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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
NASA NTRS1975

Design, fabrication, and operation of capsules for the irradiation testing of candidate advanced space reactor fuel pins

Fuel irradiation experiments were designed, built, and operated to test uranium mononitride (UN) fuel clad in tungsten-lined T-111 and uranium dioxide fuel clad in both tungsten-lined T-111 and tungsten-lined Nb-1% Zr. A total of nine fuel pins was irradiated at average cladding temperatures ranging from 931 to 1015 C. The UN experiments, capsules UN-4 and -5, operated for 10,480 and 10,037 hr, respectively, at an average linear heat generation rate of 10 kW/ft. The UO2 experiment, capsule UN-6, operated for 8333 hr at an average linear heat generation rate of approximately 5 kW/ft. Following irradiation, the nine fuel pins were removed from their capsules, externally examined, and sent to the NASA Plum Brook Facility for more detailed postirradiation examination. During visual examination, it was discovered that the cladding of the fuel pin containing dense UN in each of capsules UN-4 and -5 had failed, exposing the UN fuel to the NaK in which the pins were submerged and permitting the release of fission gas from the failed pins. A rough analysis of the fission gas seen in samples of the gas in the fuel pin region indicated fission gas release-to-birth rates from these fuel pins in the range of .00001.

Thoms, K. R.↗
DOE OSTI2024

Qualification and Quantification of Porosity at the Top of the Fuel Pins in Metallic Fuels Using Image Processing

Approximately 130,000 metal fuel pins were irradiated in the Experimental Breeder Reactor II (EBR-II) during its 30 years of operation to develop and characterize existing and prospective fuels. For many of the metal fuel irradiation experiments, neutron radiography imaging was performed to characterize fuel behavior, such as fuel axial expansion. While several fuel expansion results obtained from neutron radiography imaging have been published, the analysis of neutron radiography for the purpose of describing statistical properties of porous matter formed on top of the fuel pins, also referred to as fluff in previous publications, is significantly less represented in the literature with just a single paper so far. This study aims to validate and augment results reported in previous publications using automated image processing. The paper describes the statistical properties of the porous matter in terms of nine parameters derived from radiography images and correlates those parameters with such fuel properties as composition, expansion, temperature, and burnup. The reported results are based on 1097 fuel pins of eight different fuel compositions. For three major fuel types, U-10Zr, U-8Pu-10Zr, and U-19Pu-10Zr, a clear negative correlation is found between the Pu content and five parameters describing the amount of porous matter generated. The parameters describing granularity properties, however, showed either negative correlation or nonlinear dependency from fuel composition. The parameters describing the amount showed a positive correlation with fuel axial expansion, while granularity parameters showed a negative correlation with axial expansion. The dependency on cladding temperature was found to be weak. A positive correlation is demonstrated for volume parameters and fuel burnup. In general, reported results confirm and validate findings published in previous studies using a much larger number of pins and automated processing techniques, which easily lend themselves to reproducibility, thus avoiding subjective bias.

36 MATERIALS SCIENCE↗
DOE OSTI2019

One-way coupled simulation of FIV in a 7-pin wire-wrapped fuel pin bundle

A normal fuel geometry found in sodium cooled reactor designs is the hexagonal lattice of wire-wrapped fuel pins. The wire-wrappers, which replace the more common spacer grids, act as a spacer between the fuel pins, while simultaneously increasing the fluid mixing between subchannels. The induced transverse flow, while good for mixing, increases the force load experienced by the fuel pins, increasing the possibility of problematic flow induced vibrations. The primary source of vibrations is turbulent buffeting, so very small in amplitude, but capable of rupturing the fuel cladding by fretting. The vast majority of research on fretting has been for bare rods with spacer grids. There are several significant ways that wire-wrapped fuel pins differ from bare rods that may have significant impact on the vibrations present. The increased transverse flow and asymmetrical flow pattern may result in larger and imbalanced force loads on the pins. The helical bracing of each pin may result in unique vibration patterns, and gaps may form between pins affecting how they are braced. Simulation allows for the observation of the forces present, how the flow field affects these forces, and how the structure responds and can be repeated for multiple cases for relatively low cost. Here, simulation of the flow induced vibrations for a 7-pin wire-wrapped fuel pin bundle is carried out by coupling Nek5000, a spectral element LES/DNS solver with DIABLO, a finite element CSM solver. The small amplitude vibrations allow for the assumption that the structure motion has negligible effect on the fluid flow, permitting the much less computationally expensive one-direction coupling. In order to gather significant force history data for the 2.63 helical pitch structure, a scheme was developed to artificially create force history from the power spectrum density of the one-pitch CFD simulation forces. The vibrations could then be simulated in the structure multiple times varying the contact and gaps between various pins. This provides for the search of worst-case scenarios and informs about the types of fretting that might be present. The simulation geometry is based on an experiment for comparison. However, the viscosity of the simulation was increased by a factor of four to make the simulation computationally feasible. While validation is not possible, comparisons are still valuable.

