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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Computational and experimental search for potential polyanionic K-ion cathode materials

Discovering high-energy cathode materials is critical to construct K-ion batteries for practical applications. Owing to the great success of layered oxides in Li- and Na-ion systems, K layered cathodes have also been investigated in recent years. However, the much larger size of K + compared to Li or Na introduces strong K + –K + interaction within the layer, which results in a sloped voltage profile thereby limiting the specific capacity and operating voltage. In contrast, polyanionic materials with a three-dimensional K + arrangement can effectively mitigate K + –K + interaction. In this work, ten K polyanionic compounds with theoretical capacity >100 mA h g –1 are screened from the Inorganic Crystal Structure Database as potential cathode materials for K-ion batteries. Among the ten proposed compounds, K 2 MnP 2 O 7 , K 2 Mn 2 P 2 O 7 F 2 , K 2 Fe 2 P 2 O 7 F 2 , and K 6 V 2 (PO 4 ) 4 with average voltage <4.5 V are synthesized and evaluated electrochemically. While the re-insertion of K into these compounds is not fully reversible, it may be related to the very high migration barrier that we compute for K ions. In addition, we show the successful synthesis of a series of K 3 V 3–x Cr x (PO 4 ) 4 (x = 0, 1, 2, 3) compounds. Among these, K 3 V 2 Cr(PO 4 ) 4 exhibits the largest reversible capacity, as revealed by the in situ investigation. Lastly, we find that the redox couples in many of these compounds sit at remarkably high potential, even higher than in equivalent Li compounds, which brings both opportunities and challenges in the future research of K polyanion cathodes.

25 ENERGY STORAGE↗
DOE OSTI2022

Experimental Searches for Muon to Electron Conversion in a Nucleus: COMET, DeeMe, and Mu2e (A Contributed paper for Snowmass 21)

Searches for charged lepton flavor violation (CLFV) offer deep probes for a range of new physics scenarios, such as super-symmetric models, theories involving scalar leptoquarks or additional Higgs doublets, and models explaining the neutrino mass hierarchy and the matter-antimatter asymmetry of the universe via leptogenesis. The coherent, neutrinoless conversion of a muon to an electron in the field of a nucleus, $\mu^{-}+N\rightarrow e^{-} +N$, is one example of a muonic CLFV process which has sensitivity to this new physics. This paper details three experiments: COMET, DeeMe and Mu2e which will search for $\mu^{-}+N\rightarrow e^{-} +N$ in the coming decade. These experiments offer sensitivity up to an effective new physics mass scale of $\mathcal{O}(10^{4}$ TeV/c$^{2}$), going far beyond what can be achieved in direct, collider-based, searches. The theoretical motivation, designs and anticipated timelines for these three experiments are presented. These experiments are a crucial part of a global search for CLFV. Continued support for all planned experimental searches for muonic CLFV is strongly encouraged.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Experimental search for the chiral magnetic effect in relativistic heavy-ion collisions: A perspective

The chiral magnetic effect (CME) refers to generation of the electric current along a magnetic field in a chirally imbalanced system of quarks. The latter is predicted by quantum chromodynamics to arise from quark interaction with nontrivial topological fluctuations of the vacuum gluonic field. The CME has been actively searched for in relativistic heavy-ion collisions, where such gluonic field fluctuations and a strong magnetic field are believed to be present. The CME-sensitive observables are unfortunately subject to a possibly large non-CME background, and firm conclusions on a CME observation have not yet been reached. In this perspective, we review the experimental status and progress in the CME search, from the initial measurements more than a decade ago to the dedicated program of isobar collisions in 2018 and the release of the isobar blind analysis result in 2022 to intriguing hints of a possible CME signal in Au + Au collisions, and discuss future prospects of a potential CME discovery in the anticipated high-statistic Au + Au collision data at the Relativistic Heavy-Ion Collider by 2025. We hope such a perspective will help sharpening our focus on the fundamental physics of the CME and steer its experimental search.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Progress on the experimental search for the chiral magnetic effect, the chiral vortical effect, and the chiral magnetic wave

In quantum chromodynamics, the interactions of quarks with the topological gluon field can lead to nonconservation of local parity (P) and conjugated parity (CP) , which provides a solution to the strong CP problem and a possibility to explain the asymmetry of matter-antimatter in the current universe. Under the action of a strong magnetic field, the nonconservation of P and CP can lead to the separation of particles according to their electric charges, which is called the chiral magnetic effect (CME). An observation of the CME-induced charge separation will confirm several fundamental properties of quantum chromodynamics (QCD), namely, approximate chiral symmetry restoration, topological charge fluctuation, and local parity violation. In relativistic heavy-ion collisions, there are other chiral anomalous effects similar to the CME, such as the chiral vortical effect (CVE) and the chiral magnetic wave (CMW). This review briefly summarizes the current progress of experimental research on the CME, CVE, and CMW in relativistic heavy-ion collisions.

