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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records

Retrieval of the molecular orientation distribution from atom-pair angular distributions

Imaging laser-induced rotational dynamics is an important and active field due to its applications in capturing reactions in the molecular frame and in molecular imaging. Experimental measurement of the molecular orientation distribution, as a function of the Euler angles, has only been demonstrated for special cases when the detectable signal is generated along the molecular symmetry axis. Here we developed the general theory that maps the probability density distribution of the molecular orientation to the atom-pair angular distributions for nonlinear molecules. With the theory, the molecular orientation distribution can be retrieved from the measured atom-pair angular distribution, which we demonstrate experimentally using ultrafast electron diffractive imaging of impulsively aligned trifluoro-iodomethane molecules. Here, the retrieved molecular orientation distribution is in good agreement with direct numerical simulations of the time-dependent Schrodinger equation using the experimental conditions. Unlike the existing retrieval methods, the retrieval method does not require solving Schrodinger equation, works for any alignment method, and is in principle applicable to asymmetric top molecules.

74 ATOMIC AND MOLECULAR PHYSICS↗

Angular Distribution of Dimuons from Drell-Yan Production in p+Fe Interactions at 120 GeV Beam Energy

In the E906/SeaQuest Fermilab experiment, we report a measurement of the angular distributions by measuring the angular parameters $\lambda$, $\mu$, and $\nu$ of Drell-Yan dimuons produced using a 120 GeV proton beam incident on an iron target. The angular distribution in the naive Drell-Yan model does not show any $\cos2\phi$ dependency, where $\phi$ denotes the azimuthal angle of dimuons in the Collins-Soper frame. However, pion-induced Drell-Yan experiments, such as NA10 and E615, have observed a significant dependence on $\cos2\phi$. The Boer–Mulders function, a transverse momentum-dependent distribution function, represents the correlation between the transverse spin and the transverse momentum of the quark. A non-zero Boer-Mulders function or an improved higher-order Drell-Yan model considering QCD effects can produce a $\cos 2\phi$ modulation in the Drell-Yan angular distribution. To measure the angular distributions, we have used an event mixing method to construct the combin atorial background, which was then subtracted from the data to isolate the Drell-Yan signal. Following this, we corrected the detector, trigger, and reconstruction efficiencies using a doubly-iterative Bayesian Unfolding method. This iterative unfolding technique improves the response matrix based on the results of the previous unfolding step, ensuring robust convergence without exaggeration of uncertainties. The angular distributions of the dimuons were measured over the invariant mass range $5.0 < M_{\mu^+ \mu^-} < 8.0$ $GeV/c^2$, with dimuon transverse momentum $P_T < 2$ GeV/c and Feynman-x $-0.18 < x_F < 0.9$. The measured angular distributions are then compared with the QCD calculations for $p + \text{Fe}$ interactions, and proton-induced angular distribution measurements from other experiments. We have observed weak $\cos 2\phi$ modulations as a function of $P_T$. For $P_T > 1.0 \, \text{GeV}/c$, the predicted NNLO perturbative QCD value of $\nu$ is larger than what we have me asured at E906/SeaQuest. Moreover, we have not observed a strong dependence of $\nu$ on the kinematic variables, such as dimuon mass $M_{\mu^+ \mu^-}$ and Bjorken-$x$. The spin alignment of the virtual photon, $\lambda$, measured from the SeaQuest Drell-Yan $p+\text{Fe}$ data, is found to be strongly dependent on $P_T$, decreasing as $P_T$ increases. $\lambda$ also holds to the upper bound condition $\lambda < 1.0$ within the statistical uncertainty, showing a trend similar to that predicted by NNLO perturbative QCD. However, for $1.0 < P_T < 2.0 \, \text{GeV}/c$, the extracted $\lambda$ value from SeaQuest is smaller than that predicted by perturbative QCD at NNLO.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Effects of anisotropic electron-ion interactions in atomic photoelectron angular distributions

A summary of the angular momentum transfer formulation of the differential photoionization cross section is presented and photoionization amplitudes in LS coupling are considered. The application of the theoretical concepts and relations developed is illustrated with the aid of an example involving the calculation of the angular distribution of photoelectrons ionized from atomic sulfur according to a certain reaction. The investigation shows that anisotropic electron-ion interactions in atomic sulfur lead to measurable differences between photoelectron angular distribution asymmetry parameters corresponding to alternative ionic term levels.

