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At least 19 records

Metallography and fuel cladding chemical interaction in fast flux test facility irradiated metallic U-10Zr MFF-3 and MFF-5 fuel pins

Abstract The Mechanistic Fuel Failure (MFF) series of metal fuel irradiations conducted in the Fast Flux Test Facility (FFTF) provides an important potential comparison between data generated in the Experimental Breeder Reactor (EBR-II) and that expected in a larger-scale fast reactor. The irradiations were the beginning tests to qualify U-10wt%Zr as a driver fuel for FFTF. The FFTF core, with a 91.4 cm tall fuel column and a chopped cosine neutron flux profile, operated with a peak cladding temperature at the top of the fuel column, but developed peak burnup at the centerline of the core. This places the peak fuel temperature midway between the core center and the top of fuel, lower in the fuel column than in previous EBR-II experiments that had a 32-cm height core. The MFF-3 and MFF-5 qualification assemblies operated in FFTF to >10 at% burnup, and performed very well with no cladding breaches. The MFF-3 assembly operated to 13.8 at% burnup with a peak inner cladding temperature of 643°C, and the MFF-5 assembly operated to 10.1 at% burnup with a peak inner cladding temperature of 651°C. Because of the very high operating temperatures for both the fuel and the cladding, data from the MFF assemblies are most comparable to the data obtained from the EBR-II X447 experiment, which experienced two pin breaches. The X447 breaches were strongly influenced by a large amount of fuel/cladding chemical interaction (FCCI). The MFF pins benefitted from different axial locations of high burnup and peak cladding temperature, which helped to reduce interdiffusion between rare earth fission products and stainless steel cladding. Post-irradiation examination evidence illustrates this advantage. Comparing other performance data of the long MFF pins to prior EBR-II test data, the MFF fuel inside the cladding grew less axially, and the gas release data did not reveal a definitive difference.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Qualification and Quantification of Porosity at the Top of the Fuel Pins in Metallic Fuels Using Image Processing

Approximately 130,000 metal fuel pins were irradiated in the Experimental Breeder Reactor II (EBR-II) during its 30 years of operation to develop and characterize existing and prospective fuels. For many of the metal fuel irradiation experiments, neutron radiography imaging was performed to characterize fuel behavior, such as fuel axial expansion. While several fuel expansion results obtained from neutron radiography imaging have been published, the analysis of neutron radiography for the purpose of describing statistical properties of porous matter formed on top of the fuel pins, also referred to as fluff in previous publications, is significantly less represented in the literature with just a single paper so far. This study aims to validate and augment results reported in previous publications using automated image processing. The paper describes the statistical properties of the porous matter in terms of nine parameters derived from radiography images and correlates those parameters with such fuel properties as composition, expansion, temperature, and burnup. The reported results are based on 1097 fuel pins of eight different fuel compositions. For three major fuel types, U-10Zr, U-8Pu-10Zr, and U-19Pu-10Zr, a clear negative correlation is found between the Pu content and five parameters describing the amount of porous matter generated. The parameters describing granularity properties, however, showed either negative correlation or nonlinear dependency from fuel composition. The parameters describing the amount showed a positive correlation with fuel axial expansion, while granularity parameters showed a negative correlation with axial expansion. The dependency on cladding temperature was found to be weak. A positive correlation is demonstrated for volume parameters and fuel burnup. In general, reported results confirm and validate findings published in previous studies using a much larger number of pins and automated processing techniques, which easily lend themselves to reproducibility, thus avoiding subjective bias.

