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At least 19 records

Highly charged ion approach to measure nuclear charge radii of Fr, Ra, and Rn isotopes for precision measurements

Conventional electron scattering and muonic atom spectroscopy techniques are challenging to apply to heavy ions unless the element has at least one stable or extremely long-lived isotope. To overcome this limitation, a recently introduced method for determining nuclear charge radii relies on extreme-ultraviolet (EUV) spectroscopy of the D 1 line in highly charged Na-like ions. In this work, we present an experimental approach to measure the nuclear charge radii of isotopes of radioactive elements such as Fr, Ra, and Rn using this method at TRIUMF’s Ion Trap for Atomic and Nuclear Science (TITAN) instrument, located at the ISAC radioactive beam facility. We also explore the potential of using Na-like D 2 lines in the soft x-ray region for future measurements.

Electron beam ion trap↗

SST-TG-P1F4R3200: Decaying Stably-Stratified Turbulence (SST), Initialized Using Taylor-Green Vortices (TG) at Prandtl Number Pr=1, Froude Number Fr=4, Reynolds Number Re=3200

This dataset comprises direct numerical simulations (DNS) of decaying stably-stratified turbulence influenced by a linear background density gradient, initialized using an array of Taylor-Green vortices, as described in [Riley & de Bruyn Kops (2003)](https://doi.org/10.1063/1.1578077). The initial Prandtl, Froude, and Reynolds numbers are (Pr, Fr, Re) = (1, 4, 3200). A total of 15,000 snapshots are recorded at uniform time intervals, each with a spatial resolution of 512x512x256 grid points. Four flow variables are associated with each snapshot: the three velocity components (u,v,w) and the perturbed density field (rho) away from the background gradient. All fields are stored in binary format (32-bit little-endian), each with a size of 255 MB, yielding a total dataset size of 15.3 TB. Further details are referenced in the attached README file, and a current list of publications and associated analysis tools are provided at https://stratified-turbulence.github.io/web/.

42 ENGINEERING↗

SST-TG-P50F4R3200: Decaying Stably-Stratified Turbulence (SST), Initialized Using Taylor-Green Vortices (TG) at Prandtl Number Pr=50, Froude Number Fr=4, Reynolds Number Re=3200

This dataset comprises direct numerical simulations (DNS) of decaying stably-stratified turbulence influenced by a linear background density gradient, initialized using an array of Taylor-Green vortices, extending the Pr=1 simulations performed in [Riley and de Bruyn Kops (2003)](https://doi.org/10.1063/1.1578077). The initial Prandtl, Froude, and Reynolds numbers are (Pr, Fr, Re) = (50, 4, 3200). A total of 1,680 snapshots are recorded at uniform time intervals, each with a spatial resolution of 3584x3584x1792 grid points. Four flow variables are associated with each snapshot: the three velocity components (u,v,w) and the perturbed density field (rho) away from the background gradient. All fields are stored in binary format (32-bit little-endian), each with a size of 85.8 GB, yielding a total dataset size of 577 TB. Further details are referenced in the attached README file, and a current list of publications and associated analysis tools are provided at https://stratified-turbulence.github.io/web/.

42 ENGINEERING↗

SST-TG-P7F4R3200: Decaying Stably-Stratified Turbulence (SST), Initialized Using Taylor-Green Vortices (TG) at Prandtl Number Pr=7, Froude Number Fr=4, Reynolds Number Re=3200

This dataset comprises direct numerical simulations (DNS) of decaying stably-stratified turbulence influenced by a linear background density gradient, initialized using an array of Taylor-Green vortices, extending the Pr=1 simulations performed in [Riley and de Bruyn Kops (2003)](https://doi.org/10.1063/1.1578077). The initial Prandtl, Froude, and Reynolds numbers are (Pr, Fr, Re) = (7, 4, 3200). A total of 15,250 snapshots are recorded at uniform time intervals, each with a spatial resolution of 1280x1280x640 grid points. Four flow variables are associated with each snapshot: the three velocity components (u,v,w) and the perturbed density field (rho) away from the background gradient. All fields are stored in binary format (32-bit little-endian), each with a size of 4 GB, yielding a total dataset size of 244 TB. Further details are referenced in the attached README file, and a current list of publications and associated analysis tools are provided at https://stratified-turbulence.github.io/web/.

