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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Carbonyl Sulfide (OCS): Detections in Comets C/2002 T7 (LINEAR), C/2015 ER61 (PanSTARRS), and 21P/Giacobini–Zinner and Stringent Upper Limits in 46P/Wirtanen

Carbonyl sulfide (OCS) is one of the sulfur-bearing molecules detected in different astronomical environments, including comets. The present-day sulfur chemistry in comets may reveal much about the origin of these ices and their subsequent processing history. Cometary sulfur molecules such as H{sub 2}S, H{sub 2}CS, SO{sub 2}, SO, CS, CS{sub 2}, S{sub 2}, and NS have been detected in many comets. However, OCS, the only sulfur-bearing species with fluorescence emission lines at infrared wavelengths, is under-represented in comet volatile studies, having been reported in only six comets so far. We targeted OCS with the NASA Infrared Telescope Facility in comets 46P/Wirtanen, 21P/Giacobini–Zinner, and C/2015 ER61 (PanSTARRS) in 2017–2018 using the high-resolution iSHELL spectrograph, and in C/2002 T7 (LINEAR) in 2004 using the heritage CSHELL spectrograph. In comet C/2015 ER61, the OCS abundance was similar to those measured in bright comets such as comets C/2012 S1 (ISON) and C/1996 B2 (Hyakutake), whereas in C/2002 T7 it was relatively depleted. Our OCS measurement in 21P/Giacobini–Zinner is the first definitive detection of this molecule in a Jupiter-family comet from a ground-based facility and is close to the average OCS abundance determined in comet 67P/Churyumov–Gerasimenko by the Rosetta mission. Our 3σ upper limit for comet 46P/Wirtanen is the lowest reported OCS abundance in any comet. We present production rates and mixing ratios (with respect to H{sub 2}O) for these comets and place our results in the context of comets measured to date.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

High-resolution Optical Spectroscopic Observations of Comet 21P/Giacobini–Zinner in Its 2018 Apparition

Comet 21P/Giacobini–Zinner is a peculiar comet from the viewpoints of the chemical and physical properties of its dust grains. We conduct optical high-resolution spectroscopic observations of the comet. The intensity ratios of forbidden oxygen lines (at 557.7, 630.0, and 636.4 nm) and ortho-to-para abundance ratios (OPRs) of water cations (H{sub 2}O{sup +}) and amidogen radicals (NH{sub 2}) are obtained while only the upper limit for {sup 14}N/{sup 15}N in the amidogen radical is restricted. The OPRs of H{sub 2}O{sup +} and NH{sub 2} are similar to those of other comets, although the real meaning of these OPRs is still debated. Based on the observation of the forbidden emission lines of oxygen atoms, it can be concluded that the comet is depleted in CO{sub 2}. In consideration with the depletion in other highly volatile species found in the near-infrared region and the presence of complex organics in comet 21P/Giacobini–Zinner, this comet might form in a warmer region in the solar nebula compared with other comets.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Lyα Observations of Comet C/2013 A1 (Siding Spring) Using MAVEN IUVS Echelle

The close approach of comet C/2013 A1 (Siding Spring) to Mars in 2014 October provided a unique opportunity to observe a dynamically new Oort cloud comet with potential for interaction with a planet’s atmosphere. The water-originating hydrogen coma of the comet extended to over 20 million km from the nucleus. Determining the properties of this coma contributes to characterizing the comet’s water content and production rate. The present study analyzes a unique data set of high spectral resolution UV observations of comet C/2013 A1 Siding Spring measured by the Mars Atmosphere and Volatile Evolution spacecraft. The Siding Spring observations capture Lyα emissions from the Martian corona, the interplanetary medium, as well as the cometary H and D reservoirs. The isolated cometary spectra are analyzed to reveal a velocity distribution of H atoms that are consistent with model estimates of H{sub 2}O photodissociated H emissions and of OH photodissociated H emissions, Doppler shifted from the main comet H emission line center by 18 km s{sup −1} and 8 km s{sup −1}, respectively. The variations in comet H brightness with distance from the nucleus are used to constrain cometary water production to a rate of 0.5 × 10{sup 28} molecules s{sup −1} at a time when Siding Spring was at 1.5 au, pre-perihelion.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Physical Characterization of Interstellar Comet 2I/2019 Q4 (Borisov)

