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All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

The Diurnal Variation of the Aerosol Optical Depth at the ARM SGP Site

Abstract This study examines the diurnal variation of the aerosol optical depth (AOD) at 355 nm observed by Raman lidar (RL) at the Atmospheric Radiation Measurement Program Southern Great Plains (SGP) site under both clear and cloudy‐sky conditions. Here only cloudy‐skies when the lidar signal is not fully attenuated are considered. The daytime AOD and its variation from the RL showed an excellent agreement with the Aerosol Robotic Network, demonstrating that the RL‐retrieved AOD is not affected by solar background contamination. The climatological annual‐mean daytime‐mean AOD is only slightly larger than the nighttime‐mean AOD (by 1%–3%). However, day‐to‐day variations are observed such that the daytime‐ and nighttime‐mean AOD difference for a given day can be large (about 95% of days have differences within 0.2). The seasonal AOD diurnal range (i.e., the difference between the maximum and minimum values) relative to the mean was 10%–15% except in the winter when it was 44%. The seasonal‐mean cloudy‐sky AOD diurnal variation is similar to that for clear‐sky, except that the AODs are larger (the annual‐mean cloudy‐sky AOD is larger than the clear‐sky by 24%). The aerosol lidar ratio diurnal variations are also examined, which are 10%–20% for all seasons with a minimum near 9 a.m. to 15 p.m. for all seasons except winter. Also presented is the annual‐mean AOD from the Cloud‐Aerosol Lidar and Infrared Pathfinder Satellite at SGP site: its daytime AOD is about 0.1 smaller than nighttime AOD because of daytime solar background contamination.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Simulated Precipitation Diurnal Variation With a Deep Convective Closure Subject to Shallow Convection in Community Atmosphere Model Version 5 Coupled With CLUBB

In order to improve the physical consistency between shallow and deep convection, we modify the deep convective closure in the Community Atmosphere Model version 5 (CAM5) coupled with a third-order turbulence closure parameterization (i.e., Cloud Layers Unified by Binormals; CLUBB). The revised closure reserves a portion of the total convective available potential energy for shallow convection via utilizing the heating and moistening profiles from CLUBB to distribute moisture and energy between shallow and deep convection. Simulations at two resolutions (i.e. 2° and 0.5°, respectively) are conducted to investigate the impacts of convective closure on the simulated precipitation diurnal variations. Results from low-resolution simulations show that the revised closure suppresses deep convection until the lower troposphere is sufficiently moistened by shallow convection, which improves the precipitation diurnal variation simulations compared to the default closure, with the precipitation diurnal peak over tropical lands delayed from 12LST to 19LST. The revised closure better simulates the diurnal variations for precipitation over the Asian monsoon region, such as the delayed precipitation onset, but still fails to well capture the nighttime peak for precipitation there. This deficiency is alleviated to some extent when applying the revised closure in highresolution simulations, but nighttime precipitation is still underestimated probably because key processes responsible for nighttime convection are missing. Altogether, our results indicate that establishing the consistency between shallow and deep convection is critical for the precipitation diurnal cycle simulations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Convection-permitting hindcasting of diurnal variation of Mei-yu rainfall over East China with a global variable-resolution model

Two sets of 48-hr hindcast experiments for Mei-yu season using non-hydrostatic global variable-resolution model (MPAS-Atmosphere) with regional refinement at 4km resolution (V4km) and uniform 60km resolution (U60km) are first-time conducted to attempt at simulating the Mei-yu rainfall in 2015 over East China. The analysis focuses on the seasonal average of diurnal variation of precipitation amount (PA), intensity (PI), and frequency (PF). Both simulations reasonably reproduce the spatial distribution of PA. V4km is more skillful in simulating the spatial distributions and magnitudes of PF and PI. The diurnal cycle of Mei-yu rainfall shows a major early morning peak and a minor afternoon peak, contributed by precipitation during two sub-periods with distinct synoptic circulations. With strong Mei-yu in the first sub-period, the diurnal variation of PA is controlled by nocturnal southwesterly jet. V4km overestimates the morning peak mainly due to its bias in simulating boundary layer inertial oscillation. Although differences in PA between the simulations are small, U60km overestimates PF and underestimates PI. With weak Mei-yu in the second sub-period, the diurnal variation of PA is controlled by both synoptic circulation and local convection. At both resolutions, deviations in the large-scale circulation modulated by a few typhoons lead to positive biases in the morning peak of PA. After removing the typhoon impacts, V4km captures the observed diurnal cycle of PA well, while U60km significantly underestimates PA and PI particularly in the afternoon. Future studies focusing on advancing modeling of southwesterly jet and typhoons may further improve convection permitting simulation of Mei-yu rainfall.

