Emulating Daytime ABI Cloud Optical Properties at Night With Machine Learning
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White, Charles H.↗
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Evaluation of cloud height, optical thickness, and phase retrievals from the CHROMA algorithm applied to Sentinel-3 OLCI data
We previously developed the Cloud Height Retrieval from O 2 Molecular Absorption (CHROMA) algorithm for the Ocean Color Instrument (OCI) on the new NASA Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission. Here, we apply CHROMA to observations from the Ocean Land Colour Instrument (OLCI) to guide expectations for PACE, as it will take some time to obtain large-scale validation data for OCI. We use cloud top height (CTH), phase, and (for liquid clouds) cloud optical thickness (COT) data from the ground-based Atmospheric Radiation Measurement (ARM) network to evaluate the OLCI retrievals. We found that OLCI and Moderate Resolution Imaging Spectroradiometer (MODIS) CTH compare similarly well to the ARM reference. OLCI has a tendency to underestimate CTH as CTH increases, and algorithm assumptions about cloud geometric thickness may contribute to this. ARM COT from multifilter shadowband radiometers (MFRSR) and Sun photometers are well-correlated with one another, albeit with a roughly 30 % offset on average; OLCI and MODIS COT agree more closely with the MFRSR data. OLCI retrieval uncertainty estimates show skill at telling low-uncertainty cases from high-uncertainty ones, although CTH uncertainties are underestimated. Additionally, we compare the OLCI data to satellite retrievals based on thermal infrared measurements from MODIS and Sea and Land Surface Temperature Radiometer (SLSTR) data. Differences are broadly consistent with physical expectations based on the A-band vs. thermal techniques, although one key challenge in such aggregated comparisons is different cloud masking sensitivities and algorithm failure rates meaning additional sampling differences are introduced. We conclude by discussing the transition to and possible enhancements for PACE OCI.
Sayer, Andrew M. [Univ. of Maryland Baltimore Coun↗
Evaluating Mean State Cloud Properties in the Simple Cloud‐Resolving E3SM Atmosphere Model (SCREAM)
Accurately simulating clouds remains a key challenge in global climate models, primarily because cloud formation involves sub-grid processes that are parameterized and crudely represented in models. This study examines the performance of DOE's Simple Cloud-Resolving Energy Exascale Earth System (E3SM) Atmosphere Model (SCREAM) in simulating cloud properties and their spatio-temporal distribution by comparing against satellite observations. Two horizontal resolutions of SCREAM (3 and 12 km) are examined, and both depict a realistic spatial structure of mean-state cloud cover but underestimate its global mean magnitude. SCREAM 3 km reasonably reproduces the distribution of mean-state cloud properties across various cloud optical thickness and cloud-top pressure regimes, with performance comparable to CMIP5 and CMIP6 ensemble and marginally outperforming SCREAM 12 km. Still, SCREAM 3 km tends to underpredict low clouds and optically thin clouds, highlighting the need for continued improvement in representing unresolved processes. This study provides a basis for confidence in the representation of clouds in SCREAM, as simulating mean-state clouds is a necessary prerequisite for trusting its cloud responses to changes in aerosols and greenhouse gases.
Geosciences↗
Long-Term Trends in Aerosols, Low Clouds, and Large-Scale Meteorology Over the Western North Atlantic From 2003 to 2020
Here, a continuous decrease in aerosols over the Western North Atlantic Ocean (WNAO) on a decadal timescale provides a long-term benchmark to evaluate how various natural and anthropogenic processes affect the manifestation of aerosol-cloud interactions in this region. Furthermore, the WNAO serves as a natural laboratory with diverse aerosol sources, marine boundary layer clouds more variable than those in marine stratocumulus deck regions, and unique flow regimes established by the Gulf Stream and the semi-permanent Bermuda High. We investigate how satellite-retrieved macrophysical and microphysical properties of low clouds and the surface shortwave irradiance changed from 2003 to 2020, in tandem with this aerosol decrease. The decadal changes in large-scale meteorology related to the North Atlantic Oscillation (NAO) are also examined. We find a reduction in low-cloud optical thickness, accompanied by fewer and larger cloud droplets, yet observe no significant changes in low-cloud fraction and liquid water path. Despite the reduction in low-cloud optical thickness together with aerosol decrease, a corresponding increase in the trends of surface shortwave irradiance, also known as surface brightening, is lacking. This absence of brightening is potentially related to concomitant changes found in large-scale meteorology associated with NAO—Bermuda High strengthening, sea surface warming, and atmospheric moistening— as well as an increase in high-level cloud fraction that can counteract the surface brightening. Ultimately, our findings suggest that spatial patterns of decadal meteorological variability introduce complexities in the surface cloud radiative effect over the WNAO, thereby complicating the isolation and examination of aerosol-cloud interactions.
