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HIGH BURNUP FUEL-COOLANT INTERACTION ANALYSIS SUPPORTING FUEL SAFETY TESTING AT IDAHO NATIONAL LABORATORY

In the near future, experiments on HBu fuel under loss-of-coolant accident (LOCA) and reactivity-initiated accident (RIA) conditions will be performed within the Transient Reactor Test Facility (TREAT) at Idaho National Laboratory (INL). These experiments will be performed using the Transient Water Irradiation System for TREAT (TWIST) experiment vehicle. To support these experiments, analysis of fuel-coolant interaction (FCI) energetics is underway. This paper discusses FCIs in the context of light water reactor (LWR) safety, differentiating between the severe accident focus of commercial reactors and experimental RIA test programs where FCIs have occurred. However, it is highlighted that as the nuclear industry aims for increased burnup limits, the FCI events observed in RIA test programs may become relevant to commercial LWR safety analysis. The paper then presents developments to the UW-FCI computer program to enable simulation of FCIs initiated by solid fuel particles dispersing into the coolant during RIAs.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel-Coolant Interaction Results for High Energy In-Pile LWR Fuels Experiments

Fuel-coolant interaction (FCI) has long been a subject of interest in severe-accident reactor safety applications. Significant chemical interaction also frequently results at the high temperature associated with these events in a water environment. Historical rapid, high energy transient irradiation test results are reviewed for experiments performed in transient experimental reactors in Idaho. Though such events are not credible for any deployed nuclear reactor technology, the pressure waves produced by FCI on surrounding containment structures are of importance to advanced light water reactor designs and for transient experiment design considerations. A brief introduction to steam explosion and related studies is provided in the context of these experiments. Extensive reactivity initiated accident testing programs were carried out in the Transient REActor Test (TREAT) facility, the Special Power Excursion Reactor Test (SPERT) facility, and the Power Burst Facility (PBF) from the 1960’s through the late 1970’s. A variety of fuel forms including waterlogged rods were tested in capsules containing water coolant at standard temperature pressure. A few tests were performed at high pressure and temperature in the water loop of PBF. In many of these experiments, energy deposition was high enough to greatly exceed melting temperatures of the fuel, resulting in some fraction of the fuel being dispersed into the coolant. A purpose of many of these tests was to determine the nuclear-to-mechanical energy conversion ratio as well as the extent of metal-water reaction. Relevant data collected from these tests included transient energy deposition, pressure response of the coolant, water column velocity, total hydrogen generation, and resulting particle size distributions and particle characterization. In this paper, the mechanical configuration of each experiment facility is reviewed and discussed relative to the measured responses. The empirical results for source pressure and extent of metal-water reaction are presented in the context of the experimental conditions. The results of these experiments provide a unique understanding for behavior of fuel under severe accident conditions in a reactor environment.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Numerical simulation on pressure propagation in fuel-coolant interaction with MCBA-simple algorithm

A computer code named METRIC is developed to simulate multiphase interactions of molten fuel and coolant at pressure propagation stage, also to examine the model's ability to predict the physical process. The fluids modeled in current code are liquid coolant, vapor, non-condensable gas, molten drop and molten fragment. Conservation equations are solved by MCBA-SIMPLE method, which comes from the mass conservation-based algorithms (MCBA) group. The numerical methods and constitutive models in the code are described in this paper. Pressure wave propagation in two-phase medium is simulated to validate current two-phase model. Computational simulation of KROTOS 21 is carried out. Parameter sensitivity study is performed. Effects of void fraction, fragment size, and fragmentation model are discussed. Results of the simulations are physically reasonable and close to the experimental observations. It is suggested that the physical models still need improved to avoid the uncertainty of empirical parameters and user effect. (authors)

42 ENGINEERING↗

The Effect of Support Rod on Film Boiling Heat Transfer for Hot Metal Sphere in Subcooled Water