42 ENGINEERING↗
NASA NTRS1973

Irradiation of TZM: Uranium dioxide fuel pin at 1700 K

A fuel pin clad with TZM and containing solid pellets of uranium dioxide was fission heated in a static helium-cooled capsule at a maximum surface temperature of 1700 K for approximately 1000 hr and to a total burnup of 2.0 percent of the uranium-235. The results of the postirradiation examination indicated: (1) A transverse, intergranular failure of the fuel pin occurred when the fuel pin reached 2.0-percent burnup. This corresponds to 1330 kW-hr/cu cm, where the volume is the sum of the fuel, clad, and void volumes in the fuel region. (2) The maximum swelling of the fuel pin was less than 1.5 percent on the fuel-pin diameter. (3) There was no visible interaction between the TZM clad and the UO2. (4) Irradiation at 1700 K produced a course-grained structure, with an average grain diameter of 0.02 centimeter and with some of the grains extending one-half of the thickness of the clad. (5) Below approximately 1500 K, the irradiation of the clad produced a moderately fine-grained structure, with an average grain diameter of 0.004 centimeter.

Mcdonald, G. E.↗
DOE OSTI2021

CFD analysis of a solid pin-fueled small modular fluoride salt-cooled reactor

A computational fluid dynamics (CFD) study is performed for the pre-conceptual solid pin-fueled small modular fluoride salt-cooled reactor developed by the Oak Ridge National Laboratory (ORNL). The solid and fluid regions in a 1/12th section of a fuel assembly are modeled. The solid region includes fuel and non-fuel pins, with heat generation in the active region of the fuel pins. Two different power profiles, uniform and center-peaked, are considered. The FLiBe coolant flows from the bottom to the top of the core, parallel to the bank of fuel and non-fuel pins. The k-ω shear-stress transport (SST) model is chosen as the baseline turbulence model. The effects of grid refinement, inlet turbulence specification, and turbulence models on the temperature and pressure drop predictions are studied. Turbulence model sensitivity is investigated by comparing the results from the k-ω SST model with other two-equation models (k-ω baseline or BSL and k-ε realizable) as well as with anisotropic Reynolds stress transport models (linear pressure-strain and stress-BSL). Here the results show that the choice of turbulence model has a significant impact on the pin temperature and bundle pressure drop predictions. The results from the baseline turbulence model show good agreement between the fuel pin temperatures and bundle pressure drop values predicted using a subchannel model previously developed by the authors of the present study.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2026

EDS Analysis of FCCI in AFC-FAST Fuel Pins

The Advanced Fuel Campaign’s Fission Accelerated Steady-state Testing (FAST) program uses metallic fuel pins with small diameters to reach a desired burnup more quickly. This enables accelerated testing of advanced fuel designs and decreases the time between idea conception and commercial usage. Post-irradiation examination is critical in this process, especially with respect to the fuel-cladding chemical interactions (FCCI). In this work, energy dispersive X-ray spectroscopy (EDS) is used to track how elements from the fuel and fission products have diffused through the cladding. Elemental redistribution along the fuel-cladding interface is mapped and FCCI region thicknesses are measured. The correlations between geometry, temperature, burnup, and FCCI thickness are presented.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRS1972

Results of a preliminary experimental investigation of a vapor transport fuel pin

In-Pile experimental tests were conducted on two fuel pins mounted side-by-side in a holder assembly. The fuel pins consisted of stacked fully enriched UO2 pellets enclosed in a type 316 stainless steel clad 1/2 inch outside diameter and 3 inches in length. Each fuel pin contained four pellets for a total of 22 grams of fuel weight. The experiment was operated to maintain the maximum clad temperature at 395 K corresponding to a fuel temperature at the central void surface of 2350 K. Total primary coolant water flow past the pin holder was calculated to be 110 gallons per minute. Forty-four gallons per minute at a velocity of 36.5 feet per second flowed around each fuel pin. Calculations indicated the maximum heat flux was at the point of the highest temperature and was equal to 0.24 kW/sq cm or 7.62 Btu/hr sq ft. A series of high resolution neutron radiographs of the nuclear fueled vapor transport capsule was taken. The thermal neutrons emitted from the core of the 60 megawatt Plum Brook reactor facility were used.