36 MATERIALS SCIENCE↗

One-way coupled simulation of FIV in a 7-pin wire-wrapped fuel pin bundle

A normal fuel geometry found in sodium cooled reactor designs is the hexagonal lattice of wire-wrapped fuel pins. The wire-wrappers, which replace the more common spacer grids, act as a spacer between the fuel pins, while simultaneously increasing the fluid mixing between subchannels. The induced transverse flow, while good for mixing, increases the force load experienced by the fuel pins, increasing the possibility of problematic flow induced vibrations. The primary source of vibrations is turbulent buffeting, so very small in amplitude, but capable of rupturing the fuel cladding by fretting. The vast majority of research on fretting has been for bare rods with spacer grids. There are several significant ways that wire-wrapped fuel pins differ from bare rods that may have significant impact on the vibrations present. The increased transverse flow and asymmetrical flow pattern may result in larger and imbalanced force loads on the pins. The helical bracing of each pin may result in unique vibration patterns, and gaps may form between pins affecting how they are braced. Simulation allows for the observation of the forces present, how the flow field affects these forces, and how the structure responds and can be repeated for multiple cases for relatively low cost. Here, simulation of the flow induced vibrations for a 7-pin wire-wrapped fuel pin bundle is carried out by coupling Nek5000, a spectral element LES/DNS solver with DIABLO, a finite element CSM solver. The small amplitude vibrations allow for the assumption that the structure motion has negligible effect on the fluid flow, permitting the much less computationally expensive one-direction coupling. In order to gather significant force history data for the 2.63 helical pitch structure, a scheme was developed to artificially create force history from the power spectrum density of the one-pitch CFD simulation forces. The vibrations could then be simulated in the structure multiple times varying the contact and gaps between various pins. This provides for the search of worst-case scenarios and informs about the types of fretting that might be present. The simulation geometry is based on an experiment for comparison. However, the viscosity of the simulation was increased by a factor of four to make the simulation computationally feasible. While validation is not possible, comparisons are still valuable.

42 ENGINEERING↗

CFD analysis of a solid pin-fueled small modular fluoride salt-cooled reactor

A computational fluid dynamics (CFD) study is performed for the pre-conceptual solid pin-fueled small modular fluoride salt-cooled reactor developed by the Oak Ridge National Laboratory (ORNL). The solid and fluid regions in a 1/12th section of a fuel assembly are modeled. The solid region includes fuel and non-fuel pins, with heat generation in the active region of the fuel pins. Two different power profiles, uniform and center-peaked, are considered. The FLiBe coolant flows from the bottom to the top of the core, parallel to the bank of fuel and non-fuel pins. The k-ω shear-stress transport (SST) model is chosen as the baseline turbulence model. The effects of grid refinement, inlet turbulence specification, and turbulence models on the temperature and pressure drop predictions are studied. Turbulence model sensitivity is investigated by comparing the results from the k-ω SST model with other two-equation models (k-ω baseline or BSL and k-ε realizable) as well as with anisotropic Reynolds stress transport models (linear pressure-strain and stress-BSL). Here the results show that the choice of turbulence model has a significant impact on the pin temperature and bundle pressure drop predictions. The results from the baseline turbulence model show good agreement between the fuel pin temperatures and bundle pressure drop values predicted using a subchannel model previously developed by the authors of the present study.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

EDS Analysis of FCCI in AFC-FAST Fuel Pins

The Advanced Fuel Campaign’s Fission Accelerated Steady-state Testing (FAST) program uses metallic fuel pins with small diameters to reach a desired burnup more quickly. This enables accelerated testing of advanced fuel designs and decreases the time between idea conception and commercial usage. Post-irradiation examination is critical in this process, especially with respect to the fuel-cladding chemical interactions (FCCI). In this work, energy dispersive X-ray spectroscopy (EDS) is used to track how elements from the fuel and fission products have diffused through the cladding. Elemental redistribution along the fuel-cladding interface is mapped and FCCI region thicknesses are measured. The correlations between geometry, temperature, burnup, and FCCI thickness are presented.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Cladding Profilometry Analysis of Experimental Breeder Reactor-II Metallic Fuel Pins with HT9, D9, and SS316 Cladding