Xu, Mingyue↗
DOE OSTI2025

The sources and diurnal variations of submicron aerosols in a coastal–rural environment near Houston, US

Aerosol properties were characterized at a rural site southwest of Houston from May to September 2022 during the intensive operation periods (IOPs) of the Tracking Aerosol Convection Interactions ExpeRiment (TRACER). Backward trajectory analysis reveals three major air mass types: marine air mass from the Gulf, urban air mass influenced by urban emissions, and regional air mass. Marine aerosols typically show a bimodal size distribution and have the lowest particle number and mass concentrations of PM 1 (particulate matter with an aerodynamic diameter of less than 1 µm), while aerosols from air masses strongly influenced by urban emissions exhibit the highest concentrations. Organic aerosol (OA) accounts for more than 50 % of PM 1 for urban and regional air masses, whereas sulfate is comparable to OA in marine air masses. Positive matrix factorization (PMF) analysis of aerosol mass spectra identifies 6 OA factors: hydrocarbon-like OA (HOA), OA from the oxidation of monoterpenes (MT-SOA), OA from the reactive uptake of isoprene epoxydiols by acidic sulfate particles (isoprene-SOA), oxygenated OA arising from shipping emissions (shipping-OOA), and two oxygenated OA factors with high O : C ratios (OOA1 and OOA2). OOA2 has the highest O : C ratio and exhibits elevated mass concentration in the afternoon. Similar diurnal variation of highly oxidized OA factors was commonly observed in the Houston area during previous studies and attributed to the SOA formation by photochemistry and mixing from aloft. Here, using air mass backward trajectories and a 1-D box model, we show the diurnal trend of OOA2 mass concentration is instead driven by changes in air mass arriving at the rural site. The air mass changes are likely caused by the shift between land breezes and sea/bay breezes. Within the same air mass type (e.g., either urban or marine air mass), OOA2 mass concentration is largely independent of wind direction and shows essentially no diurnal variation, suggesting OOA2 is related to aged OA with minimal influence by local emissions. This study helps identify the major sources of OA in the Houston region and highlights the impacts of both atmospheric chemistry and meteorology on aerosol properties in the coastal–rural environment.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Diurnal variation of the fair-weather atmospheric electric field in Binchuan, China

With the purpose of understanding the variation of fair-weather atmospheric electric field, the vertical component of atmospheric electric field (recorded as Ez) has been measured in the town Binchuan (25°50'N, 100°34'E, 1438.7 m asl) of Dali city, Yunnan, China from June 14, 2017 to December 1, 2020. Automatic measured visual range is used as a proxy of aerosol concentration. The mean diurnal variation curve of the fair-weather Ez in Binchuan, having two peaks occurred at around 9LT and 20LT, shows little correlation with the well-known Carnegie Curve and other two high-latitude sites' Curves. While strong negative correlation between fair-weather Ez and visual range is found, indicating the variation of fair-weather is dominated by aerosol concentration. The main source of aerosol concentration variation probably sunrise and sunset effect. We support our findings by comparing Ez, visual range with sunrise and sunset times. The peaks (troughs) of Ez (visual range) are proved to have weak correlations with anthropogenic pollution through comparing the Ez, visual range under workdays and holidays.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Diurnal Variation of the Planetary Boundary Layer Height Observed from GNSS Radio Occultation and Radiosonde Soundings over the Southern Great Plains