Lanzo, C. D.↗
DOE OSTI2021

Cladding Profilometry Analysis of Experimental Breeder Reactor-II Metallic Fuel Pins with HT9, D9, and SS316 Cladding

BISON finite element method fuel performance simulations were conducted using an existing automated process that couples the Fuels Irradiation & Physics Database (FIPD) and the Integral Fast Reactor Materials Information System database by writing input files and comparing the BISON output to post-irradiation fuel pin profilometry measurements contained within the databases. The importance of this work is to demonstrate the ability to benchmark fuel performance metallic fuel models within BISON using Experimental Breeder Reactor-II fuel pin data for a number of similar pins, while building off previous modeling efforts. Changes to the generic BISON input file include implementing pin specific axial power and flux profiles, pin specific fluences, frictional contact, and irradiation-induced volumetric swelling models for cladding. A statistical analysis of irradiation-induced volumetric swelling models for HT9, D9, and SS316 was performed for experiments X421/X421A, X441/X441A, and X486. Between these three experiments, there were 174 post-irradiation examination (PIE) profilometries used for validating the swelling models presented using a standard error of the estimate (SEE) method. Implementation of the volumetric swelling models for D9 and SS316 claddings was found to have a significant impact on the BISON profilometry simulated, where HT9 clad pins had an insignificant change due to low fluence values. BISON profilometry simulated for HT9, D9, and SS316 fuel pins agreed with PIE profilometry measurements, with assembly SEE values being 4.4 × 10−3 for X421A, 2.0 × 10−3 for X441A, and 2.8 × 10−3 for X486. D9 clad pins in X421/X421A had the highest SEE values, which is due to the BISON simulated profilometry being shifted axially. While this work accomplished its purpose to demonstrate the modeling of multiple fuel pins from the databases to help validate models, the results suggest that the continued development of metallic fuel models is necessary for qualifying new metallic fuel systems to better capture some physical performance phenomena, such as the hot pressing of U-Pu-Zr and the fuel cladding chemical interaction.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2017

Detection of Fuel Pin Diversion via Fast Neutron Emission Tomography

Oak Ridge National Laboratory is developing a new capability to perform passive fast neutron emission tomography of spent nuclear fuel. The goal of this capability is to detect vacancies or substitutions of individual fuel pins in spent nuclear fuel assemblies for international safeguards applications, such as verifying the integrity of an assembly prior to transfer to “difficult to access” storage. Emission tomography uses collimation to isolate activity along “lines of response” through an object. By combining many collimated views through an object, the neutron emission from each fuel pin can be mathematically extracted and an image of the fuel assembly can be constructed. However, performing fast-neutron imaging is challenging for the very reason that it is desirable, namely, that fast neutrons penetrate a good deal of shielding and are consequently difficult to collimate and measure with high resolution. For spent fuel, additional challenges include the modest neutron source strength and the overwhelming gamma-ray emissions. While the International Atomic Energy Agency (IAEA) is presently investigating the use of passive gamma emission tomography for the same application, it is useful to investigate neutron emission tomography because fast neutrons better penetrate larger fuel assemblies and because fast neutrons (originating primarily from curium-244 which is mainly produced at the end of the exposure cycle) may be sensitive to replacement fuel pins that are subsequently irradiated. In the present work, we present a novel collimator concept that will enable rapid transaxial tomographic imaging of spent nuclear fuel using the spontaneous fast neutron emissions from the fuel. Initial design simulations of an imager based on this collimator indicate sufficient resolution to identify individual fuel pins. Employing such a collimator, the resulting imager can be sufficiently compact, efficient, and radiation resistant to make fast neutron emission imaging practical.