BISON finite element method fuel performance simulations were conducted using an existing automated process that couples the Fuels Irradiation & Physics Database (FIPD) and the Integral Fast Reactor Materials Information System database by writing input files and comparing the BISON output to post-irradiation fuel pin profilometry measurements contained within the databases. The importance of this work is to demonstrate the ability to benchmark fuel performance metallic fuel models within BISON using Experimental Breeder Reactor-II fuel pin data for a number of similar pins, while building off previous modeling efforts. Changes to the generic BISON input file include implementing pin specific axial power and flux profiles, pin specific fluences, frictional contact, and irradiation-induced volumetric swelling models for cladding. A statistical analysis of irradiation-induced volumetric swelling models for HT9, D9, and SS316 was performed for experiments X421/X421A, X441/X441A, and X486. Between these three experiments, there were 174 post-irradiation examination (PIE) profilometries used for validating the swelling models presented using a standard error of the estimate (SEE) method. Implementation of the volumetric swelling models for D9 and SS316 claddings was found to have a significant impact on the BISON profilometry simulated, where HT9 clad pins had an insignificant change due to low fluence values. BISON profilometry simulated for HT9, D9, and SS316 fuel pins agreed with PIE profilometry measurements, with assembly SEE values being 4.4 × 10−3 for X421A, 2.0 × 10−3 for X441A, and 2.8 × 10−3 for X486. D9 clad pins in X421/X421A had the highest SEE values, which is due to the BISON simulated profilometry being shifted axially. While this work accomplished its purpose to demonstrate the modeling of multiple fuel pins from the databases to help validate models, the results suggest that the continued development of metallic fuel models is necessary for qualifying new metallic fuel systems to better capture some physical performance phenomena, such as the hot pressing of U-Pu-Zr and the fuel cladding chemical interaction.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Detection of Fuel Pin Diversion via Fast Neutron Emission Tomography

Oak Ridge National Laboratory is developing a new capability to perform passive fast neutron emission tomography of spent nuclear fuel. The goal of this capability is to detect vacancies or substitutions of individual fuel pins in spent nuclear fuel assemblies for international safeguards applications, such as verifying the integrity of an assembly prior to transfer to “difficult to access” storage. Emission tomography uses collimation to isolate activity along “lines of response” through an object. By combining many collimated views through an object, the neutron emission from each fuel pin can be mathematically extracted and an image of the fuel assembly can be constructed. However, performing fast-neutron imaging is challenging for the very reason that it is desirable, namely, that fast neutrons penetrate a good deal of shielding and are consequently difficult to collimate and measure with high resolution. For spent fuel, additional challenges include the modest neutron source strength and the overwhelming gamma-ray emissions. While the International Atomic Energy Agency (IAEA) is presently investigating the use of passive gamma emission tomography for the same application, it is useful to investigate neutron emission tomography because fast neutrons better penetrate larger fuel assemblies and because fast neutrons (originating primarily from curium-244 which is mainly produced at the end of the exposure cycle) may be sensitive to replacement fuel pins that are subsequently irradiated. In the present work, we present a novel collimator concept that will enable rapid transaxial tomographic imaging of spent nuclear fuel using the spontaneous fast neutron emissions from the fuel. Initial design simulations of an imager based on this collimator indicate sufficient resolution to identify individual fuel pins. Employing such a collimator, the resulting imager can be sufficiently compact, efficient, and radiation resistant to make fast neutron emission imaging practical.

Iyengar, Anagha↗

Fuel pin zoning to improve the accuracy of the palisades spent fuel pool criticality analysis

Most PWR spent fuel pool criticality analyses assume that the burnup is uniformly distributed among the fuel pins in the assembly. This assumption is accurate for PWR cores that have the typical small inter-assembly gap. The Palisades reactor core, however, is different in that it uses cruciform control rods in between fuel assemblies. Every interior assembly has two sides having a wide water gap and two sides having a narrow water gap. After depleting under these conditions, the pins near the wide water gap will have a higher burnup than the pins in the center. If the burnup is distributed uniformly among the pins, the resulting k calculation will be conservative but excessively so. The excess conservatism was found to be on the order of 1% in k. For this analysis, SCALE 6.1 depletion with TRITON is used followed by the CSAS5 module for the Palisades pool analysis. Several burnup zoning arrangements (uniform enrichment) were investigated ranging from 3 zones to as many as 19 zones. The 19 zone analysis agreed well with a CASMO analysis where every pin was its own depletion zone. It was found that 8 fuel zones gave essentially the same result as 19 zones with less complexity. The depletion calculation using 8 fuel zones instead of a single zone is more complicated but the resulting k calculation no longer has the excessive conservatism seen in a one zone model. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Comparison of Subdivided Versus Full-Length Fuel Pin Burnup in the ATF-2 Safety Analysis