In fuel-coolant interaction (FCI), the heat transfer of corium has been conventionally evaluated by the correlations with a sphere developed in boiling region for subcooled film. However, these correlations do not give significant consideration on the support rod for the sphere from their developments, although Nishio et al. pointed out that the heat transfer and the vapor film collapsing mode would depend on H/D ratio. In this study, we performed experimental tests with the SS316 sphere (10 mm) and found the noticeable increase on the heat transfer in subcooled film boiling region with the deeper immersion depth and larger diameter of support rod. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effects of Coolant Void Condition on Melt Fragmentation using Simulants in Initial Phase of Metal-fueled SFR Severe Accident

Metal fuel has inherent safety characteristics, especially in severe accident conditions. However, the metal-fueled SFR severe accident scenarios need to be categorized since overall severe accident mitigation strategies have not been prepared. In addition, these mitigation strategies should be classified in specific phases. In an initial phase of metal-fueled SFR severe accident scenarios, fuel melting, and cladding failures would occur. After the occurrence of the cladding breach, the molten metal fuel would be ejected into a coolant channel due to fission gas in fuel cavity or rapid evaporation of sodium bond. This is called Ex-pin phenomena. There are few studies considering the Ex-pin phenomena of metal fuel. Related representative studies are transient reactor test facility (TREAT) M series tests. The TREAT M series tests provided fundamental metal fuel performance in transient condition. They informed partial experimental data such as the amount of melt ejected into coolant channel after the cladding failure. However, these experimental data did not examine the melt behavior during the Ex-pin phenomena. In metal-fueled SFR, it is a known fact that the negative reactivity feedback occurs in the initial phase of severe accident. In an unprotected loss-of-flow (ULOF) accident, the void-reactivity feedback may be positive depending on where in the reactor core the sodium voiding occurs. However, molten metal fuel would be better dispersed upward compared to those of an oxide fuel and significant negative reactivity feedback could be induced through such behaviors. Thus, a key safety strategy to mitigate the accident progression at the initial phase of severe accident is to discharge melt upwards out of the core. In this paper, the upward discharge of melt is defined as melt levitation. Such melt levitation could ensure early termination of severe accident. There could be different melting behaviors inside the pin depending on reactor types or the type of fuel. In case of pressurized water reactor (PWR) oxide fuel-water system, the rapid power excursion would initiate melting of fuel at the surface of the pellets. In this paper, the ULOF accident for the metal-fueled SFR is considered as an accident scenario. To induce the melt levitation, the driving force should be clarified. Heo et al. observed a built-up vapor pressure was suggested as one of the driving forces for the upward dispersion of the molten materials. The following factors also have the potential to induce the melt levitation; the pressure induced by fission gas in the cavity or rapid boiling of sodium bond, natural circulation flow of the sodium, the sodium vapor flow generated by the difference between inlet and outlet plenum in the reactor core, the built-up vapor pressure due to the fuel-coolant interaction etc. These factors are balanced each other. They should be examined through the Ex-pin experiments. Before conducting a parametric study for each factor, the general behavior of the molten metal fuel should be investigated in the coolant channel. Since rapid sodium coolant boiling could occur in the initial phase of severe accident scenarios, the molten fuel would be ejected and fragmented in voided channel. Unlike previous studies concerning an un-voided channel, differences in melt behavior in the voided channel are expected. In present study, molten material behavior was evaluated to reveal their characteristics in voided channel. The Ex-pin experiments were performed in both un-voided and voided channel, thus such behavior differences were explicitly observed. In the lab-scale experiments, the un-voided and voided channel were reflected by coolant-filled and air-filled channel, respectively. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Thermo-hydrologic processes in maar eruptions: The role of vapor transport and condensation

