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At least 19 records

GPM IMERG V07B and V06B: Evaluation Using Ground-Based Radar Observations and Application in Global Mesoscale Convective System Tracking

This study evaluates the latest Global Precipitation Measurement (GPM) Integrated Multi-satellitE Retrievals for GPM (IMERG V07B) against its predecessor V06B, for studying mesoscale convective systems (MCSs). Both versions are compared using ground-based radar and rain gauge data from five meteorologically diverse regions: the contiguous United States (including eastern coastlines), Amazon rainforest, central Argentina mountains, equatorial Indian Ocean, and northern Australia across multiple temporal (0.5–6 hours) and spatial scales (0.1°–0.25°). An updated global MCS tracking dataset is developed by integrating satellite-observed infrared brightness temperature with IMERG V07B. Comparation of IMERG against radar observations reveals that IMERG demonstrates better performance in capturing the probability distribution and quantitative contributions of rainfall (from no-rain to intense-rain conditions) over tropical oceans than over land, with marked improvements in IMERG V07B for heavy-to-intense rain (> 10 mm h-1). Over land, systematic biases persist: IMERG tends to overestimate light-to-moderate rain (1–10 mm h-1) while underestimating heavy-to-intense rain. Additionally, aggregating IMERG to coarser resolutions (3-hourly or 0.25°) improves consistency with radar observations, outperforming the 1-hourly/0.1° resolution. The new IMERG V07B-based global MCS dataset exhibits consistent statistical characteristics with the V06B-based dataset, despite lower mean rain rates and reduced heavy precipitation contributions. These findings offer valuable insights for utilizing IMERG V07B in global precipitation studies, MCS characterization, and model evaluation.

Zhang, Sihan↗

The Detection of Mesoscale Convective Systems by the GPM Ku-Band Spaceborne Radar

The Global Precipitation Measurement (GPM) core observatory satellite launched in 2014 features more extended latitudinal coverage (65 degree S-65 degree N) than its predecessor Tropical Rainfall Measuring Mission (TRMM, 35 degree S-35 degree N). The Ku-band radar onboard of the GPM is known to be capable of characterizing the 3D structure of deep convection globally. In this study, GPM’s capability for detecting mesoscale convective systems (MCSs) is evaluated. Extreme convective echoes seen by GPM are compared against an MCS database based on tracking convective entities over the contiguous US. The tracking is based on geostationary satellite and ground-based Next Generation Radar (NEXRAD) network data obtained during the 2014-2016 warm seasons. Results show that more than 70% of the GPM-detected Deep-Wide Convective Core (DWC) and Wide Convective Core (WCC) objects are part of NEXRAD identified MCSs, indicating that GPM-classified DWCs and WCCs correlate well with typical MCSs containing large convective features. By applying this method to the rest of the world, a global view of MCS distribution is obtained. This work reveals GPM’s potential in MCS detection at the global scale, particularly over remote regions without dense observation network.

3D reflectivity structure↗

Graupel and Hail Identification Algorithm for the Dual-frequency Precipitation Radar (DPR) on the GPM Core Satellite

Precipitation consists of many types of hydrometeors, such as raindrops, ice crystals, graupel, and hail. Due to their impacts, graupel and hail (GH) have received particular attention in the literature. Global Precipitation Measurement (GPM) dual-frequency radar (DPR) has proved to be a very reliable system for global precipitation retrievals. This paper aims to develop a GH identification algorithm for GPM DPR. This algorithm is constructed using a precipitation type index (PTI) defined for DPR. The PTI is effective in separating hydrometeor types and is calculated using measurements of reflectivity, dual-frequency ratio, and storm top height data. The output of the algorithm is a Boolean product representing the existence of graupel or hail along with the vertical profile for each Ku- and Ka-band matched footprint. Cross validation is performed with the Weather Service Radar (WSR-88D) network over continental United States as well as during the Remote sensing of Electrification, Lightning, and Mesoscale/Microscale Processes with Adaptive Ground Observations (RELAMPAGO) experiment. Evaluation of the GH identification algorithm is performed on a global basis, which illustrates promising comparisons with the global lightning and hail precipitation maps generated using radar and radiometer.

