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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

An Investigation of the Ice Cloud Detection Sensitivity of Cloud Radars Using the Raman Lidar at the ARM SGP Site

The ice cloud detection sensitivity of the millimeter cloud radar (MMCR) and the Ka-band Zenith radar (KAZR) is investigated using a collocated Raman lidar (RL) at the Atmospheric Radiation Measurement Program Southern Great Plains site. Only profiles that are transparent to the RL with ice clouds only are considered in this study. The MMCR underestimates the RL ice cloud optical depth (COD) by 20%. The MMCR detects no ice clouds in 37% of the profiles. These profiles where ice cloud goes undetected by the MMCR typically contain very optically thin clouds, with a mean RL ice COD of 0.03. Higher ice cloud detection sensitivity is found for the KAZR, which underestimates the RL ice COD by 15%. The decrease in the ice COD bias for the KAZR compared to the MMCR is largely due to a decrease in the ice COD bias for the situation where the transparent profiles with ice clouds are detected by both the RL and cloud radar. The climatic net ice cloud radiative effects (CREs) from the RL at the top of the atmosphere (TOA) and the surface are 3.2 W m−2 and −0.6 W m−2, respectively. The ice CREs at the TOA and surface are underestimated for the MMCR by 0.7 W m−2 and 0.16 W m−2 (21% and 29%) and underestimated for the KAZR by 0.6 W m−2 and 0.14 W m−2 (17% and 24%). The ice clouds undetected by the cloud radars led to underestimating the climatic net cloud heating rates below 150 hPa by about 0–0.04 K day−1.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation

The prediction of ice cloud formation in the atmosphere remains challenging. Free tropospheric aerosols can act as ice nucleating particles (INPs), affecting cloud properties and precipitation. The physicochemical properties of free tropospheric particles are modified upon long-range transport by different atmospheric processes. These modifications affect the ice formation potential of individual particles. We investigated free tropospheric particles collected at the remote Pico Mountain Observatory at 2225m a.s.l. in the North Atlantic Ocean using multimodal microspectroscopy and chemical imaging techniques. We probed their ice nucleation activity using an ice nucleation stage interfaced with an environmental scanning electron microscope. Retroplume analysis, chemical imaging, and micro-spectroscopy analysis indicated that the size-resolved chemical composition, mixing state, and phase state of the articles with similar aging times but different transport patterns were substantially different. Relative humidity-dependent glass transition temperatures estimated from meteorological conditions were consistent with the observed organic component of the particles' phase. More viscous (solid and semi-solid-like) particles are more ice active in deposition mode at temperature ranging from 205-220 K than those less viscous particles. Finally, this study provides a better understanding of the phase and mixing state of long range transported free tropospheric aerosols and their role in ice cloud formation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Performance of Cloud 3D Solvers in Ice Cloud Shortwave Radiation Closure Over the Equatorial Western Pacific Ocean

Abstract For retrieving cloud optical properties from satellite images or computing these properties from climate model output, computationally efficient treatments of cloud horizontal inhomogeneity include the Monte Carlo Independent Column Approximation (McICA) and the Tripleclouds method. Computationally efficient treatment of cloud horizontal radiation exchanges includes the SPeedy Algorithm for Radiative TrAnsfer through CloUd Sides (SPARTACUS). As a test to derive properties from satellite images, we collocate Moderate Resolution Imaging Spectroradiometer (MODIS) cloud retrievals with near‐nadir Cloud and the Earth's Radiant Energy System (CERES) footprints in July 2008 over an equatorial western Pacific Ocean region to compare the performance of the McICA, Tripleclouds, and SPARTACUS solvers to the conventional plane‐parallel homogeneous (PPH) treatment. PPH overestimates cloud albedo, and the three solvers effectively reduce overestimation with root mean square error of shortwave upwelling irradiance decreasing between 15.72 and 18.53 W m −2 , or about 22%–25%. Although cloud top variability does not get fed into the simulations, all three solvers also reduce the effect of cloud top variability on cloud albedo. Entrapment (energy reflected downward from clouds) and horizontal radiation transfer have opposite effects on the SPARTACUS cloud albedo simulation. The net effect depends on the cloud vertical extent, the unawareness of which limits the performance of the SPARTACUS solver.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