42 ENGINEERING↗

Materials (FR 2023 Annual Progress Report)

This document summarizes the progress of VTO Materials R&D projects supported during the fiscal year 2023. The Propulsion Materials portfolio is closely aligned with other VTO subprograms to identify critical materials needs for next-generation high-efficiency powertrains for both heavy- and light-duty vehicles. The Lightweight Materials portfolio works closely with industry through the U.S. DRIVE Partnership to understand light-duty vehicle structural weight-reduction goals and identify technical challenges that prevent the deployment of lightweight materials.

33 ADVANCED PROPULSION SYSTEMS↗

Electric-Field Manipulation of Magnetic Chirality in a Homo-Ferro-Rotational Helimagnet

Ferro-rotational (FR) materials, renowned for their distinctive material functionalities, present challenges in the growth of homo-FR crystals (i.e., single FR domain). This study explores a cost-effective approach to growing homo-FR helimagnetic RbFe(SO 4 ) 2 (RFSO) crystals by lowering the crystal growth temperature below the T FR threshold using the high-pressure hydrothermal method. Through polarized neutron diffraction experiments, it is observed that nearly 86% of RFSO crystals consist of a homo-FR domain. Notably, RFSO displays remarkable stability in the FR phase, with an exceptionally high T FR of ≈573 K. Furthermore, RFSO exhibits a chiral helical magnetic structure with switchable ferroelectric polarization below 4 K. Importantly, external electric fields can induce a single magnetic domain state and manipulate its magnetic chirality. The findings suggest that the search for new FR magnets with outstanding material properties should consider magnetic sulfates as promising candidates.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Dependence of wind-farm-induced gravity waves and wind farm performance on non-dimensional atmospheric parameters and simulation configuration

This large-eddy simulation (LES) study examines how wind-farm-induced atmospheric gravity waves (AGWs) and wind farm performance depend on non-dimensional atmospheric parameters and simulation configuration. A hypothetical aligned wind farm of actuator disks is simulated under neutral surface conditions, with a stable capping inversion and a mildly stable free atmosphere, to assess the effects of stratification beyond the atmospheric boundary layer (ABL) on ABL flow. Simulation set-ups fully resolving AGWs are validated to minimize spurious wave generation and reflection from the domain boundaries. The validated set-up is then used to analyze AGW types and characteristics, as well as stratification impacts under conventionally neutral boundary layer (CNBL) conditions. These conditions are governed by four non-dimensional parameters: the Froude numbers of the free atmosphere and capping inversion (Fr, Fr i ), and the aspect ratios of the ABL and wind farm (H̃ i , S h ). Simulation configurations that fully resolve AGWs – capturing at least one wavelength both horizontally and vertically – yield the most realistic stratification effects on ABL flow, whereas partial or unresolved configurations produce non-physical, channel-like behavior. A coherent description of the AGW phenomena is provided, highlighting the central role of capping inversion displacement in linking ABL fluctuations with AGWs. Trapped waves are confined within the capping inversion, while interfacial and internal waves aloft are identified as the AGW types most relevant to wind farm performance. The wavy inversion, analogous to an interfacial wave, forms converging and diverging zones that drive power fluctuations across the farm. The interfacial wavelength, measured over the wind farm, corresponds to one diverging, one converging, and one mildly diverging zone. As the interfacial wavelength decreases with Fr i , multiple convergence–divergence zones develop under sub-critical conditions (Fr i <1.0), while for super-critical conditions (Fr i > 1.0), the wavelength approaches the farm length. Wave amplitude increases with decreasing H̃ i (i.e., shallower capping inversions). Wind farm performance is most sensitive to H̃ i : shallow boundary layers increase blockage and reduce efficiency, while deeper layers enhance efficiency. Increasing Fr and Fr i mitigates blockage, and increasing S h mainly improves wake recovery. Although local power fluctuations arise from AGWs, overall wind farm efficiency remains nearly constant with Fr and Fr i , improving primarily with larger H̃ i and S h .