We present a study of interstellar comet 2I/2019 Q4 (Borisov) using both preperihelion and postperihelion observations spanning late September 2019 through late January 2020. The intrinsic brightness of the comet was observed to continuously decline throughout the timespan, likely due to the decreasing effective scattering cross-section as a result of volatile sublimation with a slope of −0.43 ± 0.02 km{sup 2} d{sup −1}. We witnessed no significant change in the slightly reddish color of the comet, with mean values of 〈g−r〉=0.68±0.04, 〈r−i〉=0.23±0.03, and the normalized reflectivity gradient across the g and i bands (S{sup ′})-bar (g,i)=(10.6±1.4)% per 10{sup 3} Å, all unremarkable in the context of solar system comets. Using the available astrometric observations, we confidently detect the nongravitational acceleration of the comet following a shallow heliocentric distance dependence of r{sub H}{sup −1±1}. Accordingly, we estimate that the nucleus is most likely ≲0.4 km in radius, and that a fraction of ≳0.2% of the total mass of the nucleus has been eroded due to the sublimation activity since the earliest observation of the comet in 2018 December by the time of perihelion. Our morphology simulation suggests that the dust ejection speed increased from ∼4 m s{sup −1} in 2019 September to ∼7 m s{sup −1} around perihelion for the optically dominant dust grains with β∼0.01, and that the observable dust grains are no smaller than micron size.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

A New Era of Nuclear Criticality Experiments: The First 10 Years of Comet Operations at NCERC

Comet is a general-purpose, heavy-duty, vertical-lift assembly designed for flexibility in conducting a variety of critical experiments. It is currently located at the National Criticality Experiments Research Center (NCERC) in Nevada. In the past, Comet resided at Technical Area-18 in Los Alamos, New Mexico, as part of the Los Alamos Critical Experiments Facility (LACEF). The Comet assembly was relocated to NCERC in 2008 and became fully operational in June of 2011. The first critical experiment performed on Comet at NCERC was a verification of one of the previous configurations of the Zeus experiment series. Over the next 10 years, many additional experiments followed including other Zeus configurations as well as completely new designs. This paper discusses the Comet vertical-lift assembly, the transition from LACEF to NCERC, and a selection of experiments that have been performed on Comet during its first 10 years of operation at NCERC.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Compositional evidence for chondrule origins of low‐Ca pyroxenes in comet Wild 2 and a giant cluster IDP

Abstract A literature compilation of 1136 low‐Ca pyroxene compositions from chondrules from 12 primitive type 2–3 carbonaceous, ordinary and enstatite chondrite groups define unique regions on an Al 2 O 3 and Cr 2 O 3 diagram when compared to low‐Ca pyroxenes from equilibrated type 4‐6 chondrites. Measured compositions of 100 low‐Ca pyroxenes from comet Wild 2 and a giant cluster IDP of probable cometary origin are similar to each other and fall in the type 2–3 chondrite chondrule region suggesting that most of the pyroxenes likely formed in the solar nebula like conventional chondrules. The data imply that most low Ca‐pyroxenes from comet Wild 2 and the giant cluster IDP formed from igneous crystallization processes and did not experience significant thermal metamorphism, indicating that the low‐Ca pyroxenes were unlikely incorporated into large parent bodies prior to accretion in their respective comet bodies. An intriguing group of nine low‐Ca pyroxenes from comet Wild 2 with low Cr and Al that fall where type 4–6 chondrites are located are interpreted as products of condensation. The compositional data combined with previously measured oxygen isotopes on 17 low‐Ca pyroxenes support earlier conclusions that comet samples have links with carbonaceous, ordinary, and possibly enstatite chondrite groups. Our results provide additional evidence that comets accreted materials from multiple chondrule reservoirs throughout the solar nebula.