54 ENVIRONMENTAL SCIENCES↗

Cross Validation of the Network of Ground-Based Radar with GPM during the Remote Sensing of Electrification, Lightning, And Mesoscale/Microscale Processes with Adaptive Ground Observations (RELAMPAGO) Field Campaign

The cross-validation of radars in a network is important in making consistent retrievals across the domain and assuring the product quality. During the RELAMPAGO field campaign, two C-band radars, namely the Colorado State University C-band Hydrological Instrument for Volumetric Observations ( CSU-CHIVO) and the C-band Scanning ARM Precipitation Radar (CSAPR-2), were deployed near the Sierras de Cordoba in Argentina, a region known for having some of the most intense severe weather in the world. In addition to these two radars, the operational radar of the Cordoba City, the Radar Meteorologico Argentino 1 (RMA-1), adds another instrument to the RELAMPAGO network. This study presents an intercomparison between the RELAMPAGO C-band radars using the GPM spaceborne radar as a common reference ..A method to bring ground-based radars into better agreement is also proposed. Moreover, the attenuation correction for the C-band radar is studied in the context of intercomparing two radars. The attenuation coefficients are computed for the RELAMPAGO domain using the local disdrometers deployed. during the campaign. After the attenuation correction, CSU-CHIVO, CSAPR-2, and RMA-1 compare well with GPM-DPR with a high correlation and bias less than 1 dB.

54 ENVIRONMENTAL SCIENCES↗

A Parameterization of the Cloud Scattering Polarization Signal Derived From GPM Observations for Microwave Fast Radative Transfer Models

Microwave cloud polarized observations have shown the potential to improve precipitation retrievals since they are linked to the orientation and shape of ice habits. Stratiform clouds show larger brightness temperature (TB) polarization differences (PDs), defined as the vertically polarized TB (TBV) minus the horizontally polarized TB (TBH), with ~10 K PD values at 89 GHz due to the presence of horizontally aligned snowflakes, while convective regions show smaller PD signals, as graupel and/or hail in the updraft tend to become randomly oriented. The launch of the global precipitation measurement (GPM) microwave imager (GMI) has extended the availability of microwave polarized observations to higher frequencies (166 GHz) in the tropics and midlatitudes, previously only available up to 89 GHz. This study analyzes one year of GMI observations to explore further the previously reported stable relationship between the PD and the observed TBs at 89 and 166 GHz, respectively. The latitudinal and seasonal variability is analyzed to propose a cloud scattering polarization parameterization of the PD-TB relationship, capable of reconstructing the PD signal from simulated TBs. Given that operational radiative transfer (RT) models do not currently simulate the cloud polarized signals, this is an alternative and simple solution to exploit the large number of cloud polarized observations available. Finally, the atmospheric radiative transfer simulator (ARTS) is coupled with the weather research and forecasting (WRF) model, in order to apply the proposed parameterization to the RT simulated TBs and hence infer the corresponding PD values, which show to reproduce the observed GMI PDs well.

54 ENVIRONMENTAL SCIENCES↗

Can the GPM IMERG Final Product Accurately Represent MCSs’ Precipitation Characteristics over the Central and Eastern United States?

