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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records

Student research with 400keV beams: {sup 13}N radioisotope production target development

The AN400 Van de Graaff accelerator at the Minnesota State University, Mankato, Applied Nuclear Science Lab has demonstrated utility as an accessible and versatile platform for student research. Despite the limits of low energy, the research team successfully developed projects with applications to the wider radioisotope production community. A target system has been developed for producing and extracting {sup 13}N by the {sup 12}C(d,n){sup 13}N reaction below 400keV. The system is both reusable and robust, with future applications to higher energy machines producing this important radioisotope for physiological imaging studies with Positron Emission Tomography. Up to 36({+-}1)% of the {sup 13}N was extracted from the graphite matrix when 35 A current was externally applied to the graphite target while simultaneously flushing the target chamber with CO{sub 2} gas.

07 ISOTOPE AND RADIATION SOURCES↗

Measurement of the {sup 12}C({alpha},{gamma}){sup 16}O reaction at TRIAC

We have measured the {gamma}-ray angular distribution of the {sup 12}C({alpha},{gamma}){sup 16}O reaction at TRIAC (Tokai Radioactive Ion Accelerator Complex) to accurately determine the E1 and E2 cross sections. In this experiment, we used high efficiency anti-Compton NaI(T1) spectrometers to detect a {gamma}-ray from the reaction with large S/N ratio, intense pulsed {alpha}-beams to discriminate true event from background events due to neutrons from {sup 13}C({alpha},n){sup 16}O reaction with a time-of-flight (TOF) method. We succeeded in removing a background events due to neutrons and clearly detected {gamma}-ray from the {sup 12}C({alpha}{gamma}){sup 16}O reaction with high statistics.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Study of {sup 24}Mg resonances relevant for carbon burning nucleosynthesis

We have studied decays of resonances in {sup 24}Mg at excitation energies above the {sup 12}C+{sup 12}C decay threshold, using {sup 12}C({sup 16}O,α){sup 24}Mg* reaction. This experiment has been performed at INFNLNS, using Tandem accelerator beam of 16O at E = 94 MeV. Some preliminary results are presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Two-neutron stripping in ({sup 18}O, {sup 16}O) and (t,p) reactions

The {sup 12}C({sup 18}O,{sup 16}O){sup 14}C reactions has been investigated at 84 MeV incident energy. The charged ejectiles produced in the reaction have been momentum analyzed and identified by the MAGNEX magnetic spectrometer. Q-value spectra have been extracted with an energy resolution of 160 keV (Full Width at Half Maximum) and several known bound and resonant states of {sup 14}C have been identified up to 15 MeV. In particular, excited states with dominant 2p - 4h configuration are the most populated. The absolute values of the cross sections have been extracted showing a striking similarity with those measured for the same transitions by (t,p) reactions. This indicates that the effect of the {sup 16}O core is negligible in the reaction mechanism.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Effect of {sup 12}C+{sup 12}C reaction and convective mixing on the progenitor mass of ONe white dwarfs

Stars in the mass range ∼8 - 12 M{sub ⊙} are the most numerous massive stars. This mass range is critical because it may lead to supernova (SN) explosion, so it is important for the production of heavy elements and the chemical evolution of the galaxy. We investigate the critical transition mass (M{sub up}), which is the minimum initial stellar mass that attains the conditions for hydrostatic carbon burning. Stars of masses < M{sub up} evolve to the Asymptotic Giant Branch and then develop CO White Dwarfs, while stars of masses ≥ M{sub up} ignite carbon in a partially degenerate CO core and form electron degenerate ONe cores. These stars evolve to the Super AGB (SAGB) phase and either become progenitors of ONe White Dwarfs or eventually explode as electron-capture SN (EC-SN). We study the sensitivity of M{sub up} to the C-burning reaction rate and to the treatment of convective mixing. In particular, we show the effect of a recent determination of the {sup 12}C+{sup 12}C fusion rate, as well as the extension of the convective core during hydrogen and helium burning on M{sub up} in solar metallicity stars. We choose the 9 M{sub ⊙} model to show the detailed characteristics of the evolution with the new C-burning rate.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multipolarity analysis for {sup 14}C high-energy resonance populated by ({sup 18}O,{sup 16}O) two-neutron transfer reaction