The Accident Tolerant Fuels (ATF) campaign, under the Fuel Cycle Research and Development (FCRD) Advanced Fuels program, was developed after the Fukushima Daiichi Nuclear Power Plant disaster in 2011. Under ATF, fuel and cladding concepts are to be developed and tested that may more readily withstand an accident similar to the one that occurred at Fukushima Daiichi. ATF is a combination of industry, universities, and national laboratories in an effort to develop advanced accident tolerant cladding and fuel concepts. The end goal of the ATF program is to insert a lead test rod (LTR) or lead test assembly (LTA) into an operating commercial power light water reactor by 2022. In order to meet this 2022 insertion goal, ATF is split into three separate phases: ATF-1, ATF-2, and ATF-3. The first phase of the ATF program, ATF-1, is the concept feasibility study and early irradiation testing. Feasibility, fabrication, and out-of-pile testing are happening at universities and laboratories all over the United States. Irradiation testing of these concepts is happening at the Advanced Test Reactor (ATR) at the Idaho National Laboratory (INL). Early irradiation testing involves testing clad and/or fuel in drop-in capsules in the ATR. Currently, these capsules are in the relatively low-flux positions in the ATR, but some newer concepts and concepts that require higher burnup will be moved to the higher-flux positions later on during irradiation. Currently, Oak Ridge National Laboratory (ORNL), Westinghouse Electric Company, Areva, and General Electric (GE) have inserted capsules for ATF-1, although more concepts are planned. The second phase of ATF, ATF-2, is the focus of this paper. ATF-2 is the loop testing of fuel pins with new cladding and fuel concepts to simulate pressurized water reactor (PWR) and boiling water reactor (BWR) environments. ATF-2 will concurrently be happening at the ATR and at the Halden Reactor in Norway. The ATF-2 irradiation at the ATR will only simulate a PWR environment. ATF-2 will be inserted into the ATR pressurized water loop, Loop 2A, in the Center Flux Trap (CFT), where chemistry, temperature, and pressure can all be controlled separately from the primary coolant system and other loops in ATR. Loop 2A will be borated, pressurized to 2200 psi nominal, and have an average water temperature of 300 deg. C. A borated loop with fueled rodlets is extremely rare for Nuclear Energy experiments in the ATR, so ATF-2 will demonstrate new and unique capabilities for INL. ATF-3 is the testing of fresh and irradiated ATF concepts at the Transient Reactor Test (TREAT) Facility. The TREAT Reactor is planned for restart, re-establishing U.S. transient testing capabilities after nearly 20 years of non-operations. TREAT will test ATF concepts under transient conditions, such as a reactivity insertion accident. In addition to fresh fuel pins, TREAT will use from ATF2 and do transient testing on those irradiated pins. The information TREAT will provide to the vendors to support fuel licensing will be valuable, showing that these concepts do enhance the accident tolerance of the fuel in commercial reactors. (author)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Initial demonstration of automated fuel performance modeling with 1977 EBR-II metallic fuel pins using BISON code with FIPD and IMIS databases

