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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Development of a Random-Forest Cloud-Regime Classification Model Based on Surface Radiation and Cloud Products

Various methods have been developed to characterize cloud type, otherwise referred to as cloud regime. These include manual sky observations, combining radiative and cloud vertical properties observed from satellite, surface-based remote sensing, and digital processing of sky imagers. While each method has inherent advantages and disadvantages, none of these cloud-typing methods actually includes measurements of surface shortwave or longwave radiative fluxes. Here, a method that relies upon detailed, surface-based radiation and cloud measurements and derived data products to train a random-forest machine-learning cloud classification model is introduced. Measurements from five years of data from the ARM Southern Great Plains site were compiled to train and independently evaluate the model classification performance. A cloud-type accuracy of approximately 80% using the random-forest classifier reveals that the model is well suited to predict climatological cloud properties. Furthermore, an analysis of the cloud-type misclassifications is performed. While physical cloud types may be misreported, the shortwave radiative signatures are similar between misclassified cloud types. From this, we assert that the cloud-regime model has the capacity to successfully differentiate clouds with comparable cloud–radiative interactions. Therefore, we conclude that the model can provide useful cloud-property information for fundamental cloud studies, inform renewable energy studies, and be a tool for numerical model evaluation and parameterization improvement, among many other applications.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Improvement of the Simulation of Cloud Longwave Scattering in Broadband Radiative Transfer Models

Abstract Cloud longwave scattering is generally neglected in general circulation models (GCMs), but it plays a significant and highly uncertain role in the atmospheric energy budget as demonstrated in recent studies. To reduce the errors caused by neglecting cloud longwave scattering, two new radiance adjustment methods are developed that retain the computational efficiency of broadband radiative transfer simulations. In particular, two existing scaling methods and the two new adjustment methods are implemented in the Rapid Radiative Transfer Model (RRTM). The results are then compared with those based on the Discrete Ordinate Radiative Transfer model (DISORT) that explicitly accounts for multiple scattering by clouds. The two scaling methods are shown to improve the accuracy of radiative transfer simulations for optically thin clouds but not effectively for optically thick clouds. However, the adjustment methods reduce computational errors over a wide range, from optically thin to thick clouds. With the adjustment methods, the errors resulting from neglecting cloud longwave scattering are reduced to less than 2 W m−2 for the upward irradiance at the top of the atmosphere and less than 0.5 W m−2 for the surface downward irradiance. The adjustment schemes prove to be more accurate and efficient than a four-stream approximation that explicitly accounts for multiple scattering. The neglect of cloud longwave scattering results in an underestimate of the surface downward irradiance (cooling effect), but the errors are almost eliminated by the adjustment methods (warming effect).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Uncertainty of SW Cloud Radiative Effect in Atmospheric Models Due to the Parameterization of Liquid Cloud Optical Properties

Clouds are largely responsible for the spread of climate models predictions. Here we focus on the uncertainties in cloud shortwave radiative effect due to the parameterization of liquid cloud single scattering properties (SSPs) from liquid water content (LWC) and droplet number concentration (N), named parameterization of cloud optical properties. Uncertainties arise from not accounting for the droplet size distribution (DSD)—which affects the estimation of the effective radius (r eff ) and modulates the r eff -dependency of the SSPs—and from averaging SSPs over wide spectral bands. To assess these uncertainties a series of r eff -dependent SSPs parameterizations corresponding to various DSDs and spectral averaging methods are derived and implemented in a radiative code. Combined with the DSD-dependent estimation of r eff they are used to compute the bulk radiative properties (reflectance, transmittance, absorptance) of various clouds (defined in terms of LWC and N), including a homogeneous cloud, more realistic case studies, and outputs of a climate model. The results show that the cloud radiative forcing can vary up to 20% depending on the assumed DSD. Likewise, differences up to 20% are obtained for heating rates. The estimation of r eff is the main source of uncertainty, while the SSPs parameterization contributes to around 20% of the total uncertainty. Spectral averaging is less an issue, except for atmospheric absorption. Overall, global shortwave cloud radiative effect can vary by 6 W m –2 depending on the assumed DSD shape, which is about 13% of the best observational estimate.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Process-oriented evaluation using ARM observations to improve clouds and radiation in a global atmospheric model

