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ICSBEP evaluation lessons learned and good practice

This document describes lessons learned during my nearly 20 years of experience in International Criticality Safety Benchmark Evaluation Project (ICSBEP) meetings and in the development of several evaluations employing the IPEN/MB-01 reactor. The evaluations cover a wide range of possible configurations at the reactor core of this facility. Most of the evaluations are related to critical configurations, although two of them concern subcritical measurements. Examples of the evaluations submitted and approved for ICSBEP publication are the critical configurations employed in the standard core; critical configurations employing heavy reflectors composed of stainless steel, nickel, and carbon steel; and critical configurations employing the standard fuel rods and fuel rods composed of UO 2 -Gd 2 O 3 , among several others. Additionally, this document addresses good practices for the development of ICSBEP evaluations; the intention is to help beginners who are going to start evaluations for ICSBEP. The sections of the ICSBEP evaluation are described and illustrated with several examples.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ICSBEP Benchmarking Tutorial for DNCSH

As part of the DOE/NRC Collaboration for Criticality Safety Support for Commercial-Scale HALEU for Fuel Cycles and Transportation (DNCSH), a workshop was held on Teams on how to write a ICSBEP benchmark that meets modern standards. The workshop prepared people performing experiments and writing benchmarks so that they have an increased chance of submitting a benchmark that will be accepted. The workshop was led by experts from LANL, LLNL and Sandia.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ICSBEP Benchmark Template

The purpose of this document is to demonstrate the ability of LATEX to create an ICSBEP benchmark evaluation. Creating a large document in LATEX offers many benefits, such as automatic numbering of items such as tables and figures, and easier placement of objects in the page. Additionally, it is easier to have multiple styles of pages in the same document, and in general the handling of large documents (which evaluations very commonly are) is not problematic. The formatting of this document is meant to conform to both the standards of the document and formatting guide and established practices in order to make the creation of new evaluations a more streamlined process. This will also help reduce the benchmark-to-benchmark variation in style.

97 MATHEMATICS AND COMPUTING↗

Status of HEU-Pb in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook

The Department of Energy invests tens of millions of dollars each year to develop the next generation of nuclear engineering modeling & simulation (M&S) tools. These tools are used to analyze advanced reactor designs and the safety of current nuclear operations. As computers become more powerful, we are able to enhance resolution in our calculations. This improved resolution is taking us to a point where the limitations of simulation capability are in the quality of data, including our ability to quantify the uncertainty and sensitivity of the data. In order to model systems of interest with increasing accuracy, the industry must improve key nuclear data measurements. Thus, M&S tools need evaluated and quality-assured experimental data for validation purposes. The International Criticality Safety Benchmark Evaluation Project (ICSBEP) compiles and evaluates experiment data in a handbook that can be used by criticality safety engineers and others to validate computer codes and cross-section libraries at nuclear facilities. Both critical and subcritical experiments are included in the handbook. Figure 1 organizes all the benchmark evaluations that have been performed by the isotope of interest, in this case Pb, and the average neutron energy the system. Compared to other isotopes of interest for nuclear applications, there are few benchmark evaluations for Pb systems. The lack of integral measurements to determine errors in Pb cross-section data has caused the latest nuclear cross-section libraries to over/underestimate k eff compared to experimental results. Therefore, this evaluation fills an important knowledge gap in benchmark evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Status of the CERBERUS Evaluation for the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook

Modeling & Simulation (M&S) tools are used to analyze advanced reactor designs and the safety of current nuclear operations. As computers continue to improve, we are able to enhance resolution in our calculations. Therefore, the limitations of simulation capability are in the quality of data that is being used, including our ability to quantify the uncertainty and sensitivity of that data. In order to model systems of interest with increasing accuracy, the industry must improve key nuclear data measurements. The International Criticality Safety Benchmark Evaluation Project (ICSBEP) compiles and evaluates experiment data in a handbook that can be used by criticality safety engineers and others to validate computer codes and cross section libraries at nuclear facilities. Both critical and subcritical experiments are included in the handbook. These experiments, along with differential measurements, can help improve the quality of nuclear data. Concerns regarding the accuracy of Cu nuclear data have been published. The large values and trend of C-E for the Zeus intermediate energy benchmark, being one of the primary examples. Furthermore, very few experiments have been designed to be sensitive to Cu (as shown in Figure 1), so an integral, critical experiment is needed to help resolve these differences.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Addendum to ICSBEP Logbooks 12r, 13r, 14r and 15r for Polyethylene and Graphite Reflected HEU Metal Critical Experiments