Dill, D.↗

Recent findings on angular distributions of dayside ring current energetic ions

The angular distributions observed in the equatorial region for energetic protons, helium ions, and carbon-nitrogen-oxygen ions are investigated. The anisotropy index for the ions in the equatorial magnetosphere between L shells is examined, and a variety of angular distributions different from simple pancake distributions are presented. The survey reveals unusual angular distributions which suggest for the first time a net field-aligned transport of energetic ring current ions and a sharp intensity enhancement over a pitch angle range centered at 90 deg. The latter reflects a sharp boundary of ring curent energetic ions at L of roughly 3 and 4, plausibly due to the addition of a newly injected population.

Lui, A. T. Y.↗

Probing light quark Yukawa couplings through angularity distributions in Higgs boson decay

We propose to utilize angularity distributions in Higgs boson decay to probe light quark Yukawa couplings at e + e - colliders. Angularities $τ$ a are a class of 2-jet event shapes with variable and tunable sensitivity to the distribution of radiation in hadronic jets in the final state. Using soft-collinear effective theory (SCET), we present a prediction of angularity distributions from Higgs decaying to quark and gluon states at e + e - colliders to NNLL + $\mathcal{O}$(α s ) accuracy. Due to the different color structures in quark and gluon jets, the angularity distributions from H → $q\overline{q}$ and H → gg show different behaviors and can be used to constrain the light quark Yukawa couplings. We show that the upper limit of light quark Yukawa couplings could be probed to the level of ~ 15% of the bottom quark Yukawa coupling in the Standard Model in a conservative analysis window far away from nonperturbative effects and other uncertainties; the limit can be pushed to ≲ 7 – 9% with better control of the nonperturbative effects especially on gluon angularity distributions and/or with multiple angularities.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Ion and electron angular distributions in the Io torus region of the Jovian magnetosphere

Angular distributions are presented of ion (about 0.5-2 MeV) and electron (greater than 10 MeV) fluxes measured during the Voyager 1 spacecraft passage through the inner regions of the Jovian magnetosphere. In the regions of peak flux intensities, just outside the orbit of Io, the ion angular distributions are most sharply peaked at 90 deg local pitch angle, a configuration consistent with diffusion of the particles inward from large radial distances. Inside the orbit of Io the lower-energy ions exhibit angular distributions depleted at 90 deg local pitch angles, suggesting the possibility of charge-exchange scattering loss of these particles. In the vicinity of the Io flux tube, no significant effect is observed in the flux or pitch angle distributions of the ions. The relativistic electrons are depleted in the flux tube region and exhibit an asymmetrical pitch angle distribution, with more electrons appearing to arrive from the equatorial region (the direction of Io) than from the low-altitude mirror point.

Lanzerotti, L. J.↗

Constructing angular distributions of neutrinos in core-collapse supernovae from zeroth and first moments calibrated by full Boltzmann neutrino transport

Two-moment neutrino transport methods have been widely used for developing theoretical models of core-collapse supernovae (CCSN), since they substantially reduce the computational burden inherent in the multidimensional neutrino-radiation hydrodynamical simulations. The approximation, however, comes at a price; the detailed structure of angular distribution of neutrinos is sacrificed, that is the main drawback of this approach. In this paper, we develop a novel method by which to construct angular distributions of neutrinos from the zeroth and first angular moments. In our method, the angular distribution is expressed with two quadratic functions of the neutrino angle in a piecewise fashion. We determine the best parameters in the fitting function by comparing to the neutrino data in a spherically symmetric CCSN model with full Boltzmann neutrino transport. We demonstrate the capability of our method by using our recent 2D CCSN model. In this work, we find that the essential features of the angular distributions can be well reconstructed, whereas the angular distributions of incoming neutrinos tend to have large errors that increase with flux factor ($\textit{κ}$). This issue originates from the insensitiveness of incoming neutrinos to $\textit{κ}$, that is an intrinsic limitation in moment methods. Based on the results of the demonstration, we assess the reliability of electron- neutrinos lepton number (ELN)-crossing searches with the two-moment neutrino transport. This analysis is complementary to our [L. Johns and H. Nagakura arXiv:2104.04106] that scrutinizes the limitation of crossing searches with a few moments. We find that the systematic errors of angular distributions for incoming neutrinos lead to misjudgements of the crossing at $\textit{κ}$ ≳ 0.5. This casts doubt on the results of ELN-crossing searches based on two-moment methods in some previous studies.

