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All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Nuclear Data Sheets for A = 139

The experimental nuclear spectroscopic data for known nuclides of mass number 139 (Sn, Sb, Te, I, Xe, Cs, Ba, La, Ce, Pr, Nd, Pm, Sm, Eu, Gd, Tb, Dy) have been evaluated and presented together with adopted properties for levels and gamma rays. This evaluation represents a revision of previous one (2001Bu16) by T.W. Burrows. Since then extensive new data have become available for many A=139 nuclides although, no excited state data are yet available for {sup 139}Sn, {sup 139}Sb, {sup 139}Tb, and {sup 139}Dy. The decay schemes of {sup 139}Sn, {sup 139}Sb, {sup 139}I, {sup 139}Tb and {sup 139}Dy nuclei are not known, and those for {sup 139}Gd and {sup 139}Eu are poorly known. Particle-transfer data are available for {sup 139}Ba, {sup 139}La, {sup 139}Ce and {sup 139}Pr. Limited high-spin data are available for {sup 139}Te, {sup 139}I, {sup 139}Cs, {sup 139}Ba, {sup 139}La and {sup 139}Ce, while such data are extensive for {sup 139}Pr, {sup 139}Nd, {sup 139}Pm, {sup 139}Sm, {sup 139}Eu and {sup 139}Gd. Recent {sup 139}Pm high-spin data from two independent studies using the same reaction and similar beam energy are in conflict and could be improved using state-of-the-art large gamma-detector arrays in contrast to the smaller arrays currently used. Cases for which no new experimental information are available since the last update have undergone checking resulting in some changes in the current work, but for the most part these are taken from the previous evaluations. Thus, the present work has greatly benefited from all prior NDS evaluations (2001Bu16, 1989Bu12, 1981Pe04, 1974Gr46), but at the same time data presented herein supersede those in the earlier evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Iodine Vapor Reactions with Pure Metal Wires at Temperatures of 100–139 °C in Air

In this work, I 2(g) reactions with 11 metal wires (i.e., Al, Ag, Cu, In, Mo, Nb, Ni, Pd, Pt, Sn, Ta) were evaluated at three temperatures (i.e., 100 ± 3°C, 123 ± 4°C, 139 ± 5°C) with exposure times of 24 hours at each temperature. Over these temperatures, some of the metals showed increased mass gain with higher temperatures (i.e., In, Ag, Cu), Sn showed decreased iodine capture at increased temperatures, and most metals (i.e., Mo, Nb, Ni, Pd, Pt, and Ta) showed little to no mass gain at all temperatures. Silver mordenite (AgZ) was used as a standard during these studies and showed a consistent mass gain (m% I ) of 10.6 → 12.8% over this temperature range. The values of mass of iodine captured per mass of starting metal (g g -1 ) ranged widely across the study with the highest values achieved for (in descending order) Sn-T 100°C (4.37), In-T 139°C (3.34), Sn-T 123°C (1.98), In-T 123°C (1.57), Ag-T 139°C (1.19), In-T 100°C (0.97), and Cu-T 139°C (0.71). In some cases, the metal-iodide complex was not stable at the experimental temperature and it was clear some volatility had occurred during the experiment based on discoloration in the vials. These results show that some metals can have extensive reactions with I 2(g) without showing metal-iodide preferences over metal-oxide formation based on thermodynamic predictions. It is possible that materials such as these could be implemented near nuclear facilities to getter I 2(g) in the event of a nuclear accident.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

High spin spectroscopy of near spherical nuclei: Role of intruder orbitals

High spin states of nuclei in the vicinity of neutron shell closure N = 82 and proton shell closure Z = 82 have been studied using the Clovere Ge detectors of Indian National Gamma Array. The shape driving effects of proton and neutron unique parity intruder orbitals for the structure of nuclei around the above shell closures have been investigated using light and heavy ion beams. Lifetime measurements of excited states in {sup 139}Pr have been done using pulsed-beam-γ coincidence technique. The prompt spectroscopy of {sup 207}Rn has been extended beyond the 181μs 13/2{sup +} isomer. Neutron-rich nuclei around {sup 132}Sn have been produced from proton induced fission of {sup 235}U and lifetime measurement of low-lying states of odd-odd {sup 132}I have been performed from offline decay.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Identification of the feeding arteries of hepatocellular carcinomas by performing dual arterial phase CT during pre-transarterial chemoembolization angiography

Purpose: This study evaluated the usefulness of performing dual arterial phase computed tomography (CT) during pre-transarterial chemoembolization (TACE) angiography for identifying the feeding arteries of hepatocellular carcinomas (HCC). Materials and methods: Dual arterial phase CT was performed during pre-TACE angiography in 73 patients with 139 HCC. Ten HCC underwent this procedure twice, so the total number of examined HCC was 149. Early and late arterial phase images were obtained 6 seconds after injection of an iodinated contrast material serially during a single breath-hold. The feeding artery was defined as the branch of the hepatic artery that was connected to the enhanced areas of the tumor. For HCC that could not be visualized on the early arterial phase images, fusion images superimposing the early and late arterial phase images were constructed. Furthermore, technical success defined as successful catheterization of the subsegmental or more distal feeding artery was evaluated. Results: The feeding artery was correctly identified on dual arterial phase CT in 146 of the 149 tumors (98.0%). In two HCC, the feeding arteries could not be identified due to severe motion artifacts, and in one, due to the presence of anastomosis between the right and left hepatic arteries. Catheterization of the subsegmental feeding artery was successful in all TACE procedures (technical success rate: 100%). Conclusion: Performing dual arterial phase CT during angiography appears to be useful for identifying the feeding arteries of HCC.

62 RADIOLOGY AND NUCLEAR MEDICINE↗
DOE OSTI2015

Photodissociation of Methyl Iodide via Selected Vibrational Levels of the $\tilde{B}$ ( 2 E 3/2 )6s Rydberg State

We have determined the I 2P3/2 and 2P1/2 branching fractions following the photodissociation of methyl iodide (CH3I) via a number of vibronic bands associated with the $\tilde{B}$ (2E3/2)6s Rydberg state at excitation wavelengths between 201.2 and 192.7 nm. Vacuum ultraviolet light at 118.2 nm was used to ionize both the product iodine atoms and the methyl radical cofragments, and velocity map ion imaging was used to determine the product translational energy distributions and angular distributions. The known relative photoionization cross sections for I 2P3/2 and 2P1/2 at 118.2 nm were used to determine the corresponding branching fractions. The results extend our earlier work at 193 nm by Xu et al. (J. Chem. Phys. 2013, 139, 214310), and complement the closely related work of González et al. (J. Chem. Phys. 2011, 135, 021102). We find that for most of the excited vibronic levels of the $\tilde{B}$ state studied, the I 2P3/2 branching ratio is small, but nonzero, and that this channel is associated with internally excited CH3 radicals. The results are discussed in relation to the recent theoretical results of Alekseyev et al. (J. Chem. Phys. 2011, 134, 044303).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