This report documents the experimenters’ data sheets that were recently (2023) discovered for critical experiments with highly enriched uranium metal with polyethylene and graphite reflectors. These data sheets were produced at the time of the measurements, when the dimensional inspection reports for the polyethylene and graphite were available. However, at this writing, those inspection reports are not available but may be in unmarked storage for the Y-12 National Security Complex. However, the data sheets presented herein contain sketches of the experimental configurations and other additional information that is not in the logbooks, such as dimensions and masses of the graphite measurements. This report reproduces the experimental data sheets that complement the logbooks. Some of the data on these sheets and the logbooks can be used to infer the dimensions and masses that are not documented. Some obvious mistakes in the logbook and data sheets have been corrected. In the reproduced data sheets, some of the information is not clearly visible: some information, such as average values, can be obtained from other data in the sheets or logbook. This report should be sent to the International Criticality Safety Benchmark Program at Idaho National Laboratory to complement the existing Oak Ridge Critical Facility logbooks there.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Validating ENDF/B-VIII.1beta3 with LLNL Pulsed-Sphere Experiments and ICSBEP Benchmarks [Slides]

LPS experiments are not benchmarks but can provide valuable input. 22/1/24 LPS experiments are not benchmarks but can provide valuable input. LPS (run by Denise) help validate nuclear data up to 15 MeV. They test scattering and fission data. They have incomplete uncertainties from 2-8%. I take note when: (1) I see C/E differences above the peak and before late times => 20%. (2) Simulated results between libraries change by => 20% without a good explanation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

LLNL IPD Tasks: ICSBEP and Pulsed Spheres Benchmark [Slides]

This lecture presented benchmark of the blank and polyethylene spheres at SINBAD in April 2023. In responding to comments about the building, we uncovered a large amount of additional detailed information about the building and experimental set up. We incorporated this new information into an even higher fidelity model and are working on uncertainty analysis at a low level. Scheduled to present at SINBAD meeting in April 2024.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

Status of the International Criticality Safety Benchmark Evaluation Project

The International Criticality Safety Benchmark Evaluation Project (ICSBEP) has continued its work generating evaluations of new and historical criticality benchmark experiments since the last update to the nuclear criticality safety community at the 11th International Conference on Nuclear Criticality Safety (ICNC 2019) in Paris, France. Three additional versions of the ICSBEP Handbook have been published since that update, and the Technical Review Group (TRG) held two in-person (in 2019 and 2023) and three virtual (2020 and 2021) meetings to review and approve additional benchmarks. The 2019 edition of the ICSBEP Handbook included five new evaluations with 79 new configurations, the 2020 version of the ICSBEP Handbook contained five new evaluations totaling 76 new configurations, and the 2021 version of the ICSBEP handbook contained five new evaluations with a total of 57 different configurations. The ICSBEP TRG met in October and December 2021, to review benchmarks for potential inclusion in the 2022 ICSBEP Handbook, with seven evaluations receiving provisional approval pending resolution of review group comments. Final comment resolution for some of these evaluations is currently underway and handbook publication should be completed soon. The ICSBEP TRG met again in person in April 2023 to review benchmarks for the 2023 ICSBEP Handbook, provisionally approving 7 new evaluations. The ICSBEP continues to deliver high-quality, peer reviewed evaluations of experiments relevant to the nuclear criticality safety community.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Status of the International Criticality Safety Benchmark Evaluation Project

The International Criticality Safety Benchmark Evaluation Project (ICSBEP) has continued its work generating evaluations of new and historical benchmark experiments since the last update to the nuclear criticality safety (NCS) community at the 12th International Conference on Nuclear Criticality Conference held in 2023. One additional version of the ICSBEP Handbook has been published since that update, and the Technical Review Group (TRG) held two in-person meetings to review and approve additional benchmarks. The 2022 and 2023 editions of the handbook were combined into one release (published in November 2024) and contained 13 new evaluations with 46 different configurations and two major revisions to existing evaluations. The 2024 version of the handbook, currently under publication review, will contain two new evaluations with 15 new configurations and one major revision to HEU-MET-FAST-028, the evaluation of Flattop with a uranium core. The ICSBEP TRG met again in person in April 2025 to review benchmarks for the 2025 ICSBEP Handbook and final comment resolution is currently ongoing. Many of the new benchmarks represent contemporaneous experiments that have been specifically optimized to provide validation cases relevant to the NCS community. One major area of focus for new critical experiments is to target the sparsely populated intermediate energy (or resonance) region. Another focus of many of the new benchmarks is to provide experiments sensitive to different materials, such as chlorine, hafnium, tantalum, titanium, molybdenum, chromium, and polymethyl methacrylate (PMMA, or Lucite). The ICSBEP continues to deliver high-quality, peer reviewed evaluations of integral experiments relevant to the nuclear data community.