The goal of the research is to improve understanding of cloud, radiation and precipitation processes and their representation in numerical models for weather and climate using observations from the ARM/ASR program. Global models need to represent all cloud types across different weather regimes from the tropics to the poles and ARM provides long-term observations at different geographical sites that cover these different regimes. Combined with satellite data to give a global context, the observations are used to evaluate the systematic errors in a global model for predictions of cloud, radiation and precipitation. The focus is on understanding the links to underlying physical processes to pinpoint the sources of error and improve the model representation of these processes. The research covers boundary layer cloud over the continental U.S., marine stratocumulus and shallow cumulus in the subtropics, mixed-phase clouds over the Arctic and Southern Ocean, and high-altitude cirrus ice clouds in the tropics. The model used is the operational global weather prediction system at the European Centre for Medium-range Weather Forecasts (ECMWF). The research has led to numerous developments, several of which have been implemented operationally leading to improvements in everyday forecasts. Many of the systematic errors are common across different modelling systems and the wider implications from the research for other weather and climate models are highlighted.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Understanding the Varied Influence of Midlatitude Jet Position on Clouds and Cloud Radiative Effects in Observations and Global Climate Models

This study examines the dynamical mechanisms responsible for changes in midlatitude clouds and cloud radiative effects (CRE) that occur in conjunction with meridional shifts in the jet streams over the North Atlantic, North Pacific, and Southern Oceans. When the midlatitude jet shifts poleward, extratropical cyclones and their associated upward vertical velocity anomalies closely follow. As a result, a poleward jet shift contributes to a poleward shift in high-topped storm-track clouds and their associated longwave CRE. However, when the jet shifts poleward, downward vertical velocity anomalies increase equatorward of the jet, contributing to an enhancement of the boundary layer estimated inversion strength (EIS) and an increase in low cloud amount there. Because shortwave CRE depends on the reflection of solar radiation by clouds in all layers, the shortwave cooling effects of midlatitude clouds increase with both upward vertical velocity anomalies and positive EIS anomalies. Over midlatitude oceans where a poleward jet shift contributes to positive EIS anomalies but downward vertical velocity anomalies, the two effects cancel, and net observed changes in shortwave CRE are small. Global climate models generally capture the observed anomalies associated with midlatitude jet shifts. However, there is large intermodel spread in the shortwave CRE anomalies, with a subset of models showing a large shortwave cloud radiative warming over midlatitude oceans with a poleward jet shift. In these models, midlatitude shortwave CRE is sensitive to vertical velocity perturbations, but the observed sensitivity to EIS perturbations is underestimated. Consequently, these models might incorrectly estimate future midlatitude cloud feedbacks in regions where appreciable changes in both vertical velocity and EIS are projected

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Using the Atmospheric Radiation Measurement (ARM) Datasets to Evaluate Climate Models in Simulating Diurnal and Seasonal Variations of Tropical Clouds

We use the long-term Atmospheric Radiation Measurement (ARM) datasets collected at the three Tropical Western Pacific (TWP) sites as a tropical testbed to evaluate the ability of the Community Atmosphere Model (CAM5) to simulate the various types of clouds, their seasonal and diurnal variations, and their impact on surface radiation. We conducted a series of CAM5 simulations at various horizontal grid spacing (around 2°, 1°, 0.5°, and 0.25°) with meteorological constraints from reanalysis. Model biases in the seasonal cycle of cloudiness are found to be weakly dependent on model resolution. Positive biases (up to 20%) in the annual mean total cloud fraction appear mostly in stratiform ice clouds. Higher-resolution simulations do reduce the positive bias in the frequency of ice clouds, but they inadvertently increase the negative biases in convective clouds and low-level liquid clouds, leading to a positive bias in annual mean shortwave fluxes at the sites, as high as 65 W m-2 in the 0.25° simulation. Such resolution-dependent biases in clouds can adversely lead to biases in ambient thermodynamic properties and, in turn, feedback on clouds. Both the CAM5 model and ARM observations show distinct diurnal cycles in total, stratiform and convective cloud fractions; however, they are out-of-phase by 12 hours and the biases vary by site. Our results suggest that biases in deep convection affect the vertical distribution and diurnal cycle of stratiform clouds through the transport of vapor and/or the detrainment of liquid and ice. We also found that the modelled gridmean surface longwave fluxes are systematically larger than site measurements when the grid that the ARM sites reside in is partially covered by ocean. The modeled longwave fluxes at such sites also lack a discernable diurnal cycle because the ocean part of the grid is warmer and less sensitive to radiative heating/cooling compared to land. Higher spatial resolution is more helpful is this regard. Our testbed approach can be easily adapted for the evaluation of new parameterizations being developed for CAM5 or other global or regional model simulations at high spatial resolutions.