Using the BISON fuel performance code, simulations were conducted using an automated process to read initial and operating conditions from the Fuels Irradiation and Physics Database (FIPD) and Integral Fast Reactor materials information system (IMIS) database, which contains metallic fuel data from the Experimental Breeder Reactor-II (EBR-II). This work demonstrates use of an integrated framework to access the vast majority of EBR-II experimental fuel pin data to support rapid development of fuel performance models for next-generation metallic fuel systems. With this capability, validation for fuel qualification can be performed rapidly. Between IMIS and FIPD, there is enough information to conduct 1977 unique EBR-II metallic fuel pin histories from 24 different experiments, at varying levels of detail between the two databases. Each of these histories includes a high-resolution power history, flux history, coolant channel flow rates, and coolant channel temperatures. Fission gas release (FGR), cumulative damage fraction (CDF), fuel axial swelling, cladding profilometry, and burnup were all simulated in BISON. The results were compared to post-irradiation examination (PIE) results for the initial demonstration of automated BISON modeling. BISON simulations conducted with IMIS and FIPD were in rough agreement with PIE measurements and calculations. Cladding profilometry, FGR, and fuel axial swelling were found to be in rough agreement with PIE measurements, depending on the physics used within the BISON input files. Here, the mechanical contact solver chosen was found to significantly impact axial fuel swelling and cladding strain predictions. CDF values were assessed to see whether pin failure may have been predicted (CDF ≥ 1). This work suggests that continued development of an automated tool for BISON should focus on inclusion of the Fast Flux Test Facility (FFTF) experimental data for a larger database for metallic fuel, improved physical models to better capture fuel performance, such as fuel-cladding interactions, and a more detailed comparison with available PIE data to further the BISON model development.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Engineering & Microstructure Scale PIE Report on EBR-II X441A Metallic Fuel Pins for the MORPH Experiment

The objectives of this project are to increase fundamental understanding of irradiation induced metallic U-Pu-Zr fuel behavior and to obtain data needed for the development of irradiation models for metallic fuels in MARMOT. The requested metallic fuel pins are from the X441A experiment irradiated in Experimental Breeder Reactor (EBR)-II and will be provided by the PIs for the duration of the experiment. The purpose of the pins irradiated in the X441A assembly was to vary Zr composition and fuel slug diameter in order to provide data for the metallic fuel performance code “LIFEMETAL” [ANL-IFR-125]. The fuels of interest to this project are metallic fuels with several Zr compositions (in wt.%): U-19Pu-6Zr, U-19Pu-10Zr, and U-19Pu-14Zr, which were irradiated to a peak burnup of approximately 11 at.%. The cladding was the same for all three fuel pins (austenitic stainless steel D9), which allows investigation of fuel-cladding interaction (FCI) phenomena. Varying Zr content in fuel pins enables investigation of the effect of Zr on fuel restructuring and fuel-cladding compatibility. Engineering and microstructure scale PIE activities will be focused on investigation of fundamental aspect of fuel performance such as species diffusion and migration, fission product behavior, and constituent redistribution. Obtained microstructural information will be used as the basis for the development of MARMOT models of U-Pu-Zr fuel performance at the mesoscale. Experimental data obtained through this proposal will be used to provide this fundamental understanding which will serve as the foundation of the development of radiation models for U-Pu-Zr in MARMOT. It will also provide a starting point for the design of new experiments to provide data for the validation of these MARMOT models.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel Pin Melting in a Fast Reactor and Melt Solidification: Simulation Using the SAFR/V1 Module of the EVKLID/V2 Integral Code

The approaches used in the SAFR/V1 module modeling the thermal destruction of fuel pins in fast reactors for calculating in integrated code EVKLID/V2 the melting of fuel pins and solidification of the formed melt are described. The enthalpy formulation of the heat-conduction equation is used. The numerical scheme used for the heat-conduction equation in performing the calculations is presented. The realized boundary conditions as well as a model of the gas gap in a fuel pin are described. The module’s capability of modeling heat propagation, including in the presence of a phase transition, is verified on the basis of analytical tests.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Critical and Subcritical Californium Source Driven Noise Analysis Experiments with Fresh PWR Fuels Pins