54 ENVIRONMENTAL SCIENCES↗
A Concept of a Convection–Cloud Chamber to Study Aerosol–Cloud–Drizzle Interactions
Understanding and quantifying the full chain of processes from aerosol activation to drizzle formation, and the associated feedbacks to the aerosol chemical and physical properties, all within a turbulent cloud are some of the toughest challenges in atmospheric chemistry and physics and are keys to the cloud–precipitation puzzle. This paper describes a concept for a new type of research facility consisting of a cloud chamber plus associated instrumentation and computational models, to explore aerosol–cloud interactions and processing, cloud optical properties, entrainment–cloud interactions, and quantitative assessment of drizzle onset. The envisioned design is for a 3 m × 3 m × 9 m chamber, such that the height is sufficient to achieve long lifetimes for aerosol processing and for significant drizzle growth by collision and coalescence. A suite of computational tools for simulating microphysical properties in the chamber provides a digital twin for designing the chamber and a range of example experiments. Theory and test results from novel remote sensing systems for exploring chemical and physical interactions and evolution of aerosols, cloud droplets, and drizzle within turbulent clouds are described. Testing of technology needed for the operation of a large-volume chamber, including aerosol generation methods and novel materials for water vapor boundary conditions, is described. Simulations suggest that spatially uniform turbulence and microphysical properties can be sustained in a steady state, with reasonable aerosol and water vapor fluxes, and that substantial drizzle can be produced through collision and coalescence of cloud droplets. Remaining challenges for more detailed engineering design and a discussion of possible first-light experiments are described.
54 ENVIRONMENTAL SCIENCES↗
Field Validation of Cloud Properties Sensor Field Campaign Report
The purpose of this campaign is to deploy Aerodyne Research Inc.’s extended wavelength cloud optical properties sensor (TWST-EN) in an operationally relevant environment with co-located, validated sensors. The Atmospheric Radiation Measurement (ARM) user facility’s Southern Great Plains (SGP) observatory is ideal for this deployment because of the variety of operational sensors that can measure some of the same cloud properties using different modalities. While cloud property sensors have long existed, they tend to be costly to produce and maintain. Our sensor measures absolute spectral radiance in the two bands and will retrieve cloud optical depth (COD), droplet effective radius, and thermodynamic phase. Our prototype is built predominantly from off-the-shelf components and uses uncooled spectrometers. A lower-cost, easy-to-use sensor such as this could allow deployment at many more sites for greater spatial coverage. Analysis and retrieval algorithm development using the data from this deployment has been a central technical objective of our U.S. Department of Energy Small Business Innovative Research (SBIR) Phase 2 contract (DE-SC0020473: Low-Cost Shortwave Spectroradiometer for Retrieval of Cloud Properties).
54 ENVIRONMENTAL SCIENCES↗
Assessing Clouds in GFDL's AM4.0 With Different Microphysical Parameterizations Using the Satellite Simulator Package COSP
We evaluate cloud simulations using satellite simulators against multiple observational data sets. These simulators have been run within the Geophysical Fluid Dynamics Laboratory's Atmosphere Model version 4.0 (AM4.0), as well as an alternative configuration where a fully two‐moment Morrison‐Gettelman cloud microphysical parameterization with prognostic precipitation (MG2) is applied, denoted as AM4‐MG2. The modeled cloud spatial distributions, vertical profiles, phase partitioning, cloud‐to‐precipitation transitions, and radiative effects compare reasonably well with satellite observations. Model biases include the under‐prediction of total and low‐level clouds, especially optically thin/intermediate clouds with cloud optical depth of less than 23, but the over‐prediction of thick clouds, indicating “too few, too bright” biases. These biases counteract each other, and give rise to reasonable estimates of cloud radiative effects. The underestimate of low‐level clouds is associated with too early and too frequent drizzle/precipitation formation. The precipitation bias is improved in AM4‐MG2, where the autoconversion scheme initiates the precipitation more realistically. There also exist discrepancies between models and observations for midlevel and high‐level clouds. Additional biases include the underestimate of liquid cloud fraction and the overestimate of ice cloud fraction.