Mesoscale convective systems (MCSs) play an important role in water and energy cycles as they produce heavy rainfall and modify the radiative profile in the tropics and midlatitudes. An accurate representation of MCSs’ rainfall is therefore crucial in understanding their impact on the climate system. The V06B Integrated Multisatellite Retrievals from Global Precipitation Measurement (IMERG) half-hourly precipitation final product is a useful tool to study the precipitation characteristics of MCSs because of its global coverage and fine spatiotemporal resolutions. However, errors and uncertainties in IMERG should be quantified before applying it to hydrology and climate applications. This study evaluates IMERG performance on capturing and detecting MCSs’ precipitation in the central and eastern United States during a 3-yr study period against the radar-based Stage IV product. The tracked MCSs are divided into four seasons and are analyzed separately for both datasets. IMERG shows a wet bias in total precipitation but a dry bias in hourly mean precipitation during all seasons due to the false classification of nonprecipitating pixels as precipitating. These false alarm events are possibly caused by evaporation under the cloud base or the misrepresentation of MCS cold anvil regions as precipitating clouds by the algorithm. IMERG agrees reasonably well with Stage IV in terms of the seasonal spatial distribution and diurnal cycle of MCSs precipitation. A relative humidity (RH)-based correction has been applied to the IMERG precipitation product, which helps reduce the number of false alarm pixels and improves the overall performance of IMERG with respect to Stage IV.

54 ENVIRONMENTAL SCIENCES↗

Graphene-polyelectrolyte multilayer membranes with tunable structure and internal charge

One great advantage of graphene-polyelectrolyte multilayer (GPM) membranes is their tunable structure and internal charge for improved separation performance. In this study, we synthesized GO-dominant GPM membrane with internal negatively-charged domains, polyethyleneimine (PEI)-dominant GPM membrane with internal positively-charged domains and charge-balanced dense/loose GPM membranes by simply adjusting the ionic strength and pH of the GO and PEI solutions used in layer-by-layer membrane synthesis. A combined system of quartz crystal microbalance with dissipation (QCM-D) and ellipsometry was used to analyze the mass deposition, film thickness, and layer density of the GPM membranes. The performance of the GPM membranes were compared in terms of both permeability and selectivity to determine the optimal membrane structure and synthesis strategy. One effective strategy to improve the GPM membrane permeability-selectivity tradeoff is to assemble charge-balanced dense membranes under weak electrostatic interactions. This balanced membrane exhibits the highest MgCl 2 selectivity (~86%). Another effective strategy for improved cation removal is to create PEI-dominant membranes that provide internal positively-charged barrier to enhance cation selectivity without sacrificing water permeability. Finally, these findings shine lights on the development of a systematic approach to push the boundary of permeability-selectivity tradeoff for GPM membranes.

42 ENGINEERING↗

Conversion of METL Diagnostic Flowmeters to Permanent Magnet Based Electromagnetic Flowmeters