17 WIND ENERGY↗

Beyond the visible: Accounting for ultraviolet and far‐red radiation in vegetation productivity and surface energy budgets

Photosynthetically active radiation (PAR) is typically defined as light with a wavelength within 400–700 nm. However, ultra-violet (UV) radiation within 280–400 nm and far-red (FR) radiation within 700–750 nm can also excite photosystems, though not as efficiently as PAR. Vegetation and land surface models (LSMs) typically do not explicitly account for UV's contribution to energy budgets or photosynthesis, nor FR's contribution to photosynthesis. However, whether neglecting UV and FR has significant impacts remains unknown. Here, we explored how canopy radiative transfer (RT) and photosynthesis are impacted when explicitly implementing UV in the canopy RT model and accounting for UV and FR in the photosynthesis models within a next-generation LSM that can simulate hyperspectral canopy RT. We validated our improvements using photosynthesis measurements from plants under different light sources and intensities and surface reflection from an eddy-covariance tower. Our model simulations suggested that at the whole plant level, after accounting for UV and FR explicitly, chlorophyll content, leaf area index (LAI), clumping index, and solar radiation all impact the modeling of gross primary productivity (GPP). At the global scale, mean annual GPP within a grid would increase by up to 7.3% and the increase is proportional to LAI; globally integrated GPP increases by 4.6 PgC year −1 (3.8% of the GPP without accounting for UV + FR). Further, using PAR to proxy UV could overestimate surface albedo by more than 0.1, particularly in the boreal forests. Our results highlight the importance of improving UV and FR in canopy RT and photosynthesis modeling and the necessity to implement hyperspectral or multispectral canopy RT schemes in future vegetation and LSMs.

energy budget↗

RG-CAT: Detection pipeline and catalogue of radio galaxies in the EMU pilot survey

Abstract We present source detection and catalogue construction pipelines to build the first catalogue of radio galaxies from the 270$\rm deg^2$pilot survey of the Evolutionary Map of the Universe (EMU-PS) conducted with the Australian Square Kilometre Array Pathfinder (ASKAP) telescope. The detection pipeline uses Gal-DINO computer vision networks (Gupta et al. 2024, PASA, 41, e001) to predict the categories of radio morphology and bounding boxes for radio sources, as well as their potential infrared host positions. The Gal-DINO network is trained and evaluated on approximately 5 000 visually inspected radio galaxies and their infrared hosts, encompassing both compact and extended radio morphologies. We find that the Intersection over Union (IoU) for the predicted and ground-truth bounding boxes is larger than 0.5 for 99% of the radio sources, and 98% of predicted host positions are within$3^{\prime \prime}$of the ground-truth infrared host in the evaluation set. The catalogue construction pipeline uses the predictions of the trained network on the radio and infrared image cutouts based on the catalogue of radio components identified using theSelavysource finder algorithm. Confidence scores of the predictions are then used to prioritiseSelavycomponents with higher scores and incorporate them first into the catalogue. This results in identifications for a total of 211 625 radio sources, with 201 211 classified as compact and unresolved. The remaining 10 414 are categorised as extended radio morphologies, including 582 FR-I, 5 602 FR-II, 1 494 FR-x (uncertain whether FR-I or FR-II), 2 375 R (single-peak resolved) radio galaxies, and 361 with peculiar and other rare morphologies. Each source in the catalogue includes a confidence score. We cross-match the radio sources in the catalogue with the infrared and optical catalogues, finding infrared cross-matches for 73% and photometric redshifts for 36% of the radio galaxies. The EMU-PS catalogue and the detection pipelines presented here will be used towards constructing catalogues for the main EMU survey covering the full southern sky.

