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Identification of Prompt Proton Emission in $N = Z - 1$ 61 Ga: Isospin Symmetry at the Limit of Nuclear Binding
Excited states in the proton drip line nucleus 61 Ga were populated via the fusion-evaporation reaction 24 Mg ( 40 Ca, 𝑝2𝑛) 61 Ga. The experimental setup at Argonne National Laboratory comprised a novel combination of the Gammasphere array with two CD-shaped double-sided Si-strip detectors inside the Microball CsI(Tl) charged-particle detection array, as well as the Neutron-Shell liquid scintillators and the Fragment Mass Analyzer. Owing to the setup’s unprecedented in-beam proton spectroscopy and tracking capabilities, a coincidence between a 957.6(5)-keV 𝛾 ray and a 1.876(24)-MeV proton line was observed, which identifies the quasibound proton 𝜋𝑔 9/2 single-particle state in 61 Ga at 𝐸 𝑥 = 2150(34) keV. This probes isospin symmetry at the limit of nuclear binding by providing a unique challenge for the shell-model interpretation of mirror nuclei beyond doubly magic 56 Ni .
CHICOX, a heavy-ion detection system for GRETA
The CHICOX detection system is an array of position sensitive parallel plate avalanche counters used for heavy ion detection in in-beam particle-gamma coincidence experiments. CHICOX, an upgrade of the CHICO2 array, is geometrically compatible with the GRETINA and GRETA gamma-ray arrays and provides an angular resolution sufficient to utilize the excellent position resolution of GRETINA/GRETA. CHICOX was successfully commissioned and fielded as an auxiliary detector to GRETINA in a campaign of stable-beam Coulomb excitation experiments at the ATLAS facility of Argonne National Laboratory. We report here on the design and in-beam performance of the CHICOX array.
Disentangling Centrality Bias and Final-State Effects in the Production of High-𝑝 𝑇 Neutral Pions Using Direct Photon in 𝑑+Au Collisions at $\sqrt{s_{NN}}$ = 200 GeV
Here, PHENIX presents a simultaneous measurement of the production of direct 𝛾 and 𝜋 0 in 𝑑 + Au collisions at $\sqrt{s_{NN}}$ = 200 GeV over a 𝑝 𝑇 range of 7.5 to 18 GeV/𝑐 for different event samples selected by event activity, i.e., charged-particle multiplicity detected at forward rapidity. Direct-photon yields are used to empirically estimate the contribution of hard-scattering processes in the different event samples. Using this estimate, the average nuclear-modification factor, 𝑅$^{𝜋^0}_{dAu,EXP}$, is 0.925 ± 0.023(stat) ± 0.15(scale), consistent with unity for minimum-bias (MB) 𝑑+Au collisions. For event classes with low and moderate event activity, 𝑅$^{𝜋^0}_{dAu,EXP}$ is consistent with the MB value within 5% uncertainty. This result confirms that the previously observed enhancement of high-𝑝 𝑇 𝜋 0 production found in small-system collisions with low event activity is a result of a bias in interpreting event activity within the Glauber framework. In contrast, for the top 5% of events with the highest event activity, 𝑅$^{𝜋^0}_{dAu,EXP}$ is suppressed by 20% relative to the MB value with a significance of 4.5𝜎, which may be due to final-state effects. This suppression corresponds to a 𝑝 𝑇 shift of 𝛿𝑝 𝑇 = 0.213 ± 0.055 Gev/𝑐 at 9 Gev/𝑐.
Templates of expected measurement uncertainties for neutron-induced capture and charged-particle production cross section observables
This paper provides a template of expected uncertainties and correlations for measurements of neutron-induced capture and charged-particle production cross sections. Measurements performed in-beam include total absorption spectroscopy, total energy detection, γ -ray spectroscopy, and direct charged-particle detection. Offline measurements include activation analysis and accelerator mass spectrometry. The information needed for proper use of the datasets in resonance region and high energy region evaluations is described, and recommended uncertainties are provided when specific values are not available for a dataset.