>The planetary boundary layer (PBL) height (PBLH) is a key physical parameter of the PBL affected by numerous physical processes within the boundary layer. Specifically, the PBLH over land exhibits large spatial and temporal variation across different geographical regions. In this study, the Constellation Observing System for Meteorology, Ionosphere and Climate (COSMIC) radio occultation (RO) profiles and high-resolution radiosonde profiles from 2007 to 2013 were analyzed to estimate the diurnal cycle of the PBLH over the Southern Great Plains (SGP) in the United States. Large variations in PBLH derived from radiosonde temperature, moisture, and refractivity are observed on seasonal scales. COSMIC RO is capable of observing diurnal and seasonal variations in the terrestrial PBLH over the SGP region. Annual mean diurnal amplitude of approximately 250 m in the terrestrial PBLH was observed, with maxima occurring at around 1500 local solar time (LST) in both the collocated radiosondes and COSMIC RO profiles. Seasonal changes in the PBLH diurnal cycles ranging from approximately 100 to 400 m were also observed. Such PBL diurnal and seasonal changes can be further incorporated into PBL parameterizations to help improve weather and climate model prediction. Significance Statement. The atmospheric planetary boundary layer (PBL) and its height (PBLH) control many atmospheric processes that affect our everyday lives. Observations of the PBL are usually limited to radiosondes at limited time intervals. GNSS radio occultation (RO) provide high-vertical-resolution atmospheric observations that are ideal for PBL study. This study demonstrates that the GNSS RO is capable of capturing the diurnal and seasonal variations of the PBLH over the southern Great Plains (SGP) well as compared to the collocated radiosonde observations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Relationships among diurnal variations of polar night cloud, precipitation, surface temperatures, and the fair-weather return current of the global electric circuit (GEC)

Over the past five years (June 2017-current), the vertical electric field (E z ) as well as numerous cloud, precipitation and radiation properties have been monitored at the Department of Energy-Atmospheric Radiation Measurement (DOE ARM) North Slope of Alaska (NSA) field site. Comparisons between the composite diurnal averaged fair-weather E z , and composite ceilometer derived cloud base height during the polar night, reveal a significant correlation between the parameters (r = 0.62), supporting previous studies that there is high correlation between local electric field and cloud properties. With the use of extensive instrumentation at the site, such as the Micro Pulse Lidar (MPL), Ka-band Zenith Radar (KAZR), ceilometer, SKYRAD, Precipitation Imaging Package (PIP), among others, this study provides a more comprehensive examination of the diurnal cycle of cloud and precipitation properties along with the localized fair-weather return current of the larger Global Electric Circuit (GEC) system. Comparisons between the composite diurnal averaged fair-weather E z , and cloud thickness, maximum column backscatter, and precipitation particle counts all show similar diurnal variability during the polar night, indicating that during the largest magnitude fair weather E z time periods, clouds bases tend to be higher, clouds are thicker, have a larger column backscatter, and display more precipitating particles. Furthermore, a slight diurnal variability in the polar night surface temperature was found to be highly correlated (r = 0.87) to the longwave downwelling irradiance measured by SKYRAD, indicating that the variations in the physical properties of local clouds could modulate the diurnal polar night surface temperature variability on the order of 0.5 °C/day. In conclusion, these findings emphasize the importance and global nature of the GEC system, with the global aggregate of thunderstorms and electrified clouds potentially influencing polar night cloud properties as well as diurnal wintertime polar surface temperature variation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Sub-Diurnal Methane Variations on Mars Driven by Barometric Pumping and Planetary Boundary Layer Evolution

