Investigation of the thermal and neutron irradiation response of BAM-11 bulk metallic glass
Abstract not provided
Brechtl, J.↗
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Experience by BAM in the Transport Package Safety Assessment of German Waste Containers - 18469
Transport and storage containers for low and mid-level radioactive waste are getting more and more of relevance due to the nuclear phase out decision in 2011. For higher activities Type B(U) approved waste containers will be needed for the shut down and dismantling phases of NPPs. It is expected that large quantities are required in the near future. German waste containers are generally approved for transport and interim storage and are also intended for the final disposal in the Konrad repository. BAM is involved in the authority licensing of transport package designs in Germany. In this context, BAM is responsible for the assessment of safe containment, mechanical, thermal and quality management issues. BAM also operates test facilities and performs drop as well as thermal tests during package licensing procedures. This paper summarizes our experience in the transport package design assessment of Type B(U) waste containers. A general overview of the approval process, the requirements and approaches BAM applies are described. Some examples are used to illustrate different aspects and technical issues we are addressing during the package assessment. In the first part of the paper the specific design aspects of German waste containers are described. Here, a general overview is given e.g. about closure systems, impact limiter designs, and the handling concepts. Furthermore, the wide range of radioactive content and their physical behavior including the impact on the packages assessment are described. The second part is focused on questions about the licensing and assessment process of German waste containers from the BAM authority point of view. The general approaches for the strategy of demonstration are outlined on the basis of the test conditions according to IAEA Regulations SSR-6. Furthermore, particular issues of the mechanical and thermal assessment with respect to the specific test conditions are discussed. For accident conditions of transport, aspects to be mentioned are e.g. the assessment of the lid bolts, the axial gap applied between content and lid, and the thermal behavior of the wood filled impact limiter after the fire test. However, issues of the assessment for routine and normal conditions of transport are addressed in this paper, too. The intention of this paper is introduce recent approval procedure experience in Germany, describing technical evaluation issues and so reduce rounds of questions during applications. (authors)
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
Bayesian Attack Model (BAM) User Story
This document presents a user story for the Bayesian Attack Model (BAM) tool designed to aggregate and analyze cyber-attack observables for operational technology (OT) systems. BAM aims to empower cybersecurity analysts by providing a streamlined interface for collecting observable data from various sources, enabling real-time analysis of potential adversary activity. By enhancing the response capabilities of security teams, BAM facilitates risk-informed decision-making and improves organizational security posture. This user story outlines the key functionalities, user interactions, and requirements necessary to successfully integrate BAM with other security information and event management (SIEM) technology and cybersecurity operations centers (CSOCs).
97 MATHEMATICS AND COMPUTING↗
Modeling East Asian Dust and Its Radiative Feedbacks in CAM4-BAM
East Asian dust and its radiative feedbacks are analyzed by the use of the fourth version of the Community Atmosphere Model (CAM4) with a bulk aerosol model parameterization (BAM) for the dust size distribution (CAM4-BAM). Two numerical experiments are conducted and intercompared: one with (Active) and one without (Passive) the radiative effects of dust aerosols. This CAM4-BAM captures the main spatial distribution of the dust aerosol optical depth (AOD) and the dust surface concentrations over East Asia, with positive correlations with the local observational data on annual and seasonal means. A comparative analysis of the Active and Passive experiments reveals that consideration of the dust-radiation interaction can significantly reduce dust emissions, loading, transport, and dry and wet depositions over East Asia, which is opposite to the enhanced dust cycle over North Africa. Further analysis of the contrasting dust-radiation feedbacks between North Africa and East Asia shows that over North Africa, the dust radiative forcing significantly increases the surface temperature and 10-m wind speed, whereas it decreases the surface temperature and the surface wind speeds over East Asia. These contrasting radiative effects, in turn, result in distinct dust cycle changes over these two regions. Thus, mechanistic analysis reveals that the radiative contrasts between East Asia and North Africa are mainly due to the differences in their regional surface albedo, dust vertical distribution and size distribution.