The {sup 12}C({sup 18}O,{sup 16}O){sup 14}C reaction at 84 MeV incident energy has been explored up to high excitation energy of the residual nucleus thanks to the use of the MAGNEX spectrometer to detect the ejectiles. In the region above the two-neutron separation energy, a resonance has been observed at 16.9 MeV. A multipolarity analysis of the cross section angular distribution indicates an L = 0 character for such a transition.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

THE {sup 12}C + {sup 12}C REACTION AND THE IMPACT ON NUCLEOSYNTHESIS IN MASSIVE STARS

Despite much effort in the past decades, the C-burning reaction rate is uncertain by several orders of magnitude, and the relative strength between the different channels {sup 12}C({sup 12}C, {alpha}){sup 20}Ne, {sup 12}C({sup 12}C, p){sup 23}Na, and {sup 12}C({sup 12}C, n){sup 23}Mg is poorly determined. Additionally, in C-burning conditions a high {sup 12}C+{sup 12}C rate may lead to lower central C-burning temperatures and to {sup 13}C({alpha}, n){sup 16}O emerging as a more dominant neutron source than {sup 22}Ne({alpha}, n){sup 25}Mg, increasing significantly the s-process production. This is due to the chain {sup 12}C(p, {gamma}){sup 13}N followed by {sup 13}N({beta} +){sup 13}C, where the photodisintegration reverse channel {sup 13}N({gamma}, p){sup 12}C is strongly decreasing with increasing temperature. Presented here is the impact of the {sup 12}C+{sup 12}C reaction uncertainties on the s-process and on explosive p-process nucleosynthesis in massive stars, including also fast rotating massive stars at low metallicity. Using various {sup 12}C+{sup 12}C rates, in particular an upper and lower rate limit of {approx}50,000 higher and {approx}20 lower than the standard rate at 5 Multiplication-Sign 10{sup 8} K, five 25 M {sub Sun} stellar models are calculated. The enhanced s-process signature due to {sup 13}C({alpha}, n){sup 16}O activation is considered, taking into account the impact of the uncertainty of all three C-burning reaction branches. Consequently, we show that the p-process abundances have an average production factor increased up to about a factor of eight compared with the standard case, efficiently producing the elusive Mo and Ru proton-rich isotopes. We also show that an s-process being driven by {sup 13}C({alpha}, n){sup 16}O is a secondary process, even though the abundance of {sup 13}C does not depend on the initial metal content. Finally, implications for the Sr-peak elements inventory in the solar system and at low metallicity are discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Photoproduction of {pi}{sup +}p pairs on nuclei

The photoproduction of pion-nucleon pairs on nuclei was analyzed. The contributions of both nucleonic and isobar configurations in the ground state of nuclei were taken into account. The cross section for the photoproduction of pion-proton pairs in the reactions {sup 16}O({gamma}, {pi}{sup +}p){sup 15}C and {sup 12}C({gamma}, {pi}{sup +}p){sup 11}Be were calculated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron production in collisions between carbon nuclei of energy 2 GeV per nucleon and carbon, aluminum, copper, cadmium, and lead nuclei

Double-differential cross sections for neutron production were measured by the time-of-flight method for the interactions between carbon nuclei of energy 2 GeV per nucleon and carbon, aluminum, copper, cadmium, and lead nuclei. These measurements were performed for angles of 30 Degree-Sign , 53 Degree-Sign , and 90 Degree-Sign in the neutron-energy range fromseveral hundred keVunits to 300MeV. The phenomenologicalmodel of four moving sources was used as a basis in analyzing experimental results and in estimating the contribution to neutron emission from various reaction stages. The temperature parameters determined from the slope of the neutron energy spectra proved to be 22 {+-} 2 MeV for a hot source (fireball) and 4.5 {+-} 0.3 MeV for the stage of thermal fragmentation of highly excited heavy nuclear residues. The relative contribution of these two sources to the total neutron yield is independent of the type of the target nucleus and is about 42%, on average.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

{sup 12}C+{sup 12}C reactions at astrophysical energies: Tests of targets behaviour under beam bombardment