Geochemistry & Geophysics↗
DOE OSTI2021

C/2014 UN 271 (Bernardinelli-Bernstein): The Nearly Spherical Cow of Comets

Abstract Comet C/2014 UN 271 (Bernardinelli-Bernstein), incoming from the Oort cloud, is remarkable in having the brightest (and presumably largest) nucleus of any well-measured comet and having been discovered at the heliocentric distance r h ≈ 29 au, farther than any Oort cloud comet. In this work, we describe the discovery process and observations and the properties that can be inferred from images recorded until the first reports of activity in 2021 June. The orbit has i = 95°, with a perihelion of 10.97 au to be reached in 2031 and a previous aphelion at 40,400 ± 260 au. Backward integration of the orbit under a standard Galactic tidal model and known stellar encounters suggests a perihelion of q ≈ 18 au on its previous perihelion passage 3.5 Myr ago; hence, the current data could be the first ever obtained of a comet that has not been inside Uranus’s orbit in 4 Gyr. The photometric data show an unresolved nucleus with absolute magnitude H r = 8.0, colors that are typical of comet nuclei or Damocloids, and no secular trend as it traversed the range 34–23 au. For the r -band geometric albedo p r , this implies a diameter of 150 ( p r / 0.04 ) − 0.5 km. There is strong evidence of brightness fluctuations at the ±0.2 mag level, but no rotation period can be discerned. A coma, nominally consistent with a “stationary” 1/ ρ surface brightness distribution, grew in scattering cross section at an exponential rate from A f ρ ≈ 1 to ≈150 m as the comet approached from 28 to 20 au. The activity rate is consistent with a very simple model of sublimation of a surface species in radiative equilibrium with the Sun. The inferred enthalpy of sublimation matches those of CO 2 and NH 3 . More volatile species, such as N 2 , CH 4 , and CO, must be far less abundant on the sublimating surfaces.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Investigation of the Origins of Comets as Revealed through Infrared High-resolution Spectroscopy I. Molecular Abundances

We report and analyze updated molecular abundances in 20 comets obtained by employing modern data reduction procedures and molecular models. Using box and scatter plots, we examine how the different molecular species are distributed among the comet population, while by means of pie charts, we investigate the relative proportions of these molecular species in each comet. We compare these results with the orbital parameters of the selected comets to identify trends related to their dynamical history. With these analyses, we tentatively identify at least three chemical classes based mainly on relative abundances of CO, CH{sub 3}OH, CH{sub 4}, C{sub 2}H{sub 6}, HCN, and NH{sub 3}. The combination of relative abundances and orbital parameters is then compared with recent chemical models of planetary system formation. This approach may help in investigating the origins and evolution of the material in cometary nuclei. Among other aspects, we underline the need to increase our sample size, especially for hypervolatiles (i.e., CH{sub 4} and CO) in Jupiter family comets.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Disintegration of Long-period Comet C/2019 Y4 (ATLAS). I. Hubble Space Telescope Observations

The near-Sun comet C/2019 Y4 (ATLAS) is the first member of a long-period comet group observed to disintegrate well before perihelion. Here we present our investigation into this disintegration event using images obtained in a three-day Hubble Space Telescope campaign. We identify two fragment clusters produced by the initial disintegration event, corresponding to fragments C/2019 Y4-A and C/2019 Y4-B identified in ground-based data. These two clusters started with similar integrated brightness but exhibit different evolutionary behavior. C/2019 Y4-A was much shorter-lived compared to C/2019 Y4-B and showed signs of significant mass loss and changes in size distribution throughout the three-day campaign. The cause of the initial fragmentation is undetermined by the limited evidence but crudely compatible with either the spin-up disruption of the nucleus or runaway sublimation of subsurface supervolatile ices, either of which would lead to the release of a large amount of gas as inferred from the significant bluing of the comet observed shortly before its disintegration. Gas can only be produced by the sublimation of volatile ices, which must have survived at least one perihelion passage at a perihelion distance of q = 0.25 au. We speculate that Comet ATLAS is derived from the ice-rich interior of a nonuniform, kilometer-wide progenitor that split during its previous perihelion. This suggests that comets down to a few kilometers in diameter can still possess complex, nonuniform interiors that can protect ices against intense solar heating.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Rotational symmetry relation for efficient response function generation in the coarse mesh transport method COMET