A Refined Understanding of the Ice Cloud Longwave Scattering Effects in Climate Model

Abstract Because longwave (LW) absorption by greenhouse gases and clouds is more significant than the LW scattering effect by clouds, most climate models neglect cloud LW scattering to save computational costs. Ignoring cloud LW scattering directly overestimates outgoing longwave radiation (OLR). This study included ice‐cloud LW scattering treatment in the Exascale Energy Earth System Model (E3SM) version 2 and ran fully‐coupled simulations, prescribed sea surface temperature simulations, and offline radiative transfer calculations to comprehensively assess the impact of ice‐cloud LW scattering on global climate simulation. The instantaneous effect due to ice‐cloud LW scattering reduces the OLR by ∼1 W/m 2 on the global average and 2 W/m 2 on the tropical average. Tropospheric warming and high cloud amount reduction act to partially compensate for such instantaneous OLR reduction caused by the inclusion of LW scattering. When the simulation reaches the equilibrium, the surface warms by 0.66 K on average with respect to the simulation without LW scattering, with the Arctic surface temperature differences more than twice as large as that of the global mean. The impact of including LW scattering on the simulated climate change in response to 4 × CO 2 is also assessed. While including the cloud LW scattering does not significantly modify radiative forcing and total radiative feedback under such a scenario, it results in a 10% more positive cloud feedback.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Seasonal Dependent Impact of Ice Cloud Longwave Scattering on the Polar Climate

Most climate models neglect cloud longwave (LW) scattering because scattering is considered negligible compared to strong LW absorption by clouds and greenhouse gases. While this rationale is valid for simulating extrapolar regions, it is questionable for the polar regions, where the atmosphere is dry and hence has weak absorption, and ice clouds that have strong scattering capability frequently occur. Using the slab-ocean Community Earth System Model, we show that ice cloud LW scattering can warm winter surface air temperature by 0.8–1.8 K in the Arctic and 1.3–1.9 K in the Antarctic, while this warming becomes much weaker in polar summer. Such scattering effect cannot be correctly assessed when sea surface temperature and sea ice are prescribed as this effect is manifested through a surface-atmosphere coupling. Furthermore, cloud LW scattering is a necessity for the correct simulation of polar climate and surface radiation budget, especially in the winter.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

The correlation between Arctic sea ice, cloud phase and radiation using A-Train satellites

Abstract. Climate warming has a stronger impact on Arctic climate and sea ice cover (SIC) decline than previously thought. Better understanding and characterization of the relationship between sea ice and clouds and the implications for surface radiation is key to improving our confidence in Arctic climate projections. Here we analyze the relationship between sea ice, cloud phase and surface radiation over the Arctic, defined as north of 60° N, using active- and passive-sensor satellite observations from three different datasets. We find that all datasets agree on the climatology of and seasonal variability in total and liquid-bearing (liquid and mixed-phase) cloud covers. Similarly, our results show a robust relationship between decreased SIC and increased liquid-bearing clouds in the lowest levels (below 3 km) for all seasons (strongest in winter) but summer, while increased SIC and ice clouds are positively correlated in two of the three datasets. A refined map correlation analysis indicates that the relationship between SIC and liquid-bearing clouds can change sign over the Bering, Barents and Laptev seas, likely because of intrusions of warm air from low latitudes during winter and spring. Finally, the increase in liquid clouds resulting from decreasing SIC is associated with enhanced radiative cooling at the surface. Our findings indicate that the newly formed liquid clouds reflect more shortwave (SW) radiation back to space compared to the surface, generating a cooling effect of the surface, while their downward longwave (LW) radiation is similar to the upward LW surface emission, which has a negligible radiative impact on the surface. This overall cooling effect should contribute to dampening future Arctic surface warming as SIC continues to decline.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Characteristics of Ice Cloud–Precipitation of Warm Season Mesoscale Convective Systems over the Great Plains