Physics↗
DOE OSTI2022

Experimental Search for Neutron to Mirror Neutron Oscillations as an Explanation of the Neutron Lifetime Anomaly

We report an unexplained >4σ discrepancy persists between “beam” and “bottle” measurements of the neutron lifetime. A new model proposed that conversions of neutrons n into mirror neutrons n', part of a dark mirror sector, can increase the apparent neutron lifetime by 1% via a small mass splitting Δm between n and n' inside the 4.6 T magnetic field of the National Institute of Standards and Technology Beam Lifetime experiment. A search for neutron conversions in a 6.6 T magnetic field was performed at the Spallation Neutron Source which excludes this explanation for the neutron lifetime discrepancy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Probing lepton flavor violation in meson decays with LHC data

Abstract In this letter, we use LHC data from the Drell–Yan processes $$pp\rightarrow \ell _i\ell _j$$ p p → ℓ i ℓ j (with $$i\ne j$$ i ≠ j ) to derive model-independent upper limits on lepton-flavor-violating meson decays. Our analysis is based on an Effective Field Theory (EFT) approach and it does not require a specific assumption regarding the basis of effective operators. We find that current LHC data (140 $$\textrm{fb}^{-1}$$ fb - 1 ) already provides competitive limits on $${\mathcal {B}}(B\rightarrow \pi e \tau )$$ B ( B → π e τ ) and $${\mathcal {B}}(B\rightarrow \pi \mu \tau )$$ B ( B → π μ τ ) with respect to the ones obtained through experimental searches at the B -factories. Moreover, we derive upper limits on several decays that have not been searched for experimentally yet, such as $$D^0\rightarrow e\tau $$ D 0 → e τ in the charm sector, and various semileptonic decays such as $$B\rightarrow \rho \mu \tau $$ B → ρ μ τ , $$B_s\rightarrow K \mu \tau $$ B s → K μ τ and $$B_s\rightarrow \phi \mu \tau $$ B s → ϕ μ τ . Lastly, we discuss the validity of the EFT description of LHC data and the impact of loop corrections in our analysis.

Descotes-Genon, S.↗
DOE OSTI2022

Superconducting detectors for rare event searches in experimental astroparticle physics

Superconducting detectors have become an important tool in experimental astroparticle physics, which seeks to provide a fundamental understanding of the Universe. In particular, such detectors have demonstrated excellent potential in two challenging research areas involving rare event search experiments, namely, the direct detection of dark matter (DM) and the search for neutrinoless double beta decay. Here, we review the superconducting detectors that have been and are planned to be used in these two categories of experiments. We first provide brief histories of the two research areas and outline their significance and challenges in astroparticle physics. Then, we present an extensive overview of various types of superconducting detectors with a focus on sensor technologies and detector physics, which are based on calorimetric measurements and heat flow in the detector components. Finally, we introduce leading experiments and discuss their future prospects for the detection of DM and the search for neutrinoless double beta decay employing superconducting detectors.

transition edge sensors↗
DOE OSTI2021

Manipulating strong electromagnetic fields with the average transverse momentum of relativistic nuclear collisions

Abstract We show that an event-shape engineering based on the mean transverse momentum of charged hadrons, $$[p_t]$$ [ p t ] , provides an optimal handle on the strength of the magnetic field created in central heavy-ion collisions at high energy. This is established through quantitative evaluations of the correlation existing between the event-by-event magnetic field produced by the spectator protons in 5.02 TeV Pb + Pb collisions and the event-by-event $$[p_t]$$ [ p t ] at a given collision centrality. We argue that the event selection based on $$[p_t]$$ [ p t ] provides a better handle on the magnetic field than the more traditional selection based on the event ellipticities. Advantages brought by this new method for the experimental search of the chiral magnetic effect are discussed.