79 ASTRONOMY AND ASTROPHYSICS↗

Anisotropy in fission fragment and prompt neutron angular distributions

Several physics mechanisms can lead to the deviation from an isotropic angular distribution for both fission fragments and the neutrons that are emitted during the fission event. Two of these effects have recently been implemented into CGMF, the Monte Carlo fission event generator developed at Los Alamos National Laboratory: angular distribution sampling for fission fragments and pre-equilibrium neutrons (those emitted before the compound nucleus forms). Using these new developments, we show that the anisotropy of the neutrons reflects the anisotropy of the fission fragments, in particular as the outgoing energy of neutrons increases. Correlations between the fission fragment and neutron anisotropies could be used to extract the fission fragment anisotropy from the neutron angular distributions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Electron angular distributions during charging events

The angular distribution of electrons and ions at times of spacecraft charging were examined for several charging events. Generally it was found that electrons measured perpendicular to the Earth's magnetic field are more intense and more energetic than those measured parallel to the magnetic field during charging events. During the substorm charging injection, the electron spectra harden at all angles to the magnetic field as the evolution of the charging spectra is monitored by the P78-2 satellites. An example of the onset of charging and the changes in the electron distributions is examined. The evolution of the electrons from a 'soft' plasma sheet distribution to a 'hard' charging distribution is compared with the charging of Kapton on the satellite and the spacecraft frame potential. The ions are used to determine the spacecraft potential. Evidence of periodic surface potential variations related to particle anisotropies are presented and discussed.

Fennell, J. F.↗

Incorporating new evaluation on angular distributions and energy spectra of neutron-induced charged particle reactions into the next ENDF library release (Technical Progress Report)

This project aims to provide the improved Evaluated Nuclear Data File (ENDF) using the newly measured data as well as the latest nuclear reaction model for calculating angular distributions and energy spectra on neutron-induced charged particle reactions through the collaboration of Korea Atomic Energy Research Institute (KAERI) and Los Alamos National Laboratory (LANL). The LANL group will provide the experimental data for angular distributions and spectra of (n,p) and (n,α) on several structural materials such as Fe, Ni and Zn isotopes using the Low Energy Neutron-induced Charged-particle (Z) Chamber (LENZ) instrument at Los Alamos Neutron Science Center (LANSCE). The KAERI group will provide the improved evaluated nuclear library which is based on the LANL experimental data, and further will predict angular distributions and spectra of (n,p) and (n,α) reactions on unmeasured nuclides, such as Cr, Mn, Co, Cu and so on. For the first year of this project, we planned to analyze (n,p) and (n,α) reactions for 54,56 Fe and perform new measurements on those reactions for 58,60 Ni isotopes with the LENZ instrument at LANSCE. For improving our evaluation quality, we have studied reaction models to reproduce LANL’s experimental angular distributions and energy spectra using the full Hauser-Feshbach model code, CoH3 with no approximations used. As the first year’s deliverables, we provided the experimental (n,p) and (n,α) reaction cross sections for 54,56 Fe and incorporate new evaluation on angular distributions and energy spectra of neutron-induced charged particle reactions into the current ENDF/B-VIII.0.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Photoelectron angular distributions as a probe of anisotropic electron-ion interactions

Expressions are given for atomic photoelectron angular distributions in LS coupling in which the role of anisotropic final state electron-ion interactions emerges explicitly. Calculations of photoelectron angular distributions for atomic sulfur are presented in which these anisotropic interactions produce pronounced deviations from the predictions of the Cooper-Zare model. Such effects are expected to be a general feature of photoelectron angular distributions for most open shell atoms.

Dill, D.↗

Photoelectron angular distributions as a probe of anisotropic electron-ion interactions

Expressions are given for atomic photoelectron angular distributions in LS coupling in which the role of anisotropic final state electron-ion interactions emerges explicitly. Calculations of photoelectron angular distributions for atomic sulfur are presented in which these anisotropic interactions produce clear deviations from the predictions of the Cooper-Zare model. Such effects are expected to be a general feature of photoelectron angular distributions for most open-shell atoms.

Dill, D.↗

Changes in TOA SW Fluxes over Marine Clouds When Estimated via Semiphysical Angular Distribution Models

Top-of-atmosphere (TOA) shortwave (SW) angular distribution models (ADMs) approximate—per angular direction of an imagined upward hemisphere—the intensity of sunlight scattered back from a specific Earth–atmosphere scene. ADMs are, thus, critical when converting satellite-borne broadband radiometry into estimated radiative fluxes. This paper applies a set of newly developed ADMs with a more refined scene definition and demonstrates tenable changes in estimated fluxes compared to currently operational ADMs. Newly developed ADMs use a semiphysical framework to consider cloud-top effective radius (¯¯R_e) and above-cloud water vapor (ACWV), in addition to accounting for surface wind speed and clouds’ phase, fraction, and optical depth. In effect, instantaneous TOA SW fluxes for marine liquid-phase clouds had the largest flux differences (of up to 25 W m−2) for lower solar zenith angles and cloud optical depth greater than 10 due to extremes in ¯¯R_e or ACWV. In regions where clouds had persistently extreme levels of ¯¯R_e (here mostly for ¯¯R_e < 7μm and ¯¯R_e > 15μm) or ACWV, instantaneous fluxes estimated from Aqua, Terra, Meteosat-8, and Meteosat-9 satellites using the two ADMs differed systematically, resulting in significant deviations in daily mean fluxes (up to ±10 W m^(−2)) and monthly mean fluxes (up to ±5 W m^(−2)). Flux estimates using newly developed, semiphysical ADMs may contribute to a better understanding of solar fluxes over low-level clouds. It remains to be seen whether aerosol indirect effects are impacted by these updates.