Abstract In this study, the mesoscale convective systems (MCSs) are tracked using high-resolution radar and satellite observations over the U.S. Great Plains during April–August from 2010 to 2012. The spatiotemporal variability of MCS precipitation is then characterized using the Stage IV product. We found that the spatial variability and nocturnal peaks of MCS precipitation are primarily driven by the MCS occurrence rather than the precipitation intensity. The tracked MCSs are further classified into convective core (CC), stratiform rain (SR), and anvil clouds regions. The spatial variability and diurnal cycle of precipitation in the SR regions of MCSs are not as significant as those of MCS precipitation. In the SR regions, the high-resolution, long-term ice cloud microphysical properties [ice water content (IWC) and ice water paths (IWPs)] are provided. The IWCs generally decrease with height. Spatially, the IWC, IWP, and precipitation are all higher over the southern Great Plains than over the northern Great Plains. Seasonally, those ice and precipitation properties are all higher in summer than in spring. Comparing the peak timings of MCS precipitation and IWPs from the diurnal cycles and their composite evolutions, it is found that when using the peak timing of IWPSR as a reference, the heaviest precipitation in the MCS convective core occurs earlier, while the strongest SR precipitation occurs later. The shift of peak timings could be explained by the stratiform precipitation formation process. The IWP and precipitation relationships are different at MCS genesis, mature, and decay stages. The relationships and the transition processes from ice particles to precipitation also depend on the low-level humidity.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Broadband and filter radiometers at Ross Island, Antarctica: detection of cloud ice phase versus liquid water influences on shortwave and longwave radiation

Abstract. Surface radiometer data from Ross Island, Antarctica, collected during the austral summer 2015–2016 by the US Department of Energy Atmospheric Radiation Measurement (ARM) program West Antarctic Radiation Experiment (AWARE), are used to evaluate how shortwave and longwave irradiance respond to changing cloud properties as governed by contrasting meteorological regimes. Shortwave atmospheric transmittance is derived from pyranometer measurements, and cloud conservative-scattering optical depth is derived from filter radiometer measurements at 870 nm. With onshore flow associated with marine air masses, clouds contain mostly liquid water. With southerly flow over the Transantarctic Mountains, orographic forcing induces substantial cloud ice water content. These ice and mixed-phase clouds attenuate more surface shortwave irradiance than the maritime-influenced clouds and also emit less longwave irradiance due to colder cloud base temperature. These detected irradiance changes are in a range that can mean onset or inhibition of surface melt over ice shelves. This study demonstrates how basic and relatively low-cost broadband and filter radiometers can be used to detect subtle climatological influences of contrasting cloud microphysical properties at very remote locations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Processes Associated with Boundary Layer Cloud Ice Phase Precipitation in the High Southern Latitudes (Final Technical Report)

This is a final technical report for DOE Award No. DE-SC0018995. Using data collected during the MARCUS deployment of the 2nd ARM mobile facility, this project sought to address the following scientific questions: 1. What are the conditions that govern phase partitioning in supercooled boundary layer clouds over the high latitude Southern Oceans? 2. To what extent are supercooled mixed phase clouds responsible for the high cloud fractions over the Southern Ocean and do these mixed phase clouds contribute to the model biases in absorbed shortwave radiation? 3. Can the cloud properties and phase partitioning over the Southern Ocean be linked to the underlying aerosol environment? 4. How do the aerosol properties at the surface vary spatially and seasonally over the high latitude Southern Ocean and what processes control these features? 5. How well defined are the atmospheric compositional boundaries between Southern Ocean marine, Antarctic free tropospheric, and Antarctic surface airmasses, and how does this influence the chemistry and physics of the Southern Ocean atmosphere? In this project we published three peer review journal articles that address these questions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Sizing ice hydrometeor populations using the dual-wavelength radar ratio