The coarse mesh transport code COMET is a continuous energy hybrid stochastic-deterministic neutronics solver with high fidelity and formidable computation speed in solving reactor core problems. Its method is based on the incident flux expansion theory. In this work, we take advantage of the local geometric symmetry in many reactor cores lattices (e.g., fuel lattices and reflector blocks) to develop relations among the flux response expansion coefficients for symmetric surfaces to further improve the computational efficiency of the COMET response function generation tool (method). This is done by a rigorous derivation of the transformation matrices for the angular and spatial expansion moments resulting from a rotation of a coarse mesh by an arbitrary angle. The relations for the response coefficients for the symmetric surfaces can be then written as the Kronecker product of those transformation matrices. The method is implemented into COMET and tested on two advanced high temperature reactor (AHTR) full-length single assembly benchmark problems. The COMET results using the response function library based on the symmetry relations were compared to those using the library directly generated by continuous energy Monte Carlo for all surfaces. It was found that the eigenvalues and stripe-wise fission densities using the two libraries are in statistical agreement as expected. This indicates that the new method maintains the high fidelity of the original COMET method while improving the computational efficiency in the response function generation by 270% to 400%, depending on the local geometric symmetry. This method also reduces the size of the response function library by the same magnitude (270% to 400%). (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2022

Physical and dynamical characterization of hyperbolic comet C/2017 U7 (PANSTARRS)

Here we present here a dynamical and observational study of the comet C/2017 U7 (PANSTARRS). This comet was discovered in 2017 and found to have a hyperbolic orbit. Our dynamical analysis shows that the object has probably originated in the Oort cloud, however an interstellar origin cannot be discarded. The observations were obtained in 2018 and 2019 using the Goodman High Throughput Spectrograph (GHTS) at the SOAR telescope. We obtained visible spectra covering the wavelength range of 0.5 - 0.9 μm and also images in the SDSS filters system. Both the low-resolution reflectance spectrum and the reflectance spectra derived from the SDSS filters show an atypical band at ~ 0.595 μm. We conducted a comparative study of the colors and reflectance spectra of different small body populations (e.g., comets, Centaurs, and trans-Neptunian objects or TNOs) from the literature and concluded that the spectra and the colors of this comet are atypical, showing only some overlap with those of some known members of the TNOs and Centaurs, within the large uncertainties of the measurements of those populations. It is found that the feature and overall spectral shape can be reproduced by laboratory spectra of kerite, a template for aliphatic-rich hydrocarbons that has been previously identified in NIR cometary spectra absorptions. It is tentatively proposed that the unusual spectral shape is the result of a particle size distribution of dust grains in the coma or on the surface that has arisen due to a low grain ejection velocity from the surface and large nucleus size.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Characterization of the Nucleus, Morphology, and Activity of Interstellar Comet 2I/Borisov by Optical and Near-infrared GROWTH, Apache Point, IRTF, ZTF, and Keck Observations

We present visible and near-infrared (NIR) photometric and spectroscopic observations of interstellar object (ISO) 2I/Borisov taken from 2019 September 10 to 2019 December 20 using the GROWTH, the Apache Point Observatory Astrophysical Research Consortium 3.5 m, and the NASA Infrared Telescope Facility 3.0 m combined with pre- and postdiscovery observations of 2I obtained by the Zwicky Transient Facility from 2019 March 17 to 2019 May 5. Comparison with imaging of distant solar system comets shows an object very similar to mildly active solar system comets with an outgassing rate of ∼10{sup 27} mol s{sup −1}. The photometry, taken in filters spanning the visible and NIR range, shows a gradual brightening trend of ∼0.03 mag day{sup −1} since 2019 September 10 UTC for a reddish object becoming neutral in the NIR. The light curve from recent and prediscovery data reveals a brightness trend suggesting the recent onset of significant H{sub 2}O sublimation with the comet being active with super volatiles such as CO at heliocentric distances >6 au consistent with its extended morphology. Using the advanced capability to significantly reduce the scattered light from the coma enabled by high-resolution NIR images from Keck adaptive optics taken on 2019 October 4, we estimate a diameter for 2I’s nucleus of ≲1.4 km. We use the size estimates of 1I/’Oumuamua and 2I/Borisov to roughly estimate the slope of the ISO size distribution, resulting in a slope of ∼3.4 ± 1.2, similar to solar system comets and bodies produced from collisional equilibrium.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Systematics and Consequences of Comet Nucleus Outgassing Torques

