 particles from several transport events, this study shows the occurrences of individual particles including compositions, size distributions, number fractions, and possible sources of materials that mix with other particles. Aerosol particles during the wet season were from both natural sources such as the Amazon forest, Saharan desert, Atlantic Ocean, and African biomass burning and anthropogenic sources such as Manaus and local emissions. These particles mix together at an individual particle scale. The number fractions of mineral dust and sea-salt particles increased almost 3-fold when long-range transport (LRT) from the African continent occurred. Nearly 20 % of mineral dust and primary biological aerosol particles had attached sea salts on their surfaces. Sulfates were also internally mixed with sea-salt and mineral dust particles. The TEM element mapping images showed that several components with sizes of hundreds of nanometers from different sources commonly occur within individual LRT aerosol particles. We conclude that many aerosol particles from natural sources change their compositions by mixing during transport. The compositions and mixing states of these particles after emission result in changes in their hygroscopic and optical properties and should be considered when assessing their effects on climate.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Mixing states of Amazon-basin aerosol particles transported over long distances using transmission electron microscopy

The Amazon basin is important for understanding the global climate both because of its carbon cycle and as a laboratory for obtaining basic knowledge of the continental background atmosphere. Aerosol particles play an important role in the climate and weather, and knowledge of their compositions and mixing states is necessary to understand their influence on the climate. For this study, we collected aerosol particles from the Amazon basin during the Green Ocean Amazon (GoAmazon2014/5) campaign (February to March 2014) at the T3 site, which locates about 70 km from Manaus, and analyzed using transmission electron microscopy (TEM). TEM has better spatial resolution than other instruments, which enables us to analyse the occurrences of components that attach to or are embedded within other particles. Based on the TEM results of more than 10,000 particles from several transport events, this study shows the occurrences of individual particles including compositions, size distributions, number fractions, and possible sources of materials that mix with other particles. Aerosol particles during the wet season were from both natural sources such as the Amazon forest, Saharan desert, Atlantic Ocean, and African biomass burning and anthropogenic sources such as Manaus and local emissions. These particles mix together at an individual particle scale. The number fractions of mineral dust and sea-salt particles increased almost three-fold when long-range transport (LRT) from the African continent occurred. Nearly 20 % of mineral dust and primary biological aerosol particles attached sea salts on their surfaces. Sulfates were also internally mixed with sea-salt and mineral dust particles. The TEM element mapping images showed that several components with sizes of hundreds of nanometres from different sources commonly occur within individual LRT aerosol particles. We conclude that many aerosol particles from natural sources change their compositions by mixing during transport. The compositions and mixing states of these particles after emission result in changes in their hygroscopic and optical properties and should be considered when assessing their effects on climate.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1988

Boundary layer ozone - An airborne survey above the Amazon Basin

Ozone data obtained over the forest canopy of the Amazon Basin during July and August 1985 in the course of NASA's Amazon Boundary Layer Experiment 2A are discussed, and ozone profiles obtained during flights from Belem to Tabatinga, Brazil, are analyzed to determine any cross-basin effects. The analyses of ozone data indicate that the mixed layer of the Amazon Basin, for the conditions of undisturbed meteorology and in the absence of biomass burning, is a significant sink for tropospheric ozone. As the coast is approached, marine influences are noted at about 300 km inland, and a transition from a forest-controlled mixed layer to a marine-controlled mixed layer is noted.