A parallel-plate avalanche counter for the prompt fission neutron spectrum measurement
Neutrons, gamma’s, and fission fragments are among the prompt fission observables. Their precision measurements are fundamental to advance our understanding of fission and any application of fission. For our programmatic need, the χ matrix, which defines as the outgoing neutron spectrum as a function of incoming neutron energy, is sparsely populated and poorly measured for 233,235,238 U and 239,240 Pu. To improve the quality of those χ matrices, a joint LANLLLNL project was undertaken to measure their prompt fission neutron spectra at the LANSCE/WNR facility using neutron detector arrays and a charged-particle detector for the fission-fragment detection. A typical setup is shown in Fig. 1, where one of neutron detector array with a charged-particle detector is given.
Alpha/beta-gated gamma–gamma spectroscopy of mixed fission products for trace analysis
This experiment demonstrated that some hard-to-detect fission products can be quantified directly from mixed fission product samples using advanced radio-emission spectroscopy techniques. A gamma/gamma coincidence detector was combined with a custom liquid scintillation counter to evaluate the benefits of alpha and beta coincident and anti-coincident analysis of mixed fission product samples. Reduction factors in the minimum detectable activity (MDA) relative to traditional gamma counting were quantified for a set of radionuclides. For isotopes like 91Y, 144Ce, 147Nd, and 153Sm MDA reductions of factors of 1-2 were observed using optimized beta thresholds. Using beta anti-coincidence counting reductions of factors 3-5 were observed for isotopes like 89Sr, 95mNb, 115Cd, and 137Cs and factors of 5-7 for isotopes like 235U using alpha coincidence counting. The selectivity of gamma/gamma coincidence and reduction in backgrounds using beta gating were also demonstrated with 136Cs and 153Sm. The improvements observed in the detection sensitivity of fission products and actinides achieved by combining time-correlated radiation signatures is significant and of value to applications such as nuclear fission physics, environmental monitoring for nuclear waste, reactor accidental releases, and nuclear forensics.
Two bright, optically clear, intrinsic fast-neutron and charged-particle detector materials for neutron imaging and other applications
Two optically clear, bright, scintillating ZnS materials have been identified that, like previous opaque ZnS scintillators, are excellent charged particle detectors. We show that ZnS is a good fast-neutron-to charged-particle converter making optically clear ZnS an intrinsic fast-neutron detector that does not require layering or mixing of converter materials and scintillator materials, and removes the limitations imposed by opaque ZnS scintillator materials used for more than a century. Thermal neutron detection using optically clear 6 LiF or 10 BN and clear ZnS may benefit from improved spatial resolution and light transmission. Properties and tests of clear scintillating ZnS are described. Fast-neutron imaging applications benefit from increased efficiency of these scintillators, minimal scattering in the scintillator, and increased useful detector volume. Charged particle and fast-neutron detectors have numerous applications in nuclear non-proliferation and security, nuclear and particle physics, and non-destructive testing and environmental measurements.
Understanding hadronic interactions using advanced reconstruction techniques
ProtoDUNE-SP served as the prototype of the future Deep Underground Neutrino Experiment (DUNE). With a total liquid argon mass of 0.77 kt, it stood as the most extensive monolithic single-phase Liquid Argon Time Projection Chamber (LArTPC) ever constructed. Strategically located and operated at CERN, ProtoDUNE-SP benefited from a specialized charged-particle test beam, offering a momentum range of 0.3 - 7 GeV/c. This setup provided a unique opportunity to conduct in-depth studies on hadronic interactions within argon. Hadronic interactions play a fundamental role in neutrino physics, particularly in the intricacies of neutrino detection. We depend on analyzing the outcomes of these interactions to accurately determine both the flavor and energy of the interacting neutrinos. Pions, as one of the primary byproducts of neutrino interactions, are crucial for understanding the overall dynamics and kinematics of these processes. Accurately characterizing and understanding the interaction of pions with argon can significantly enhance the precision of neutrino simulations and measurements.Being a Liquid Argon Time Projection Chamber (LArTPC), ProtoDUNE-SP is distinguished by its ability to produce high-definition images of charged particles as they traverse through the detector's active volume. Yet, accurately reconstructing these particle interactions and determining their kinematic attributes remains a challenging task. The successes of deep learning in diverse domains, especially in image recognition, provide a promising approach for addressing this challenge in ProtoDUNE. This thesis discusses a measurement of the Piplus - argon inelastic cross section in the energy range of 2400 to 3000 MeV, using data taken by protoDUNE during the fall of 2018. Additionally, panoptic segmentation, a machine learning technique, is introduced and validated through its application in the reconstruction of the neutral pion rest mass. The aim is to showcase how these advanced methods can enhance the quality of event reconstruction.