Wang, Hailong↗
DOE OSTI2016

Numerical simulations of turbulent molecular clouds regulated by radiation feedback forces. I. Star formation rate and efficiency

Radiation feedback from stellar clusters is expected to play a key role in setting the rate and efficiency of star formation in giant molecular clouds. To investigate how radiation forces influence realistic turbulent systems, we have conducted a series of numerical simulations employing the Hyperion radiation hydrodynamics solver, considering the regime that is optically thick to ultraviolet and optically thin to infrared radiation. Our model clouds cover initial surface densities between Σ{sub cl,0}∼10--300 M{sub ⊙} pc{sup −2}, with varying initial turbulence. We follow them through turbulent, self-gravitating collapse, star cluster formation, and cloud dispersal by stellar radiation. All our models display a log-normal distribution of gas surface density Σ; for an initial virial parameter α{sub vir,0}=2, the log-normal standard deviation is σ{sub lnΣ}=1--1.5 and the star formation rate coefficient ε{sub ff, ρ-bar }=0.3--0.5, both of which are sensitive to turbulence but not radiation feedback. The net star formation efficiency (SFE) ε{sub final} increases with Σ{sub cl,0} and decreases with α{sub vir,0}. We interpret these results via a simple conceptual framework, whereby steady star formation increases the radiation force, such that local gas patches at successively higher Σ become unbound. Based on this formalism (with fixed σ{sub lnΣ}), we provide an analytic upper bound on ε{sub final}, which is in good agreement with our numerical results. The final SFE depends on the distribution of Eddington ratios in the cloud and is strongly increased by the turbulent compression of gas.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Separating radiative forcing by aerosol–cloud interactions and rapid cloud adjustments in the ECHAM–HAMMOZ aerosol–climate model using the method of partial radiative perturbations

Using the method of offline radiative transfer modeling within the partial radiative perturbation (PRP) approach, the effective radiative forcing by aerosol–cloud interactions (ERF aci ) in the ECHAM–HAMMOZ aerosol climate model is decomposed into a radiative forcing by anthropogenic cloud droplet number change and adjustments of the liquid water path and cloud fraction.The simulated radiative forcing by anthropogenic cloud droplet number change and liquid water path adjustment are of approximately equal magnitude at –0.52 and –0.53 W m –2 , respectively, while the cloud-fraction adjustment is somewhat weaker at –0.31 W m –2 (constituting 38 %, 39 %, and 23 %of the total ERFaci, respectively); geographically, all three ERF aci components in the simulation peak over China, the subtropical eastern ocean boundaries,the northern Atlantic and Pacific oceans, Europe, and eastern North America (in order of prominence). Spatial correlations indicate that the temporal-mean liquid water path adjustment is proportional to the temporal-mean radiative forcing, while the relationship between cloud-fraction adjustment and radiative forcing is less direct. While the estimate of warm-cloud ERF aci is relatively insensitive to the treatment of ice and mixed-phase cloud overlying warm cloud, there are indications that more restrictive treatments of ice in the column result in a low bias in the estimated magnitude of the liquid water path adjustment and a high bias in the estimated magnitude of the droplet number forcing. Since the present work is the first PRP decomposition of the aerosol effective radiative forcing into radiative forcing and rapid cloud adjustments, idealized experiments are conducted to provide evidence that the PRP results are accurate. The experiments show that using low-frequency(daily or monthly) time-averaged model output of the cloud property fields underestimates the ERF, but 3-hourly mean output is sufficiently frequent.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Light Transfers Through a Koch Shape Cloud

Abstract Modeling radiative transfer in a 3D cloudy atmosphere is critical to climate projections. A recently developed fast 3D radiation parameterization scheme gains some success in quantifying horizontal radiative transfer through cloud sides using cloud area fraction. Based on 3D Monte Carlo simulations of radiative transfer through an idealized single‐layer cloud with Koch‐shaped fractal geometry edges, here we show that radiative energy transport through cloud sides correlates more significantly with cloud area fraction than with cloud perimeter length. The results exemplify the importance of accounting for the horizontal radiative energy exchanges between cloud‐free and cloudy regions with cloud area fraction. Results from additional sensitivity simulations show that increased cloud vertical extent often enhances cloud‐side sunlight leak more significantly than cloud‐side sunlight interception. At low sun elevations, cloud‐side sunlight interception is enhanced more than cloud‐side sunlight leak does with the increase of cloud mass.