Gregory, Gerald L.↗

NASA NTRS2002

Space-Time Controls on Carbon Sequestration Over Large-Scale Amazon Basin

A major research focus of the LBA Ecology Program is an assessment of the carbon budget and the carbon sequestering capacity of the large scale forest-pasture system that dominates the Amazonia landscape, and its time-space heterogeneity manifest in carbon fluxes across the large scale Amazon basin ecosystem. Quantification of these processes requires a combination of in situ measurements, remotely sensed measurements from space, and a realistically forced hydrometeorological model coupled to a carbon assimilation model, capable of simulating details within the surface energy and water budgets along with the principle modes of photosynthesis and respiration. Here we describe the results of an investigation concerning the space-time controls of carbon sources and sinks distributed over the large scale Amazon basin. The results are derived from a carbon-water-energy budget retrieval system for the large scale Amazon basin, which uses a coupled carbon assimilation-hydrometeorological model as an integrating system, forced by both in situ meteorological measurements and remotely sensed radiation fluxes and precipitation retrieval retrieved from a combination of GOES, SSM/I, TOMS, and TRMM satellite measurements. Brief discussion concerning validation of (a) retrieved surface radiation fluxes and precipitation based on 30-min averaged surface measurements taken at Ji-Parana in Rondonia and Manaus in Amazonas, and (b) modeled carbon fluxes based on tower CO2 flux measurements taken at Reserva Jaru, Manaus and Fazenda Nossa Senhora. The space-time controls on carbon sequestration are partitioned into sets of factors classified by: (1) above canopy meteorology, (2) incoming surface radiation, (3) precipitation interception, and (4) indigenous stomatal processes varied over the different land covers of pristine rainforest, partially, and fully logged rainforests, and pasture lands. These are the principle meteorological, thermodynamical, hydrological, and biophysical control paths which perturb net carbon fluxes and sequestration, produce time-space switching of carbon sources and sinks, undergo modulation through atmospheric boundary layer feedbacks, and respond to any discontinuous intervention on the landscape itself such as produced by human intervention in converting rainforest to pasture or conducting selective/clearcut logging operations.

Smith, Eric A.↗

NASA NTRS1988

The cycle of biogenic sulfur compounds over the Amazon Basin. I - Dry season

The concentrations of SO2, methylmercaptan, dimethylsulfide, H2S, aerosol sulfate, and methanesulfonate over the Amazon Basin during the July/August dry season were determined from samples collected by the NASA research aircraft. The results indicate that biogenic emissions represent an important, if not the dominant, source of sulfur to the atmosphere over Amazonia. Per unit area, the wet continental tropics appear to have about the same reduced sulfur emission flux as the oceanic area average (about 6 nmol/sq m per min), consistent with the fact that the aerosol sulfate concentration over the Amazon Basin is similar to the excess sulfate levels over the remote oceans. However, since the wet tropical continents represent only about 3 percent of the earth's surface, their global contribution is modest; it is also small relative to the anthropogenic emissions from fossil fuel burning.

Andreae, M. O.↗

NASA NTRS1988

Carbon monoxide over the Amazon Basin during the 1985 dry season

During the Amazon Boundary Layer Experiment, approximately 100 hours of in situ carbon monoxide measurements were obtained using a tunable diode laser sensor that provided continuous, fast-response (about 1 s) measurements. This data set, taken on board the NASA Electra between July 12 and August 12, 1985, characterizes the temporal and spatial changes in the CO distribution over the Amazon Basin as meteorological conditions progressed from the early to middle phases of the 1985 day season. Early dry-season CO values of 75-95 ppbv were generally observed in the PBL. As the dry season became well established, biomass burning and a persistent capping inversion at about 3 km profoundly altered the CO distribution, with PBL values typically reaching 150-275 ppbv. Concentrations as high as 800 ppbv were measured within identifiable haze layers. An analysis of satellite imagery shows that biomass burning was occurring along the Amazon River system and in savannah areas located more than 1000 km south of the region sampled.

Sachse, G. W.↗

NASA NTRS2007

Theorizing Land Cover and Land Use Change: The Peasant Economy of Colonization in the Amazon Basin

This paper addresses deforestation processes in the Amazon basin. It deploys a methodology combining remote sensing and survey-based fieldwork to examine, with regression analysis, the impact household structure and economic circumstances on deforestation decisions made by colonist farmers in the forest frontiers of Brazil. Unlike most previous regression-based studies, the methodology implemented analyzes behavior at the level of the individual property. The regressions correct for endogenous relationships between key variables, and spatial autocorrelation, as necessary. Variables used in the analysis are specified, in part, by a theoretical development integrating the Chayanovian concept of the peasant household with spatial considerations stemming from von Thuenen. The results from the empirical model indicate that demographic characteristics of households, as well as market factors, affect deforestation in the Amazon. Thus, statistical results from studies that do not include household-scale information may be subject to error. From a policy perspective, the results suggest that environmental policies in the Amazon based on market incentives to small farmers may not be as effective as hoped, given the importance of household factors in catalyzing the demand for land. The paper concludes by noting that household decisions regarding land use and deforestation are not independent of broader social circumstances, and that a full understanding of Amazonian deforestation will require insight into why poor families find it necessary to settle the frontier in the first place.

