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Aerodynamic effects on outer ash deposition rates in second generation atmospheric pressure oxy-coal combustion systems
Recent measurements in scenarios representative of second generation atmospheric pressure oxy-coal combustion systems have shown a significant increase in ash deposition rates in comparison to combustion in air. However, the causative mechanisms behind this increase have not been well understood. To fill this void, well-characterized experiments including fuel and deposit particle size distributions (PSDs) were coupled with highly resolved numerical simulations to isolate the aerodynamic effects impacting the deposition process such that mechanisms could be hypothesized. Three combustion scenarios (AIR, OXY27, OXY70) spanning a factor of three variation in flue gas volumetric flow rates were simulated and the deposition characteristics (impaction rates, deposit PSD, temperature, residence times, capture rates) tracked/predicted using a customized deposition module. The measured deposit PSD was significantly different from the PSD of the parent fuel indicating significant physio-chemical transformations (coalescence and particle growth in particular) at play. The use of simplistic modeling approaches (swelling parameter variations) to model particle growth led to inaccurate deposit ash PSD and rate predictions. A more satisfactory agreement between the measurements and simulations was obtained when the functional form of the parent fuel PSD (spread parameter) was modified to conform closely to the deposit PSD while still ensuring the fidelity of temperature and velocity predictions. Based on the measured ash compositions, identical capture criteria were employed across all three scenarios. Here this study further supports the theory that the ash deposition rates in these systems are dominated by aerodynamic effects with the ash PSD playing a dominant role.
Measurements and Prediction of Ash Deposition in a Cyclone-Fired Boiler Operating under Variable Load Conditions
Measurements of ash deposition rates were made between the secondary superheater and reheater sections of a 450 MW cyclone-fired lignite boiler as the operational load varied from 33 to 100%. Significant reductions in deposition rates with a decrease in operational load were observed. To uncover the causative mechanisms behind these observations, operational data from the power plant were used to carry out computational fluid dynamic (CFD) simulations of the boiler. After ascertaining that the gas temperatures and velocities at various sections within the boiler were being represented adequately, decoupled simulations of the ash deposition process on the deposit probe were carried out using a finely resolved boundary layer mesh. Fly ash particle size distribution (PSD) and its concentration for the decoupled calculations were determined from stand-alone cyclone barrel simulations. The ash partitioning (mass %) between the fly ash and slag was found to be ~50:50, which was in line with previous field observations, and it did not vary significantly across different cyclone loads. The predicted PSD of the deposit ash was concentrated in the size range 10–30 microns, which was in agreement with cross-sectional images of the deposit obtained from the measurements. At lower loads, sharp variations in the deposition rates were predicted in the gas temperature range 950–1150 K. The particle kinetic energy—particle viscosity-based capture methodology utilized in this study in conjunction with appropriate ash compositions, ash viscosity models and gas temperature estimates can help estimate slagging propensities at different loads reasonably well in these systems.
Modeling ash deposition and shedding during oxy-combustion of coal/rice husk blends at 70% inlet O2
Abstract Co-firing rice husk (RH) and coal with carbon capture using oxy-combustion presents a net carbon negative energy production opportunity. In addition, the high fusion temperature of the non-sticky, silica rich, RH can mitigate ash deposition as well as promote shedding of deposits. To identify the optimum operating conditions, fuel particle sizes, and blend ratios that minimize ash deposition, a Computational Fluid Dynamic methodology with add-on ash deposition and shedding models were employed to predict outer ash deposition and shedding rates during co-combustion of coal/RH in AIR and O 2 /CO 2 (70/30 vol%, OXY70) oxidizer compositions. After ensuring that the fly-ash particle size distributions and particle Stokes numbers near the deposition surface were accurately represented (to model impaction), appropriate models for coal ash and RH ash viscosities that were accurate in the temperature region (1200–1300 K) of interest in this study were identified. A particle viscosity and kinetic energy (PKE) based capture criterion was enforced to model the ash capture. An erosion/shedding criterion that takes the deposit melt fraction and the energy consumed during particle impact into account was also implemented. Deposition rate predictions as well as the deposition rate enhancement (OXY70/AIR) were in good agreement with measured values. While the OXY70 scenario was associated with a significant reduction (60%–70%) in flue gas velocities, it also resulted in larger fly-ash particles. As a result, the PKE distributions of the erosive RH ash were similar in both scenarios and resulted in similar shedding rates.
