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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records

Stability and dissociation dynamics of N{sub 2}{sup ++} ions following core ionization studied by an Auger-electron–photoion coincidence method

An Auger-electron–photoion coincidence (AEPICO) method has been applied to study the stability and dissociation dynamics of dicationic states after the N K-shell photoionization of nitrogen molecules. From time-of-flight and kinetic energy analyses of the product ions, we have obtained coincident Auger spectra associated with metastable states of N{sub 2}{sup ++} ions and dissociative states leading to N{sub 2}{sup ++} → N{sup +} + N{sup +} and N{sup ++} + N. To investigate the production of dissociative states, we present two-dimensional AEPICO maps which reveal the correlations between the binding energies of the Auger final states and the ion kinetic energy release. These correlations have been used to determine the dissociation limits of individual Auger final states.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

A method for coincidence timing resolution enhancement

A method including the coincidence time resolution improvement for a TOF/positron emission tomography system was suggested. The spectrometer for this aim was composed of two NaI(Tl) and two plastic scintillation detectors. Experimental results were supported by FLUKA Monte Carlo simulation program by constructing the detector setup in software medium. Present experimental results verified our previous results and conclusions obtained from the suggested method. It was concluded that better resolutions would help the improvement not only on the TOF gain but also on the spatial resolution, leading to better images and helping the Physician in his/her diagnosis and treatment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Passive Neutron Instrumentation and Applications

This chapter presents a description of most of the instruments that are currently in use for the measurement of plutonium and uranium using passive methods (without an external source). This includes the acquisition electronics as well as Singles counting methods, coincidence counting methods and multiplicity counting methods. The Singles counting applications include the measurement of waste and curium bearing materials. The coincidence counting applications include bulk plutonium, bulk uranium, waste and holdup measurements and fresh fuel assemblies. The multiplicity application description includes advantages and disadvantages and multiplicity detector design. There is also a description of some non-3He systems. The chapter concludes with a description of additional concepts: neutron imagers, list-mode data analysis, distributed source term analysis, unattended monitoring and MCNP modeling for detector design.

Coincidence shift register↗

Low-Noise Free-Running High-Rate Photon-Counting for Space Communication and Ranging

We present performance data for low-noise free-running high-rate photon counting method for space optical communication and ranging. NASA GSFC is testing the performance of two types of novel photon-counting detectors 1) a 2x8 mercury cadmium telluride (HgCdTe) avalanche array made by DRS Inc., and a 2) a commercial 2880-element silicon avalanche photodiode (APD) array. We successfully measured real-time communication performance using both the 2 detected-photon threshold and logic AND-gate coincidence methods. Use of these methods allows mitigation of dark count, after-pulsing and background noise effects without using other method of Time Gating The HgCdTe APD array routinely demonstrated very high photon detection efficiencies (50) at near infrared wavelength. The commercial silicon APD array exhibited a fast output with rise times of 300 ps and pulse widths of 600 ps. On-chip individually filtered signals from the entire array were multiplexed onto a single fast output. NASA GSFC has tested both detectors for their potential application for space communications and ranging. We developed and compare their performances using both the 2 detected photon threshold and coincidence methods.

Photons↗

Low-Noise Free-Running High-Rate Photon-Counting for Space Communication and Ranging

We present performance data for low-noise free-running high-rate photon counting method for space optical communication and ranging. NASA GSFC is testing the performance of two types of novel photon-counting detectors 1) a 2x8 mercury cadmium telluride (HgCdTe) avalanche array made by DRS Inc., and a 2) a commercial 2880-element silicon avalanche photodiode (APD) array. We successfully measured real-time communication performance using both the 2 detected-photon threshold and logic AND-gate coincidence methods. Use of these methods allows mitigation of dark count, after-pulsing and background noise effects without using other method of Time Gating The HgCdTe APD array routinely demonstrated very high photon detection efficiencies ((is) greater than 50%) at near infrared wavelength. The commercial silicon APD array exhibited a fast output with rise times of 300 ps and pulse widths of 600 ps. On-chip individually filtered signals from the entire array were multiplexed onto a single fast output. NASA GSFC has tested both detectors for their potential application for space communications and ranging. We developed and compare their performances using both the 2 detected photon threshold and coincidence methods.