Dual-wavelength (3.2 and 0.32 cm, i.e., X- and W-radar bands) radar ratio (DWR) measurements in ice clouds and precipitation using Canada's National Research Council Institute for Aerospace Research airborne radar are compared to closely collocated particle microphysical in situ sampling data in order to develop relations between DWR and characteristic hydrometeor size. This study uses the radar and in situ data sets collected during the In-Cloud ICing and Large-drop Experiment (ICICLE) campaign in midlatitude frontal clouds. Since atmospheric particle scattering at X band is predominantly in the Rayleigh regime and the W-band frequency is the highest frequency usually used for hydrometeor remote sensing, the X–W-band combination provides a relatively strong dual-wavelength reflectivity difference. This study considers radar and in situ measurements conducted in relatively homogeneous cloud and precipitation conditions. Measurements show that under these conditions, the difference between the X-band radar reflectivities observed with vertical and horizontal pointing of the radar beam are generally small and often negligible. However, W-band reflectivities at vertical beam pointing are, on average, larger than those for horizontal beam pointing by about 4 dB, which is a non-Rayleigh scattering effect from preferentially oriented non-spherical particles. A horizontal radar beam DWR–mean volume particle size relation, D v , provides robust estimates of this characteristic size for populations of particles with different habits. Uncertainties of D v retrievals using DWR are around 0.6 mm when D v is greater than approximately 1 mm. Size estimates using vertical radar beam DWRs have larger uncertainties due to smaller dual-wavelength signals and stronger influences of hydrometeor habits and orientations at this geometry of beam pointing. Mean relations among different characteristic sizes, which describe the entire particle size distribution (PSD), such as D v , and other sizes used in various applications (e.g., the mean, effective, and median sizes) are derived, so the results of this study can be used for estimating different PSD characteristic sizes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Development of a triple-moment ice-phase cloud microphysics scheme and its application to the Single Column Atmosphere Model

Parameterization of cloud microphysics is critical for accurate simulation of weather and climate, in which the characteristics of cloud particle spectrum inevitably further affect climate simulation by changing the cloud evolution and cloud radiation effects. The popular currently used double-moment cloud microphysics schemes in numerical models can predict the intercept (N 0 ) and slope (λ) parameters of cloud particle spectrum but cannot predict the spectral shape parameter (μ), which hinders accurate description of cloud physical processes in climate models. Therefore, in the present study, we built upon the ideas of previously developed triple-moment cloud microphysics scheme, considered radar reflectivity factor as the third predictor in addition to number and mass concentration, and introduced its related prediction equation to the Single Column Atmosphere Model Version 5.3 (SCAM5.3). Moreover, the relevant microphysical process formulas in the model were revised, and a triple-moment ice-cloud microphysics scheme was constructed to predict the μ of ice particle spectrum. Based on this model, a 29-day case of the Atmospheric Radiation Measurement Program in the summer of 1997 (ARM97) was simulated, and the differences in cloud fraction and radiation simulations between the double- and triple-moment schemes were analysed. The μ of ice particle spectrum predicted by the triple-moment scheme mainly ranged from 0 to 4; the peak value was around 2, and at least 85% of the μ values were greater than the default 0. Therefore, the μ=0 setting in the double-moment scheme is unreasonable. Moreover, the developed triple-moment ice-cloud microphysics scheme yielded a narrower ice particle spectrum, which was closer to the observation results of previous studies, than the double-moment cloud microphysics scheme (e.g., height=233 hPa). Furthermore, compared with the double-moment scheme, the triple-moment scheme achieved closer simulations of the cloud fraction observations, particularly for ice clouds in the upper levels. Considering the close association between cloud fraction and radiation, the error with the triple-moment scheme was smaller than that with the double-moment scheme regardless of the shortwave (surface downward shortwave radiation, net downward shortwave radiation at the top of the atmosphere, and net shortwave radiation at the surface) or longwave (surface downward longwave radiation and net longwave radiation at the surface) flux density. Finally, the improvement mechanism of the triple-moment scheme on cloud fraction and radiation simulations was explored. The major reason is that the triple-moment scheme weakens the autoconversion of ice crystal to form snow and enhances the growth process of ice crystal deposition, thereby increasing the mass concentration of ice crystals and ice cloud fraction. Overall, the developed triple-moment ice-cloud microphysics scheme can help improve the simulation ability of models for cloud-climate feedback and other processes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Sensitivity of Arctic Clouds to Ice Microphysical Processes in the NorESM2 Climate Model