HEU-MET-FAST-028↗

Preliminary Design of Critical Experiments Involving Commercially Available B 4 C Neutron Absorber Plates with Low-Enriched UO 2 Fuel

The International Criticality Safety Benchmark Evaluation Project (ICSBEP) is an initiative to provide high-quality benchmark data in a standardized format for criticality safety analysts to use to validate calculational tools and nuclear data. In the last released 2022 version, the ICSBEP handbook contains over 5,000 critical experiment descriptions, results, and associated models. This paper describes the critical configurations proposed and calculations performed as part of the conceptual design phase of Integral Experiment Request (IER) 554 (IER-554). The goal of IER-554 is to add to the benchmark experiments available to the criticality safety community by designing critical experiments that can analyze how adding commercially available Boralcan plates to an assembly of low-enriched UO2 fuel rods affects the effective neutron multiplication factor (k eff ). Boralcan, a neutron absorber product developed by Rio Tinto, is made of B4C in an Al 1100 matrix and is commonly used for criticality suppression in fuel storage pools. In the current version of the ICSBEP handbook, only a few dated critical experiments involve B4C materials, and none involve Boralcan in a thin plate shape. The experiments designed as part of IER-554 are intended to be performed at the Sandia Pulsed Reactor Facility/Critical Experiments (SPRF/CX) apparatus at Sandia National Laboratories. SPRF/CX is a well-characterized assembly considered trustworthy by the benchmarking community because of the numerous high-quality evaluations with very low experimental uncertainties included in the ICSBEP handbook. Figure 1 illustrates the assembly for a particular configuration from LCT-078, one of the published benchmarks in the ICSBEP handbook. The experiments will be moderated and reflected by light water at ambient atmospheric pressure. Before the plates are inserted in the critical assembly, they will be characterized with x-ray computed tomography (XCT) to identify the sizes and distribution of the B 4 C powder particles inside the plates. The preliminary design calculations were performed with SCALE 6.3.0 using the KENO V.a sequence for the criticality calculations, the CE-TSUNAMI-3D sequence for the sensitivity and uncertainty studies, and the ENDF/B-VII.1 Continuous Energy cross section library. All the calculation results presented have 10 pcm statistical uncertainties. A set of critical experiments with Boralcan plates could increase the confidence of the criticality safety community in its modeling methods when using this type of neutron absorber material. Experiments would also help validate k eff calculations, and the industry could use these validations to change the B loading credit limits from the US Nuclear Regulatory Commission standard review plan for dry cask storage of spent nuclear fuel. This paper summarizes only part of the analysis documented in the preliminary design report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Jemima Plate Characterization

The HEU Jemima plates have been utilized in numerous International Criticality Safety Benchmark Evaluation Project (ICSBEP) evaluations. ICSBEP evaluations are a vital com ponent of nuclear data validation for applications across the nuclear community. In the past, different combinations of mass, caliper measurements, and drawing dimensions have been used to define the HEU Jemima plates in ICSBEP evaluations. Some of these combinations result in large density ranges (17 g/cm 3 to 19 g/cm 3 ) or unrealistic densities (greater than 19 g/cm 3 ). Additionally, oxidation of the plates has led to questioning the flatness of each plate, which can add additional gaps in experiment configurations. This work proposes a standardized method of defining the commonly used HEU Jemima plates across different experiments.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Delayed Critical Highly Enriched Uranium Metal Cylinders with Thin Graphite Top and Bottom Reflectors

Nine 7, 11, and 15 in. diam highly enriched uranium (HEU, 93.15 wt % 235 U) metal cylinders were assembled on the vertical assembly machine in the Oak Ridge Critical Experiments Facility (ORCEF) and had 1, 2, or 3 in. thick HLM graphite reflectors on the top and bottom. The experiments, which were performed between April 3, 1970, and February 18, 1971, used 23 operational days at ORCEF. Before those experiments were carried out, unreflected and unmoderated, graphite- and polyethylene-reflected, and polyethylene-moderated HEU metal cylinders had been assembled to obtain delayed criticality at ORCEF in the 1960s and reported by the International Criticality Safety Benchmark Evaluation Project (ICSBEP) at the Nuclear Energy Agency (NEA)*. The data from the nine critical experiments are acceptable for use as criticality safety benchmark experiments for the NEA’s ICSBEP once the uncertainty analysis is completed. Based on previous ICSBEP benchmarks with HEU metal at ORCEF, the uncertainties in k eff are expected to be as low as ±0.0004.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Final Design for Thermal/Epithermal eXperiments (TEX) with Lithium Absorbers to Provide Validation Benchmarks for Y-12 Electrorefining Facility