Iyengar, Anagha↗
DOE OSTI2017

Fuel pin zoning to improve the accuracy of the palisades spent fuel pool criticality analysis

Most PWR spent fuel pool criticality analyses assume that the burnup is uniformly distributed among the fuel pins in the assembly. This assumption is accurate for PWR cores that have the typical small inter-assembly gap. The Palisades reactor core, however, is different in that it uses cruciform control rods in between fuel assemblies. Every interior assembly has two sides having a wide water gap and two sides having a narrow water gap. After depleting under these conditions, the pins near the wide water gap will have a higher burnup than the pins in the center. If the burnup is distributed uniformly among the pins, the resulting k calculation will be conservative but excessively so. The excess conservatism was found to be on the order of 1% in k. For this analysis, SCALE 6.1 depletion with TRITON is used followed by the CSAS5 module for the Palisades pool analysis. Several burnup zoning arrangements (uniform enrichment) were investigated ranging from 3 zones to as many as 19 zones. The 19 zone analysis agreed well with a CASMO analysis where every pin was its own depletion zone. It was found that 8 fuel zones gave essentially the same result as 19 zones with less complexity. The depletion calculation using 8 fuel zones instead of a single zone is more complicated but the resulting k calculation no longer has the excessive conservatism seen in a one zone model. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRS1973

Examination of T-111 clad uranium nitride fuel pins irradiated up to 13,000 hours at a clad temperature of 990 C

The examination of 27 fuel pins irradiated for up to 13,000 hours at 990 C is described. The fuel pin clad was a tantalum alloy with uranium nitride as the nuclear fuel. Two nominal fuel pin diameters were tested with a maximum burnup of 2.34 atom percent. Twenty-two fuel pins were tested for fission gas leaks; thirteen pins leaked. Clad ductility tests indicated clad embrittlement. The embrittlement is attributed to hydrogen from an n,p reaction in the fuel. Fuel swelling was burnup dependent, and the amount of fission gas release was low, generally less than 0.5 percent. No incompatibilities between fuel, liner, and clad were in evidence.

Slaby, J. G.↗
NASA NTRS1973

EXFILE: A program for compiling irradiation data on UN and UC fuel pins

A FORTRAN-4 computer program for handling fuel pin data is described. Its main features include standardized output, easy access for data manipulation, and tabulation of important material property data. An additional feature allows simplified preparation of input decks for a fuel swelling computer code (CYGRO-2). Data from over 300 high temperature nitride and carbide based fuel pin irradiations are listed.

Mayer, J. T.↗
DOE OSTI2021

Initial demonstration of automated fuel performance modeling with 1977 EBR-II metallic fuel pins using BISON code with FIPD and IMIS databases

Using the BISON fuel performance code, simulations were conducted using an automated process to read initial and operating conditions from the Fuels Irradiation and Physics Database (FIPD) and Integral Fast Reactor materials information system (IMIS) database, which contains metallic fuel data from the Experimental Breeder Reactor-II (EBR-II). This work demonstrates use of an integrated framework to access the vast majority of EBR-II experimental fuel pin data to support rapid development of fuel performance models for next-generation metallic fuel systems. With this capability, validation for fuel qualification can be performed rapidly. Between IMIS and FIPD, there is enough information to conduct 1977 unique EBR-II metallic fuel pin histories from 24 different experiments, at varying levels of detail between the two databases. Each of these histories includes a high-resolution power history, flux history, coolant channel flow rates, and coolant channel temperatures. Fission gas release (FGR), cumulative damage fraction (CDF), fuel axial swelling, cladding profilometry, and burnup were all simulated in BISON. The results were compared to post-irradiation examination (PIE) results for the initial demonstration of automated BISON modeling. BISON simulations conducted with IMIS and FIPD were in rough agreement with PIE measurements and calculations. Cladding profilometry, FGR, and fuel axial swelling were found to be in rough agreement with PIE measurements, depending on the physics used within the BISON input files. Here, the mechanical contact solver chosen was found to significantly impact axial fuel swelling and cladding strain predictions. CDF values were assessed to see whether pin failure may have been predicted (CDF ≥ 1). This work suggests that continued development of an automated tool for BISON should focus on inclusion of the Fast Flux Test Facility (FFTF) experimental data for a larger database for metallic fuel, improved physical models to better capture fuel performance, such as fuel-cladding interactions, and a more detailed comparison with available PIE data to further the BISON model development.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2022

Engineering & Microstructure Scale PIE Report on EBR-II X441A Metallic Fuel Pins for the MORPH Experiment