Anisotropic outgassing from comets exerts a torque sufficient to rapidly change the angular momentum of the nucleus, potentially leading to rotational instability. Here, we use empirical measures of spin changes in a sample of comets to characterize the torques, and to compare them with expectations from a simple model. Both the data and the model show that the characteristic spin-up timescale, τ {sub s}, is a strong function of nucleus radius, r {sub n}. Empirically, we find that the timescale for comets (most with perihelion 1–2 au and eccentricity ∼0.5) varies as τ{sub s}∼100r{sub n}{sup 2}, where r {sub n} is expressed in kilometers, and τ {sub s} is in years. The fraction of the nucleus surface that is active varies as f{sub A}∼0.1r{sub n}{sup −2}. We find that the median value of the dimensionless moment arm of the torque is k {sub T} = 0.007 (i.e., ∼0.7% of the escaping momentum torques the nucleus), with weak (<3σ) evidence for a size dependence k{sub T}∼10{sup −3}r{sub n}{sup 2}. Sub-kilometer nuclei have spin-up timescales comparable to their orbital periods, confirming that outgassing torques are quickly capable of driving small nuclei toward rotational disruption. Torque-induced rotational instability likely accounts for the paucity of sub-kilometer short-period cometary nuclei, and for the pre-perihelion destruction of sungrazing comets. Torques from sustained outgassing on small active asteroids can rival YORP torques, even for very small (≲1 g s{sup −1}) mass-loss rates. Finally, we highlight the important role played by observational biases in the measured distributions of τ {sub s}, f {sub A}, and k {sub T}.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

A metabolic modeling platform for the computation of microbial ecosystems in time and space (COMETS)

Genome-scale stoichiometric modeling of metabolism has become a standard systems biology tool for modeling cellular physiology and growth. Extensions of this approach are emerging as a valuable avenue for predicting, understanding and designing microbial communities. Computation of microbial ecosystems in time and space (COMETS) extends dynamic flux balance analysis to generate simulations of multiple microbial species in molecularly complex and spatially structured environments. Here we describe how to best use and apply the most recent version of COMETS, which incorporates a more accurate biophysical model of microbial biomass expansion upon growth, evolutionary dynamics and extracellular enzyme activity modules. In addition to a command-line option, COMETS includes user-friendly Python and MATLAB interfaces compatible with the well-established COBRA models and methods, as well as comprehensive documentation and tutorials. Overall, this protocol provides a detailed guideline for installing, testing and applying COMETS to different scenarios, generating simulations that take from a few minutes to several days to run, with broad applicability to microbial communities across biomes and scales.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2021

The Encounter of the Parker Solar Probe and a Comet-like Object Near the Sun: Model Predictions and Measurements

The Parker Solar Probe (PSP) aims to explore the nascent solar wind close to the Sun. Meanwhile, PSP is also expected to encounter small objects like comets and asteroids. Here, we survey the ephemerides to find the chance of a recent encounter and then model the interaction between released dusty plasmas and solar wind plasmas. On 2019 September 2, a comet-like object, the 322P/Solar and Heliosphere Observatory, just passed its perihelion flying to a heliocentric distance of 0.12 au and swept by PSP at a relative distance as close as 0.025 au. We present the dynamics of the dust particles released from 322P, forming a curved dust tail. Along the path of PSP in the simulated inner heliosphere, the states of plasma and magnetic field are sampled and illustrated, with the magnetic field sequences from simulation results being compared directly with the in situ measurements from PSP. Through the comparison, we suggest that 322P might be at a deficient activity level releasing limited dusty plasmas on its way to becoming a "rock comet." We also present images of solar wind streamers as recorded by the Wide-field Imager for Solar Probe Plus, showing an indication of dust bombardment for the images superposed with messy trails. We observe from the Large Angle and Spectrometric Coronagraph that 322P was transiting from a dimming region to a relatively bright streamer during its perihelion passage, and perform a simulation to confirm that 322P was flying from relatively faster to slower solar wind streams, modifying the local plasma states of the streams.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