Abstract Ice formation remains one of the most poorly represented microphysical processes in climate models. While primary ice production (PIP) parameterizations are known to have a large influence on the modeled cloud properties, the representation of secondary ice production (SIP) is incomplete and its corresponding impact is therefore largely unquantified. Furthermore, ice aggregation is another important process for the total cloud ice budget, which also remains largely unconstrained. In this study, we examine the impact of PIP, SIP, and ice aggregation on Arctic clouds, using the Norwegian Earth System Model, version 2 (NorESM2). Simulations with both prognostic and diagnostic PIP show that heterogeneous freezing alone cannot reproduce the observed cloud ice content. The implementation of missing SIP mechanisms (collisional breakup, drop shattering, and sublimation breakup) in NorESM2 improves the modeled ice properties, while improvements in liquid content occur only in simulations with prognostic PIP. However, results are sensitive to the description of collisional breakup. This mechanism, which dominates SIP in the examined conditions, is very sensitive to the treatment of the sublimation correction factor, a poorly constrained parameter that is included in the utilized parameterization. Finally, variations in ice aggregation treatment can also significantly impact cloud properties, mainly through their impact on collisional breakup efficiency. Overall, enhancement in ice production through the addition of SIP mechanisms and the reduction in ice aggregation (in line with radar observations of shallow Arctic clouds) result in enhanced cloud cover and decreased TOA radiation biases, compared to satellite measurements, especially during the cold months. Significance Statement Arctic clouds remain a large source of uncertainty in projections of the future climate due to the poor representation of the microphysical processes that govern their life cycle. Ice formation is among the least understood processes. While it is widely recognized that better constraints on primary ice production (PIP) are needed to improve existing parameterizations, we show that secondary ice production (SIP) and ice aggregation can have also a significant impact on ice number concentrations. Constraining ice formation through the addition of missing SIP mechanisms and reducing ice aggregation can improve the representation of the cloud macrophysical properties and enhance total cloud cover in the Arctic region, which in turn contributes to decreased TOA radiation biases in the cold months.

Meteorology & Atmospheric Sciences↗
DOE OSTI2020

CERES MODIS Cloud Product Retrievals for Edition 4--Part I: Algorithm Changes

The Edition 2 (Ed2) cloud property retrieval algorithm system was upgraded and applied to the MODerate-resolution Imaging Spectroradiometer (MODIS) data for the Clouds and the Earth's Radiant Energy System (CERES) Edition 4 (Ed4) products. New calibrations for solar channels and the use of the 1.24-μm channel for cloud optical depth (COD) over snow improve the daytime consistency between Terra and Aqua MODIS retrievals. Use of additional spectral channels and revised logic enhanced the cloud-top phase retrieval accuracy. A new ice crystal reflectance model and a CO₂-channel algorithm retrieved higher ice clouds, while a new regional lapse rate technique produced more accurate water cloud heights than in Ed2. Ice cloud base heights are more accurate due to a new cloud thickness parameterization. Overall, CODs increased, especially over the polar (PO) regions. The mean particle sizes increased slightly for water clouds, but more so for ice clouds in the PO areas. New experimental parameters introduced in Ed4 are limited in utility, but will be revised for the next CERES edition. As part of the Ed4 retrieval evaluation, the average properties are compared with those from other algorithms and the differences between individual reference data and matched Ed4 retrievals are explored. Part II of this article provides a comprehensive, objective evaluation of selected parameters. More accurate interpretation of the CERES radiation measurements has resulted from the use of the Ed4 cloud properties.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

