Diode laser-CO2 laser heterodyne spectrometer - Measurement of 2sQ/1,1/ in 2 nu 2-nu 2 of NH3
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Hillman, J. J.↗
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Heterodyne frequency measurements with a tunable diode laser-CO2 laser spectrometer - Spectroscopic reference frequencies in the 9.5-micron band of carbonyl sulfide
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Wells, J. S.↗
LaRC-developed catalysts for CO2 lasers
Pulsed CO2 lasers have many remote sensing applications from space, airborne, and ground platforms. The NASA Laser Atmospheric Wind Sounder (LAWS) system will be designed to measure wind velocities from polar earth orbit for a period of up to three years. Accordingly, this and other applications require a closed-cycle pulsed CO2 laser which necessitates the use of an efficient CO-O2 recombination catalyst for these dissociation products which otherwise would degrade the laser operation. The required catalyst must not only operate at low temperatures but also must operate efficiently for long time periods. The research effort at NASA LaRC has centered around development and testing of CO oxidation catalysts for closed-cycle, pulsed, common and rare-isotope CO2 lasers. Researchers examined available commercial catalysts both in a laser and under simulated closed-cycle laser conditions with efforts aimed toward a thorough understanding of the fundamental catalytic reaction. These data were used to design and synthesize new catalyst compositions to better meet the catalyst requirements for closed-cycle pulsed CO2 lasers. Syntheses and test results for catalysts developed at Langley Research Center which have significantly better long-term decay characteristics than previously available catalysts and at the same time operate quite well under lower temperature conditions are discussed.
Upchurch, Billy T.↗
A computer program for the design of optimum catalytic monoliths for CO2 lasers
Pulsed CO2 lasers have many applications in aeronautics, space research, weather monitoring and other areas. Full exploitation of the potential of these lasers is hampered by the dissociation of CO2 that occurs during laser operation. The development of closed-cycle CO2 lasers requires active CO-O2 recombination (CO oxidation) catalysts and design methods for implementation of catalysts inside lasers. The performance criteria and constraints involved in the design of catalyst configurations for use in a closed-cycle laser are discussed, and several design studies performed with a computerized design program that was written are presented. Trade-offs between catalyst activity and dimensions, flow channel dimensions, pressure drop, O2 conversion and other variables are discussed.
Guinn, K.↗
'Design of CO-O2 recombination catalysts for closed-cycle CO2 lasers'
Pulsed CO2 lasers have many applications in aeronautics, space research, weather monitoring and other areas. Full exploitation of the potential of these lasers is hampered by the dissociation of CO2 that occurs during laser operation. The development of closed-cycle CO2 lasers requires active CO-O2 recombination (CO oxidation) catalysts and design methods for implementation of catalysts inside lasers. This paper will discuss the performance criteria and constraints involved in the design of monolith catalyst configurations for use in a closed-cycle laser and will present a design study performed with a computerized design program that had been written. Trade-offs between catalyst activity and dimensions, flow channel dimensions, pressure drop, O2 conversion and other variables will be discussed.
Guinn, K.↗
A curve-fitting technique for the determination of gain and saturation intensity in homogeneously-broadened gas lasers: Application to a waveguide CO2 laser
A least squares curve-fitting algorithm is derived which allows the simultaneous estimation of the small signal gain and the saturation intensity from an arbitrary number of data points relating power output to the incidence angle of an internal coupling plate. The method is used to study the dependence of the two parameters on tube pressure and discharge current in a waveguide CO2 laser having a 2 mm diameter capillary. It is found that, at pressures greater than 28 torr, rising CO2 temperature degrades the small signal gain at current levels as low as three milliamperes.