One of the main goals of the Thermal/Epithermal eXperiments (TEX) project is to use existing Nuclear Criticality Safety Program (NCSP) assets to create critical experiment plutonium and uranium test beds for materials important to criticality safety that have insufficient benchmark evaluations. The plutonium test bed experiments were completed in 2018 and are published in the 2020 edition of the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. The uranium test bed assemblies were completed in 2023 and accepted in the 2024 edition of the ICSBEP Handbook. The Nuclear Criticality Safety (NCS) group at Y-12 National Security Complex has identified programmatic need for validation cases for uranium electrorefining operations at Y-12. The electrorefining operation credits lithium enriched in 6 Li in addition to 35 Cl as absorbers in the design criticality safety evaluation for precluding criticality under upset conditions in the large and geometrically unfavorable electro-refiner. There is, however, inadequate experimental validation for the 6 Li absorbers. As an extension of the TEX uranium test bed, TEX-Cl critical experiments were performed with sodium chloride salt to address the 35 Cl thermal absorption as well as other validation needs at Los Alamos National Laboratory (LANL). These experiments were completed in 2024 and accepted into the 2025 ICSBEP Handbook. To continue the methodology used in TEX-Cl, TEX-Li aims to accomplish the same. The overall design of both experiments was to use commercially available, high purity, salts with polyethylene moderator and HEU plates to configure a critical assembly. Three experiments are planned for TEX-Li using encapsulated lithium carbonate (Li 2 CO 3 ), with natural 6 Li abundance. For all experiments, the highly enriched uranium (HEU) Jemima plates will be used as fissile material. Multiple layers will be stacked together with encapsulated Li 2 CO 3 alternated with polyethylene in standard configurations. Standard stacking was found to be optimal in matching the different sensitivity profiles provided by the Y-12 models. Three configurations are proposed with varying polyethylene moderation and a constant 1/4” absorber thickness. The first uses 11 layers of 5/4” polyethylene, the second uses 9 layers of 3/4” polyethylene, and the third uses 10 layers of 1/2” polyethylene. Calculations showed that some alternative forms of lithium-based materials provided slightly less-optimal sensitivity profiles when compared to lithium carbonate but come with other drawbacks. These alternatives included lithium aluminate (LiAlO 2 ), Aluminum-2050 alloy, Aluminum-8090, Aluminum-2095, lithium hydride (LiH), and lithium fluoride (LiF). Lithium aluminate and aluminum-2050 provided comparable sensitivity profiles when compared to lithium carbonate and can be used instead if lithium carbonate cannot be readily procured. After a broad material study, lithium carbonate outperformed any alternative material with a balance in affordability and workability. The assessment of experimental uncertainties of the non-absorber and absorber components was predicted to be 0.00089 and 0.00093 Δk eff , respectively. The largest uncertainties may be reduced with precision dimensional inspection of the components. Many of the parts and equipment for IER 575 have already been fabricated or procured for previous projects and therefore do not contribute significantly to the overall cost of this experiment. This includes the Jemima plates and Comet critical assembly machine, which are existing NCSP assets, as well as the aluminum platen and polyethylene reflector rings, which were fabricated and authorized for the TEX experiment involving HEU with polyethylene. Lithium carbonate containers will be procured by LANL and will be filled by LLNL. The total material costs for TEX-Li experiments are estimated to be on the order of $\$$47,400. Precision inspection, including dimensional, mass, density, and impurity, is recommended for all components for an estimated cost of $\$$12,000.