Photons↗

Thermometry of an open spatially inhomogeneous flame by diode laser absorption spectroscopy

Features of a single-beam variant of diode laser absorption spectroscopy (DLAS) used for temperature measurements in a spatially inhomogeneous hot zone are studied. A flame temperature of a commercial burner is measured by using water molecule absorption lines. The flame is probed by a diode laser radiation at various heights and in various directions. The correctness of DLAS measurement results is verified by comparing DLAS data with temperatures measured by the method of coherent anti-Stokes scattering (CARS). It is shown that in homogeneous flame domains the temperatures obtained by both the methods coincide. Temperature inhomogeneity along the probe beam direction is a principal problem of DLAS, in which case the method yields information about some effective temperature along the light trace. The difference in data obtained by DLAS and CARS is estimated. In probing traces with temperature gradients the difference reaches 700 K. Possibilities of accounting for temperature inhomogeneities along the trace in DLAS measurements are discussed. A method of differential spectra is suggested, which in certain conditions can provide substantially better coincidence of results for the two methods. (laser spectroscopy)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

X-ray escape peaks in gamma-ray spectrum acquired by perovskite detector

The X-ray escape peaks are clearly visible in the high-resolution gamma spectra acquired by CsPbBr 3 , credit to the rapidly improving energy resolution of perovskite gamma detectors. But it also raises concerns. If this peak remains as significant as it is, perovskite gamma detectors would have very limited use in complex gamma spectrometry applications. This paper discusses the origin of the escape peaks in CsPbBr 3 detectors, benchmarked against Ge and CZT detectors. The Pb escape peak consists of four escape peaks that are merged together, while the Cs and Br escape peaks are hidden inside the photopeak of 137 Cs (662 keV). These combined effects either create a noticeable gamma peak observed to the left of the 662 keV photopeak when acquired using a high-resolution CsPbBr 3 detector or raise the left slope of the photopeak. We also explore potential methods to mitigate these peaks, such as applying anti-coincidence method. The height of the escape peaks diminishes as the detector volume increases but will not go away entirely. The relationship between the observed Pb escape peak and the detector's dimensions is demonstrated through Monte Carlo simulation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Identification of $^{3}$He–$^{3}$H clusters in the $^{6}$Li+$^{89}$Y experiment using particle-$\gamma$ coincidence measurement

The 6 Li+ 89 Y experiment was performed to explore the reaction mechanism induced by a weakly bound nucleus 6 Li and its cluster configuration. Here, the particle-$\gamma$ coincidence method was used to identify the different reaction channels. The $\gamma$-rays coincident with 3 He/ 3 H indicate that the 3 H/ 3 He stripping reaction plays a significant role in the formation of Zr/Nb isotopes. The obtained results support the existence of a 3 He- 3 H cluster in 6 Li. Direct and sequential transfer reactions are adequately discussed, and the FRESCO code is used to perform precise finite-range cyclic redundancy check calculations. In the microscopic calculation, direct cluster transfer is more predominant than sequential transfer in 3 H transfer. However, the direct cluster transfer is of comparable magnitude to the sequential transfer in the 3 He transfer.

CRC calculations↗

Photoelectron spectroscopy in molecular physical chemistry

Photoelectron spectroscopy has long been a powerful method in the toolbox of experimental physical chemistry and molecular physics. Recent improvements in coincidence methods, charged-particle imaging, and electron energy resolution have greatly expanded the variety of environments in which photoelectron spectroscopy can be applied, as well as the range of questions that can now be addressed. In this Perspectives Article, we focus on selected recent studies that highlight these advances and research areas. Furthermore, the topics include reactive intermediates and new thermochemical data, high-resolution comparisons of experiment and theory using methods based on pulsed-field ionisation (PFI), and the application of photoelectron spectroscopy as an analytical tool to monitor chemical reactions in complex environments, like model flames, catalytic or high-temperature reactors.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Entrance channel effects on the quasifission reaction channel in Cr + W systems

Background: Formation of a fully equilibrated compound nucleus is a critical step in the heavy-ion fusion reaction mechanism but can be hindered by orders of magnitude by quasifission, a process in which the dinuclear system breaks apart prior to full equilibration. Furthermore, to provide a complete description of heavy-ion fusion it is important to characterize the quasifission process. In particular, the impact of changing the neutron richness on the quasifission process is not well known. A previous study of Cr + W reactions at a constant 13% above the Coulomb barrier concluded that an increase in neutron richness leads to a decrease in the prominence of the quasifission reaction channel. Purpose: The dynamics of quasifission for reactions with varying neutron richness was explored at a constant excitation energy, closer to the interaction barrier than the previous work, to see if the correlation between neutron richness and quasifission is valid at lower energies. Methods: Mass distributions were measured at the Australian National University for eight different combinations of Cr + W reactions, using the kinematic coincidence method. To eliminate the effect of differing excitation energies, measurements were made at beam energies chosen to give 52 MeV of excitation energy in all the compound nuclei. Results: A curvature parameter, describing the shape of the mass distributions, was determined for the fission-like fragment mass distributions for each reaction, and compared to various reaction parameters known to influence quasifission. Conclusions: The present work demonstrates that, at energies near the interaction barrier, the beam energy with respect to the barrier is as important as neutron-richness effects in determining the quasifission characteristics in these Cr + W reactions involving statically deformed target nuclei, and both are important considerations for future heavy and superheavy element production reactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Radiative decay rate of excitons in square quantum wells: Microscopic modeling and experiment

