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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Impact of dynamical chiral symmetry breaking and dynamical diquark correlations on proton generalized parton distributions

We calculate the leading-twist, helicity-independent generalized parton distributions (GPDs) of the proton, at finite skewness, in the Nambu–Jona-Lasinio (NJL) model of quantum chomodynamics (QCD). The NJL model reproduces low-energy characteristics of QCD, including dynamical chiral symmetry breaking (DCSB). The proton bound-state amplitude is solved for using the Faddeev equation in a quark-diquark approximation, including both dynamical scalar and axial vector diquarks. GPDs are calculated using a dressed non-local correlator, consistent with DCSB, which is obtained by solving a Bethe-Salpeter equation. The model and approximations used observe Lorentz covariance, and as a consequence the GPDs obey polynomiality sum rules. Extractions of electromagnetic and gravitational form factors are performed. We find a D-term of -1.08 when the non-local correlator is properly dressed, and 0.85 when the bare correlator is used instead, suggesting that within this framework proton stability requires the constituent quarks to be dressed consistently with DCSB. In conclusion, we also find that the anomalous gravitomagnetic moment vanishes, as required by Poincare symmetry.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

High-quality axion from exact SUSY chiral dynamics

We use supersymmetric chiral dynamics perturbed by anomaly-mediated supersymmetry breaking to obtain a high-quality, composite axion that solves the strong problem. The strong dynamics arises from a supersymmetric SU(10) chiral gauge theory with massless matter chiral superfields. This leads to a stable, nonsupersymmetric vacuum, calculated exactly, where a spontaneously broken global symmetry, identified with the Peccei-Quinn (PQ) symmetry, gives rise to a composite QCD axion. The chiral gauge theory also admits a discrete (or ) gauge symmetry that forbids PQ-violating operators up to dimension eight. An extension to an chiral gauge theory incorporates grand unification where the unification scale is identified with the PQ-breaking scale and PQ-violating operators are forbidden up to dimension 20. The supersymmetry breaking scale, near 100 TeV, ameliorates the Higgs hierarchy problem, while colored Nambu–Goldstone bosons may be detected at future colliders via decays to gluons or form heavy isotopes.

Gherghetta, Tony↗
DOE OSTI2024

Real-time chiral dynamics at finite temperature from quantum simulation

In this study, we explore the real-time dynamics of the chiral magnetic effect (CME) at a finite temperature in the (1+1)-dimensional QED, the massive Schwinger model. By introducing a chiral chemical potential μ 5 through a quench process, we drive the system out of equilibrium and analyze the induced vector currents and their evolution over time. The Hamiltonian is modified to include the time-dependent chiral chemical potential, thus allowing the investigation of the CME within a quantum computing framework. We employ the quantum imaginary time evolution (QITE) algorithm to study the thermal states, and utilize the Suzuki-Trotter decomposition for the real-time evolution. This study provides insights into the quantum simulation capabilities for modeling the CME and offers a pathway for studying chiral dynamics in low-dimensional quantum field theories.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Ninth International Workshop on Chiral Dynamics, 2018

The Ninth International Workshop on Chiral Dynamics (CD18) was hosted by the Triangle Universities Nuclear Laboratory (TUNL) and held on the campus of Duke University in Durham, NC. The workshop was from September 17 th to 21 st , 2018. This series of workshops, which started at MIT in 1994, brings together theorists and experimentalists every three years to discuss the status and challenges in the physics of low-energy quantum chromodynamics (QCD), Goldstone Boson dynamics, meson-baryon interactions, few-body physics, lattice QCD and Chiral Perturbation Theory. The last workshop was jointly hosted by the Department of Physics of the University of Pisa and the Pisa branch of the Istituto Nazionale di Fisica Nucleare in July 2015. Previous hosts of the workshop include MIT in 1994, the University of Mainz in 1997, Jefferson Lab in 2000 and 2012, the University of Bonn in 2003, TUNL and Duke University in 2006, and the University of Bern in 2009. Hosting this workshop is an important and substantial service to the international low-energy QCD physics community. Nearly 120 participants attended the workshop, which delivered twenty plenary talks, and over ninety parallel presentations. Proceedings of the workshop are published in Proceedings of Science at https://pos.sissa.it/317/. These proceedings present topics convened in this 9 th workshop and provide a comprehensive review of the field, highlighting recent accomplishments and discussing challenges that will motivate research in the coming years.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Dynamically Chiral Expanded Helicenes

Expanded helicenes are a class of chiral nanographenes with a screw-shaped skeleton and a larger diameter than their classical ortho-fused counterparts. The flexibility of this internal cavity results in helicenes that are often difficult to isolate as single enantiomers. Expanded helicenes are therefore an intriguing target for exploration of dynamic chirality, a phenomenon resulting from introduction of chiral auxiliaries to control structure in a racemic system. This contribution describes installation of chiral amine substituents into the cavity of a diformyl expanded [11]-helicene by mild, efficient, and reversible imine condensations. The resulting helicenes display strong molar circular dichroism up to |Δε| = 300 M -1 cm -1 and absorption dissymmetry factors of |g abs | = 0.010. The magnitude of circular dichroism can be varied by using different chiral amine substituents, which is correlated to the diastereomeric ratios of the helicenes. In conclusion, this is the first instance of dynamic chirality being used to observe a chiroptic response in expanded helicenes and is a significant synthetic improvement over methods which require conventional enantiomer resolution.