58 GEOSCIENCES↗
DOE OSTI2023

Assessment of CMIP5 and CMIP6 AMIP Simulated Clouds and Surface Shortwave Radiation Using ARM Observations over Different Climate Regions

The simulations of clouds and surface radiation from 10 CMIP6 models and their CMIP5 predecessors are compared to the ARM ground-based observations over different climate regions. Compared to the ARM radar-lidar derived total cloud fractions (CFT) and cloud fraction vertical distributions over the six selected sites, both CMIP5 and CMIP6 significantly underestimated CFT and low-level CF over the Northern Hemispheric midlatitude sites (SGPC1 and ENAC1), although the biases are generally smaller in CMIP6. Over the tropical oceanic site (TWPC2), 5 out of 10 CMIP6 models better simulated low-level CF than their CMIP5 predecessors. CMIP6 simulations generally agreed well with the ARM observations in CFT and cloud fraction vertical distributions over the tropical continental (MAOM1) and coastal (TWPC3) sites but missed the transitions between dry and wet seasons, similar to CMIP5 simulations. The improvements in downwelling shortwave fluxes (SWdn) at the surface from the majority of CMIP6 compared to CMIP5 primarily resulted from the improved cloud fraction simulations, especially over the SGPC1, ENAC1, and TWPC3 sites. By contrast, both CMIP5 and CMIP6 models exhibited diverse performances of clouds and shortwave radiation over the Arctic site (NSAC1), where CMIP6 models produced more clouds than CMIP5 models, especially for the low-level clouds. The comparisons between observations and CMIP5 and CMIP6 simulations provide valuable quantitative assessments of the accuracy of mean states and variabilities in the model simulations and shed light on general directions to improve climate models in different regions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Clouds and Radiation Processes in Regional Climate Models Evaluated Using Observations Over the Ice‐free Arctic Ocean

Abstract The presence of clouds in the Arctic regulates the surface energy budget (SEB) over the sea‐ice surface and the ice‐free ocean. Following several previous field campaigns, the cloud‐radiation relationship, including cloud vertical structure and phase, has been elucidated; however, modeling of this relationship has matured slowly. In recognition of the recent decline in the Arctic sea‐ice extent, representation of the cloud system in numerical models should consider the effects of areas covered by sea ice and ice‐free areas. Using an in situ stationary meteorological observation data set obtained over the ice‐free Arctic Ocean by the Japanese Research Vessel Mirai (September 2014), coordinated evaluation of six regional climate models (RCMs) with nine model runs was performed by focusing on clouds and the SEB. The most remarkable findings were as follows: (1) reduced occurrence of unstable stratification with low‐level cloud water in all models in comparison to the observations, (2) significant differences in cloud water representations between single‐ and double‐moment cloud schemes, (3) extensive differences in partitioning of hydrometeors including solid/liquid precipitation, and (4) pronounced lower‐tropospheric air temperature biases. These issues are considered as the main sources of SEB uncertainty over ice‐free areas of the Arctic Ocean. The results from a coupled RCM imply that the SEB is constrained by both the atmosphere and the ocean (and sea ice) with considerable feedback. Coordinated improvement of both stand‐alone atmospheric and coupled RCMs would promote a more comprehensive and improved understanding of the Arctic air‐ice‐sea coupled system.