Phreatomagmatic eruptions occur when magma interacts directly with water or slurries, commonly from groundwater in the shallow crust, resulting in rapid conversion of thermal energy to mechanical energy in a set of processes known as molten fuel-coolant interaction (MFCI). The efficiency of MFCI is controlled by properties of the magma and coolant, contact surface geometry, and system conditions, such as pressure and temperature; phreatomagmatic behavior can range from passive thermal granulation to violent thermohydraulic explosions (Zimanowski et al., 2015). Maar-diatreme eruptions, characterized by repetitive phreatomagmatic explosions, can form in a wide range of near-surface environments, from soft sediment substrate (e.g., Tecuitlapa, Mexico, Ort and Carrasco-Núñez, 2009; Hopi Buttes, AZ, Lefebvre et al., 2013) to hard, fractured country rock (e.g., West Eifel volcanic field, Germany and Massif Central, France, Lorenz, 2003). Country-rock structure, including faults and joints, rock type, and shallow crustal hydrologic properties, can influence an eruption’s behavior by controlling how much and at what rate water can be supplied to the magma (hydraulic flow rate), and determining the sediment: water ratio in the case of soft-sediment substrate eruptions. In a “soft” substrate environment, volcanic tremor can lead to liquefaction of saturated sediment, producing a slurry that may then interact with magma in unique ways (White, 1996; Auer, et al., 2006).

58 GEOSCIENCES↗

Severe Accident Phenomena: A Comparison Among the NuScale SMR, Other Advanced LWR Designs, and Operating LWRs

During a severe accident in a nuclear reactor, there are a number of phenomenological events which can present a challenge to containment integrity. These include the generation and combustion of hydrogen, energetic fuel-coolant interactions, thermal attack of fission product barriers, core-concrete interactions, direct containment heating, and gradual overpressurization. The advanced design of the NuScale small modular reactor has resulted in the reduced likelihood and severity of severe accident challenges to containment. This paper discusses the features of the NuScale design that reduce the likelihood of occurrence of these severe accident phenomena, and discusses the ability of containment to survive in the unlikely event that they do occur. Here, the impact of severe accident phenomena for the NuScale design is compared and contrasted against other advanced light water reactors, such as AP1000 and ESBWR, as well as the existing fleet, using information from publicly available documents.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Research plan for the development of optical fiber pressure sensors for nuclear applications

Fiber optic pressure sensors are desirable for nuclear applications because they are low mass/small size, immune to electromagnetic interference, high sensitivity, and have multiplexing and multimodal measurement capabilities. Much research and development has been conducted on developing fiber optic based sensors and they are now considered a class of standard instrumentation in many industries. Specifically, for pressure sensing, a wide range of fiber based sensors have been developed for various pressure ranges and environments. This vast body of research will be leveraged for the development of pressure sensors for nuclear applications. Four pressure measurement scenarios were considered which would benefit from a fiber optic based pressure sensor. These scenarios include pressure measurement in the fuel rod plenum, coolant pressure during LOCA testing, advanced coolant (helium, sodium, molten salt) pressure for flow loop operation, and high pressures resulting for direct fuel-coolant interaction. Each scenario has unique pressure, temperature, and material requirements for the sensor. From a survey of commercially available sensors and a literature review; it has been determined that an extrinsic Fabry-Perot interferometer approach is the most appropriate for the various measurement requirements. The experience and knowledge base for Fabry-Perot interferometers can be leveraged since they are the most common fiber optic based pressure sensors available commercially and found in literature. These pressure sensors rely on the interference of light in a gas filled cavity, which minimizes the impact of radiation induced attenuation and compaction on the measurement, compared to intrinsic sensing techniques. The measurement range of these sensors is based on the stiffness of the diaphragm that deflects under pressure. This allows for a suite of fiber based sensors to be developed by interchanging this diaphragm for the requirements of each application. Key material and design considerations have been identified for the development of a Fabry-Perot interferometry pressure measurement for nuclear applications. These include high temperature bonding between the glass fiber optic and metal housing, identifying diaphragm materials & geometry, and minimizing cross sensitivity to temperature or implementing compensation techniques found in literature. Overcoming these challenges will develop a pathway for a fiber optic based pressure sensor for nuclear applications, and additionally can be leveraged for other sensing application based on Fabry-Perot interferometers, such as temperature, strain (creep & deformation), vibration, and index of refraction.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Trigger - and heat-transfer times measured during experimental molten-fuel-interactions