54 ENVIRONMENTAL SCIENCES↗
Breaking Barriers in Chalcogenide Perovskite Synthesis: A Generalized Framework for Fabrication of BaMS 3 (M═Ti, Zr, Hf) Materials
Abstract Chalcogenide perovskites have garnered increasing attention as stable, non‐toxic alternatives to lead halide perovskites. However, their conventional synthesis at high temperatures (>1000 °C) has hindered widespread adoption. Recent studies have developed low‐to‐moderate temperature synthesis methods (<600 °C) using reactive precursors, yet a comprehensive understanding of the pivotal factors affecting reproducibility and repeatability remains elusive. This study delineates the critical factors in the low‐temperature synthesis of BaMS 3 (M═Zr, Hf, Ti) compounds and presents a generalized framework. Innovative approaches are developed for synthesizing BaMS 3 compounds using this framework involving organometallics for solution deposition. The molecular precursor routes, employing metal acetylacetonates to generate soluble metal–sulfur bonded complexes and metal–organic compounds to produce soluble metal‐thiolate, metal‐isothiocyanate, and metal‐trithiocarbonate species, are demonstrated to yield carbon‐free BaMS 3 . These methods have achieved the most contiguous films of BaZrS 3 and BaHfS 3 using solution deposition to date. Furthermore, a hybrid solution processing method involving stacking sputter‐deposited Zr and solution‐deposited BaS layers is employed to synthesize a contiguous, oxygen‐free BaZrS 3 film. The diffuse reflectance measurements indicate a direct bandgap of ≈ 1.85 eV for the BaZrS 3 films and ≈ 2.1 eV for the BaHfS 3 film under investigation.
25 ENERGY STORAGE↗
Bayesian Attack Model (BAM)
The Bayesian Attack Model (BAM) is an analytical tool designed to enhance the comprehension of adversarial activity in OT environments. BAM leverages both expert cybersecurity insights and historical data to characterize the likelihood of adversarial behavior given anomalous observable events.
99 GENERAL AND MISCELLANEOUS↗
Structural and magnetic properties of Ni-Zn doped BaM nanocomposite via citrate precursor
Ni-Zn substituted M-type barium ferrite nanocomposite has been prepared via citrate precursor method. Nanocomposite having composition BaNi{sub 0.5}Zn{sub 0.5}Fe{sub 11}O{sub 19} was sintered at 900°C for 3hrs and characterized by using different characterization techniques. X-ray diffraction (XRD) confirmed the formation of double phase with most prominent peak at (114). Average crystallite size for pure BaM and BNZFO were found to be 36 nm & 45 nm. Field emission scanning electron microscopy (FESEM) confirmed the formation of hexagonal platelets with a layered structure. Magnetic properties of these samples were investigated by using vibrating sample magnetometer (VSM). Magnetic parameters like saturation magnetization (M{sub s}), coericivity (H{sub c}) and squareness ratio (SQR) of nanocomposite were found to be 60 emu/g, 3663 Oe and 0.6163 respectively. These values were noticed to be higher as compared to pure BaM. Enhanced magnetic properties of nanocomposite were strongly dependent on exchange coupling. Therefore these properties make this nanocomposite a suitable candidate for magnetic recording and high frequency applications.
77 NANOSCIENCE AND NANOTECHNOLOGY↗
A Comparative Study of Two BAM Designs for Friction Sensitivity Testing of Explosives
A new commercial design of BAM friction tester that utilizes a programmable servo motor was tested in comparison to the traditional cam-driven model. Displacement and velocity profiles were analyzed for both designs; significant differences were found between the two designs, most notable of which is that the traditional cam-driven unit has plate velocities that can be 50–75 % greater than those seen on the servo-driven model. Five energetic materials were also tested on each machine, including PETN, RDX, HMX, CL-20, and HNAB. Finally, results from the servo-driven model generally showed slightly less sensitivity when compared to the cam driven model, though the magnitude of the difference is not significant enough to require modification of safe handling procedures for the materials tested.
45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
BAM: bias assignment method to generate mock catalogues
Combining the statistics of dark matter tracers from a high-resolution cosmological N-body simulation and the dark matter density field calculated from down-sampled initial conditions using efficient structure formation solvers, we extract the halo-bias relation on a mesh of a 3$h^{-1}$ Mpc cell side resolution as a function of properties of the dark matter density field (e.g. local density, cosmic web type), automatically including stochastic, deterministic, local and non-local components. We use this information to sample the halo density field, accounting for ignored dependencies through an iterative process. By construction, our approach reaches ~1% accuracy in the majority of the k-range up to the Nyquist frequency without systematic deviations for power spectra (about $k ~ 1h$ Mpc -1 ) using either particle mesh or Lagrangian perturbation theory based solvers. When using phase-space mapping to compensate the low resolution of the approximate gravity solvers, our method reproduces the bispectra of the reference within 10% precision studying configurations tracing the quasi-non-linear regime. BAM has the potential to become a standard technique to produce mock halo and galaxy catalogues for future galaxy surveys and cosmological studies being highly accurate, efficient and parameter free.