Rothenberger, August J. [University of California,↗
DOE OSTI2024

Lattice QED in an external magnetic field: Evidence for dynamical chiral symmetry breaking

We simulate quantum electrodynamics (QED) in a strong constant homogeneous external magnetic field on a Euclidean space-time lattice using the rational hybrid Monte Carlo method, developed for simulating lattice quantum chromodynamics (QCD). Our primary goal is to measure the chiral condensate in the limit when the input electron mass m is zero. We observe a nonzero value, indicating that the external magnetic field catalyzes chiral symmetry breaking as predicted by approximate truncated Schwinger-Dyson methods. Such behavior is associated with dominance by the lowest Landau level which causes the effective dimensional reduction from 3 + 1 dimensions to 1 + 1 dimensions for charged particles (electrons and positrons) where the attractive forces of QED can produce chiral symmetry breaking with a dynamical electron mass and associated chiral condensate. Since our lattice simulations use bare (lattice) parameters, while the Schwinger-Dyson analyses work with renormalized quantities, direct numerical comparison will require renormalization of our lattice results. Published by the American Physical Society 2024

Kogut, J. B. (ORCID:000000030151548X)↗
DOE OSTI2021

Crystalline Supramolecular Polymers: Dynamics, Chirality, and Function

Inspired by biological systems, supramolecular polymers have emerged over the past three decades as an important way to form functional structures with potential to tune the internal order and dynamics and to create materials with the potential for responsiveness, reconfigurability, and recyclability. We focus here on several recent examples of ordered supramolecular polymers with a significant extent of internal order that results in crystalline molecular packing, or with dynamics that allow them to undergo structural reconfiguration. These examples highlight the spectrum of molecular mobility that the noncovalently bound constituents can experience. Furthermore, these materials have found interesting functions in their interaction with chiral biological systems and in their ability to form materials with interesting optoelectronic and photocatalytic behavior.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Quantum‐Classical Simulation of Quantum Field Theory by Quantum Circuit Learning

Abstract Quantum circuit learning is employed to simulate quantum field theories (QFTs). Typically, when simulating QFTs with quantum computers, significant challenges are encountered due to the technical limitations of quantum devices when implementing the Hamiltonian using Pauli spin matrices. To address this challenge, quantum circuit learning is leveraged, employing a compact configuration of qubits and low‐depth quantum circuits to predict real‐time dynamics in quantum field theories. The key advantage of this approach is that a single‐qubit measurement can accurately forecast various physical parameters, including fully‐connected operators. To demonstrate the effectiveness of this method, it is used to predict quench dynamics, chiral dynamics and jet production in a 1+1‐dimensional model of quantum electrodynamics. It is found that our predictions closely align with the results of rigorous classical calculations, exhibiting a high degree of accuracy. This hybrid quantum‐classical approach illustrates the feasibility of efficiently simulating large‐scale QFTs on cutting‐edge quantum devices.

Ikeda, Kazuki [Department of Physics University of↗
DOE OSTI2025

Attosecond control and measurement of chiral photoionization dynamics

Many chirality-sensitive light–matter interactions are governed by chiral electron dynamics. Therefore, the development of advanced technologies making use of chiral phenomena would critically benefit from measuring and controlling chiral electron dynamics on their natural attosecond timescales. Such endeavours have so far been hampered by the lack of characterized circularly polarized attosecond pulses, an obstacle that has recently been overcome. Here we introduce chiroptical spectroscopy with attosecond pulses and demonstrate attosecond coherent control over photoelectron circular dichroism (PECD), as well as the measurement of chiral asymmetries in the forward–backward and angle-resolved photoionization delays of chiral molecules. We show that co-rotating attosecond and near-infrared (IR) pulses can nearly double the PECD and even change its sign compared with single-photon ionization. We demonstrate that chiral photoionization delays depend on both polar and azimuthal angles of photoemission in the light-propagation frame, requiring 3D momentum resolution. We measure forward–backward chiral-sensitive delays of up to 60 as and polar-angle-resolved photoionization delays of up to 240 as, which include an asymmetry of about 60 as originating from chirality in the continuum–continuum transitions. Attosecond chiroptical spectroscopy opens the door to quantitatively understanding and controlling the dynamics of chiral molecules on the electronic timescale.