54 ENVIRONMENTAL SCIENCES↗
Marine and continental stratocumulus cloud microphysical properties obtained from routine ARM Cimel sunphotometer observations
This study investigates marine and continental stratocumulus (Sc) cloud properties obtained from an automated implementation of a multispectral photometer retrieval. Photometer methods simultaneously retrieve cloud optical depth (τ) and cloud droplet effective radius (r e ), with estimates for liquid water path (LWP) calculated on the availability of those quantities. These applied methods evaluate retrieved cloud properties for Sc identified during a recent 6 year period over the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program sites in Oklahoma, USA (SGP) and in the Azores, Portugal (ENA). Modest agreement in key quantity retrievals is found between the routine photometer products and multisensor collocated profiling references. Cumulative breakdowns contingent on cloud thickness indicate increases in all retrieved quantities in thicker clouds, with larger discrepancies in the relative performance between the retrievals collected in the presence of drizzle. Under continental cloud conditions, the clouds of a similar thickness and r e to those sampled under marine conditions report a factor of 1.5 larger τ and LWP. An r 2 ≅0.65 is found between photometer τ retrievals and shadowband radiometer measurements, with photometer retrievals reporting a high (relative) bias. The τ intercomparisons indicate that variability between retrievals is a factor of three larger than errors reported from individual retrieval input perturbation tests. Photometer r e retrievals suggest a low r 2 (< 0.1) having a standard deviation ≅ 3 µm when compared to ARM baseline multi-sensor radar/radiometer references (accounting for offsets in the cloud droplet number concentration assumptions of the latter). However, photometer LWP calculations remain relatively unbiased in non-drizzling conditions, with errors O (50 g m −2 ) and r 2 ≅0.5 to collocated radiometer and interferometer references. Additional sensitivity tests for island influences on marine Sc properties suggest that while island-influenced winds may promote larger cloud LWP or thickness, the influence could be within retrieval method uncertainty and/or collocated instrument variability.
54 ENVIRONMENTAL SCIENCES↗
Constraining dark matter-proton scattering from molecular cloud ionization
Optically dense clouds in the interstellar medium composed predominantly of molecular hydrogen, known as molecular clouds, are sensitive to energy injection in the form of photon absorption, cosmic-ray scattering, and dark matter (DM) scattering. The ionization rates in dense molecular clouds are heavily constrained by observations of abundances of various molecular tracers. Recent studies have set constraints on the DM-electron scattering cross section using measurements of ionization rates in dense molecular clouds. Here we calculate the analogous bounds on the DM-proton cross section using the molecular Migdal effect, recently adapted from the neutron scattering literature to the DM context. These bounds may be the strongest limits on a strongly coupled DM subfraction, and represent the first application of the Migdal effect to astrophysical systems. Published by the American Physical Society 2024
Astronomy & Astrophysics↗
Three-Channel Sunphotometer Cloud Mode Value-Added Product Report
A primary source of uncertainty in Earth system model (ESM) predictions is the representation of cloud processes and associated cloud feedback. Several fundamental cloud properties critical to the understanding of aerosol-cloud interactions are poorly constrained by observations, with key deficiencies in our observations of cloud and precipitation droplet sizes and cloud optical depth. Observations of these cloud properties are often challenging to estimate from remote-sensing platforms and costly to obtain from in situ aircraft. Nevertheless, observations of boundary-layer clouds, and improved knowledge of stratocumulus cloud (Sc) processes, are especially important to ESM advancement. This is because these clouds have extensive coverage and exert controls on boundary-layer dynamics and the global radiative energy balance.
54 ENVIRONMENTAL SCIENCES↗
Implementation and Evaluation of Physics-Driven Dynamic Entrainment-Mixing Parameterization in a Climate Model and Its Impact on Low-Cloud Simulation
The turbulent entrainment-mixing process in the Community Earth System Model version 1.2 (CESM1.2) is assumed to follow the extremely inhomogeneous entrainment-mixing. However, different entrainment-mixing scenarios can occur in real clouds. To address this deficiency, a unifying parameterization that represents different entrainment-mixing processes is implemented and evaluated in CESM1.2. The results indicate that the homogeneous mixing degree values simulated by the new parameterization in CESM1.2 are predominantly greater than 50%, suggesting a tendency toward homogeneous mixing. Compared to the extremely inhomogeneous mixing mechanism, the new parameterization increases the cloud droplet number concentration (Nc). More importantly, the new parameterization improves low-cloud fraction (CLDLOW) simulation in Northwest Pacific (NWP) and Southeast Pacific (SEP) regions, with relative improvements of 2.95% and 4.17%, respectively. Furthermore, the improvements reach up to 44.6% and 16.2% in the NWP and SEP regions, respectively, when considering the relationship between N c and CLDLOW. Further analysis reveals that the new parameterization enhances cloud optical depth, longwave radiative cooling effect, net condensation rate, cloud water mixing ratio, lower-troposphere stability, and CLDLOW by increasing N c . Additionally, these results underscore the importance of improving entrainment-mixing parameterization in climate models.
