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Full‐Waveform Simulation of Infrasound Propagation in the Atmosphere: A Case Study of the 2023 April 20 SpaceX Starship Explosion

Infrasound, low‐frequency sound below 20 Hz, has been a key technology to monitor explosion events in the atmosphere. The International Monitoring System (IMS) of the Comprehensive Nuclear‐Test‐Ban Treaty Organization provides the means for continuous monitoring of infrasonic events worldwide. Infrasonic techniques for event location and size estimation can also complement other observational techniques for the detection and characterization of the entry of asteroids or large meteoroids. In this study, we describe the detection capability of IMS infrasound stations for an explosive event in the middle of the atmosphere. Full‐waveform simulations are performed with the specification of atmospheric conditions and incorporated into the event location and explosion yield estimation. We applied it to the 2023 April 20 SpaceX Starship explosion at 29 km altitude. Starship is a super heavy‐lift space vehicle constructed by SpaceX and known as the largest and most powerful rocket ever built. The Starship explosion created huge pressure disturbances in the atmosphere, and its infrasound was detected by the IMS arrays in North America between 2000 and 4000 km. Independent observational data and available ground‐truth information provide a rare opportunity to evaluate the monitoring capability of the IMS network for elevated sources in the atmosphere. We also demonstrate the capability of full‐waveform simulation for infrasound wavefield characterization and prediction to improve event location and yield estimation.

Geosciences

PySolate : A Python‐Based Thresholding Tool to Denoise or Designal Seismic Waveforms Based on the Continuous Wavelet Transform

PySolate is a Python‐based toolset that implements the continuous wavelet transform and nonlinear thresholding operations to denoise or designal seismic data, following Langston and Mousavi (2019). This filtering approach can remove microseismic noise to isolate intermediate‐period seismic signals that are key to enabling full‐waveform modeling and analysis of smaller‐magnitude regional events. This approach is best for the application to signals with frequency or time separation of signal and noise, in contrast to Fourier analysis, which is effective when signal and noise are separated in frequency. We demonstrate the Python toolset using the six announced Democratic People’s Republic of Korea declared nuclear tests, showing the effectiveness of isolating the seismic signal compared to standard bandpass filtering. In conclusion, we also demonstrate the ease of using the toolset with any Python processing tools.

Asia

127 Xe quantification method development and intercomparison exercise

Monitoring of the atmosphere for fission products ( 131m Xe, 133m Xe, 133 Xe, and 135 Xe) is performed by various laboratories to detect nuclear explosions. Quantification of 127 Xe is not routinely performed by laboratories measuring atmospheric radioxenon because it is not a fission product. 127 Xe was recently detected by a ground-based beta-gamma air monitoring system. When measured using beta-gamma coincidence detector systems, such as those in use on the International Monitoring System (IMS) of the Comprehensive Nuclear-Test-Ban Treaty (CTBT), 127 Xe can interfere with the quantification of fission product radioxenon due to overlap of the 127 Xe beta-gamma coincidence signatures with those of fission product radioxenon. Here, this work demonstrates quantification of 127 Xe at different laboratories with different measurement techniques. Production and purification of 127 Xe was performed by neutron activation of enriched 126 Xe. The purified 127 Xe was then split between laboratories, and detection and quantification methods were developed. At Idaho National Laboratory, a quantification method involving high purity germanium detectors was devised that included self-attenuation correction. At AWE, a beta-gamma coincidence counting method, as used in support of the IMS, was modified to enable the measurement and analysis of the 127 Xe samples. Corrections were made for self-attenuation, which showed a strong xenon volume dependency, for some coincidence signatures. The gas sample activity concentration was used as the comparison metric and it showed excellent agreement between the methods.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P

Development and validation of a software for simulating γ-γ coincidence emission and detection probabilities

Gamma-gamma coincidence spectrometers have the potential to significantly enhance detection sensitivity for ultra-trace radionuclide measurements. The implementation of these spectrometers, however, is limited by the complexity of acquisition hardware, data processing and quantification. This work reports development of a novel radionuclide quantification software for γ-γ coincidence measurements. For any radionuclide, the software parses the Evaluated Nuclear Structure Data File (ENSDF) database, recursively simulating all possible γ-γ coincidence signatures and their respective emission and detection probabilities. Implemented using Python programming language, the software employs several strategies to boost overall computational performance. Since coincidence-based spectrometers are of notable interest in monitoring compliance for the Comprehensive Nuclear-Test-Ban Treaty (CTBT), the software’s execution was tested for 84 CTBT-relevant radionuclides. To date, the software has been experimentally validated for 15 radionuclides using the Advanced Radionuclide Gamma spectrOmeter (ARGO) at Pacific Northwest National Laboratory, USA (PNNL). Notably, the software can be operated in convergence mode, whereby coincidence detection efficiency’s convergence behavior can help avoid unreliable radionuclide activity estimates. With growing number of coincidence spectrometers worldwide, this paper aims to assist the radiation metrology community in developing similar software for their system.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND

Computational Optimization of 133m Xe Production via Neutron Irradiation in a TRIGA Reactor