In recent years, the Tunable Laser Spectrometer within the Sample Analysis at Mars (TLS-SAM) instrument on board the Mars Science Laboratory (MSL) Curiosity rover has detected methane variations in the atmosphere at Gale crater. Methane concentrations appear to fluctuate seasonally as well as sub-diurnally, which is difficult to reconcile with an as-yet-unknown transport mechanism delivering the gas from underground to the atmosphere. To potentially explain the fluctuations, we consider barometrically induced transport of methane from an underground source to the surface, modulated by temperature-dependent adsorption. The subsurface fractured-rock seepage model is coupled to a simplified 1-D atmospheric mixing model to provide insights on the pattern of atmospheric methane concentrations in response to transient surface methane emissions, as well as to predict sub-diurnal variation in methane abundance for the northern summer period, which is a candidate time frame for a MSL Curiosity sampling campaign. Our analysis suggests that there is a lower limit to the subsurface fracture density that can produce the observed methane patterns, below which the atmospheric methane variations would be out of phase with the observations. The best-performing model scenarios indicate a significant, short-lived methane pulse just prior to sunrise, the detection of which by TLS-SAM would be a potential indicator of the contribution of barometric pumping to Mars' atmospheric methane variations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Statistically Resolved Planetary Boundary Layer Height Diurnal Variability Using Spaceborne Lidar Data

The Planetary Boundary Layer Height (PBLH) significantly impacts weather, climate, and air quality. Understanding the global diurnal variation of the PBLH is particularly challenging due to the necessity of extensive observations and suitable retrieval algorithms that can adapt to diverse thermodynamic and dynamic conditions. This study utilized data from the Cloud-Aerosol Transport System (CATS) to analyze the diurnal variation of PBLH in both continental and marine regions. By leveraging CATS data and a modified version of the Different Thermo-Dynamics Stability (DTDS) algorithm, along with machine learning denoising, the study determined the diurnal variation of the PBLH in continental mid-latitude and marine regions. The CATS DTDS-PBLH closely matches ground-based lidar and radiosonde measurements at the continental sites, with correlation coefficients above 0.6 and well-aligned diurnal variability, although slightly overestimated at nighttime. In contrast, PBLH at the marine site was consistently overestimated due to the viewing geometry of CATS and complex cloud structures. The study emphasizes the importance of integrating meteorological data with lidar signals for accurate and robust PBLH estimations, which are essential for effective boundary layer assessment from satellite observations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Comparative Evaluation of the Ability of the MYNN‐EDMF PBL Scheme in WRF Model to Reproduce Near Surface Wind Speed Over Different Topographical Types

Abstract This study systematically evaluates the performance of the Mellor‐Yamada‐Nakanishi‐Niino‐Eddy‐Diffusion‐Mass‐Flux planetary boundary layer (PBL) scheme within the Weather Research and Forecasting (WRF) model in simulating near‐surface wind speeds across various topographies in New York State (NYS). Simulated wind speeds are compared with in‐situ measurements from 22 surface sites, grouped into six topographic categories: continental plain (CT), lakeside (LS), river valley (RV), Long Island (LI), Block Island (BI), and offshore ocean (OO). A quantitative evaluation based on Relative Euclidean Distance shows that wind speeds at the OO site are the most accurately reproduced, followed by those at LI sites, while the model performs less accurately for the remaining topographic groups. Wind speeds over CT sites tend to be overestimated by approximately 1 m/s, although their diurnal variability (DV) is well captured. In contrast, the model underestimates wind DV at LS, RV, LI, and BI sites, with the largest biases occurring at LI and BI, resulting in underestimated daytime wind speed and/or overestimated nighttime wind speed. The OO winds exhibit minimal diurnal variation, accurately captured by our WRF model. The surface wind diurnal variation is closely linked to PBL development. Among the indicators of PBL development, surface potential temperature biases most strongly correlate with wind speed biases. Our WRF model faces challenges in capturing the distinctions between winds influenced by local circulations and those over continental plains, and the significantly stronger winds at OO compared to BI. Potential causes for these biases are discussed, offering pathways for improving surface wind simulations in future.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Quasi-Two-Day and Diurnal Cloud Variation Timescales over Convectively Active Regions