Giacalone, Giuliano (ORCID:0000000287761034)↗
DOE OSTI2022

Lattice QCD and the Computational Frontier

The search for new physics requires a joint experimental and theoretical effort. Lattice QCD is already an essential tool for obtaining precise model-free theoretical predictions of the hadronic processes underlying many key experimental searches, such as those involving heavy flavor physics, the anomalous magnetic moment of the muon, nucleon-neutrino scattering, and rare, second-order electroweak processes. As experimental measurements become more precise over the next decade, lattice QCD will play an increasing role in providing the needed matching theoretical precision. Achieving the needed precision requires simulations with lattices with substantially increased resolution. As we push to finer lattice spacing we encounter an array of new challenges. They include algorithmic and software-engineering challenges, challenges in computer technology and design, and challenges in maintaining the necessary human resources. In this white paper we describe those challenges and discuss ways they are being dealt with. Overcoming them is key to supporting the community effort required to deliver the needed theoretical support for experiments in the coming decade.

Boyle, Peter↗
DOE OSTI2021

Investigation of experimental observables in search of the chiral magnetic effect in heavy-ion collisions in the STAR experiment *

The chiral magnetic effect (CME) is a novel transport phenomenon, arising from the interplay between quantum anomalies and strong magnetic fields in chiral systems. In high-energy nuclear collisions, the CME may survive the expansion of the quark-gluon plasma fireball and be detected in experiments. Over the past two decades, experimental searches for the CME have attracted extensive interest at the Relativistic Heavy Ion Collider (RHIC) and the Large Hadron Collider (LHC). The main goal of this study is to investigate three pertinent experimental approaches: the $γ$ correlator, the R correlator, and the signed balance functions. We exploit simple Monte Carlo simulations and a realistic event generator (EBE-AVFD) to verify the equivalence of the core components among these methods and to ascertain their sensitivities to the CME signal and the background contributions for the isobar collisions at the RHIC.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Chiral Magnetic Effects in Nuclear Collisions

The interplay of quantum anomalies with strong magnetic fields and vorticity in chiral systems could lead to novel transport phenomena, such as the chiral magnetic effect (CME), the chiral magnetic wave (CMW), and the chiral vortical effect (CVE). In high-energy nuclear collisions, these chiral effects may survive the expansion of a quark–gluon plasma fireball and be detected in experiments. The experimental searches for the CME, the CMW, and the CVE have aroused extensive interest over the past couple of decades. The main goal of this article is to review the latest experimental progress in the search for these novel chiral transport phenomena at the Relativistic Heavy Ion Collider at Brookhaven National Laboratory and the Large Hadron Collider at CERN. Future programs to help reduce uncertainties and facilitate the interpretation of the data are also discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Superconductivity in La and Y hydrides: Remaining questions to experiment and theory

Recent reports of the superconductivity in hydrides of two different families (covalent lattice, as in SH3 and clathrate-type H-cages containing La and Y atoms, as in LaH10 and YH6) have revealed new families of high-Tc materials with Tc’s near room temperature values. These findings confirm earlier expectations that hydrides may have very high Tc’s due to the fact that light H atoms have very high vibrational frequencies, leading to high Tc values within the conventional Bardeen–Cooper–Schrieffer phonon mechanism of superconductivity. However, as is pointed out by Ashcroft, it is important to have the metallic hydrogen “alloyed” with the elements added to it. This concept of a metallic alloy containing a high concentration of metal-like hydrogen atoms has been instrumental in finding new high-Tc superhydrides. These new superhydride “room-temperature” superconductors are stabilized only at very high pressures above 100 GPa, making the experimental search for their superconducting properties very difficult. We will review the current experimental and theoretical results for LaH10−x and YH6−x superhydrides.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Baryon Number Violation Search

Understanding the fundamental forces and symmetries of nature has long been a central goal of particle physics. While the Standard Model (SM) provides a successful framework, it does not guarantee the conservation of baryon number B or lepton number L, thus motivating searches for their violation. Proton decay, a fundamental process violating B, has been at the forefront of experimental searches for decades.The discovery of the weak neutral current in 1973 unified the electromagnetic and weak forces and inspired the creation of Grand Unified Theories (GUTs) that also unify the strong force. In 1974, the first-ever GUT, proposed by Georgi and Glashow, naturally predicted proton decay. This prediction led to an experimental push to validate these theories, and a large underground detector boom was born. Initially designed for proton decay searches, these detectors later proved invaluable to neutrino physics.Although no evidence for proton decay has yet been observed, next-generation large detectors, such as the Deep Underground Neutrino Experiment (DUNE), offer the opportunity to improve on current experimental limits. Utilizing its Liquid Argon Time Projection Chamber (LArTPC) technology, DUNE is positioned to probe rare processes such as proton decay with increased sensitivity.This thesis presents a sensitivity study for the dominant proton decay mode predicted by Supersymmetric GUTs, p → K+ν, utilizing machine learning approaches. Two methods are explored in this thesis: a Boosted Decision Tree (BDT) analysis and a Graphical Neural Network (GNN) analysis with NuGraph. A lifetime limit of 5.36 ± 0.69 × 1033 years for 400 kt-yrs is found using the BDT, while the GNN achieves a lifetime limit of 6.19±1.26×1033 years for 400-kt-yrs. The NuGraph result offers better sensitivity compared to the current limit set by Super-Kamiokande of 5.90 × 1033 while the BDT result offers a slightly lower sensitivity.Additionally, this thesis discusses cross-section work, a first-ever foray into proton decay and atmospheric neutrinos in a vertical drift (VD) DUNE detector, and extensive hardware contributions to the DUNE Far Detector (FD) 1 Module-0, ProtoDUNE-2, which serves as a testbed for the final detector design and installation.