{sup 12}C({sup 12}C,α){sup 20}Ne and {sup 12}C({sup 12}C,p){sup 23}Na are the most important reactions during the carbon burning phase in stars. Direct measurements at the relevant astrophysical energy (E=1.5±0.3MeV) are very challenging because of the extremely small cross sections involved and of the high beam-induced background originating from impurities in the targets. In addition, persistent resonant structures at low energies are not well understood and make the extrapolation of the cross section from high energy data very uncertain. As a preliminary step towards the measurements of the {sup 12}C({sup 12}C,α){sup 20}Ne and {sup 12}C({sup 12}C,p){sup 23}Na reactions we intend to investigate the behaviour of targets under beam bombardment, specifically the quantitative measurement of hydrogen and deuterium content of highly pure stable carbon targets in relation to target temperature. Experiments are taking place at the CIRCE accelerator in Caserta, Italy and preliminary results are presented here.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutrino-nucleus reactions based on recent structure studies

Neutrino-nucleus reactions are studied with the use of new shell model Hamiltonians, which have proper tensor components in the interactions and prove to be successful in the description of Gamow-Teller (GT) strengths in nuclei. The new Hamiltonians are applied to obtain new neutrino-nucleus reaction cross sections in {sup 12}C, {sup 13}C, {sup 56}Fe and {sup 56}Ni induced by solar and supernova neutrinos. The element synthesis by neutrino processes in supernova explosions is discussed with the new cross sections. The enhancement of the production yields of {sup 7}Li, {sup 11}B and {sup 55}Mn is obtained while fragmented GT strength in {sup 56}Ni with two-peak structure is found to result in smaller e-capture rates at stellar environments. The monopole-based universal interaction with tensor force of π+ρ meson exchanges is used to evaluate GT strength in {sup 40}Ar and ν-induced reactions on {sup 40}Ar. It is found to reproduce well the experimental GT strength in {sup 40}Ar.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Determination of Energy and Fluences of Protons Collectively Accelerated in a Luce Diode Accelerator

Plates of boron carbide B{sub 4}C were used as refractory targets for determination of energy and fluences of protons collectively accelerated in a Luce diode accelerator by control of {sup 7}Be and {sup 13}N gamma radioactivity induced by nuclear reactions {sup 10}B(p, α){sup 7}Be and {sup 12}C(p, γ){sup 13}N, respectively. The Luce diode exploited a cylindrical tungsten rod as a cathode and a polyethylene washer as an anode, producing pulsed electron beams with durations and currents of up to 100 ns and 30 kA at voltages of 250 kV. The technique allows controlling proton energies within the range of 500–1500 keV and fluences of up to 5 × 10{sup 13} protons per cm{sup 2} per pulse.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Investigating {sup 13}C+{sup 12}C reaction by the activation method. Sensitivity tests

We have performed experiments to check the limits of sensitivity of the activation method using the new 3 MV Tandetron accelerator and the low and ultra-low background laboratories of the “Horia Hulubei” National Institute of Physics and Nuclear Engineering (IFIN-HH). We have used the {sup 12}C+{sup 13}C reaction at beam energies E{sub lab}= 6, 7 and 8 MeV. The knowledge of this fusion cross section at deep sub-barrier energies is of interest for astrophysical applications, as it provides an upper limit for the fusion cross section of {sup 12}C+{sup 12}C over a wide energy range. A {sup 13}C beam with intensities 0.5–2 particleμA was provided by the accelerator and used to bombard graphite targets, resulting in activation with {sup 24}Na from the {sup 12}C({sup 13}C,p) reaction. The 1369 and 2754 keV gamma-rays from {sup 24}Na de-activation were clearly observed in the spectra obtained in two different laboratories used for measurements at low and ultralow background: one at the surface and one located underground in the Unirea salt mine from Slanic Prahova, Romania. In the underground laboratory, for E{sub lab} = 6 MeV we have measured an activity of 0.085 ± 0.011 Bq, corresponding to cross sections of 1–3 nb. This demonstrates that it is possible to measure {sup 12}C targets irradiated at lower energies for at least 10 times lower cross sections than before β–γ coincidences will lead us another factor of 10 lower, proving that this installations can be successfully used for nuclear astrophysics measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear fragmentation measurements for hadrontherapy and space radiation protection