Caldas, Marcellus↗

NASA NTRS1990

The atmospheric sulfur cycle over the Amazon Basin. II - Wet season

The fluxes and concentrations of atmospheric sulfur species were determined at ground level and from aircraft over the Amazon Basin during the 1987 wet season, providing a comprehensive description of the sulfur cycle over a remote tropical region. The vertical profile of dimethylsulfide (DMS) during the wet season was found to be very similar to that measured during the dry season, suggesting little seasonal variation in DMS fluxes. The concentrations of H2S were almost an order of magnitude higher than those of DMS, which makes H2S the most important biogenic source species in the atmosheric sulfur cycle over the Amazon Basin. Using the gradient-flux approach, the flux of DMS at the top of the tree canopy was estimated. The canopy was a source of DMS during the day, and a weak sink during the night. Measurements of sulfur gas emissions from soils, using the chamber method, showed very small fluxes, consistent with the hypothesis that the forest canopy is the major source of sulfur gases. The observed soil and canopy emission fluxes are similar to those measured in temperate regions. The concentrations of SO2 and sulfate aerosol in the wet season atmosphere were similar to dry season values.

Andreae, M. O.↗

NASA NTRS1988

Carbon dioxide in the atmosphere over the Amazon Basin

As a part of the NASA's Amazon Boundary Layer Experiment 2A mission, the cycle of atmospheric CO2 over the Amazon Basin was examined using measured vertical profiles of CO2 concentrations in the canopy and aloft, and direct measurements of CO2 emissions from soils. The results provide a detailed picture of daily exchanges of air between the tropical forest (0-30) and the atmospheric boundary layer (30-2000 m). A comparison of atmospheric CO2 distributions over forests, wetlands, and rivers shows that the lower atmosphere over forests functions separately from that over rivers or wetlands during the night and to some extent during the day; the basic diurnal cycle of CO2 over wetlands is much weaker than over forests, and the cycle is almost absent over rivers. This result is consistent with expectations based on the biogeochemistry of organic carbon in these systems.

Wofsy, Steven C.↗

NASA NTRS2013

Surface Freshwater Storage and Variability in the Amazon Basin from Multi-Satellite Observations, 1993-2007

The amount of water stored and moving through the surface water bodies of large river basins (river, floodplains, wetlands) plays a major role in the global water and biochemical cycles and is a critical parameter for water resources management. However, the spatio-temporal variations of these freshwater reservoirs are still widely unknown at the global scale. Here, we propose a hypsographic curve approach to estimate surface freshwater storage variations over the Amazon basin combining surface water extent from a multi-satellite-technique with topographic data from the Global Digital Elevation Model (GDEM) from Advance Spaceborne Thermal Emission and Reflection Radiometer (ASTER). Monthly surface water storage variations for 1993-2007 are presented, showing a strong seasonal and interannual variability, and are evaluated against in situ river discharge and precipitation. The basin-scale mean annual amplitude of approx. 1200 cu km is in the range of previous estimates and contributes to about half of the Gravity Recovery And Climate Experiment (GRACE) total water storage variations. For the first time, we map the surface water volume anomaly during the extreme droughts of 1997 (October-November) and 2005 (September-October) and found that during these dry events the water stored in the river and flood-plains of the Amazon basin was, respectively, approx. 230 (approx. 40%) and 210 (approx. 50%) cu km below the 1993-2007 average. This new 15year data set of surface water volume represents an unprecedented source of information for future hydrological or climate modeling of the Amazon. It is also a first step toward the development of such database at the global scale.