79 ASTRONOMY AND ASTROPHYSICS↗
Radiative feedbacks of dust in snow over eastern Asia in CAM4-BAM
Dust in snow on the Tibetan Plateau (TP) could reduce the visible snow albedo by changing surface optical properties and removing the snow cover through increased snowmelt, which leads to a significant positive radiative forcing and remarkably alters the regional energy balance and the eastern Asian climate system. This work extends our previous investigation in dust–radiation interactions to investigate the dust-in-snow radiative forcing (SRF) and its feedbacks on the regional climate and the dust cycle over eastern Asia through the use of the Community Atmosphere Model version 4 with a Bulk Aerosol Model parameterizations of the dust size distribution (CAM4-BAM). Our results show that SRF increases the eastern Asian dust emissions significantly by 13.7% in the spring, countering a 7.6% decrease in the regional emissions by the dust direct radiative forcing (DRF). SRF also remarkably affects the whole dust cycle, including transport and deposition of dust aerosols over eastern Asia. The simulations indicate an increase in dust emissions of 5.1%, due to the combined effect of DRF and SRF. Further analysis reveals that these results are mainly due to the regional climatic feedbacks induced by SRF over eastern Asia. By reducing the snow albedo over the TP, the dust in snow mainly warms the TP and influences its thermal effects by increasing the surface sensible and latent heat flux, which in turn increases the aridity and westerly winds over northwestern China and affects the regional dust cycle. Additionally, the dust in snow also accelerates the snow-melting process, reduces the snow cover and then expands the eastern Asian dust source region, which results in increasing the regional dust emissions. Hence, a significant feature of SRF on the TP is the creation of a positive feedback loop that affects the dust cycle over eastern Asia.
54 ENVIRONMENTAL SCIENCES↗
Structure-property relationship in layered BaM n 2 S b 2 and B a 2 M n 3 S b 2 O 2
Layered transition-metal compounds have received great attention owing to their physical properties. In this work, we present the structural, electronic, thermal, and magnetic properties of BaMn 2 Sb 2 and Ba 2 Mn 3 Sb 2 O 2 single crystals, both with the layered structure analogous to high-temperature Cu- and Fe-based superconductors. While the Mn moment in the MnSb 4 tetrahedral environment forms a long-range G-type antiferromagnetic (AFM) ordering in both BaMn 2 Sb 2 (T N1 ≈443K) and Ba 2 Mn 3 Sb 2 O 2 (T N1 ≈314K), a short-range AFM order is found in the intercalated MnO 2 layer at a much lower temperature (T N2 ≈60K) coexisting with long-range G-type order in MnSb 4 layer in Ba 2 Mn 3 Sb 2 O 2 . The directions of the ordered moments in these two magnetic sublattices of Ba 2 Mn 3 Sb 2 O 2 are perpendicular to each other, even though the system is electrically conductive. The G-type AFM order in MnSb 4 layers in both compounds is distinct from the stripe-like order in Fe-based superconductors, but the in-plane magnetic structure in MnO 2 layers of Ba 2 Mn 3 Sb 2 O 2 is found to be similar to that in the cuprates. Our study acknowledges the significant and distinct roles of the CuO 2 - and FeAs 4 -type transition metal layers in the structure and their magnetic and electronic properties.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
First-principles study of crystalline and amorphous AlMgB{sub 14}-based materials
We report first-principles investigations of crystalline and amorphous boron and M1{sub x}M2{sub y}X{sub z}B{sub 14−z} (M1, M2 = Al, Mg, Li, Na, Y; X = Ti, C, Si) phases (so-called “BAM” materials). Phase stability is analyzed in terms of formation energy and dynamical stability. The atomic configurations as well as the electronic and phonon density states of these phases are compared. Amorphous boron consists of distorted icosahedra, icosahedron fragments, and dioctahedra, connected by an amorphous network. The presence of metal atoms in amorphous BAM materials precludes the formation of icosahedra. For all the amorphous structures considered here, the Fermi level is located in the mobility gap independent of the number of valence electrons. The intra-icosahedral vibrations are localized in the range of 800 cm{sup −1}, whereas the inter-icosahedral vibrations appear at higher wavenumbers. The amorphization leads to an enhancement of the vibrations in the range of 1100–1250 cm{sup −1}. The mechanical properties of BAM materials are investigated at equilibrium and under shear and tensile strain. The anisotropy of the ideal shear and tensile strengths is explained in terms of a layered structure of the B{sub 12} units. The strength of amorphous BAM materials is lower than that of the crystalline counterparts because of the partial fragmentation of the boron icosahedra in amorphous structures. The strength enhancement found experimentally for amorphous boron-based films is very likely related to an increase in film density, and the presence of oxygen impurities. For crystalline BAM materials, the icosahedra are preserved during elongation upon tension as well as upon shear in the (010)[100] slip system.