54 ENVIRONMENTAL SCIENCES↗
Can We Rely on Satellite Visible/Infrared Microphysical Retrievals of Boundary Layer Clouds in Partially Cloudy Scenes? Implications for Climate Research
This study addresses the longstanding question of the reliability of gridded visible/infrared satellite cloud properties in partially cloudy scenes. By using in-situ cloud probes and airborne Research Scanning Polarimeter (RSP) observations, we analyze bias changes in satellite retrievals from the Spinning Enhanced Visible Infra-Red Imager (SEVIRI) geostationary sensor during the ORACLES campaign. Biases in cloud optical depth (τ) and droplet effective radius (r e ) modestly change for cloud area fraction greater than 35%. The agreement between SEVIRI and RSP r e substantially improves when the retrievals are averaged after removing pixels with τ < 3.0, yielding biases indistinguishable from overcast scenes. In addition, satellite and RSP show an excellent agreement for closed- and open-cell stratocumulus clouds, showing that the satellite retrievals capture spatial changes of r e , and confirming that satellites can faithfully reproduce real physical features for optically thick and partially cloudy scenes. We demonstrate that a simple methodology can minimize uncertainties in satellite-based climate studies.
Painemal, David [NASA Langley Research Center, Ham↗
High-resolution lidar observations of sedimentation-induced size sorting of droplets near a laboratory cloud top
Cloud optical properties and precipitation, which are crucial to weather and climate, are strongly influenced by cloud microphysical properties that are still poorly understood. Here, we develop a high-resolution time-correlated single-photon-counting lidar and apply it to observe cloud microphysical properties at one-centimeter range resolution in a convection chamber under well-controlled conditions. Together with concurrent in-situ measurements and theoretical analysis, our lidar observations indicate that although turbulent mixing tends to homogenize the cloud in the bulk region, entrainment and sedimentation cause inhomogeneities in droplet concentrations near the cloud top. Specifically, the topmost region is directly affected by entrainment, and lidar profiles show clear evidence of entrained air and detrained cloud filament. The transition region below exhibits vertical size sorting of cloud droplets caused by sedimentation. Our results suggest that using a single sedimentation velocity for all cloud droplets, as is done in many atmospheric models, overlooks key physics relevant to the microphysical structure near the cloud top. In conclusion, our conceptual model used to describe these measurements can serve as a step toward improving the current modeling of processes in the cloud top region.
54 ENVIRONMENTAL SCIENCES↗
Diurnal evolution of non-precipitating marine stratocumuli in a large-eddy simulation ensemble
Abstract. We explore the cloud system evolution of non-precipitating marine stratocumuli with a focus on the impacts of the diurnal cycle and free-tropospheric (FT) humidity based on an ensemble of 244 large-eddy simulations generated by perturbing initial thermodynamic profiles and aerosol conditions. Cases are categorized based on their degree of decoupling and the cloud liquid water path (LWPc, based on model columns with cloud optical depths greater than one). A budget analysis method is proposed to analyze the evolution of cloud water in both coupled and decoupled boundary layers. More coupled clouds start with a relatively low LWPc and cloud fraction (fc) but experience the least decrease in LWPc and fc during the daytime. More decoupled clouds undergo greater daytime reduction in LWPc and fc, especially those with higher LWPc at sunrise because they suffer from faster weakening of net radiative cooling. During the nighttime, a positive correlation between FT humidity and the LWPc emerges, consistent with higher FT humidity reducing both radiative cooling and the humidity jump, both of which reduce entrainment and increase LWPc. The LWPc is more likely to decrease during the nighttime for a larger LWPc and greater inversion base height (zi), conditions under which entrainment dominates as turbulence develops. In the morning, the rate of the LWPc reduction depends on the LWPc at sunrise, zi, and the degree of decoupling, with distinct contributions from subsidence and radiation.
Chen, Yao-Sheng (ORCID:0000000208354132)↗
Interconnection of Aerosol‐Cloud Interactions and Cloud Feedback Through Warm Rain Process
Recent research has revealed a correlation within the Coupled Model Intercomparison Project Phase 6 (CMIP6) simulations: models exhibiting more pronounced warming due to positive cloud feedback simultaneously show enhanced cooling from aerosol‐cloud interactions (ACI). However, the interplay between ACI and cloud feedback is not well understood in these models. Our study addresses this gap by modifying the autoconversion rate in two Earth system models (ESMs), elucidating how ACI could connect with cloud feedback through the warm rain process. We find that higher autoconversion rates, which are associated with stronger ACI, suppress the increase in cloud liquid water path (LWP) and cloud optical depth with warming by enhancing the precipitation efficiency over the extratropical regions, leading to a larger positive cloud feedback. This study offers new insights into the compensatory mechanism between ACI and cloud feedback through the warm rain process and highlights the importance of constraining the autoconversion parameterization in models.