A modified setup featuring high speed high resolution data and video recording was developed to obtain detailed information on trigger and heat transfer times during explosive molten fuel-coolant-interaction (MFCI). MFCI occurs predominantly in configurations where water is entrapped by hot melt. The setup was modified to allow direct observation of the trigger and explosion onset. In addition the influences of experimental control and data acquisition can now be more clearly distinguished from the pure phenomena. More precise experimental studies will facilitate the description of MFCI thermodynamics.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

BWR ex-vessel steam explosion analysis with MC3D code

A steam explosion may occur, during a severe reactor accident, when the molten core comes into contact with the coolant water. A strong enough steam explosion in a nuclear power plant could jeopardize the containment integrity and so lead to a direct release of radioactive material to the environment. To resolve the open issues in steam explosion understanding and modeling, the OECD program SERENA phase 2 was launched at the end of year 2007, focusing on reactor applications. To verify the progress made in the understanding and modeling of fuel coolant interaction key phenomena for reactor applications a reactor exercise has been performed. In this paper the BWR ex-vessel steam explosion study, which was carried out with the MC3D code in conditions of the SERENA reactor exercise for the BWR case, is presented and discussed. The premixing simulations were performed with two different jet breakup modeling approaches and the explosion was triggered also at the expected most challenging time. For the most challenging case, at the cavity wall the highest calculated pressure was {approx}20 MPa and the highest pressure impulse was {approx}90 kPa.s. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Analysis of the KROTOS KFC test by coupling X-Ray image analysis and MC3D calculations

During a hypothetical severe accident sequence in a Pressurized Water Reactor (PWR), the hot molten materials (corium) issuing from the degraded reactor core may generate a steam explosion if they come in contact with water and may damage the structures and threaten the reactor integrity. The SERENA program is an international OECD project that aims at helping the understanding of this phenomenon also called Fuel Coolant Interaction (FCI) by providing data. CEA takes part in this program by performing tests in its KROTOS facility where steam explosions using prototypic corium can be triggered. Data about the different phases in the premixing are extracted from the KROTOS X-Ray radioscopy images by using KIWI software (KROTOS Image analysis of Water-corium Interaction) currently developed by CEA. The MC3D code, developed by IRSN, is a thermal-hydraulic multiphase code mainly dedicated to FCI studies. It is composed of two applications: premixing and explosion. An overall FCI calculation with MC3D requires a premixing calculation followed by an explosion calculation. The present paper proposes an alternative approach in which all the features of the premixing are extracted from the X-Ray pictures using the KIWI software and transferred to an MC3D dataset for a direct simulation of the explosion. The main hypothesis are discussed as well as the first explosion results obtained with MC3D for the KROTOS KFC test. These results are rather encouraging and are analyzed on the basis of comparisons with the experimental data. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Accuracy Enhancement of Nuclear Power Plant Simulators Utilizing High Accuracy Simulation Predictions