The objectives of this project are to increase fundamental understanding of irradiation induced metallic U-Pu-Zr fuel behavior and to obtain data needed for the development of irradiation models for metallic fuels in MARMOT. The requested metallic fuel pins are from the X441A experiment irradiated in Experimental Breeder Reactor (EBR)-II and will be provided by the PIs for the duration of the experiment. The purpose of the pins irradiated in the X441A assembly was to vary Zr composition and fuel slug diameter in order to provide data for the metallic fuel performance code “LIFEMETAL” [ANL-IFR-125]. The fuels of interest to this project are metallic fuels with several Zr compositions (in wt.%): U-19Pu-6Zr, U-19Pu-10Zr, and U-19Pu-14Zr, which were irradiated to a peak burnup of approximately 11 at.%. The cladding was the same for all three fuel pins (austenitic stainless steel D9), which allows investigation of fuel-cladding interaction (FCI) phenomena. Varying Zr content in fuel pins enables investigation of the effect of Zr on fuel restructuring and fuel-cladding compatibility. Engineering and microstructure scale PIE activities will be focused on investigation of fundamental aspect of fuel performance such as species diffusion and migration, fission product behavior, and constituent redistribution. Obtained microstructural information will be used as the basis for the development of MARMOT models of U-Pu-Zr fuel performance at the mesoscale. Experimental data obtained through this proposal will be used to provide this fundamental understanding which will serve as the foundation of the development of radiation models for U-Pu-Zr in MARMOT. It will also provide a starting point for the design of new experiments to provide data for the validation of these MARMOT models.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2018

Fuel Pin Melting in a Fast Reactor and Melt Solidification: Simulation Using the SAFR/V1 Module of the EVKLID/V2 Integral Code

The approaches used in the SAFR/V1 module modeling the thermal destruction of fuel pins in fast reactors for calculating in integrated code EVKLID/V2 the melting of fuel pins and solidification of the formed melt are described. The enthalpy formulation of the heat-conduction equation is used. The numerical scheme used for the heat-conduction equation in performing the calculations is presented. The realized boundary conditions as well as a model of the gas gap in a fuel pin are described. The module’s capability of modeling heat propagation, including in the presence of a phase transition, is verified on the basis of analytical tests.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2021

Critical and Subcritical Californium Source Driven Noise Analysis Experiments with Fresh PWR Fuels Pins

These experiments were performed in 1983 between August 1 and September 16 and used 35 operational days of critical facility time at the Babcock & Wilcox critical facility in Lynchburg, Va. These measurements were to assess the capability of the Cf source driven noise analysis method to measure the subcriticality of light water reactor fresh fuel configurations. This report documents the experiments of 1983 that were not reported at that time. These measurement with 2.459 wt. % 235 U enriched uranium oxide fresh fuel pins started at the delayed critical configuration of the fully assembled pressurized water reactor (PWR) core configuration with 1511 parts per million (ppm) natural boron (19.8 wt. % 10 B) in the water. This was a cylindrical configuration of 4961 fuel pins. After the initial measurements at delayed criticality, subcritical measurements by the Cf source driven noise analysis method were performed in which the number of detectors and Cf source locations were varied. Additional boron was added to the water moderator and reflector to reduce the neutron multiplication factor, with resulting boron concentrations of 1561, 1613, 1765, 1880, 2104, 2384, 2975, 3606, and 4303 ppm. After the completion of these measurements the increased, the boron concentration was returned to that at delayed critical (1511 ppm) and the reactivity was decreased by reducing the number of fuel pins in steps to 3713, 2553, 1281, 749, and 333 fuel pins and then to that (289) of a s ingle square 17 x 17 pin array, corresponding to a single PW fuel element. For all measurement that started at delayed criticality and then reduced the neutron multiplication factor to various subcritical states, inverse kinetics rod drop measurements at the higher reactivities were also performed but not reported here. At all subcritical states the break frequency noise analysis data was fitted to obtain the prompt neutron decay constant. Some data presented in this report are from notes not in the logbook. The purpose of this report is to document the experimental information for the measurements performed so that a later date someone could perform the required uncertainty and calculational analyses and documentation to use these data for an International Nuclear Criticality Safety Benchmark Program (INCSBEP) or Nuclear Energy Agency (NEA) benchmark. The data from these measurements is available from the Laboratory Records Department of Oak Ridge National Laboratory and the logbook is available from INCSBEP at Idaho National Laboratory.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