Degnan, J. J.↗
An analytical and experimental investigation of limited operational life of CO2 lasers to achieve a non flowing sealed CO2 gas laser Final report
Carbon dioxide dissociation in gas discharge, water vapor and xenon effects on dissociation, and electrode material influence on clean-up rate related to nonflowing sealed gas laser
Fantasia, J. F.↗
Monitoring of catalyst performance in CO2 lasers using frequency modulation spectroscopy with diode lasers
Closed-cycle CO2 laser operation with removal of O2 and regeneration of CO2 can be achieved by catalytic CO-O2 recombination. Both parametric studies of the optimum catalyst formulation and long-term performance tests require on line monitoring of CO, O2 and CO2 concentrations. There are several existing methods for molecular oxygen detection. These methods are either intrusive (such as electrochemical method or mass spectrometry) or very expensive (such as CARS, UV laser absorption). Researchers demonstrated a high-sensitivity spectroscopic measurement of O2 using the two-tone frequency modulation spectroscopy (FMS) technique with a near infrared GaAlAs diode laser. Besides its inexpensive cost, fast response time, nonintrusive measurements and high sensitivity, this technique may also be used to differentiate between isotopes due to its high spectroscopic resolution. This frequency modulation spectroscopy technique could also be applied for the on-line monitoring of CO and CO2 using InGaAsP diode lasers operation in the 1.55 microns region and H2O in the 1.3 microns region. The existence of single mode optical fibers at the near infrared region makes it possible to combine FMS with optical fiber technology. Optical fiber FMS is particularly suitable for making point-measurements at one or more locations in the CO2 laser/catalyst system.
Wang, Liang-Guo↗
CO2 lasers and applications II; Proceedings of the Third European Congress on Optics, The Hague, Netherlands, Mar. 12-14, 1990
Recent advances in CO2 laser technology and its applications are examined. Topics discussed include the excitation of CO2 lasers by microwave discharge, a compact RF-excited 12-kW CO2 laser, a robotic laser for three-dimensional cutting and welding, three-dimensional CO2-laser material processing with gantry machine systems, and a comparison of hollow metallic waveguides and optical fibers for transmitting CO2-laser radiation. Consideration is given to an aerodynamic window with a pump cavity and a supersonic jet, cutting and welding Al using a high-repetition-rate pulsed CO2 laser, speckle reduction in CO2 heterodyne laser radar systems, high-power-laser float-zone crystal growth, melt dynamics in surface processing with laser radiation, laser hardfacing, surface melting of AlSi10Mg with CO2 laser radiation, material processing with Cu-vapor lasers, light-induced flow at a metal surface, and absorption measurements in high-power CW CO2-laser processing of materials.
Opower, Hans↗
NO2 heterodyne frequency measurements with a tunable diode laser, a CO laser transfer oscillator and CO2 laser standards
Heterodyne frequency measurements have been made on selected groups of nitrogen dioxide rovibronic transitions between 1580.8 and 1650.7/cm. The groups are separated by 7 to 10/cm, and the intent is to provide a limited (and interim) calibration table for the region. In addition to a table of measured frequencies in the region, figures of spectra in the vicinity of the measured lines are included to provide a map for identifying the transitions measured.
Zink, L. R.↗
CO2 laser modeling
The topics covered include the following: (1) CO2 laser kinetics modeling; (2) gas lifetimes in pulsed CO2 lasers; (3) frequency chirp and laser pulse spectral analysis; (4) LAWS A' Design Study; and (5) discharge circuit components for LAWS. The appendices include LAWS Memos, computer modeling of pulsed CO2 lasers for lidar applications, discharge circuit considerations for pulsed CO2 lidars, and presentation made at the Code RC Review.
Johnson, Barry↗
Cold cathodes for sealed-off CO2 lasers
Cold cathodes for CO2 lasers should possess a very low sputtering rate, have a minimum of negative ions in the sputtering products, and consume no oxygen. These conditions can be satisfied by selecting cathode materials from those elements of group I in the periodic table which form semiconducting oxide layers and then exposing these elements to a reducing gas mixture. Experimental results show that silver, internally oxidized silver-copper alloys, and pure copper satisfy most of these requirements in He-CO2-CO-Xe gas mixtures. Infrared CO and CO2 gas analysis performed on simple gas discharge tubes using such cathodes indicate that laser lives of 10,000 hr can be expected.