Storage↗

NASA NTRS1988

Tropospheric nitric oxide measurements over the Amazon Basin

Horizontal and vertical distributions of nitric oxide (NO) were measured over the Amazon Basin during NASA's Global Tropospheric Experiment (GTE) Amazon Boundary Layer Experiment mission in July-August 1985. During transit flights between the Virginia coast and Manaus, Brazil, NO mixing ratios were 12-15 pptv at 5 km altitude. Values up to 200 pptv were observed in electrically active clouds. During longitudinal surveys over the Amazon region, NO mixing ratios in the lower planetary boundary layer decreased from 25-60 pptv over the central basin to 10-12 pptv in coastal regions. In the convective cloud layer or free troposphere, NO mixing ratios averaged 13 pptv in regions not influenced by biomass burning. No longitudinal trend above the mixed layer could be detected. A steep negative gradient with increasing altitude was noted within the mixed layer before midday. Mixing ratios decreased from 60 pptv at 0.2 km to about 15 pptv at the top of the mixed layer (1 km). By midday, growth of the mixed layer height and enhanced mixing reduced the gradient, and evidence for mixing of NO into the convective cloud layer was noted.

Torres, A. L.↗

NASA NTRS1984

Deforestation, floodplain dynamics, and carbon biogeochemistry in the Amazon Basin

Three aspects of the physical geographic environment of the Amazon Basin are considered: (1) deforestation and reforestation, (2) floodplain dynamics, and (3) fluvial geomorphology. Three independent projects are coupled in this experiment to improve the in-place research and to ensure that the Shuttle Imaging Radar-B (SIR-B) experiment stands on a secure base of ongoing work. Major benefits to be obtained center on: (1) areal and locational information, (2) data from various depression angles, and (3) digital radar signatures. Analysis will be conducted for selected sites to define how well SIR-B data can be used for: (1) definition of extent and location of deforestation in a tropical moist forest, (2) definition and quantification of the nature of the vegetation and edaphic conditions on the (floodplain) of the Amazon River, and (3) quantification of the accuracy with which the geometry and channel shifting of the Amazon River may be mapped using SIR-B imagery in conjunction with other remote sensing data.

Bryan, M. L.↗

NASA NTRS1994

Precipitation recycling in the Amazon basin

Precipitation recycling is the contribution of evaporation within a region to precipitation in that same region. The recycling rate is a diagnostic measure of the potential for interactions between land surface hydrology and regional climate. In this paper we present a model for describing the seasonal and spatial variability of the recycling process. The precipitation recycling ratio, rho, is the basic variable in describing the recycling process. Rho is the fraction of precipitation at a certain location and time which is contributed by evaporation within the region under study. The recycling model is applied in studyiing the hydrologic cycle in the Amazon basin. It is estimated that about 25% of all the rain that falls in the Amazon basin is contributed by evaporation within the basin. This estimate is based on analysis of a data set supplied by the European Centre for Medium-range Weather Forecasts (ECMWF). The same analysis is repeated using a different data set from the Geophysical Fluid Dynamics Laboratory (GFDL). Based on this data set, the recycling ratio is estimated to be 35%. The seasonal variability of the recycling ratio is small compared with the yearly average. The new estimates of the recycling ratio are compared with results of previous studies, and the differences are explained.

Eltahir, E. A. B.↗

DOE OSTI2022

Sulfuric acid in the Amazon basin: measurements and evaluation of existing sulfuric acid proxies

Abstract. Sulfuric acid is a key contributor to new particle formation, though measurements of its gaseous concentrations are difficult to make. Several parameterizations to estimate sulfuric acid exist, all of which were constructed using measurements from the Northern Hemisphere. In this work, we report the first measurements of sulfuric acid from the Amazon basin. These measurements are consistent with concentrations measured in Hyytiälä, Finland, though, unlike Hyytiälä, there is no clear correlation of sulfuric acid with global radiation. There was a minimal difference in sulfuric acid observed between the wet and dry seasons in the Amazon basin. We also test the efficacy of existing proxies to estimate sulfuric acid in this region. Our results suggest that nighttime sulfuric acid production is due to both a stabilized Criegee intermediate pathway and oxidation of SO2 by OH, the latter of which is not currently accounted for in existing proxies. These results also illustrate the drawbacks of the common substitution of radiation for OH concentrations. None of the tested proxies effectively estimate sulfuric acid measurements at night. For estimates at all times of day, a recently published proxy based on data from the boreal forest should be used. If only daytime estimates are needed, several recent proxies that do not include the Criegee pathway are sufficient. More investigation of nighttime sulfuric acid production pathways is necessary to close the gap between measurements and estimates with existing proxies.

54 ENVIRONMENTAL SCIENCES↗