An Integrated Approach to Predicting Ash Deposition and Heat Transfer in Coal-Fired Boilers
The overall goal of this project is to develop via measurements and simulations an advanced online technology to predict, monitor and manage fireside ash deposition in a coal-fired boiler allowing for more efficient operations under a range of load conditions and fuel property variability. With this in place fuel sorting and blending can be done upstream and operations can be optimized to compensate for load and fuel properties. In support of this objective, three experimental campaigns were undertaken during the course of the project to measure ash deposition rates within the boiler at different fuel flow rates and its ash composition variability. Simulations of the experimental conditions representing actual geometry, operational scenarios in terms of air flow rates, coal flow rates as well as coal compositions, heating values, and particle size distributions were also carried out. Deposition rates were predicted using a unique particle kinetic energy and viscosity based ash deposition methodology whose validity was ascertained by comparing against deposition rate measurements for widely varying operating conditions and ash compositions in a lab-scale furnace. With a unique end-to-end combustion modeling methodology established and different simulation scenarios carried out, the results from our computational fluid dynamic (CFD) simulations in conjunction with the plant data summarized in this report were used to refine Microbeam Technology Incorporated’s MTI CSPI-CT Tool to predict and monitor fire-side ash deposition under a range of load conditions and fuel property variability in real time.
Correlation of volcanic ash deposits by activation analysis of glass separates
Cascade mountains volcanic ash deposits elemental abundances correlation by computerized gamma ray spectra analysis of TRIGA reactor activated glass separates
Particle Size Distribution and Its Impacts on Ash Deposition and Radiative Transfer during Oxy-Combustion of Rice Husk–Natural Gas
Rice husk (RH) co-combustion with natural gas in highly oxygen-enriched concentrations presents a net carbon-negative energy production opportunity while minimizing flue gas recycling. However, recent experiments have shown enhanced ash deposition rates in oxygen-enriched conditions, with deposition/shedding also being dependent on the particle size distribution (PSD) of the parent RH fuel. To uncover the causative mechanisms behind these observations, add-on models for ash deposition/shedding and radiative properties were employed in computational fluid dynamics simulations. The combustion scenarios investigated encompassed two types of RH (US RH, Chinese RH) with widely varying ash contents (by % mass) and inlet fuel PSD with air and O2/CO2 (70/30 vol %, OXY70) as oxidizers. Utilizing the measured fly-ash PSDs near the deposit surface and modeling the particle viscosity accurately, particle kinetic-energy (PKE)-based capture and shedding criteria were identified as the keys to accurate deposition/shedding rate predictions. The OXY70 scenarios showed higher ash-capturing propensities due to their lower PKE. Conversely, higher erosion rates were predicted in the AIR firing scenarios. In addition, the radiative characteristics across all the scenarios were dominated by the gases and were not sensitive to the fly-ash PSD. Therefore, the higher particle concentrations in the OXY70 conditions did not negatively impact the heat extraction.
Update on Mitigation of Aerosol Impacts on Ash Deposition and Emission from Coal Combustion
Barr, in partnership with the University of North Dakota, Microbeam Technologies Inc., Envergex LLC, and MLJ Consulting, worked to develop a transformational technology that controls the formation of alkali aerosols found in coal ash. This technology mitigates ash deposition by injecting sorbents into the boiler and capturing volatile species responsible for boiler fouling, the primary cause for boiler outages. In this session, we’ll explore the science behind this technology and see some real-world results of its implementation.
Mitigation of Aerosol Impacts of Ash Deposition and Emissions from Coal Combustion (Final Technical Report)
This project was selected under FOA-0001989 Area of Interest (AOI) 2 – Power Plant Component Improvement. The objective of this AOI was to test and validate technologies and methodologies that can improve the efficiency, reliability, and/or flexibility of individual power plant components in existing plants. The aerosol mitigation technology comprises injection of sorbent into the boiler through injection lances using a positive-pressure blower. The injected sorbent interacts with flame-vaporized aerosolforming components produced during combustion reducing the abundance of sub-micrometer (< 1 micron) particles and fireside ash deposits in the boiler. The primary objective of this project was to validate a sorbent-based technology for mitigating fireside heat transfer surface fouling-related challenges in a full-scale coal-fired power generation facility, thereby, improving plant performance and reliability.
Chemically frozen multicomponent boundary layer theory of salt and/or ash deposition rates from combustion gases
There is increased interest in, and concern about, deposition and corrosion phenomena in combustion systems containing inorganic condensible vapors and particles (salts, ash). To meet the need for a computationally tractable deposition rate theory general enough to embrace multielement/component situations of current and future gas turbine and magnetogasdynamic interest, a multicomponent chemically 'frozen' boundary layer (CFBL) deposition theory is presented and its applicability to the special case of Na2SO4 deposition from seeded laboratory burner combustion products is demonstrated. The coupled effects of Fick (concentration) diffusion and Soret (thermal) diffusion are included, along with explicit corrections for effects of variable properties and free stream turbulence. The present formulation is sufficiently general to include the transport of particles provided they are small enough to be formally treated as heavy molecules. Quantitative criteria developed to delineate the domain of validity of CFBL-rate theory suggest considerable practical promise for the present framework, which is characterized by relatively modest demands for new input information and computer time.