Hochuli, U. E.↗
Aircraft wake vortex velocity measurements using a scanning CO2 laser Doppler velocimeter
A CO2 laser Doppler velocimeter was employed in the study of pairs of counterrotating vortices trailing aircraft in an airport air space. A laser positioned on an extended runway centerline scans a vertical plane perpendicular to the centerline. Vortex location, measurement of vortex transport, and measurement of the properties of aircraft wake vortex flow fields are achieved via spectral analysis of the data. Highest amplitude in the spectrum, the associated maximum velocity, the highest velocity above the amplitude threshold, and the total number of frequency (velocity) cells above thresholds are studied as parameters in analysis of the vortex-associated flow field. The profile of the radial variation of tangential velocity is studied, and two special problems are examined: location of the vortex center and error introduced by crosswind.
Dimarzio, C. A.↗
Mode selection and frequency tuning by injection in pulsed TEA-CO2 lasers
An analytical model characterizing pulsed-TEA-CO2-laser injection locking by tunable CW-laser radiation is presented and used to explore the requirements for SLM pulse generation. Photon-density-rate equations describing the laser mechanism are analyzed in terms of the mode competition between photon densities emitted at two frequencies. The expression derived for pulsed dye lasers is extended to homogeneously broadened CO2 lasers, and locking time is defined as a function of laser parameters. The extent to which injected radiation can be detuned from the CO2 line center and continue to produce SLM pulses is investigated experimentally in terms of the analytical framework. The dependence of locking time on the detuning/pressure-broadened-halfwidth ratio is seen as important for spectroscopic applications requiring tuning within the TEA-laser line-gain bandwidth.
Flamant, P. H.↗
Catalytic recombination of dissociation products with Pt/SnO2 for rare and common isotope long-life, closed-cycle CO2 lasers
This paper reports results on recombination of pulsed CO2 laser dissociation products with Pt/SnO2 catalysts, and supporting studies in a surrogate laboratory catalyst reactor. The closed-cycle, pulsed CO2 laser has been continuously operated for one million pulses with an overall power degradation of less than 5 percent by flowing the laser gas mixture through a 2-percent Pt/SnO2 catalyst bed. In the surrogate laboratory reactor, experiments have been conducted to determine isotopic exchange with the catalyst when using rare-isotope gases. The effects of catalyst pretreatment, sample weight, composition, and temperature on catalyst efficiency have also been determined.
Brown, Kenneth G.↗
Pumping mechanism of CO2 laser and formation rate of CO2 from CO and O
Time delay in pulsed optical carbon dioxide laser pumping mechanism in high current gaseous discharge
Chen, C. J.↗
CO2 laser design procedure.
A simple but powerful formalism is presented that allows one to physically design a sealed CO2 laser of any specified fundamental transverse-mode output power. The design material presented, graphically whenever possible, also allows one to determine the effect on the others of varying one design parameter. Although the formalism presented is based on some empirical and some theoretical parametric interrelationships pertinent to the CO2 laser, the treatment is general and with appropriate adjustments can be applied to other laser systems as well. The design of a 5-W sealed CO2 laser is presented to illustrate the use of the formalism developed.
Fahlen, T. S.↗
Development of tunable high pressure CO2 laser for lidar measurements of pollutants and wind velocities, January 1976 to December 1977
A tunable multiatmospheric pulsed CO2 laser with emphasis on experimental features and supporting theoretical analyses important to differential absorption lidar and Doppler lidar measurement of pollutants and wind velocities is reported. The energy deposition and the means to produce the uniform high density plasma in the multiatmospheric medium, through UV preionization of an organic seed gas is discussed. Design features of the pulsed CO2 laser are presented. The radiative processes which are operative and prevent the laser from breaking into oscillations in a large number of modes over its broad amplification bandwidth are described. The mode competition for the transient pulsed laser oscillation in a standing wave and traveling wave ring laser configuration is discussed and contrasted with the approach to steady state oscillations. The latter findings are important to transient injection locking for production of a highly stable pulsed CO2 laser output.
Javan, A.↗