Fast-neutron response of LaBr 3 (Ce) and LaCl 3 (Ce) scintillators
The response of LaBr 3 (Ce) and LaCl 3 (Ce) scintillators to fast neutrons is investigated. Neutron-induced charged-particle reactions are observed in both materials when exposed to the fast neutrons produced by an AmBe source, with pulse-shape discrimination used to separate channels. LaBr 3 (Ce) is found to have the best separation between reaction channels, while LaCl 3 (Ce) has a significantly higher efficiency.
Level Structure of {sup 31}S Via {sup 32}S({ital p,d}) {sup 31}S
Background: Properties of proton-unbound S-31 states determine the P-30(p, gamma) S-31 reaction rate, which has a significant impact on explosive hydrogen burning in classical novae and type-I x-ray bursts. Despite several previous studies, uncertainties still remain with respect to the nuclear structure of S-31 near the proton threshold. Purpose: The level structure of S-31 has been presently investigated via a charged-particle spectroscopy experiment using the S-32(p, d) S-31 reaction. Method: Deuterons corresponding to S-31 excited states with 3.285 <= E-x <= 10.8 MeV were momentum analyzed via an Enge split-pole spectrograph at six laboratory angles between 10 degrees and 62 degrees. Differential cross sections of the S-32(p, d)S-31 reaction were measured at E-p = 34.5 MeV. Distorted-wave Born approximation calculations were performed to constrain the spin-parity assignments of several of the observed levels. Results: We have detected 72 excited states of S-31, out of which 17 are within the astrophysical region of interest corresponding to the temperature range of 0.1-1.5 GK. We have resolved the discrepancy in the spin and parity of an excited state with E-x = 6542 keV, showing that is it not J(pi) = 3/2(-), and therefore the contribution of this state to the P-30(p, gamma) reaction rate is likely much less significant than previously thought owing to the larger angular-momentum transfer required to populate this excited state. Moreover, our measurement results help consolidate the spin-parity assignments for the 6377 and 6636 keV states in S-31. Conclusions: This work presents the most comprehensive spin-parity assignments to date from a single-neutron transfer reaction on S-32 to S-31 excited states in the region between 6 to 7 MeV excitation energy. This region is significant for the determination of the P-30(p, gamma)S-30 reaction rate over the temperatures characteristic of explosive hydrogen burning in novae.
Source characterization of a detector for heavy and superheavy nuclei
A new focal plane detector system for the Berkeley Gas-filled Separator (BGS) was designed, constructed, and tested offline with various α-decay and conversion-electron sources. The SuperHeavy RECoils (SHREC) detector comprises sets of double-sided silicon strip detectors arranged in an open-faced cuboid geometry. Alongside the detector upgrade new digital data acquisition electronics have been commissioned offline. This setup aims to detect separated recoiling heavy and superheavy nuclei as well as their correlated radioactive decay paths with improved energy resolution and overall sensitivity.