54 ENVIRONMENTAL SCIENCES↗
Examining astrophysical gas cloud collapse using an optical depth-scaled, x-ray-irradiated, carbon-foam sphere
When stellar radiation interacts with a molecular cloud, the cloud's fate depends on the strength of the incident radiation and the radiation's mean-free-path within the cloud [F. Bertoldi, Astrophys. J. 346, 735–755 (1989)]. Under the right conditions, the radiation compresses the cloud and a star formation may occur. Where and when the stellar formation occurs in the cloud's collapse are open questions. Direct observation of the complete star–cloud lifecycle is nearly impossible due to the immense timescales and distances over which the interaction occurs. Laboratory astrophysics offers a way to investigate such a system by scaling the important astrophysical parameters to the laboratory. This work describes laboratory experiments to study the radiation-driven implosion of clouds, using x rays from a laser-irradiated, thin, gold foil as a surrogate star and a carbon-foam sphere as a surrogate cloud. An optically thick system, theoretically corresponding to a star-forming regime, was selected by choice of the foam density. Gold foil and sphere motions were imaged by x-ray radiography. Radiographic images show the formation of an interface between rarefied gold and carbon plasmas, a shock moving into the sphere, and a blunting of the initial sphere's shape. Measurements show that the shock moved linearly around 64 μm/ns into the sphere, and the gold–carbon interface formed by 2 ns at the sphere edge remained stationary. The deformation of the sphere was driven by the incident radiation and not by mechanical pressures applied by gold plasma. The blunting of the sphere was likely due to the geometric reduction of flux near the sphere's poles. Higher x-ray flux near the sphere's equator caused high compression and a faster shock, which flattened the sphere. We will discuss the results and implications of our observations.
VanDervort, R. W. [University of Michigan 1 , Ann ↗
Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation
Abstract. The Weather Research Forecasting (WRF) version 4.3 model is configured within a Lagrangian framework to quantify the impact of aerosols on evolving cloud fields. Kilometer-scale simulations utilizing meteorological boundary conditions are based on 10 case study days offering diverse meteorology during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA). Measurements from aircraft, the ground-based Atmosphere Radiation Measurement (ARM) site at Graciosa Island in the Azores, and A-Train and geostationary satellites are utilized for validation, demonstrating good agreement with the WRF-simulated cloud and aerosol properties. Higher aerosol concentration leads to suppressed drizzle and increased cloud water content in all case study days. These changes lead to larger radiative cooling rates at cloud top, enhanced vertical velocity variance, and increased vertical and horizontal wind speed near the base of the lower-tropospheric inversion. As a result, marine cloud cell area expands, narrowing the gap between shallow clouds and increasing cloud optical thickness, liquid water content, and the top-of-atmosphere outgoing shortwave flux. While similar aerosol effects are observed in lightly to non-raining clouds, they tend to be smaller by comparison. These simulations show a relationship between cloud cell area expansion and the radiative adjustments caused by liquid water path and cloud fraction changes. The adjustments are positive and scale as 74 % and 51 %, respectively, relative to the Twomey effect. While higher-resolution large-eddy simulations may provide improved representation of cloud-top mixing processes, these results emphasize the importance of addressing mesoscale cloud-state transitions in the quantification of aerosol radiative forcing that cannot be attained from traditional climate models.
54 ENVIRONMENTAL SCIENCES↗
Glaciation of liquid clouds, snowfall, and reduced cloud cover at industrial aerosol hot spots
The ability of anthropogenic aerosols to freeze supercooled cloud droplets remains debated. Here, in this work, we present observational evidence for the glaciation of supercooled liquid-water clouds at industrial aerosol hot spots at temperatures between -10° and -24°C. Compared with the nearby liquid-water clouds, shortwave reflectance was reduced by 14% and longwave radiance was increased by 4% in the glaciation-affected regions. There was an 8% reduction in cloud cover and an 18% reduction in cloud optical thickness. Additionally, daily glaciation-induced snowfall accumulations reached 15 millimeters. Glaciation events downwind of industrial aerosol hot spots indicate that anthropogenic aerosols likely serve as ice-nucleating particles. However, rare glaciation events downwind of nuclear power plants indicate that factors other than aerosol emissions may also play a role in the observed glaciation events.
54 ENVIRONMENTAL SCIENCES↗