Inoue, Jun↗
DOE OSTI2016

A radiation closure study of Arctic stratus cloud microphysical properties using the collocated satellite-surface data and Fu-Liou radiative transfer model

Retrievals of cloud microphysical properties based on passive satellite imagery are especially difficult over snow-covered surfaces because of the bright and cold surface. To help quantify their uncertainties, single-layered overcast liquid-phase Arctic stratus cloud microphysical properties retrieved by using the Clouds and the Earth's Radiant Energy System Edition 2 and Edition 4 (CERES Ed2 and Ed4) algorithms are compared with ground-based retrievals at the Atmospheric Radiation Measurement North Slope of Alaska (ARM NSA) site at Barrow, AK, during the period from March 2000 to December 2006. A total of 206 and 140 snow-free cases (Rsfc ≤ 0.3), and 108 and 106 snow cases (R sfc > 0.3), respectively, were selected from Terra and Aqua satellite passes over the ARM NSA site. The CERES Ed4 and Ed2 optical depth (τ) and liquid water path (LWP) retrievals from both Terra and Aqua are almost identical and have excellent agreement with ARM retrievals under snow-free and snow conditions. In order to reach a radiation closure study for both the surface and top of atmosphere (TOA) radiation budgets, the ARM precision spectral pyranometer-measured surface albedos were adjusted (63.6% and 80% of the ARM surface albedos for snow-free and snow cases, respectively) to account for the water and land components of the domain of 30 km × 30 km. Most of the radiative transfer model calculated SW↓ sfc and SW↑ TOA fluxes by using ARM and CERES cloud retrievals and the domain mean albedos as input agree with the ARM and CERES flux observations within 10 W m -2 for both snow-free and snow conditions. Sensitivity studies show that the ARM LWP and r e retrievals are less dependent on solar zenith angle (SZA), but all retrieved optical depths increase with SZA.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Understanding Global Model Systematic Shortwave Radiation Errors in Subtropical Marine Boundary Layer Cloud Regimes

Abstract Global numerical weather prediction and climate models are subject to long‐standing systematic shortwave radiation errors due to deficiencies in the representation of boundary layer clouds over the ocean. In the subtropics, clouds are typically too reflective in the cumulus regime and not reflective enough in the stratocumulus regime. Potential sources of error include cloud cover, liquid water path, effective radius, and subgrid heterogeneity, but diagnosing the absolute contributions of each to the radiation bias is hampered by uncertainties and sometimes contradictory information from different observational products. This paper draws on a set of ship‐based observations of boundary layer clouds obtained during the ARM MAGIC campaign along a northeast Pacific Ocean transect, crossing both stratocumulus and shallow cumulus cloud regimes. The surface‐based observations of cloud properties are compared with various satellite products, taking account of the diurnal cycle, to provide an improved quantitative assessment of the deficiencies in the European Centre for Medium‐Range Weather Forecasts global numerical weather prediction model. A series of off‐line radiation calculations are then performed to assess the impact on the shortwave radiation bias of correcting each of the model's deficiencies in cloud characteristics along the transect. A reduction in the bias is achieved by improving the agreement between modeled and observed in‐cloud liquid water path frequency distributions. In the cumulus regime, this is accomplished primarily by reducing the all‐sky water path, while for the stratocumulus regime, an underestimate of cloud cover and liquid water and an overestimate in effective radius and subgrid heterogeneity all contribute to a lack of reflected shortwave radiation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Advancing cloud lifecycle representation in numerical models using innovative analysis methods that bridge arm observations over a breadth of scales

From its location on the subtropics-midlatitude boundary, the Azores is influenced by both the subtropical high pressure and the midlatitude baroclinic storm regimes, and therefore experiences a wide range of cloud structures, from fair-weather scenes to stratocumulus sheets to deep convective systems. This project combined three types of data sets to study cloud variability in the Azores: a satellite analysis of cloud regimes, a reanalysis characterization of storminess, and a 19-month field campaign that occurred on Graciosa Island. Combined analysis of the three data sets provides a detailed picture of cloud variability and the respective dynamic influences, with emphasis on low clouds that constitute a major uncertainty source in climate model simulations. The satellite cloud regime analysis shows that the Azores cloud distribution is similar to the mean global distribution and can therefore be used to evaluate cloud simulation in global models. Regime analysis of low clouds shows that stratocumulus decks occur under the influence of the Azores high-pressure system, while shallow cumulus clouds are sustained by cold-air outbreaks, as revealed by their preference for post-frontal environments and northwesterly flows. An evaluation of CMIP5 climate model cloud regimes over the Azores shows that all models severely underpredict shallow cumulus clouds, while most models also underpredict the occurrence of stratocumulus cloud decks. It is demonstrated that carefully selected case studies can be related through regime analysis to climatological cloud distributions, and a methodology is suggested utilizing process-resolving model simulations of individual cases to better understand cloud-dynamics interactions and attempt to explain and correct climate model cloud deficiencies.