microbase.c1

MICROBASE is a baseline retrieval of cloud microphysical properties. It uses a combination of observations from the cloud radar, ceilometer, micropulse lidar, microwave radiometer, and balloon-borne radiosonde soundings in order to produce instantaneous vertical profiles of cloud liquid water content (LWC), cloud ice water content (IWC), liquid cloud particle effective radius (LIQRE), and ice cloud particle effective radius (ICERE). Uncertainites are also produced by the VAP. The inputs are by the following VAPs: Active Remote Sensing of Clouds (ARSCL) Merged Sounding (MERGESONDE) Microwave Radiometer Retrievals (MWRRET) The output are daily files.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Tethered balloon-borne observations of thermal-infrared irradiance and cooling rate profiles in the Arctic atmospheric boundary layer

Clouds play an important role in controlling the radiative energy budget of the Arctic atmospheric boundary layer. To quantify the impact of clouds on the radiative heating or cooling of the lower atmosphere and of the surface, vertical profile observations of thermal-infrared irradiances were collected using a radiation measurement system carried by a tethered balloon. We present 70 profiles of thermal-infrared radiative quantities measured in summer 2020 during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition and in autumn 2021 and spring 2022 in Ny-Ålesund, Svalbard. Measurements are classified into four groups: cloudless, low-level liquid-bearing cloud, elevated liquid-bearing cloud, and elevated ice cloud. Cloudless cases display an average radiative cooling rate of about —2 K d—1 throughout the atmospheric boundary layer. Instead, low-level liquid-bearing clouds are characterized by a radiative cooling up to —80 K d—1 within a shallow layer at cloud top, while no temperature tendencies are identified underneath the cloud layer. Radiative transfer simulations are performed to quantify the sensitivity of radiative cooling rates to cloud microphysical properties. In particular, cloud top cooling is strongly driven by the liquid water path, especially in optically thin clouds, while for optically thick clouds the cloud droplet number concentration has an increased influence. Additional radiative transfer simulations are used to demonstrate the enhanced radiative importance of the liquid relative to ice clouds. To analyze the temporal evolution of thermal-infrared radiation profiles during the transitions from a cloudy to a cloudless atmosphere, a respective case study is investigated.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Impact of Cloud Longwave Scattering on Radiative Fluxes Associated With the Madden-Julian Oscillation in the Indian Ocean and Maritime Continent

Previous studies suggested that cloud longwave radiation contributes to the development and maintenance of the Madden-Julian Oscillation (MJO) and model-based convection is highly sensitive to the radiation scheme. However, currently used radiation schemes do not take cloud longwave scattering into account, resulting in an overestimation of the outgoing longwave radiation (OLR) and an underestimation of the downward longwave flux at the surface. We use combined active and passive satellite cloud property retrievals to quantify the one-layer cloud OLR and heating rate (HR) biases introduced by neglecting cloud longwave scattering in the Indian Ocean and Maritime Continent in the context of MJO, with a focus on its phases 3, 5, and 6. Here, the results show that the satellite-detected one-layer cloud area consists primarily of ice clouds, particularly during the boreal winter in the 4-year study period. An increased ice cloud area fraction of one-layer cloud groups is present up to 5 days before the onset of MJO events. If longwave scattering is neglected, the composite mean OLR overestimation over the one-layer ice cloud area from 5 days before to 4 days after the MJO passage is approximately 3.5 to 5.0 W m –2 . Neglecting longwave scattering also leads to a HR underestimation at cloud base and an overestimation at cloud top, making the base-to-top heating gradient less sharp at the cloud-resolving scale.

54 ENVIRONMENTAL SCIENCES↗