Atomic and molecular interactions with photons↗
DOE OSTI2022

Pump-probe spectroscopy of chiral vibrational dynamics

A planar molecule may become chiral upon excitation of an out-of-plane vibration, changing its handedness during half a vibrational period. When exciting such a vibration in an ensemble of randomly oriented molecules with an infrared laser, half of the molecules will undergo the vibration phase-shifted by π compared to the other half, and no net chiral signal is observed. This symmetry can be broken by exciting the vibrational motion with a Raman transition in the presence of a static electric field. Subsequent ionization of the vibrating molecules by an extreme ultraviolet pulse probes the time-dependent net handedness via the photoelectron circular dichroism. Our proposal for pump-probe spectroscopy of molecular chirality, based on quantum-chemical theory and discussed for the example of the carbonyl chlorofluoride molecule, is feasible with current experimental technology.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Nambu and Compositeness

The Nambu--Jona-Lasinio model is the simplest field theory of a composite scalar boson, consisting of a pair of chiral fermions. A bound state emerges from an assumed point-like 4-fermion interaction and is described by local effective field, $\Phi(x)$. We review this in the context of the renormalization group and show some its phenomenological successes, such as the QCD chiral dynamics and the prediction of stable heavy-light resonances that reveal the single light quark chiral dynamics. We also review some NJL--inspired composite Higgs models. We then describe a novel UV completion of the NJL model, to an extended interaction, where the solution is described by a bilocal effective, Yukawa field, $\Phi(x,y)$. I conclude with a personal recollection of Yoichiro Nambu.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Observation of Topological Chirality Switching Induced Freezing of a Skyrmion Crystal

Magnetic skyrmions are topologically protected quasi-particles with a well-defined chirality. Control over their chirality is proposed as an additional feature for encoding data bits or as qubits in quantum computing due to their high efficiency and stability against achiral magnetic textures. Here it is shown that an in-plane magnetic field can be utilized to reshape the energy barriers between different skyrmionic bubbles (e.g., Bloch type, type-II) enabling spontaneous chirality fluctuations with a frequency that increases with the strength of the in-plane field. The insulating van der Waals ferromagnet CrBr3 is used as an archetypal system for low damping, reduced energy dissipation and a high number of magnetic phases to capture the chirality dynamics in real time through cryo-Lorentz transmission electron microscopy. It is observed that the interplay between the intrinsic Dzyaloshinskii–Moriya interaction and out-of-plane field biased the chirality dynamics, favoring one handedness over the other. A remarkable consequence of the spontaneous chirality switching mechanism is that it induces a freezing (or crystallization) process in the skyrmion lattice. As the bubbles fluctuate between Bloch and type-II they elongate and shrink parallel to the in-plane field. Subsequently, the overall lattice crystallizes along the in-plane field direction, inducing a phase transition from a disordered liquid state to a hexatic phase where skyrmions are highly ordered resembling that of a solid. The results indicate chirality as an active element in the creation of topologically protected skyrmion crystals unveiling pathways toward chiral spintronic device platforms with tunable embedded configuration.

2D Phase Transition↗
DOE OSTI2020

Ultrafast photoinduced band splitting and carrier dynamics in chiral tellurium nanosheets

Trigonal tellurium (Te) is a chiral semiconductor that lacks both mirror and inversion symmetries, resulting in complex band structures with Weyl crossings and unique spin textures. Detailed time-resolved polarized reflectance spectroscopy is used to investigate its band structure and carrier dynamics. The polarized transient spectra reveal optical transitions between the uppermost spin-split H4 and H5 and the degenerate H6 valence bands (VB) and the lowest degenerate H6 conduction band (CB) as well as a higher energy transition at the Lpoint. Surprisingly, the degeneracy of the H6 CB (a proposed Weyl node) is lifted and the spin-split VB gap is reduced upon photoexcitation before relaxing to equilibrium as the carriers decay. Using ab initio density functional theory (DFT) calculations, we conclude that the dynamic band structure is caused by a photoinduced shear strain in the Te film that breaks the screw symmetry of the crystal. The band-edge anisotropy is also reflected in the hot carrier decay rate, which is a factor of two slower along the c-axis than perpendicular to it. The majority of photoexcited carriers near the band-edge are seen to recombine within 30 ps while higher lying transitions observed near 1.2 eV appear to have substantially longer lifetimes, potentially due to contributions of intervalley processes in the recombination rate. These new findings shed light on the strong correlation between photoinduced carriers and electronic structure in anisotropic crystals, which opens a potential pathway for designing novel Te-based devices that take advantage of the topological structures as well as strong spin-related properties.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