58 GEOSCIENCES↗
DOE OSTI2024

An overview of cloud–radiation denial experiments for the Energy Exascale Earth System Model version 1

Abstract. The interaction between clouds and radiation is a key process within the climate system, and assessing the impacts of that interaction provides valuable insights into both the present-day climate and future projections. Many modeling experiments have been designed over the years to probe the impact of the cloud radiative effect (CRE) on the climate, including those that seek to disrupt the mean CRE effect and those that only disrupt the covariance of the CRE with the circulation. Seven such experimental designs have been added to the Energy Exascale Earth System Model version 1 (E3SMv1) of the US Department of Energy. These experiments include both the first and second iterations of the Clouds On/Off Klimate Intercomparison Experiment (COOKIE) experimental design, as well as the cloud-locking method. This paper documents the code changes necessary to implement such experiments and also provides detailed instructions for how to run them. Analyses across experiment types provide valuable insights and confirm the findings of prior studies, including the role of cloud radiative heating toward intensifying the monsoon, intensifying rain rates, and poleward expansion of the general circulation owing to cloud feedbacks.

Harrop, Bryce E. (ORCID:0000000339524525)↗
DOE OSTI2016

THE GLOBAL IMPLICATIONS OF THE HARD EXCESS. II. ANALYSIS OF THE LOCAL POPULATION OF RADIO-QUIET AGNs

Active galactic nuclei (AGNs) show evidence for reprocessing gas, outflowing from the accreting black hole. The combined effects of absorption and scattering from the circumnuclear material likely explain the “hard excess” of X-ray emission above 20 keV, compared with the extrapolation of spectra from lower X-ray energies. In a recent Suzaku study, we established that the ubiquitous hard excess in hard, X-ray-selected, radio-quiet type 1 AGNs is consistent with a reprocessing of the X-ray continuum in an ensemble of clouds, located tens to hundreds of gravitational radii from the nuclear black hole. Here we add hard X-ray-selected, type 2 AGNs to extend our original study and show that the gross X-ray spectral properties of the entire local population of radio-quiet AGNs may be described by a simple unified scheme. We find a broad, continuous distribution of spectral hardness ratio and Fe Kα equivalent width across all AGN types, which can be reproduced by varying the observer's sightline through a single, simple model cloud ensemble, provided that the radiative transfer through the model cloud distribution includes not only photoelectric absorption but also three-dimensional (3D) Compton scattering. Variation in other parameters of the cloud distribution, such as column density or ionization, should be expected between AGNs, but such variation is not required to explain the gross X-ray spectral properties.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Simulating Southern Ocean Aerosol and Ice Nucleating Particles in the Community Earth System Model Version 2

Southern Ocean (SO) low-level mixed phase clouds have been a long-standing challenge for Earth system models to accurately represent. While improvements to the Community Earth System Model version 2 (CESM2) resulted in increased supercooled liquid in SO clouds and improved model radiative biases, simulated SO clouds in CESM2 now contain too little ice. Previous observational studies have indicated that marine particles are major contributor to SO low-level cloud heterogeneous ice nucleation, a process that initiates a number of cloud processes that govern cloud radiative properties. In this study, we utilize detailed aerosol and ice nucleating particle (INP) measurements from two recent measurement campaigns to assess simulated aerosol abundance, number size distributions, and composition and INP parameterizations for use in CESM2. Our results indicate that CESM2 has a positive bias in simulated surface-level total aerosol surface area at latitudes north of 58°S. Measured INP populations were dominated by marine INPs and we present evidence of refractory INPs present over the SO assumed here to be mineral dust INPs. Results highlight a critical need to assess simulated mineral dust number and size distributions in CESM2 in order to adequately represent SO INP populations and their response to long-term changes in atmospheric transport patterns and land use change. Furthermore, we also discuss important cautions and limitations in applying a commonly used mineral dust INP parameterization to remote regions like the pristine SO.

58 GEOSCIENCES↗