Here, the Comprehensive Nuclear-Test-Ban Treaty bans all nuclear tests worldwide. As part of treaty compliance, the concentration of radioactive nuclides in the atmosphere is monitored to detect nuclear weapons tests. Radioactive noble gas fission products, specifically radioxenon, can vent into the atmosphere after a nuclear weapons test, even if the test is well contained underground or underwater. Radioxenon thus serves as a signal for nuclear weapons tests. All atmospheric monitoring systems require samples of radioxenon isotopes for detector calibration, quality control, and certification. Here, we present a novel, improved method for creating samples of 133m Xe via neutron irradiation of 132 Xe in the Washington State University TRIGA reactor. 132 Xe neutron absorption results in either 133 Xe or 133m Xe—thermal neutron absorption results in 133m Xe 12% of the time, while fast neutron absorption (above ~1 MeV) results in 133m Xe ~50% of the time. To optimize the production of 133m Xe via neutron absorption in 132 Xe in the thermal TRIGA reactor, spectral tuning using an irradiation chamber is required to maximize the fraction of fast neutrons being absorbed and minimize the number of thermal neutrons interacting with the 132 Xe. We used MCNP to tally 132 Xe absorptions with the isotopic tally function, flux tallies and neutron attenuation to estimate the number of neutrons reaching the 132 Xe through the irradiation chamber, and the adjoint importance function to improve the source strength estimate. Additionally, we performed a heat transfer analysis for safety considerations. It was determined that the use of a 96% enriched 10 B boron carbide chamber, placed next to the fuel elements in reactor position D8, increases the 133m Xe/ 133 Xe activity ratio from a baseline value of 0.3 to 1.0, a 233% increase. Additionally, it was determined that the alpha heating produced in the boron does not become an unmanageable problem in the Washington State University reactor.

37 - INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL C

Measurements of radioxenon activities during periods of gaseous release from an advanced gas-cooled reactor

Activities of radioxenon isotopes are reported from an Advanced Gas-cooled Reactor (AGR) during periods of gaseous release. Xenon isotopes are relevant to the monitoring regime of the Comprehensive Nuclear-Test-Ban Treaty (CTBT). These releases may affect detections from the International Monitoring System (IMS) by influencing the radioxenon background. Time series activity plots have been produced from both in-core monitoring and direct measurement at the point of release using a stack monitor system. Ratio plots using both data sets have been produced with results compared with a commonly chosen nuclear explosion “discrimination line.” The reported results improve the understanding of radionuclide emissions from civil nuclear power plants. This work is being performed as part of the Xenon Environmental Nuclide Analysis at Hartlepool (XENAH) collaboration between the Atomic Weapons Establishment (AWE, UK), EDF Energy (UK), Pacific Northwest National Laboratory (PNNL, USA), and the Swedish Defence Research Agency (FOI).

22 GENERAL STUDIES OF NUCLEAR REACTORS

2023 Reftek Wrangler Digitizer Type Approval Evaluation

Sandia National Laboratories has tested and evaluated the Reftek Wrangler digitizer. The Wrangler digitizers are intended to record sensor output for seismic and infrasound monitoring applications. The purpose of this digitizer evaluation is to measure the performance characteristics in such areas as power consumption, input impedance, sensitivity, full scale, self-noise, dynamic range, system noise, response, passband, and timing. The Wrangler digitizers are being evaluated for potential use in the International Monitoring System (IMS) and On-site Inspection (OSI) components of Comprehensive Nuclear-Test-Ban Treaty (CTBT).

58 GEOSCIENCES

2023 Reftek Colt Seismometer Exploratory Evaluation

Sandia National Laboratories has tested and evaluated three Colt broadband seismometers designed and manufactured by Reftek. The purpose of this seismometer evaluation is to measure performance characteristics in areas such as power consumption, sensitivity, frequency response, full scale, self-noise, dynamic range, calibration system response, and passband. The Colt model of sensors are being evaluated to explore the potential for a future seismometer Type Approval process in the International Monitoring System (IMS) of the Comprehensive Nuclear-Test-Ban Treaty (CTBT).

47 OTHER INSTRUMENTATION

2023 T120 Horizon and Slim Posthole Seismometer Exploratory Evaluation

Sandia National Laboratories has tested and evaluated a suite of four T120 broadband seismometers designed and manufactured by Nanometrics. Specifically, two T120 Horizon V2 sensors, one T120 Horizon V1 sensor and one T120 Slim Posthole (PH) sensor were evaluated. The purpose of this seismometer evaluation is to measure performance characteristics in areas such as power consumption, sensitivity, frequency response, full scale, self-noise, dynamic range, calibration system response, and passband. The T120 model of sensors are being evaluated to explore the potential for a future seismometer Type Approval process in the International Monitoring System (IMS) of the Comprehensive Nuclear-Test-Ban Treaty (CTBT).

47 OTHER INSTRUMENTATION

Photonuclear Production of Radioxenon for Air Samples

Radioxenon plays an important role in ensuring compliance with the Comprehensive Nuclear-Test-Ban Treaty due to its ability to be transported through the atmosphere, as well as the fact that the half-lives of its isotopes provide a window long enough to be detected but not long enough that it could become background radiation. This allows it to be correlated with specific events that indicate the testing of nuclear weapons. Idaho National Laboratory supports this mission by providing spiked air samples for monitoring stations to enable instrument calibration and ensure measurement accuracy. We tested a photonuclear method of producing one of the main isotopes of radioxenon, Xe-135. We also tested the separation of Xe-135 from the parent isotope Xe-136 using the method of kinematic recoil. Aluminum coils were placed in quartz ampoules filled with enriched Xe-136 and were irradiated by a bremsstrahlung beam with an endpoint energy of 21 MeV. The results showed that we were not only successful in producing Xe-135 but also that the Xe-135 was deposited into the coil allowing it to be removed from the Xe-136 gas. The coil and the Xe-135 can then be chemically separated. At the time of counting the coil, it was calculated that there was about 18 Bq of activity from Xe-135 remaining in the coil. Future work includes determining the optimal material and geometry of the catcher to maximize the amount of Xe-135 captured.

07 ISOTOPE AND RADIATION SOURCES