Nuclear fragmentation measurements are necessary in hadrontherapy and space radiation protection, to predict the effects of the ion nuclear interactions within the human body. Nowadays, a very limited set of carbon fragmentation cross sections has been measured and in particular, to our knowledge, no double differential fragmentation cross sections at intermediate energies are available in literature. We have measured the double differential cross sections and the angular distributions of the secondary fragments produced in the {sup 12}C fragmentation at 62 AMeV on a thin carbon target. The experimental data have been also used to benchmark the prediction capability of the Geant4 Monte Carlo code at intermediate energies, where it was never tested before.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

Reaction dynamics of {sup 34-38}Mg projectile with carbon target using Glauber model

We have studied nuclear reaction cross-sections for {sup 34-38}Mg isotopes as projectile with {sup 12}C target at projectile energy 240AMeV using Glauber model with the conjunction of densities from relativistic mean filed formalism. We found good agreement with the available experimental data. The halo status of {sup 37}Mg is also investigated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Verification of Monte Carlo transport codes against measured small angle p-, d-, and t-emission in carbon fragmentation at 600 MeV/nucleon

Momentum spectra of hydrogen isotopes have been measured at 3.5° from 12 C fragmentation on a Be target. Momentum spectra cover both the region of fragmentation maximum and the cumulative region. Differential cross sections span five orders of magnitude. The data are compared to predictions of four Monte Carlo codes: QMD, LAQGSM, BC, and INCL++. There are large differences between the data and predictions of some models in the high momentum region. The INCL++ code gives the best and almost perfect description of the data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Comparing modern measurements of the {sup 11}B(d,n{gamma}{sub 15.1}){sup 12}C excitation function with previous values

A possible means of active interrogation of special nuclear materials is detection of signature emissions following induced photofission. This method requires a probe gamma-ray beam to induce the photofission. The {sup 11}B(d,n{gamma}{sub 15.1}){sup 12}C reaction is a candidate for the source of this probe beam. The reaction is prolific and the produced 15.1 MeV gamma-ray is close to a photofission cross-section peak for {sup 235,238}U and {sup 238,239}Pu. In order to model an active interrogation system using the {sup 11}B(d,n{gamma}{sub 15.1}){sup 12}C reaction as a source probe an accurate value for its differential crosssection must be included in data libraries. Measurements of the differential cross-section for the {sup 11}B(d,n{gamma}{sub 15.1}){sup 12}C reaction have been carried out with a BGO detector and found to differ from previous measurements reported by Kavanagh (1958) and Kuan (1964). The discrepancy in the measurements may be explained by examining the detector response function used by Kavanagh and presumably Kuan to that modeled with MCNP5. A comparison of the MCNP5 and Kavanagh detector response functions normalized to the 15.1 MeV gamma-ray peak pulse height shows a factor of approximately 1.7 difference in integrated counts. Applying this correction to the differential cross-section previously reported by Kuan brings the values into agreement, within uncertainties, to the more recent measurements. The evaluation of the detector response function for the 15.1 MeV gamma-ray signal in the NaI detector reported by Kavanagh to that modeled by MCNP5 is shown. This result is applied to the comparison of recent measurements on the {sup 11}B(d,n{gamma}{sub 15.1}){sup 12}C reaction differential cross-section to those previously reported.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

eA Pion Production at CLAS Aimed at Neutrinos

Preliminary results on semi-inclusive charged pion production in eA collisions at E{sub beam} = 5 GeV/c{sup 2} are presented. The data were collected using the CLAS detector, which is a multipurpose, large acceptance, magnetic spectrometer located in Hall B at the Thomas Jefferson National Accelerator Facility. Distributions in W, Q{sup 2}, p{sub {pi}}, and {theta}{sub {pi}} are shown for data produced using deuterium and carbon targets. Preliminary comparisons with data simulated using the GENIE generator are made. The motivation for this work is to provide distributions useful for tuning the hadronic production models used in extracting results from current and next-generation neutrino oscillation experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