The Mechanisms Engineering Test Loop (METL) uses three flowmeters to monitor sodium circulation through the main loop, the Cold Trap leg, and the Plugging Meter leg. When constructed, the Cold Trap flowmeter (CTFM) and Plugging Meter flowmeter (PMFM) were equipped with permanent magnets and Hall Sensors. By October of 2019, during normal operations, both the CTFM and PMFM failed, producing either erroneous or zero signals. Repairs to the flowmeters were attempted in January of 2020 but failed to resolve the issues. Therefore, starting in March of 2021, a plan was developed to convert the installed flowmeters to more robust permanent magnet based electromagnetic flowmeters (EMFMs). The Cold Trap EMFM (CT EMFM) and Plugging Meter EMFM (PM EMFM) were fully installed by August of 2021. Initial testing and commissioning were completed in November of 2021. Finally, the first calibration runs were finished in March of 2022. This report discusses the design, conversion, and calibration of the as-built CTFM and PMFM to robust permanent magnet based EMFMs. During the design phase, theoretical models were used to estimate the signal output and required magnet sizes. Then, the CTFM and PMFM were disassembled and converted to EMFMs. After commissioning, the CT EMFM and PM EMFM were calibrated using a ‘Time Transfer Procedure’ carried out with METL Expansion Vessels and Test Vessel Two. The accuracy of the calibration was estimated through an uncertainty analysis. Finally, the report describes some lessons learned for future flowmeter conversions and follow-up work. In total, both METL EMFM’s met the desired performance targets. Testing data showed that the METL EMFMs provide a output signal of roughly 2 mV at 1 GPM and 250 °C. During calibration, flowrates between 0.7 GPM and 2.4 GPM were achieved. In this flow range, calibration coefficients of 0.485 and 0.935 were measured as with errors ranging from 15-5% and 16-5% for the CT EMFM and PM EMFM, respectively. Above 1.5 GPM, the error was assumed to be about 5% for both METL EMFMs. Several points will be considered for future follow-up work on the METL EMFM’s. First, the signal noise issues in the PM EMFM will be addressed. It is likely the source of the noise is due to some stray EMF from a heater. Secondly, the NdFeB magnets will be replaced with a grade that has a Curie temperature above 80 °C. For example, a few grades of NeFeB magnets have Curie temperatures which exceed 150 °C and some SmCo magnets have Curie temperatures as high as 500 °C. Third, more calibration runs will be completed in the range of 0.5-2.5 GPM. This will further improve the accuracy of the calibration coefficient. Fourth, calibration runs will be completed up to 5 GPM. This requires a larger pressure relief valve to be installed on the Expansion Vessel and Test Vessel 2, as well as a revised calibration procedure. Lastly, calibration runs will be completed to account for cold spots in the system, which reduced the inlet temperature of the METL EMFMs. Overall, these points will improve the calibration coefficients derived in this work and also improve the performance of the METL EMFMs.

42 ENGINEERING↗

Managing an Aging Pump-and-Treat Groundwater Remediation System at the Fernald Preserve - 19557

The Fernald Preserve, Ohio, Site underwent restoration and remediation under the Comprehensive Environmental Response, Compensation, and Liability Act (CERCLA). With the exception of the Great Miami Aquifer, the CERCLA remediation was declared physically complete on October 29, 2006, and the site was turned over to the US Department of Energy Office of Legacy Management for long-term care and maintenance. The Record of Decision under CERCLA specifies a concentration-based cleanup that requires the extraction and treatment of Great Miami Aquifer groundwater above Final Remediation Levels (FRLs) until the full, beneficial use potential of the aquifer is achieved, including use as a drinking water source. The area of the aquifer targeted for remediation is 126.5 hectares (312.70 acres). The groundwater pumping remediation was designed by modeling cleanup with the Variable Saturated Analysis Model in 3 Dimensions (VAM-3D) modeling code, developed by Hydrogeologic Inc. The original design called for 23 extraction wells operating at 379 liters per minute (lpm) (100 gallons per minute [gpm]) to 1135 lpm (300 gpm) each for a system total of 18,073 lpm (4775 gpm). In 2014, the system was optimized down to 20 extraction wells operating at 379 to 1893 lpm each for a system total of 19,180 lpm (5075 gpm). To date, pumping has been an effective remediation technology for the aquifer. At the end of 2017, the area of the aquifer remaining above FRLs was down to 38.2 hectares (94.4 acres). From August 1993 through December 2017 (24 years), 6235 kilograms (kg) (13,733 pounds) of uranium were removed from the aquifer by the pumping of 1.74 x 10{sup 11} liters (46.2 billion gallons) of water. Since 2010, treatment of groundwater to achieve regulatory discharge limits at the Great Miami River has not been needed on a routine basis. The ongoing remediation is now essentially a pumping operation, and this water does not require treatment. Metrics reported in the annual Site Environmental Report for the groundwater remediation indicate that, based on the model-predicted estimate of the mass of uranium that needs to be removed from the aquifer to achieve a concentration-based cleanup, the cleanup is approximately 86% - 87% complete. Current model predictions indicate that pumping will need to continue an additional 16 years (until 2035) in some of the wells. During the additional 16 years, it is estimated that approximately 1012 kg (2231 pounds) of uranium will be removed from the aquifer. System pumping rates are designed to decrease over the course of the remaining 16 years, dropping down to a system total of 11,638 lpm (3075 gpm) in 2022 and a system total of 4163 lpm (1100 gpm) in 2033. Even with the designed decreases in pumping rates, it is estimated that approximately 1 x 10{sup 11} liters (26.6 billion gallons) of water will be pumped from the aquifer to remove 1012 kg (2231 pounds) of uranium. This indicates that the remaining 16 years of operation will be much less efficient than the first 24 years. Decreasing efficiency is common for pumping operations. The worst-case scenario is that decreasing concentration trends stabilize above the cleanup FRLs and remediation goals are never achieved. Performance assessments of the pumping remedy will need to be routinely conducted to determine if pumping should be discontinued, if it should be continued but optimized, or if the pumping technology can be supplemented with a different technology that will improve the outcome of the remediation and make the operation more efficient and successful. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Tank 27 Solids Disturbance Testing Using M-Star for the Impact of CSMP Usage on Blend Tank Mixing Effectiveness