James Clerk Maxwell Telescope Spectral and Continuum Imaging of Hyperactive Comet 46P/Wirtanen

The Jupiter-family comet (JFC) 46P/Wirtanen passed the Earth at a distance of 0.077 au on 2018 December 16 UT, presenting a rare opportunity to study the chemical structure of its coma. With the James Clerk Maxwell Telescope we achieved a resolution of 800 km, which is smaller than the scale lengths of some distributed cometary molecules at the comet’s heliocentric distance of 1 au. Spectroscopic observations of the J = 4 - 3 transition of HCN showed generally uniform levels of outgassing activity during the observing period, 2018 December 14–20. Gas expansion velocities were ~0.6 km s{sup -1}, and the derived average HCN production rate was 7.4 × 10{sup 24} mol s{sup -1}. HCN and CH{sub 3}OH emissions were detected at least 30" (1600 km) from the nucleus, and the abundances of these species were typical for a JFC. The radial distribution of CH{sub 3}OH is consistent with an extended source of sublimation such as a population of icy grains—cometary halo ice primaries, or CHIPs—as has been invoked previously to explain hyperactivity in comets. The abundance of H{sub 2}CO is normal if it is a daughter species. HNC and CO were not detected, but a sensitive nondetection of CS implies an unusually low CS:H{sub 2}O ratio of <0.02%. The peak brightness of the 850 μm continuum emissions from icy coma dust particles of size ~1 mm fell from (52 ± 6) to (40 ± 3) mJy beam{sup -1} through the week, while the size of the dust coma remained essentially constant, with dust extending to ~1000 km from the nucleus. The total mass of those particles was ~2 × 10{sup 8} kg.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Meteoroid Stream of Comet C/1961 T1 (Seki) and Its Relation to the December ρ-Virginids and γ-Sagittariids

We answer the question of whether long-period comet C/1961 T1 (Seki) is the parent body of a meteor shower observed in Earth’s atmosphere. We model discrete parts of a meteoroid stream associated with this comet and follow the orbital evolution of its particles via a numerical integration of their orbits. The gravitational perturbations of major planets and the Poynting–Robertson effect, which influences the motion of the particles, are taken into account. We predict two showers which are related to C/1961 T1. One of these showers was identified with the December ρ-Virginids, #502. This identification confirms an earlier suggested relationship between the shower and the comet. The second predicted shower was identified with the γ-Sagittariids, #657. The radiant areas of both showers are symmetrical in respect to the apex of Earth’s heliocentric motion.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

New Insights into the Chemical Composition of Five Oort Cloud Comets after Re-analysis of Their Infrared Spectra

We present revised results for the main molecular species in five Oort Cloud comets observed with near-infrared echelle grating spectrometer (NIRSPEC) at the Keck Observatory between 1999 and 2012 (C/1999 S4 (LINEAR), C/2001 A2 (LINEAR), C/2007 W1 (Boattini), C/2012 F6 (Lemmon), and C/2012 S1 (ISON)). The re-evaluation of these data shows the improvement of results in some of the data sets, in particular for comets observed and analyzed before the advent of new and revised fluorescence models and terrestrial retrieval methods introduced since 2011. We observe significant improvements in the resulting rotational temperatures and the production rates for all species, and in mixing ratios of minor species (relative to water). The re-analysis also allowed us to quantify species not analyzed previously, mostly due to the lack of molecular models (e.g., ammonia and formaldehyde). We note, however, that the improvement of these revised values is less substantial for comets observed (and/or analyzed) since 2010.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