Climatological features of the cloud variability on quasi-two-day (Q2D) and diurnal cycle (DC) timescales are investigated by utilizing the high-resolution satellite infrared brightness temperature (IRBT) observations from January 1998 to December 2019. A distinct land-sea contrast between the distributions of Q2D and DC signals is evident. Diurnally driven cloud activity mainly occurs over land and mountainous regions, and the Q2D timescale is more prominent over tropical ocean basins and land where organized convection is usually observed, e.g., Congo and Amazon Rainforests, the U.S. and subtropical South America during warm seasons. The long-term relationship between the Q2D variability and sea surface temperature (SST) shows that the clouds are more active on Q2D timescales over higher SST environments. The Q2D variability correlates well with both the Indian Ocean Dipole (IOD) and El Niño/Southern Oscillation (ENSO) from 1998 to 2019. The cloud variability associated with a range of convective available potential energy (CAPE) values is analyzed. The result over land shows that increased Q2D cloud variability emerges with higher CAPE, suggesting the coincidence of Q2D and organized convection, particularly given that this effect is strongest over regions with frequent mesoscale convective systems (MCSs) around the world. The cloud variability and the Q2D timescale analyses provide an alternative perspective to understand the global features of mesoscale convective systems. Overall, this study objectively examines the global variability of convective timescales related to the diurnal cycle and longer-lived convective systems to provide a greater understanding of how the global convection population varies in space and time.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

The Summertime Precipitation Bias in E3SM Atmosphere Model Version 1 over the Central United States

This study analyzes the summertime precipitation bias over the Central United States and its relationship to the simulated large-scale environment and the convection scheme in the Energy Exascale Earth System Model Atmosphere Model version 1. This relationship is mainly examined in a set of short-term hindcasts initialized with realistic large-scale conditions for the summer of 2011. Besides the uniform 1° model resolution, we adopt Regionally Refined Meshes to increase the model resolution to 0.25°over the contiguous United States. Additional five-year Atmospheric Model Intercomparison Project simulations are conducted to confirm that the results from the hindcasts are consistent with the climate runs. We find that the summertime dry precipitation bias over the Great Plains and the wet bias over the Rockies cannot be reduced simultaneously by changing resolution or tuning parameters. As for the diurnal cycle, Energy Exascale Earth System Model Atmosphere Model version 1 captures the general diurnal variation of the large-scale moisture transport and the large-scale upward motion over the Central United States. However, the diurnal cycle of precipitation over the Great Plains is out of phase with the diurnal variation of the large-scale environment because the convective precipitation dominates the total precipitation and its diurnal cycle, and it does not directly respond to the local moisture convergence and the large-scale upward motion. These results reemphasize the importance of improving the coupling of the convection to the large-scale environment in reducing the summer precipitation bias over the Central United States in climate models with the resolution of ~0.25°.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

The diurnal susceptibility of subtropical clouds to aerosols

The diurnal susceptibility of clouds and their radiative properties to aerosols is examined during their Lagrangian transition from subtropical stratocumulus to shallow cumulus regimes. Using large-eddy simulations, we analyze the six-day evolution of an air mass along a 3800 km observed trajectory from the coast of Peru toward the equator. Pristine and polluted scenarios are simulated with forcing imposed from weather reanalysis. The polluted scenario exhibits stronger diurnal variations in cloud water, cloud fraction, and albedo, with enhanced nighttime entrainment and suppressed precipitation. The overall response of cloud properties and outgoing shortwave radiation to droplet number concentration follows a distinct diurnal pattern: strong positive cloud adjustments dominate at night and in the morning, while weak negative adjustments prevail in the afternoon. This cycle is driven by the competition between precipitation suppression, which enhances cloud water and coverage, and entrainment drying, which depletes them. In polluted conditions, enhanced entrainment leads to a deeper and more decoupled boundary layer that cannot be sustained by surface fluxes in the afternoon, resulting in negative cloud adjustments. The enhanced entrainment rate under polluted conditions is caused by the reduced sedimentation of cloud and precipitation water from the entrainment zone. While the Twomey effect dominates the diurnal average albedo response, the diurnal variation in the competing cloud adjustments lead to a near-neutral net susceptibility in the afternoon, highlighting the critical role of diurnally varying processes in aerosol-cloud interactions.