Savannah River Mission Completion (SRMC) plans to operate Tank 27as a blend tank for future waste disposal operations. It is desirable to avoid additional worker exposure by using the planned commercial submersible mixing pump (CSMP) installations in Risers B2 and B4 to function as the blend pumps for prolonged blend tank operations. The purpose of this task is to evaluate the impacts to mixing across a range of pump installation heights from 1 to 201 inches above the tank floor. The CSMPs shall maintain adequate blending within a 24 hour maximum timeframe and an adequate nozzle discharge velocity as outlined in U-ESR-G-00030, using the specifications of the planned CSMPs listed in PO SRRA149971 and M-DS-G-00081. Specifications include: maximum pump diameter of D=22.5 in., dual nozzles placed tangentially opposed with nominal inside diameter of 2 in., total flow range (both nozzles combined) of 500 to 1950 GPM and maximum RPM of 1800. Tank 27 is expected to have a fill height maximum of 360". This analysis began by using results from the 2010 testing and applying them to the Tank 27 design to calculate a mixing time as a function of pump flow rate. These results were modified to account for the higher liquid level in Tank 27. Once the liquid level was increased to 360 inches, the results were modified to account for a higher viscosity in Tank 27 than in the testing. Once the viscosity was increased, the effect of changing pump elevation was applied to calculations of the mixing time in Tank 27. Finally, the uncertainty from the testing was included in the analysis to recommend a blend time as a function of pump flow rate and elevation. The conclusion from this study is that the particles in tank 27 will be suspended at both the 600 and 900 gpm flow rates. Only particles above 90 micron will not be suspended in significant amounts when the flow rate is 600 gpm. At 900 gpm even 100 micron particles were thoroughly suspended in the tank. From the series of simulations it has been concluded that it will not be possible to mix tank 27 at the proposed fluid flow rates and not suspend the solid particles at the bottom of the tank.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Comparison of atmospheric radionuclide dispersion models for a risk-informed consequence-driven advanced reactor licensing framework

Current nuclear facility emergency planning zones (EPZs) are based on outdated distance-based criteria, predating comprehensive dose and risk-informed frameworks. Recent advancements in simulation tools have permitted the development of site-specific, dose, and risk-based consequence-driven assessment frameworks. This study investigated the computation of advanced reactor (AR) EPZs using two atmospheric dispersion models: a straight-line Gaussian plume model (GPM) and a semi-Lagrangian Particle in Cell (PIC). Two case studies were conducted: (1) benchmarking the NRC SOARCA study for the Peach Bottom Nuclear Generating Station and (2) analyzing an advanced INL Heat Pipe Design A microreactor's end-of-cycle inventory. The dose criteria for both cases were 10 mSv at mean weather conditions and 50 mSv at 95th percentile weather conditions at 96 h post-release. Results demonstrated that GPM and PIC estimated similar mean peak dose levels for large boiling water reactors in the farfield case, placing EPZ limits beyond current regulations. For ARs with source terms remaining in the nearfield, PIC modeling without specific nearfield considerations could result in excessively high doses and inaccurate EPZ designations. PIC dispersion demonstrated an order of magnitude higher estimate of nearfield inhalation dose contribution when compared to GPM results. Furthermore, both models significantly reduced EPZ sizing within the nearfield. Thus, reductions in the AR source term may eliminate the need for a separate EPZ.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗

Produced Water and Waste Heat-aided Blowdown Water Treatment: Using Chemical and Energy Synergisms for Value Creation

The project objective was to develop a cooling blowdown water (BDW) treatment process utilizing produced water (PW) and low-grade heat to maximize water reuse and saleable by-product generation while reducing chemical and energy footprints of the treatment. The proposed treatment process consists of mixing, softening, organics and suspended solids removal, reverse osmosis (RO), thermal desalination, and brine electrolysis. BDW samples collected from a local coal-fired power plant and PW samples from two shale gas production wells were used in this study. Each treatment unit was first designed and tested to quantify its treatment efficiency, and its chemical and energy requirements. In addition, a process model was developed and model simulations were conducted based on the experimental results and literature data to optimize the treatment process. A techno-economic analysis was conducted to quantify chemical and energy savings as well as production of 10-lb brine as a saleable product. With the field-collected BDW and PW samples, mixing experiments determined a volumetric mixing ratio 10:1 (BDW:PW) resulted in the best performance of multivalent ions removal and largest chemical savings for softening. Softening of the BDW/PW mixtures using alkaline chemicals (Na 2 CO 3 and NaOH) achieved 95%-100% removal of scaling-forming cations (Ca, Mg, Fe, Ba, Sr) and 60% of silicon, and 10% of total organic carbon (TOC). The mixing and softening treatments yielded an effluent with total dissolved solids (TDS) concentration of 23 g/L. Activated carbon (AC) filtration removed TOC to a low level (< 3 mg/L) and further removed remaining scale-forming divalent metals and silica from the softened water. The AC filtration resulted in a slight reduction of TDS from 23 g/L to 20 g/L, leaving behind only mostly monovalent ions (i.e., sodium and chloride) in the filtered water. These pretreatments yielded a feed water that met the criteria of the downstream reverse osmosis (RO) to prevent membrane fouling. A cross-flow RO system was used to further concentrate the TDS of the AC effluent. Various factors including TDS, pH, and applied pressure were examined and optimal conditions were determined for the co-treatment process. An integrated process consisting of mixing, softening, AC filtration and RO was used to treat a continuous flow (0.25 – 1.2 L/min, or 0.07 – 0.32 gpm) and successfully generated RO permeate as product water (TDS < 0.5 g/L) for reuse in cooling operation, and a concentrate (TDS ~ 45 g/L) to be further treated in a thermal desalination unit. These flow rates meet the FOA’s criterion of 0.01 – 1 gpm. Overall, the co-treatment of BDW/PW allowed shorter ramp-up time compared to treatment of BDW alone. It resulted in 40% and 55% savings of Na 2 CO 3(s) and NaOH, respectively, compared to treating the BDW and PW individually for the same level of softening. The co-treatment also resulted in a 29% energy saving compared to treatment of BDW only for the level of TDS concentration. A thermal desalination system was designed using CFD simulations and manufactured in the WVU Innovation Hub for further treatment of the RO concentrate to generate 10-lb brine. The system has a design flow rate of 2 gpm and has been successfully tested. A bench-scale brine electrolysis system was developed for on-site generation of chlorine/hypochlorite (Cl 2 /OCl - ) and caustic soda (NaOH) as useful chemicals for the co-treatment process. Using salt solutions (0.5 M and 1 M), the system achieved faradaic efficiencies of 93%-97% and 70%-77% for caustic soda and chlorine/hypochlorite generation, respectively. An economic analysis showed that the electricity costs for on-site generation of these chemicals were significantly lower than the chemical prices offered by suppliers. An industrial-scale process model consisting of mixing, softening, AC filtration, RO, thermal desalination, and brine electrolysis was developed using the Aspen Plus V9 in conjunction with Aspen Custom Modeler V9. The model serves as a solvable Aspen Plus model and as basis to form the costing infrastructure. In addition, techno-economic analysis considering capital, operating, and transportation costs was conducted. An optimization solution showed that produced water for mixing is still advantageous in low quantities. The optimum solution approaches a leveled cost of water (LCW) of 2 $/m 3 which becomes cost competitive with nominal water treatment prices.