These experiments were performed in 1983 between August 1 and September 16 and used 35 operational days of critical facility time at the Babcock & Wilcox critical facility in Lynchburg, Va. These measurements were to assess the capability of the Cf source driven noise analysis method to measure the subcriticality of light water reactor fresh fuel configurations. This report documents the experiments of 1983 that were not reported at that time. These measurement with 2.459 wt. % 235 U enriched uranium oxide fresh fuel pins started at the delayed critical configuration of the fully assembled pressurized water reactor (PWR) core configuration with 1511 parts per million (ppm) natural boron (19.8 wt. % 10 B) in the water. This was a cylindrical configuration of 4961 fuel pins. After the initial measurements at delayed criticality, subcritical measurements by the Cf source driven noise analysis method were performed in which the number of detectors and Cf source locations were varied. Additional boron was added to the water moderator and reflector to reduce the neutron multiplication factor, with resulting boron concentrations of 1561, 1613, 1765, 1880, 2104, 2384, 2975, 3606, and 4303 ppm. After the completion of these measurements the increased, the boron concentration was returned to that at delayed critical (1511 ppm) and the reactivity was decreased by reducing the number of fuel pins in steps to 3713, 2553, 1281, 749, and 333 fuel pins and then to that (289) of a s ingle square 17 x 17 pin array, corresponding to a single PW fuel element. For all measurement that started at delayed criticality and then reduced the neutron multiplication factor to various subcritical states, inverse kinetics rod drop measurements at the higher reactivities were also performed but not reported here. At all subcritical states the break frequency noise analysis data was fitted to obtain the prompt neutron decay constant. Some data presented in this report are from notes not in the logbook. The purpose of this report is to document the experimental information for the measurements performed so that a later date someone could perform the required uncertainty and calculational analyses and documentation to use these data for an International Nuclear Criticality Safety Benchmark Program (INCSBEP) or Nuclear Energy Agency (NEA) benchmark. The data from these measurements is available from the Laboratory Records Department of Oak Ridge National Laboratory and the logbook is available from INCSBEP at Idaho National Laboratory.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Wire-Wrapped Fuel Pin Effect of Bundle Size on Temperature Distribution for Uniform Heat Flux

A common fuel arrangement for Sodium Fast Reactors (SFR) designs are hexagonal arrays of wire wrapped fuel pins. The helically wound wires redirect coolant to neighboring subchannels and increases mixing. The increased mixing of the coolant is beneficial to heat transfer from the fuel and prevents temperature peaking in hot channels that may occur. The purpose of this study is to observe the effect of bundle size on the temperature distribution of a coolant when a constant heat flux is implemented. Bundles of 19, 37, 61, and 91 pins were modeled. The wire-wrapping on fuel pins encourages interchannel mixing. With a constant heat flux the enhanced interchannel mixing has little observable effect. The temperature distributions of the subchannels has negligible dependence on radial or angular position. The temperature distribution additionally shows negligible dependence on the bundle size. The subchannel average temperatures further illustrate the homogeneity of the temperature across the bundles. Similarly oriented subchannels differ by less than two Kelvin. The temperature distribution within a single subchannel is fairly uniform, differing by about 15 K between the wall and the bulk flow, with the exception of two hot spots. The two hot spots, however, occur in two non-geometrically accurate locations, so little analysis can be performed. To better illustrate the effect of the enhanced mixing of the wire-wrapped fuel pins, a hot pin analysis should be performed to observe how the additional, non-uniform heat is dispersed. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Conjugate Heat Transfer Modeling of Salt-Filled Fuel Pins for Stable Salt Reactor Safety Analysis