Aerodynamic influences on the outer ash deposition rates during oxy-coal combustion
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Enrichment mechanism of arsenic in fine ash deposits during co-combustion of rice husk and coal
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Modelling Outer Ash Deposition Rates in Second Generation Atmospheric Pressure Oxy-Fuel Combustion Systems
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Large-eddy simulation of coal combustion in 15 MW pilot-scale boiler-simulation facility
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Gaussian Process Emulators for Volcanic Ash Dispersion Model Tephra2
It is necessary to predict volcanic ash deposition since falling ash is harmful to human activities. Because simulators built for this purpose are computationally expensive, it is popular to use statistical emulators for geophysical hazard analyses, where a large number of simulations are required. Gaussian stochastic process emulators are able to approximate expensive simulations in an accurate and efficient way. Using a relatively small number of simulation runs, a well-trained emulator can accurately predict simulation outputs at massive new input points in a few seconds. Under different explosive eruption conditions, we constructed Gaussian stochastic process emulators for Tephra2, a simulation tool for estimating the accumulation of volcanic ash over a region. Historical wind records are used as input wind data, without assuming a Gaussian wind speed profile or common wind direction among elevations. While there are several inputs for Tephra2, we use no more than three physically motivated variables as emulator inputs to reduce the computational cost of emulations. The emulator outputs predict the mass of tephra per unit area at 50281 grid points around a predetermined vent location.
Stratigraphic Evidence for Early Martian Explosive Volcanism in Arabia Terra
Several large paterae in Arabia Terra are suggested to be calderas that produced colossal explosive eruptions (i.e., supereruptions). If these features are indeed explosive calderas, dispersion modeling suggests extensive ash deposits should be common throughout the region. However, such deposits have not previously been linked with the suggested calderas. Here, we describe layered deposits containing minerals both consistent with and diagnostic of altered volcanic ash throughout Arabia Terra. These deposits include Al-dominant minerals such as montmorillonite, imogolite, and allophane among others. Altered ash deposits are found to thin (from 1-km to 100-m thickness) away from the suggested calderas. We estimate that the volcanic ash observed in Arabia Terra is the result of between 1,000 and 2,000 individual explosive eruptions over 500-million years. Our observations support the hypothesis that Arabia Terra hosted supereruptions in the late Noachian-early Hesperian that repeatedly blanketed the region with layers of ash.
Geologic setting of diverse volcanic materials in northern Elysium Planitia, Mars
Geologic mapping of high-resolution (30-50 m/pixel) Viking Orbiter images of northern Elysium Planitia has identified seven sites where current problems in martian volcanology, chronology, and stratigraphy can be resolved. These sites, which are discussed in the context of a potential Mars rover/sample return mission, would permit the following investigations: (1) the dating of Lower Amazonian lava flows from Elysium Mons (thereby providing absolute calibration for global crater size/frequency relative chronologies, (2) the petrologic investigation of long run-out lava flows, (3) the geologic interpretation of materials that may either be lava flows or lahar deposits, (4) the analysis of materials believed to be ash deposits produced by explosive eruptions of Hecates Tholus, and (5) the investigation of the stratigraphy of fractured terrain along the boundary between northern Elysium Planitia and southern Utopia Planitia.
Deposition and dose from the 18 May 1980 eruption of Mount St. Helens
The downwind deposition and radiation doses was calculated for the tropospheric part of the ash cloud from the May 18, 1980 eruption of Mount St. Helens, by using a large cloud diffusion model. The naturally occurring radionnuclides of radium and thorium, whose radon daughters normally seep very slowly from the rocks and soil, were violently released to the atmosphere. The largest dose to an individual from these nuclides is small, but the population dose to those affected by the radioactivity in the ash is about 100 person rem. This population dose from Mount St. Helens is much greater than the annual person rem routinely released by a typical large nuclear power plant. It is estimated that subsequent eruptions of Mount St. Helens have doubled or tripled the person rem calculated from the initial large eruption. The long range global ash deposition of the May 18 eruption is estimated through 1984, by use of a global deposition model. The maximum deposition is nearly 1000 kg square km and occurs in the spring of 1981 over middle latitudes of the Northern Hemisphere.