20 FOSSIL-FUELED POWER PLANTS↗

Hydraulic and Thermal Stimulation Program at Raft River Idaho, A DOE EGS

A Department of Energy Enhanced Geothermal System (EGS) stimulation program has injected over 254 million gallons of water into the well RRG-9 ST1 since the summer of 2013. Three major stimulations have been conducted during the program increasing injection flow rates from less than 20 gpm to 550 gpm. Geologic, water chemistry, microseismic activity, and borehole imaging data have been used to develop a conceptual model describing possible flow paths of this injected water. This model contains two major fracture zones one of which intersects the RRG-9 ST1 wellbore. Modified Hall and injectivity index plots constructed using injection flow rates, surface temperatures, and wellhead pressures show steady improvement in the injectivity of the well. Here, the injectivity index has risen from 0.15 gpm/psi to 2.0 gpm/ psi. A pressure falloff test conducted on April 28, 2015 indicates a reservoir permeability of 1,220 md and -5.38 skin factor. The well stimulation program was simulated numerically using an Idaho National Laboratory reservoir simulation code, FALCON. These simulations show a significant increase in the permeability of connecting fracture pathways after each stimulation event.

Enhanced geothermal system↗

Wastewater Treatment at the Fernald Preserve-Past, Present, and Future - 19555

Industrial wastewater treatment at the Fernald Preserve, Ohio, Site has been ongoing since a uranium metals refinery was constructed there at the beginning of the Cold War in 1951. Initially, the primary purpose of treatment was to recover uranium for reuse. Later, when cleanup of the site was progressing in the 1990's, wastewater treatment efforts greatly expanded. Large treatment facilities were constructed to handle contaminated surface water, groundwater, remediation wastewater, and leachate from the on-site disposal facility. These new facilities were designed to reduce uranium concentration to meet the US Environmental Protection Agency (EPA) drinking water standard and not generate large quantities of contaminated waste. Anion-exchange resin was chosen as the treatment media. The centerpiece of these facilities was the Advanced Wastewater Treatment facility, which had a treatment capacity of 10,978 liters per minute (lpm) (2900 gallons per minute [gpm]). Forecasts estimated that with the exception of groundwater the site's remediation would be completed in 2006. In 2003, the US Department of Energy (DOE) Office of Environmental Management began negotiations with the EPA and Ohio Environmental Protection Agency to reduce wastewater treatment capacity at the Fernald Environmental Management Project. These negotiations resulted in the site's treatment capacity being reduced to 6814 lpm (1800 gpm) via the Converted Advanced Wastewater Treatment facility (CAWWT). By 2010, the uranium concentration in the groundwater being pumped had been reduced to the degree that only intermittent treatment for uranium removal was needed. As a result, the CAWWT was considerably oversized. Increased maintenance on the aging CAWWT equipment led the DOE Office of Legacy Management (LM) to commission an assessment of the facility, which was completed in early 2015. The condition assessment identified numerous components at or near the end of their design life. Based on the assessment's findings and the fact that the current facility's treatment capacity was substantially greater than needed, LM began looking at options for an appropriately sized treatment system to handle the site's needs until the groundwater remediation was completed (currently projected for 2039). Options were evaluated in the spring of 2015, and LM presented the recommended changes to regulators and stakeholders. Approvals for a new, smaller system with a 189 lpm (50 gpm) capacity were obtained through a series of meetings in the summer of 2015. After more detailed planning in the fall of 2015, LM initiated the project in 2016. The project comprises the following four phases: (1) Removal and disposal of used media, piping, and tanks to make room for the new system in the existing building (completed in January 2017); (2) design of the new system (completed in April 2017); (3) construction, installation, and startup of the new system (completed in May 2018); and (4) backwash basin refurbishment (yet to be completed). In the late 2030's, when groundwater remediation is projected to be completed at the site, it is anticipated that the only remaining wastewater treatment need will be for small quantities of leachate from the on-site disposal facility. Results of leachate treatment testing in 2003 indicate it may be feasible to utilize a small passive treatment system for this leachate. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Industrial scale mesofluidic particle separation