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
Energy, greenhouse gas, and water life cycle analysis of synthetic graphite anode production in the United States
This study presents a comprehensive life cycle analysis of potential synthetic graphite battery anode material (BAM) production in the U.S. based on industrial-scale data. The analysis focuses on three impacts: greenhouse gas (GHG) emissions, total energy use, and water consumption. We also conducted sensitivity analyses to evaluate the effect of variation in process parameters and energy sources used for synthetic graphite BAM production on its life cycle GHG emissions. A detailed supply chain analysis of graphite BAM in the U.S. was also undertaken, along with a study of its associated GHG emissions. The results show GHG emissions of 29.7 kg CO 2 -eq. per kg BAM, total energy use of 580 MJ kg −1 BAM, and water consumption of 121 L kg −1 BAM for the baseline condition. The graphitization step is a major process hotspot, contributing to over 74% of all impacts. This is attributed to the energy and material input requirements for this step, particularly through the use of crucibles. Across the entire synthetic graphite production process, electricity is the primary contributor, followed by crucibles used in graphite block production, and then calcined petroleum coke. Sensitivity analyses indicate that improvement in micronization yield, reuse of crucibles, and use of low-carbon nuclear energy can significantly reduce GHG emissions of potential domestic graphite production (by ∼70%). Supply chain analysis identified major graphite BAM sources in the U.S. and showed that the U.S. has a competitive advantage in domestic production of synthetic graphite BAM in terms of reduced life cycle GHG emissions compared to present-day imported sources (by ∼20%).
Battery anode↗
Outlook on texture evolution in additively manufactured stainless steels: Prospects for hydrogen embrittlement resistance, overview of mechanical, and solidification behavior
Abstract Realizing application specific manufacture with fusion-based additive manufacturing (F-BAM) processes requires understanding of the physical phenomena that drive evolution of microstructural attributes, such as texture. Current approaches for understanding texture evolution in F-BAM are majorly considerate of the phenomena occurring only during solidification. This hinders the comprehensive understanding and control of texture during F-BAM. In this perspective article, we discuss several physical phenomena occurring during and after solidification that can determine texture in F-BAM processed stainless steels (SS). A crystal plasticity-coupled hydrogen adsorption-diffusion modeling framework is also leveraged to demonstrate the prospects of grain boundary engineering with F-BAM for enhanced hydrogen embrittlement resistance of SS. Implications of varying thermokinetics in F-BAM for solidification behavior of SS are discussed. Additionally, microstructural attributes that are key to high temperature mechanical performance of SS are highlighted. Considerations as outlined in this perspective article will enable grain boundary engineering and application specific microstructural design of SS with F-BAM. Graphical abstract
36 MATERIALS SCIENCE↗
Structure of maize BZR1-type β-amylase BAM8 provides new insights into its noncatalytic adaptation
Plant β-amylase (BAM) proteins play an essential role in growth, development, stress response, and hormone regulation. Despite their typical (β/α) 8 barrel structure as active catalysts in starch breakdown, catalytically inactive BAMs are implicated in diverse yet elusive functions in plants. Further, the noncatalytic BAM7/8 contain N-terminal BZR1 domains and were shown to be involved in the regulation of brassinosteroid signaling and possibly serve as sensors of yet an uncharacterized metabolic signal. While the structures of several catalytically active BAMs have been reported, structural characterization of the catalytically inactive BZR1-type BAMs remain unknown. Here, we determine the crystal structure of β-amylase domain of Zea mays BAM8/BES1/BZR1-5 and provide comprehensive insights into its noncatalytic adaptation. Using structural-guided comparison combined with biochemical analysis and molecular dynamics simulations, we revealed conformational changes in multiple distinct highly conserved regions resulting in rearrangement of the binding pocket. Altogether, this study adds a new layer of understanding to starch breakdown mechanism and elucidates the acquired adjustments of noncatalytic BZR1-type BAMs as putative regulatory domains and/or metabolic sensors in plants.
59 BASIC BIOLOGICAL SCIENCES↗