The binding energy and the corresponding wave function of excitons in GaAs-based finite square quantum wells (QWs) are calculated by the direct numerical solution of the three-dimensional Schrödinger equation. The precise results for the lowest exciton state are obtained by the Hamiltonian discretization using the high-order finite-difference scheme. The microscopic calculations are compared with the results obtained by the standard variational approach. The exciton binding energies found by two methods coincide within 0.1 meV for the wide range of QW widths. The radiative decay rate is calculated for QWs of various widths using the exciton wave functions obtained by direct and variational methods. The radiative decay rates are confronted with the experimental data measured for high-quality GaAs/AlGaAs and InGaAs/GaAs QW heterostructures grown by molecular beam epitaxy. The calculated and measured values are in good agreement, though slight differences with earlier calculations of the radiative decay rate are observed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

A virtual element generalization on polygonal meshes of the Scott-Vogelius finite element method for the 2-D Stokes problem

The virtual element method (VEM) is a Galerkin approximation method that extends the finite element method to polytopal meshes. In this paper, we present a conforming formulation that generalizes the Scott-Vogelius finite element method (FEM) for the numerical approximation of the Stokes problem to polygonal meshes in the framework of the virtual element method. In particular, we consider a straightforward application of the virtual element approximation space for scalar elliptic problems to the vector case and approximate the pressure variable through discontinuous polynomials. We assess the effectiveness of the numerical approximation by investigating the convergence on a manufactured solution problem and a set of representative polygonal meshes. We numerically show that this formulation is convergent with optimal convergence rates except for the lowest-order case on triangular and square meshes where the method coincides with the P 1 - P 0 Scott-Vogelius scheme, which is well-known to be unstable.

97 MATHEMATICS AND COMPUTING↗

A virtual element generalization on polygonal meshes of the Scott-Vogelius finite element method for the 2-D Stokes problem

The Virtual Element Method (VEM) is a Galerkin approximation method that extends the Finite Element Method (FEM) to polytopal meshes. In this paper, we present a conforming formulation that generalizes the Scott-Vogelius finite element method for the numerical approximation of the Stokes problem to polygonal meshes in the framework of the virtual element method. In particular, we consider a straightforward application of the virtual element approximation space for scalar elliptic problems to the vector case and approximate the pressure variable through discontinuous polynomials. We assess the effectiveness of the numerical approximation by investigating the convergence on a manufactured solution problem and a set of representative polygonal meshes. Finally, we numerically show that this formulation is convergent with optimal convergence rates except for the lowest-order case on triangular meshes, where the method coincides with the $\mathbb{P}_1$ – $\mathbb{P}_0$ Scott-Vogelius scheme, and on square meshes, which are situations that are well-known to be unstable.

97 MATHEMATICS AND COMPUTING↗

A solvable problem in statistical mechanics: The dipole-type Hamiltonian mean field model

The present study documents a type of mean field approximation inspired by the dipole interaction model, which is analytically solved in the canonical and microcanonical ensembles. The current calculations were derived from the Hamiltonian mean field model developments. After describing the canonical partition function, the free and internal energies, magnetization, and specific heat are derived and graphically depicted. In the microcanonical ensemble, the entropy is calculated as well as other thermodynamic properties. The system shows a second-order phase transition emphasizing that both methods coincide, which is only valid only in equilibrium. In addition, the current model represents a nonsymmetric Hamiltonian mean field model that shows a phase transition.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Comparative Architecture Analysis: Using Laminar Structure to Unify Multiple Grid Architectures

A great many architectures for various aspects of electric grids have been proposed over recent years and new ones continue to be suggested. Generally speaking, there is no means except ad hoc analysis by which one can reduce these architectures to some common basis, or extract common elements. This leads to confusion in choosing an architecture for implementation, as well as making it difficult to identify core product or platform opportunities with sufficient potential markets to encourage vendors to provide or develop them. The discipline of Grid Architecture as defined for the US Department of Energy (DOE) in 2014 has multiple purposes. Among them are two that are relevant here: Providing rigorous bases for architectural structures and Identifying common aspects of apparently divergent architectural structures. For the first of these, mathematical methods are applied where possible to provide the rigorous basis for structure. For the second, mapping of architectural structures to a canonical structure puts apparently disparate architectures onto a common basis. In the best case, these two methods coincide. In this paper, Laminar Coordination structure serves as the rigorously defined common basis for analysis of several real and proposed grid architectures.

24 POWER TRANSMISSION AND DISTRIBUTION↗