Stokes, Tyler D. [Louisiana State U.] (ORCID:00000↗
DOE OSTI2024

Search for anomalous neutral current coherent-like single-photon production in MicroBooNE

This note describes progress towards the first experimental search for neutrino-induced neutral current coherent single-photon production (NC coherent 1γ). The search makes use of data from the MicroBooNE’s 85-tonne active mass liquid argon time projection chamber detector, situated in Fermilab’s Booster Neutrino Beam, with an average neutrino energy of $\langle$E ν $\rangle$ ~ 0.8 GeV. A selection targeted on candidate neutrino interactions with a single photon-like electromagnetic shower in the final state and no visible vertex activity was developed to search for this rare NC coherent 1γ process.

43 PARTICLE ACCELERATORS↗
DOE OSTI2021

Slot-die-coating operability windows for polymer electrolyte membrane fuel cell cathode catalyst layers

Roll-to-roll (R2R) slot-die coating of polymer electrolyte membrane fuel cell (PEMFC) catalyst layers represents a scalable deposition method for producing 10–20 m 2 ·min -1 of catalyst-coated gas diffusion layers (GDLs). This high-throughput production technique will help lower the cost of PEMFC catalyst layers. The uniformity of the wet layer applied by slot die deposition is affected by process parameters such as substrate speed, vacuum pressure applied at the upstream meniscus, gap between the slot die lips and substrate, ink rheology, and other ink and substrate properties. The set of conditions for producing a defect-free coating with a dilute ink typically requires little to no upstream vacuum pressure, so suitable operating conditions can be found easily through trial and error and operator intuition. However, the higher viscosity of more concentrated inks dramatically shifts the range of settings that result in a homogeneous coating to higher vacuum levels, which are harder to find through hit or miss. A predictive model showing the range of operable conditions decreases material wastage inherent in experimentally searching for suitable parameters. In this study, the defect-free coating parameter window is explored experimentally and theoretically for two concentrations of PEFC cathode inks. Both a full capillary hydrodynamic model and a computationally cheaper viscocapillary model successfully predict the experimentally determined coating window within the experimental and model uncertainty limits for inks with 5.3 wt% and 12.0 wt% solids ink while maintaining the 0.1 mg Pt ·cm -2 Pt areal loading target. Here, this paper demonstrates a viable pathway for meeting the $30/kW net ultimate cost target of the United States Department of Energy (U.S. DOE) Hydrogen Fuel Cells Technologies Office (HFTO). The concentrated ink lowers the thermal energy and capital expenditure (CapEx) budget of the coating process by decreasing the amount of time, energy, and floorspace required for drying the coating.

25 ENERGY STORAGE↗
DOE OSTI2020

Searching for the Higgsino-Bino sector at the LHC

We study the search for electroweakinos at the 13 TeV LHC in the case of heavy scalar superpartners. We consider both the direct production mode and the one associated with the decay of heavy Higgs bosons, and concentrate on the case of light Higgsinos and Binos. In this case, the direct production searches becomes more challenging than in the light Wino scenario. In the direct production mode, we use the current experimental searches to set the reach for these particles at larger luminosities, and we emphasize the relevance of considering both the neutral gauge boson and the neutral Higgs decay modes of the second and third lightest neutralino. We show the complementarity of these searches with the ones induced by the decay of the heavy Higgs bosons, which are dominated by the associated production of the lightest neutralino with the second and third lightest ones, with the latter decaying into gauge bosons. We show that, depending on the value of tan β , the Higgs boson decay channel remains competitive with the direct production channel up to heavy Higgs boson masses of about 1 TeV. Moreover, this search is not limited by the same kinematic considerations as the ones in the direct production mode and can cover masses up to the kinematic threshold for the decay of the heavier electroweakinos into the lightest neutralino. This decay mode provides also an alternative way of looking for heavy Higgs bosons in this range of masses and hence should be a high priority for future LHC analyses.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