35Cl↗

Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Integral Experiment Execution (CED-3b Report)

This report documents the experimental configurations and measurements for IER-518: Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Experiments. These measurements involved a series of subcritical configurations at the Sandia Critical Experiments (SCX) facility at Sandia National Laboratories (SNL). The purpose of these measurements was to produce time tagged neutron count data of configurations that exceed a subcritical multiplication of 20, which is the high end of the fundamental physics benchmarks currently available in the International Criticality Safety Benchmark Evaluation Project Handbook (ICSBEP). These measurements leverage experimental configurations 1 and detector systems 2 from previously accepted ICSBEP benchmark evaluations, allowing evaluations of these measurements to be performed at greatly reduced cost.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Impact of recent ENDF nuclear data update, high initial enrichment and high burnup fuel on critical experiments applicability determination via the integral index c k for burnup credit validation

In 2012, NUREG/CR-7109 reported on the validation of burnup credit calculations involving major and minor actinides and major fission products which was investigated for pressurized and boiling water reactor (PWR and BWR) fuel enrichments up to 5 wt% 235 U and assembly-average burnups up to 60 GWd/MTU. Recently, there has been interest in increasing the maximum enrichment used in PWR fuel as high as 8 wt% 235 U and correspondingly increasing the maximum assembly-average burnups to approximately 75 GWd/MTU. These proposed increases in enrichment and burnup necessitate reinvestigation of the validation basis for k eff calculations for this expanded application space. Additionally, the 2012 study was performed by using the Evaluated Nuclear Data File (ENDF)/B-VII.0 nuclear data with the SCALE 6 covariance library, and the effects of using the newly released ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear data and covariance libraries should be evaluated. In this work, published in NUREG/CR-7309 in 2025, the validation assessment was performed consistently with NUREG/CR-7109: modeling irradiated fuel assemblies in the Generic Burnup Credit (GBC)-32 cask defined in NUREG/CR-6747. The TSUNAMI-3D sequence was used to generate sensitivity data for the application model, and the data were compared with sensitivity data from select benchmark models. The integral parameter c k is the metric of similarity used in this study and is consistent with NUREG/CR-7109, where a c k value in excess of 0.8 indicates sufficient similarity for use in validation. A new set of benchmark experiments with sensitivity data has been assembled for this effort. The number of experiments with available sensitivity data is now 2,104, compared to 474 in NUREG/CR-7109. This increase was facilitated by the efforts of the Nuclear Energy Agency to generate sensitivity data for a majority of the experiments in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook to supplement the data available in the Oak Ridge National Laboratory (ORNL) Verified, Archived Library of Inputs and Data (VALID). The complete set of benchmarks considered here includes experiments for low-enriched uranium (LEU), intermediate enriched uranium (IEU), and a mixture of uranium and plutonium (MIX) from the ICSBEP Handbook and VALID, as well as ORNL models of the Haut Taux de Combustion (HTC) experiments and other potentially relevant models not included in VALID. The updated similarity study shows that none of the extended burnup and higher enrichment combinations considered show a significant decrease in the number of potentially applicable experiments, meaning sufficient critical experiments exist for the validation of BUC criticality safety calculations, with initial enrichments up to 8 wt% 235 U and burnups up to 80 GWd/MTU. Additionally, both the ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear data libraries can be used for validation since the number of critical experiments applicable for validation increases for most cases with the most recent nuclear data compared to the previous one. As in previous BUC validation studies, the French HTC experiments are the most similar in a majority of the application cases studied, especially from representative discharge burnups ranging from 40 to 80 GWd/MTU. In conclusion, these results match the conclusions presented in NUREG/CR-7109 regarding validation of the primary actinides in BUC analyses.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

HEU Pancake (Jemima) Plate Preliminary Characterization Report

The HEU pancake (Jemima) plates have been used in multiple International Criticality Safety Benchmark Evaluation Project (ICSBEP) evaluations, including: HEU-MET-FAST-072, HEU-MET-FAST-073, HEU MET-FAST-102, HEU-MET-INTER-006, HEU-MET-INTER-011, HEU-MET-MIXED-021, and IEU MET-FAST-025. This report only focuses on the physical dimension characterization, since concerns have been identified about reliable diameter and height measurements. Historically, height measurements with calipers and mass measurements have been performed for every plate. However, the combination of previous measurements (mass and caliper height measurements) with the drawing dimensions for the diameters led to unrealistic densities (>19 g/cm 3 ) or large ranges of densities for parts that were manufactured at the same time (17 g/cm 3 to >19 g/cm 3 ). Due to the oxidation of the plates, questions about the flatness of each plate and what gaps are introduced into the system have been discussed, since gaps tend to be one of the largest sources of uncertainty in stacked benchmark experiments. The purpose of this report is to characterize a subset of this commonly used fuel. A uniform method for how to define the HEU pancake plates for ICSBEP evaluations will also be proposed with a discussion on what measurements should be performed on the remaining HEU pancake plates in the NCERC inventory.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