Astronomy & Astrophysics↗

Use of Fisher's Ratio assisted multivariate curve resolution- alternating least squares for discovery-based analysis using ultrahigh pressure liquid chromatography-high resolution mass spectrometry

Non-targeted analysis of complex chemical mixtures can be difficult considering the convoluted nature of the matrix and the potential unknown chemical differences between samples or classes of samples. Ultrahigh pressure liquid chromatography coupled to quadrupole time-of-flight mass spectrometry (UHPLC-QTOF) is an ideal technique to probe chemical differences for a wide variety of samples. While UHPLC-QTOF can discover minute chemical differences down to low part per billion (ppb) concentrations with a high degree of confidence, the application of high-resolution mass spectrometry can yield massive amounts of information (∼ 10 gb per sample) that cannot be analyzed manually. Therefore, the application of chemometric techniques is mandatory for the interrogation of complex samples. Fisher's ratio (FR) assisted multivariate curve resolution-alternating least squares (MCR-ALS) was used to the discover and identify the chemical differences between two classes of materials: 1) a pond water matrix and 2) the matrix spiked with a pharmaceutical standard mix containing 17 compounds. Thirteen of the seventeen spiked compounds were discovered using FR analysis, and then five were successfully deconvoluted using MCR-ALS wherein the number of curves chosen were automatically determined using singular value decomposition (SVD). In conclusion, the use of an automated FR assisted MCR-ALS will aid in discovering trace levels of chemical components without the need for the researcher to provide potentially biased input which will aid in non-targeted workflow.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Front-Surface Potential of Platinized p -InP Photocathodes Probed by Dual-Working-Electrode Measurements

The front-surface potential (E fr ) of p-InP/Pt photocathodes performing the hydrogen-evolution reaction has been probed under operating conditions using a dual-workingelectrode (DWE) method. The DWE data are consistent with expectations for proposed stability mechanisms for p-InP photocathodes. Specifically, E fr for Pt-modified p-InP adopts a value near the reversible hydrogen electrode (RHE) potential, consistent with kinetic suppression of metallic In 0 formation. The data provide a rapid, operando metric of interfacial catalyst activity, and indicate that E fr for the p-InP/Pt junction is governed by surface catalytic kinetics rather than by the applied back-contact potential (E b ).

Catalysts↗

Investigation of Fe-Ni Battery/Module for Grid Service Duty Cycles

Iron–nickel (Fe-Ni) batteries are renowned for their durability and resilience against overcharging and operating temperatures. However, they encounter challenges in achieving widespread adoption for energy storage applications due to their low efficiency and the need for regular maintenance and electrolyte replacement, which adds to maintenance costs. This study evaluates and demonstrates the capabilities of Fe-Ni batteries for participating in grid energy storage applications. Stable performance was observed frequency regulation (FR) testing at 100% and 50% state of charge (SOC)s, while at 50% SOC, there was a 14% increase in efficiency compared to 100% SOC. Although 25% SOC achieved higher efficiency, limited cyclability was observed due to reaching the discharge cutoff voltage. Optimal SOC selection, battery monitoring, maintenance, and appropriate charging strategies of Fe-Ni batteries seem to be crucial for their FR applications. Fe-Ni batteries exhibit stable peak shaving (PS) results, indicating their suitability and reliability under various load conditions for PS testing. Extended cycling tests confirm their potential for long-term grid-scale energy storage, enhancing their appeal for PS and FR applications.

25 ENERGY STORAGE↗

Recommendations on setup in simulating atmospheric gravity waves under conventionally neutral boundary layer conditions

Wind farm-induced atmospheric gravity waves have been the subject of recent research as they can impact wind farm performance. Pressure variations associated with gravity waves can contribute to the global blockage effect and wind farm wake recovery. Therefore, accurate numerical simulation of flow fields, where wind-farm-induced gravity waves may be produced, is important. Three main considerations in such simulations are the overall domain size, the use of Rayleigh damping near domain boundaries to dampen gravity waves, and advection damping at the inlet to prevent spurious oscillations. Often these considerations are treated ad hoc rather than systematically. This work aims to test and extend the systematic modelling of internal gravity waves proposed in a preliminary investigation to modelling of both internal and trapped gravity waves. The preliminary study identifies the length scales to set the domain and damping layer sizes and the time scale to configure the Rayleigh damping coefficient but under linearly stratified conditions. Large eddy simulations of flow through a wind farm canopy are performed under conventionally neutral boundary layer (CNBL) conditions to test the validity of proposed setups for CNBL conditions. Background atmospheric parameters, such as Froude number (Fr), inversion height (H i ), and inversion layer Froude number (Fr i ) control most of the atmospheric gravity wave characteristics. We validated for CBNL conditions that the effective wavelengths of the internal gravity waves are the correct length scale to configure the domain size and damping layer thickness. Likewise, the optimum damping coefficient to dampen the internal gravity waves relates to the free atmosphere's buoyancy frequency or buoyant perturbations' time scale. We infer that the damping coefficient in the inversion layer may relate to the inversion buoyancy frequency to effectively dampen the trapped gravity waves. Moreover, the advection damping length is linked to the horizontal wavelength of the trapped gravity waves in the inversion layer to prevent spurious waves at the inlet by retaining wave energy accumulation.