More recently, reactor core simulators for core designs associated with commercial nuclear power plants that utilize what is believed to be higher fidelity models have been developed. Features such as neutronics models that utilize transport equation solvers with fine spatial meshes and many energy-groups, thermal-hydraulic models that utilize sub-channel solvers with fine spatial mesh and capable of treating a wide range of fluid conditions, and fuel-coolant chemistry interaction models capable of treating CRUD deposition are to be found in these higher fidelity core simulators. These reactor core simulators require access to higher performance computers, characterized by many processors, cores and large memory. So associated with utilization of these simulators is access to high performance computers and ability to accommodate in one’s workflow longer execution times. By contrast, currently used core simulators by the nuclear industry can execute on engineering workstations and have execution times of seconds to minutes. The desirability for having short execution times is not only desired for support of time critical tasks but supports the mental process of decision making by engineers. The goal of the work reported upon here has the objective of retaining the fidelity of higher fidelity models while retaining the ability to utilize engineering workstations. Beyond the core simulator goal, additional goals of this work include incorporating the just described core simulator capability into a Nuclear Steam Supply System (NSSS) simulator, and to incorporate the resulting capability into an environment supportive of design and operational decision making associated with nuclear power stations. The model selected for the core neutronics model is the NESTLE code, for the core thermal-hydraulic model is the CTF code utilizing coarse mesh, and for the NSSS model is the RELAP5-3D code. WSC’s proprietary 3KEYMASTERTM platform is being used to provide software coupling, user interface, visualization, and reporting. The NESTLE core neutronics simulator was first integrated with the CTF core thermal-hydraulic simulator using CTF developed communication commands which are also used for CTF to communicate with RELAP5-3D under WSC’s proprietary 3KEYMASTERTM platform. To assure NESTLE prediction consistency with higher fidelity core neutronic simulators, buffer codes have been created to automatically generate from output files written by the VERA core simulator the NESTLE nodal neutronic parameter’ library, geometry, and pin-power reconstruction input files, thereby avoiding a number of challenges associated with utilizing lattice physics codes and providing consistency with VERA predictions. To treat absorber rod effects a multi-set library is utilized, where a set refers to a specific absorber rod fully inserted pattern. A coarse spatial mesh CTF model was developed with features added that support using CTF as envisioned in the engineering quality simulator. A hybrid meshing approach was implemented to allow for automated construction of models with mixed levels of refinement. Specifically, a core model could resolve some assemblies at a nodal level (4 subchannels per assembly) and others at a pin-resolution (one subchannel per coolant subchannel in the assembly). The intention is that this will allow for better resolution of limiting conditions such as DNBR and PCT, which are based on local rod and subchannel conditions. Further development was done of features that enhance the capabilities for the envisioned engineering quality simulator that has been developed, but now for RELAP-3D. The RELAP5-3D code development includes ability to model more than 999 components and the addition of the cross-channels turbulence mixing model and the void drift model that are implemented in CTF, aiming to achieve closer prediction agreement of the two codes for transient simulations, specifically, more accurate matches of the overall mass, momentum, and energy exchanges of both the liquid and gas phases between the neighboring core assemblies. Graphics were also developed for the Instructor Station for this project under WSC’s proprietary 3KEYMASTERTM platform to facilitate design and operational decision making.

42 ENGINEERING↗

Conceptual Design of a CERMET NTR Fission Core Using Multiphysics Modeling Techniques

An initial pre-conceptual CERMET Nuclear Thermal Propulsion reactor system is investigated within this paper. Reactor configurations are investigated where the fuel consists of 60 vol.% UO2 and 40 vol.% W where the UO2 consists of Gd2O3 concentrations of 5 and 10 mol.%.Gd2O3. The fuel configuration consisting of 5 mol.% UO2 was found to have a total mass of 2761 kg and a thrust to weight ratio of 4.10 and required a coolant channel surface area to fueled volume ratio of approximately 15.0 in order to keep the centerline temperature below 3000 K. The configuration consisting of 10 mol.% Gd2O3 required a surface area to volume ratio of approximately 12.2 to cool the reactor to a peak temperature of 3000 K and had a total mass of 3200 kg and a thrust to weight ratio of 3.54. It is not known yet what concentration of Gd2O3 is required to maintain fuel stability at 3000 K; however, both reactors offer the potential for operations at 25,000 lb, and at a specific impulse which may range from 900 to 950 seconds.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Criticality characteristics of MCCI products possibly produced in reactors of Fukushima Daiichi nuclear power station - 14408

The damaged Unit 1-3 reactors of the Fukushima Daiichi Nuclear Power Station may contain fuel debris of a significant amount that is in a form of molten-core-concrete-interaction (MCCI) product with porous structure. Such low density MCCI product including fissile material is a great concern for its criticality control, especially under submerged condition, due to its fairly good neutron moderation. This report shows computation results of basic criticality characteristics of the MCCI product, which will facilitate criticality risk assessments during decommissioning of the reactors. The results imply that water bound in concrete may raise the risk from the viewpoints of possibility of criticality events and of effectiveness of mitigation measures such as neutron poison injection into coolant water. (authors)

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