Geosciences↗
DOE OSTI2022

Impact of Measured Spectrum Variation on Solar Photovoltaic Efficiencies Worldwide

In photovoltaic power ratings, a single solar spectrum, AM1.5, is the de facto standard for record laboratory efficiencies, commercial module specifications, and performance ratios of solar power plants. More detailed energy analysis that accounts for local spectral irradiance, along with temperature and broadband irradiance, reduces forecast errors to expand the grid utility of solar energy. Here, ground-level measurements of spectral irradiance collected worldwide have been pooled to provide a sampling of geographic, seasonal, and diurnal variation. Applied to nine solar cell types, the resulting divergence in solar cell efficiencies illustrates that a single spectrum is insufficient for comparisons of cells with different spectral responses. Cells with two or more junctions tend to have efficiencies below that under the standard spectrum. Silicon exhibits the least spectral sensitivity: relative weekly site variation ranges from 1% in Lima, Peru to 14% in Edmonton, Canada.

energy yield↗
DOE OSTI2025

Linking large-scale weather patterns to observed and modeled turbine hub-height winds offshore of the US West Coast

The US West Coast holds great potential for wind power generation, although its potential varies due to the complex coastal climate. Characterizing and modeling turbine hub-height winds under different weather conditions are vital for wind resource assessment and management. This study uses a two-stage machine learning algorithm to identify five large-scale meteorological patterns (LSMPs): post-trough, post-ridge, pre-ridge, pre-trough, and California high. The LSMPs are linked to offshore wind patterns, specifically at lidar buoy locations within lease areas for future wind farm development off Humboldt and Morro Bay. While each LSMP is associated with characteristic large-scale atmospheric conditions and corresponding differences in wind direction, diurnal variation, and jet features at the two lidar sites, substantial variability in wind speeds can still occur within each LSMP. Wind speeds at Humboldt increase during the post-trough, pre-ridge, and California-high LSMPs and decrease during the remaining LSMPs. Morro Bay has smaller responses in mean speeds, showing increased wind speed during the post-trough and California-high LSMPs. Besides the LSMPs, local factors, including the land–sea thermal contrast and topography, also modify mean winds and diurnal variation. The High-Resolution Rapid Refresh model analysis does a good job of capturing the mean and variation at Humboldt but produces large biases at Morro Bay, particularly during the pre-ridge and California-high LSMPs. The findings are anticipated to guide the selection of cases for studying the influence of specific large-scale and local factors on California offshore winds and to contribute to refining numerical weather prediction models, thereby enhancing the efficiency and reliability of offshore wind energy production.

17 WIND ENERGY↗
DOE OSTI2024

Establishing reference ranges for circulating biomarkers of drug‐induced liver injury in healthy human volunteers 1

Aims The potential of mechanistic biomarkers to improve prediction of drug‐induced liver injury (DILI) and hepatic regeneration is widely acknowledged. We sought to determine reference intervals for new biomarkers of DILI and regeneration, as well as to characterize their natural variability and impact of diurnal variation. Methods Serum samples from 227 healthy volunteers were recruited as part of a cross‐sectional study; of these, 25 subjects had weekly serial sampling over 3 weeks, while 23 had intensive blood sampling over a 24h period. Alanine aminotransferase (ALT), MicroRNA‐122 (miR‐122), High Mobility Group Box‐1 (HMGB1), total Keratin‐18 (K18), caspase‐cleaved Keratin‐18 (ccK18), Glutamate Dehydrogenase (GLDH) and Macrophage Colony‐Stimulating Factor‐1 (CSF‐1) were assayed. Results Reference intervals were established for each biomarker based on the 97.5% quantile (90% CI) following the assessment of fixed effects in univariate and multivariable models. Intra‐individual variability was found to be non‐significant, and there was no significant impact of diurnal variation. Conclusion Reference intervals for novel DILI biomarkers have been described. An upper limit of a reference range might represent the most appropriate mechanism to utilize these data. These data can now be used to interpret data from exploratory clinical DILI studies and to assist their further qualification as required by regulatory authorities.

Jorgensen, Andrea L. [Department of Health Data Sc↗