17 WIND ENERGY↗

Characterization of a multi-kW, large-aperture gas-cooled Faraday rotator

We characterize a large-aperture gas-cooled Faraday rotator (FR) designed to mitigate stress-induced depolarization in high-energy, high-power laser systems. The rotator, based on ceramic TGG, was tested using a 150 mW probe beam at 1047 nm and a pump beam at 1070 nm. Compensating for the birefringence induced by the surrogate depolarization plate at 3.3 kW of effective pump power, the rotator reduces the spatially in-homogeneous depolarized light containing linear, circular, and elliptical polarization states to nearly linear with approximately 0.8% (or −21 dB) of residual depolarized energy. The FR demonstrated effective depolarization compensation across its 58×58 mm 2 aperture.

47 OTHER INSTRUMENTATION↗

Recommended Nuclear Structure and Decay Data for A=206 Isobars

Here, evaluated nuclear structure and decay data for all nuclei with mass number A=206 ( 206 Pt, 206 Au, 206 Hg, 206 Tl, 206 Pb, 206 Bi, 206 Po, 206 At, 206 Rn, 206 Fr, 206 Ra and 206 Ac), are presented. All available experimental data are compiled and evaluated, and best values for level and γ-ray energies, quantum numbers, lifetimes, γ-ray intensities and transition probabilities, as well as other nuclear properties, are recommended. Inconsistencies and discrepancies that exist in the literature are discussed. A number of computer codes (https://www-nds.iaea.org/public/ensdf_pgm/) developed by members of the NSDD network were used during the evaluation process. This work supersedes the earlier evaluation by F.G. Kondev (2008Ko21), published in Nuclear Data Sheets 109, 1527 (2008).

Kondev, F. G. [Argonne National Laboratory (ANL), ↗

Nuclear Structure and Decay Data for A=220 Isobars

Here, this work presents a comprehensive and critical evaluation of experimental nuclear spectroscopic data from reactions and decays for all 11 known nuclides with mass number A=220 (Pb, Bi, Po, At, Rn, Fr, Ra, Ac, Th, Pa, and Np). Recommended values are produced for level energies, spins and parities, half-lives, and radiation properties including energies, branching ratios, and multipolarities of γ rays, as well as characteristics of β and α radiation decays, based on all available experimental data. This work supersedes previous A=220 evaluations: 2011Br05, 1997Ar04, 1986Ma45, 1976El04.

Chen, J. [Michigan State University, East Lansing,↗

Radiative lifetime of the A Π 1 / 2 2 state in RaF with relevance to laser cooling

The radiative lifetime of the A Π 1 / 2 2 ( v = 0 ) state in radium monofluoride (RaF) is measured to be 35(1) ns. The lifetime of this state and the related decay rate Γ = 2.86 ( 8 ) × 10 7 s − 1 are of relevance to the laser cooling of RaF via the optically closed A Π 1 / 2 2 ← X Σ 1 / 2 2 transition, which makes the molecule a promising probe to search for new physics. RaF is found to have a comparable photon-scattering rate to homoelectronic laser-coolable molecules. Owing to its highly diagonal Franck-Condon matrix, it is expected to scatter an order of magnitude more photons than other molecules when using just three cooling lasers, before it decays to a dark state. The lifetime measurement in RaF is benchmarked by measuring the lifetime of the 8 P 3 / 2 state in Fr to be 83(3) ns, in agreement with literature. Published by the American Physical Society 2024

Optics↗