The Stable Salt Reactor (SSR) combines the proven structural design of light water reactor fuel assemblies with the inherent safety and fuel-cycle advantages of molten salt technology. In its fast reactor configuration, the SSR utilizes recycled nuclear waste as fuel, sealed within narrow salt-filled fuel pins and cooled by a surrounding liquid salt coolant. Reliable transfer of heat from the molten fuel salt through the cladding to the external coolant is essential for both reactor safety and performance. This work investigates conjugate heat transfer (CHT) in the SSR’s salt-filled fuel pins using NekRS, a high-fidelity spectral element computational fluid dynamics (CFD) solver. The analyses capture internal natural convection within the molten fuel salt and external forced convection in the coolant, under steady-state and transient operating conditions. Parametric studies evaluate how variations in reactor power and coolant flow rate influence heat transfer distributions and system response. The high-fidelity CFD results are time-averaged and post-processed for direct comparison with moderate-fidelity Reynolds-averaged Navier–Stokes (RANS) models, and for the development of reduced-order models within the SAM system code. These validated models support fast-running safety analyses of normal and off-normal transients, improving predictive capability for key safety margins. By integrating advanced CFD with system-level safety tools, this study strengthens the modeling framework for SSR design, reduces uncertainty in molten salt CHT simulations, and accelerates the engineering and licensing of next-generation nuclear reactors.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Characterization of a minor actinides bearing metallic fuel pin irradiated in EBR-II

The X501 transmutation experiment irradiated in Experimental Breeder Reactor II (EBR-II) was intended to evaluate the safety and performance of the addition of minor actinides (Am, Np) into the metallic nuclear fuel system. The irradiation of this experiment is also of paramount importance for comparisons between true fast spectrum irradiations (e.g. EBR-II) and shrouded irradiation capsules performed at the thermal neutron spectrum Idaho National Laboratory Advanced Test Reactor. The X501 experimental fuel pins were irradiated to a peak measured burnup of 6.2% fission per initial heavy metal atom. This paper reports and discusses Postirradiation Examination results for one of two minor actinide bearing pins from the EBR-II X-501 experiment (X501-G591) with a focus on fuel microstructure evolution. Additionally, fuel swelling, fission product distribution, cladding strain, fission gas release, fuel microstructure and fuel cladding chemical interaction were all evaluated. The fission gas release was 79.9% and the microstructure along the fuel pin presented several characteristics very similar to other EBR-II U-Pu-Zr ternary metallic fuel experience. Minor actinides seem to not dramatically affect the overall performance of this candidate transmutation fuel. Scanning Electron Microscopy was also performed and an in-depth characterization of the different regions and phases is presented. Performance data from these irradiations can be used to inform the feasibility of minor actinide transmutation in future reactor systems.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel Performance Analysis of Fast Flux Test Facility MFF-3 and -5 Fuel Pins Using BISON with Post Irradiation Examination Data

Using the BISON fuel-performance code, simulations were conducted of an automated process to read initial and operating conditions from the Pacific Northwest National Laboratory (PNNL) database and reports, which contain metallic-fuel data from the Fast Flux Test Facility (FFTF) MFF Experiments. This work builds on previous modeling efforts involving 1977 EBR-II metallic fuel pins from experiments. Coupling the FFTF PNNL reports to BISON allowed for all 338 pins from MFF-3 and MFF-5 campaigns to be simulated. Each BISON simulation contains unique power and flux histories, axial power and flux profiles, and coolant-channel flow rates. Fission-gas release (FGR), fuel axial swelling, cladding profilometry, and burnup were all simulated in BISON and compared to available post-irradiation examination (PIE) data. Cladding profilometry, FGR, and fuel axial swelling simulation results for full-length MFF metallic pins were found to be in agreement with PIE measurements using FFTF physics and models used previously for EBR-II simulations. The main two peaks observed within the cladding profilometry were able to be simulated, with fuel-cladding mechanical interaction (FCMI), fuel-cladding chemical interaction (FCCI), and thermal and irradiation-induced creep being the cause. A U-Pu-Zr hot-pressing model was included in this work to allow pore collapse within the fuel matrix. This allowed better agreement between BISON-simulated cladding profilometry and PIE measurements for the peak caused by FCMI. This work shows that metallic fuel models used to accurately represent fuel performance for smaller EBR-II pins may be used for full-length metallic fuel, such as FFTF MFF assemblies and the Versatile Test Reactor (VTR). As new material models and PIE measurements become available, FFTF MFF assessment cases will be reassessed to further BISON model development.

36 MATERIALS SCIENCE↗