angular distribution models (ADMs)↗

Energy spreading and angular distribution of a beam of electrons in molecular hydrogen

A Monte Carlo approach is used to obtain the energy spreading and angular distribution of initially monoenergetic and monodirectional beams of electron incident on a gas of molecular hydrogen. Several beams of primary electrons and the resultant secondaries are degraded in a step-by-step procedure which utilizes a detailed set of cross sections, together with reasonable approximations for the creation of secondary electrons. Particular attention is paid to the initial angular distribution of secondary electrons. An analytic function which characterizes current experimental differential cross-section data is used to provide realistic inputs into our calculations. The results for energy distribution as a function of distance and angular distribution at selected energies and distances are illustrated.

Heaps, M. G.↗

Angular distributions of electrons of energy E sub e greater than 0.06 MeV in the Jovian magnetosphere

The results of an angular distribution analysis of the electron intensity data recorded near Jupiter for the period from 26 November to 14 December 1973 are presented. The data were from three directional particle detectors with effective integral electron energy thresholds of 0.06, 0.55, and 5.0 Mev, respectively. It was found that the central core of the magnetosphere, within 12 Jupiter radii, is dominated by pitch angle distributions strongly peaked at alpha = 90 deg, while the region from 12 to 25 Jupiter radii shows bidirectional and approximately equal maxima at alpha = 0 and 180 deg. Bidirectional angular distributions in the magnetodisc out to the radius of the magnetopause strongly suggest quasi-trapping on closed field lines as the predominant situation. Substantial field aligned, unidirectional streaming was detected on only two occasions. No distinctive effects on angular distributions were discerned near the L-shells of satellites.

Sentman, D. D.↗

Developing an Aircraft-Based Angular Distribution Model of Solar Reflection from Wildfire Smoke to Aid Satellite-Based Radiative Flux Estimation

This study examines the angular distribution of scattered solar radiation associated with wildfire smoke aerosols observed over boreal forests in Canada during the ARCTAS (Arctic Research of the Composition of the Troposphere from Aircraft and Satellites) campaign. First, it estimates smoke radiative parameters (550 nm optical depth of 3.9 and single scattering albedo of 0.90) using quasi-simultaneous multiangular and multispectral airborne measurements by the Cloud Absorption Radiometer (CAR). Next, the paper estimates the broadband top-of-atmosphere radiances that a satellite instrument such as the Clouds and the Earth’s Radiant Energy System (CERES) could have observed, given the narrowband CAR measurements made from an aircraft circling about a kilometer above the smoke layer. This estimation includes both an atmospheric correction that accounts for the atmosphere above the aircraft and a narrowband-to-broadband conversion. The angular distribution of estimated radiances is found to be substantially different than the angular model used in the operational data processing of CERES observations over the same area. This is because the CERES model is a monthly average model that was constructed using observations taken under smoke-free conditions. Finally, a sensitivity analysis shows that the estimated angular distribution remains accurate for a fairly wide range of smoke and underlying surface parameters. Overall, results from this work suggest that airborne CAR measurements can bring some substantial improvements in the accuracy of satellite-based radiative flux estimates.

Varnai, Tamas↗

Angular distribution of 𝛾 rays from a neutron-induced 𝑝-wave resonance of 132 Xe

A neutron-energy dependent angular distribution was measured for individual 𝛾 rays from the 3.2 eV 𝑝-wave resonance of 131 Xe+⁢𝑛, that shows enhanced parity violation owing to a mixing between 𝑠- and 𝑝-wave amplitudes. The 𝛾-ray transitions from the 𝑝-wave resonance were identified, and the angular distribution with respect to the neutron momentum was evaluated as a function of the neutron energy for 7132 keV 𝛾 rays, which correspond to a transition to the 1807 keV excited state of 132 Xe. The angular distribution is considered to originate from the interference between 𝑠- and 𝑝-wave amplitudes, and will provide a basis for a quantitative understanding of the enhancement mechanism of the fundamental parity violation in compound nuclei.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