Low Energy Neutron-induced Charged-particle (Z) (LENZ) instrument development with a focus on pulse shape discrimination for low-energy charged particles
To study neutron-induced charged-particle reactions with high precision, the Low Energy Neutron-induced Charged-particle (Z) instrument (LENZ) was developed at the Los Alamos Neutron Science Center. For the interest of measuring (n,p) and (n, α) reactions simultaneously, Pulse Shape Discrimination methods were investigated to identify different charged particles in the energy range of 3 - 20 MeV and improve signal-to-background ratios using Double-sided Silicon Strip Detectors and waveform digitizers. The risetime and pulse shape properties of detected charged particles were characterized for various silicon detector’s thickness with different orientations. During the post-processing of waveforms, we implemented different digital filters for effective particle identifications and improved energy- and timing- resolutions. We validated the optimized digital filters and pulse shape analyses, via measurements with 228 Th and 229 Th calibration sources, proton-induced reactions on a 7 LiF target, and neutron-induced reactions on CH 2 , Ta 2 O 5 , 58 Ni, and 6 LiF/ 59 Ni targets at the time-of-flight facility, LANSCE. In conclusion, the summary of effective thresholds and Figure of Merits on separating different charged particles is reported.
Augmented signal processing in Liquid Argon Time Projection Chambers with a deep neural network
The Liquid Argon Time Projection Chamber (LArTPC) is an advanced neutrino detector technology widely used in recent and upcoming accelerator neutrino experiments. It features a low energy threshold and high spatial resolution that allow for comprehensive reconstruction of event topologies. In current-generation LArTPCs, the recorded data consist of digitized waveforms on wires produced by induced signal on wires of drifting ionization electrons, which can also be viewed as two-dimensional (2D) (time versus wire) projection images of charged-particle trajectories. For such an imaging detector, one critical step is the signal processing that reconstructs the original charge projections from the recorded 2D images. For the first time, we introduce a deep neural network in LArTPC signal processing to improve the signal region of interest detection. By combining domain knowledge (e.g., matching information from multiple wire planes) and deep learning, this method shows significant improvements over traditional methods. This work details the method, software tools, and performance evaluated with realistic detector simulations.
Critical thermonuclear reactions in classical novae and type I X-ray bursts
The goal of this project was to experimentally constrain the nuclear reaction rates whose uncertainties have the largest impact on models of classical novae and Type-I X-ray bursts. These astrophysical events occur when a white dwarf or neutron star, respectively, accretes hydrogen and helium from a companion star until a thermonuclear runaway ensues. The primary reactions of interest to this project for novae and X-ray bursts are 30 P(ρ,γ) 31 S and 15 O(α,γ) 19 Ne. The project methodology was to develop a new radiation detection system in two phases to measure the low-energy beta-delayed particle emissions of 31 Cl and 20 Mg at the National Superconducting Cyclotron Laboratory (NSCL) in order to constrain these two reaction rates. In particular, a gas-filled charged-particle detector was to be designed, constructed and operated, in concert with the SeGA array.
PIXE – State of the Art, Systems, Challenges
Particle-induced X-ray emission (PIXE) is an analytical technique for elemental analysis in which a charged-particle beam (most commonly protons, but also alpha particles or heavier ions) ionizes inner-shell electrons in target atoms. When these vacancies are filled by outer-shell electrons, the atom emits characteristic X-rays (e.g., Kα, Kβ, L-series) whose energies are unique to each element. Measuring the X-ray spectrum therefore enables identification of the elements present and, with appropriate calibration and modeling, their concentration. PIXE provides rapid, simultaneous, quantitative multi-element detection with trace-level sensitivity for many mid- to high-Z elements, often with minimal sample preparation. It is widely used across materials science (thin films, alloys, corrosion), geology (mineral chemistry, provenance) and environmental monitoring (aerosols, particulates, soils); semiconductor contamination analysis (wafer surface/trace metals), cultural heritage (pigments, inks, archaeological artifacts) and forensics (gunshot residue, glass/pain), and biological/medical studies (tissue/biomaterial trace-element mapping).