Here we explore the potential of a mesofluidic separator that fits within industrial piping and is designed to remove large aspherical particles out of an abrasive slurry at fast flow rates. Mesofluidic separators have recently demonstrated separation of spherical particles at flow rates of ~1 gallon/min (gpm) (6.3.10 -5 m 3 /s). Yet, the performance of these separators at flow rates achievable within industrial piping have not been explored. Here we evaluate the permeate flowrate fraction, large particle mass fraction, and pressure drop from approximately 35-100 gpm (2.2.10-3-6.3.10-3 m 3 /s) in a three inch tube using an abrasive and modestly non-spherical slurry. Faster flow rates may be achieved with larger pumps and larger diameters. We find the permeate fraction and pressure drop both increase with flow rate, though the pressure drop remains modest. Only two feet of inserts removed 97.6±2.1% of large particles for conditions tested. Separation was demonstrated in both vertical and horizontal orientations with the horizontal orientation benefiting marginally from gravitational settling.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Development of experimental and computational frameworks to predict subcooled flow boiling in the LANL Isotope Production Facility

Cooling is crucial to maintain the integrity of target systems in isotope production facilities. At Los Alamos National Laboratory (LANL)’s Isotope Production Facility (IPF), multiple encapsulated targets are stacked and irradiated in tandem with a 100 MeV, ~250μA proton beam. To facilitate effective heat removal, these stacked targets are separated and cooled via a series of water channels. At these beam currents, this high-energy proton beam heats the target system, likely initiating subcooled flow boiling in the cooling channels. However, in-beam monitoring of the IPF target system is not possible due to the extreme radiation environment, and the necessarily significant shielding. To better understand high-power target performance, we developed ex-situ experimental and computational frameworks to predict the behavior of subcooled flow boiling at IPF. Subcooled flow boiling experiments on Inconel 625 samples under IPF conditions (2 bar pressure, 10 GPM flow rate (i.e., 2249 kg/m 2 /s), 85 K subcooling) revealed that IPF's average operating power is at the early stage of boiling with a heat transfer coefficient of 48,000 W/m 2 /s. The proposed modeling framework enables us to predict a complete boiling curve, i.e., single-phase heat transfer, onset of nucleate boiling, two-phase heat transfer, and critical heat flux (CHF), with specification of input boiling parameters up to intermediate heat flux levels. The estimated CHF under IPF conditions is 5.2 MW/m 2 . Experimental data under reduced conditions (2 bar pressure, 1.5 GPM flow rate (i.e., 337 kg/m 2 /s), 45 K subcooling) served as validation cases for the computational modeling. This computational model can be further extended to more complicated systems replicating the real IPF configuration, for instance, to study void distribution as a function of the incident proton beam profile and coolant velocity profile of multiple cooling channels. Finally, the proposed experimental and computational frameworks provide a means to better understand cooling systems in the isotope production facilities at different accelerators, where in-beam monitoring of the cooling process is not available.

07 ISOTOPE AND RADIATION SOURCES↗