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NASA NTRS2017

Improving the Plasticity of LIMS Implementation: LIMS Extension through Microsoft Excel

A Laboratory Information Management System (LIMS) is a databasing software with many built-in tools ideal for handling and documenting most laboratory processes in an accurate and consistent manner, making it an indispensable tool for the modern laboratory. However, a lot of LIMS end users will find that in the performance of analyses that have unique considerations such as standard curves, multiple stages incubations, or logical considerations, a base LIMS distribution may not ideally suit their needs. These considerations bring about the need for extension languages, which can extend the functionality of a LIMS. While these languages do provide the implementation team the functionality required to accommodate these special laboratory analyses, they are usually too complex for the end user to modify to compensate for natural changes in laboratory operations. The LIMS utilized by our laboratory offers a unique and easy-to-use choice for an extension language, one that is already heavily relied upon not only in science but also in most academic and business pursuits: Microsoft Excel. The validity of Microsoft Excel as a pseudo programming language and its usability and versatility as a LIMS extension language will be discussed. The NELAC implications and overall drawbacks of this LIMS configuration will also be discussed.

LIMS↗
NASA NTRS2006

On the Quality of the Nimbus 7 LIMS Version 6 Ozone for Studies of the Middle Atmosphere

The Nimbus 7 Limb Infrared Monitor of the Stratosphere (LIMS) radiance profile dataset of 1978/79 was reconditioned and reprocessed to Version 6 (V6) profiles of temperature and species that are improved significantly over those from Version 5 (V5). The LIMS V6 dataset was archived for public use in 2002. Improvements for its ozone include: (1) a more accurate accounting for instrument and spacecraft motion effects in the radiances, (2) the use of better spectroscopic line parameters for its ozone forward model, (3) retrievals of all its scans, (4) more accurate and compatible temperature versus pressure profiles (or T(p)), which are needed for the registration of the ozone radiances and for the removal of temperature effects from them, and (5) a better accounting for interfering species in the lower stratosphere. The retrieved V6 ozone profiles extend from near cloud top altitudes to about 80 km and from 64S to 84N latitude with better sampling along the orbit than for the V5 dataset. Calculated estimates of the single-profile precision and accuracy are provided for the V6 ozone from this study. Precision estimates based on the data themselves are of order 3% or better from 1 to 30 hPa. Estimates of total systematic error for a single profile are hard to generalize because the separate sources of error may not all be of the same sign and they depend somewhat on the atmospheric state. It is estimated that the V6 zonal mean ozone distributions are accurate to within 9% to 7% from 50 hPa to 3 hPa, respectively. Effects of a temperature bias can be significant and may be present at 1 to 2 hPa though. There may be ozone biases of order 10% at those levels due to possible biases of up to +2 K, but there is no indication of a similar problem elsewhere in the stratosphere. Simulation studies show that the LIMS retrievals are also underestimating slightly the small amplitudes of the atmospheric temperature tides, which affect its retrieved day/night ozone differences. There are small biases in the middle to lower stratosphere for the ascending versus descending node LIMS ozone, due principally to not accounting for the asymmetric weighting of its radiances across the tangent layer. The estimates of total accuracy were assessed by comparing the daily zonal mean LIMS ozone distributions against those from the Nimbus 7 SBUV Version 8 (V8) dataset for the same period. Generally, the LIMS V6 ozone agrees well with SBUV, except perhaps in the tropical lower stratosphere where the LIMS ozone is less. Still, the accuracy for LIMS V6 ozone in the lower stratosphere is improved over that found for LIMS V5, as indicated by several LIMS comparisons with ECC ozonesonde profiles. The LIMS V6 ozone is considered especially suitable for detailed studies of large-scale stratospheric processes above the 100-hPa level. Comparison of diurnal, photochemical model calculations with the monthly-averaged, upper stratospheric ozone observed from LIMS V6 indicates only a slight ozone deficit for the model at about 2 hPa. However, that deficit exhibits little to no seasonal variation and is in good agreement with similar model comparisons for a seasonal time series of ozone obtained with ground-based microwave instruments. Because the LIMS V6 ozone in the lower stratosphere has improved accuracy and sampling versus that of V5, it should now be possible to conduct quantitative studies of ozone transport and chemistry for the northern hemisphere, polar stratospheric winter of 1978/79 a time period when the catalytic loss of ozone due to reactive chlorine should not have been a major factor for the Arctic region.

Remsberg, Ellis↗
NASA NTRS2009

On the Quality of the Nimbus 7 LIMS Version 6 Water Vapor Profiles and Distributions

This report describes the quality of the Nimbus 7 Limb Infrared Monitor of the Stratosphere (LIMS) water vapor (H2O) profiles of 1978/79 that were processed with a Version 6 (V6) algorithm and archived in 2002. The V6 profiles incorporate a better knowledge of the instrument attitude for the LIMS measurements along its orbits, leading to improvements for its temperature profiles and for the registration of its water vapor radiances with pressure. As a result, the LIMS V6 zonal-mean distributions of H2O exhibit better hemispheric symmetry than was the case from the original Version 5 (V5) dataset that was archived in 1982. Estimates of the precision and accuracy of the V6 H2O profiles are developed and provided. Individual profiles have a precision of order 5% and an estimated accuracy of about 19% at 3 hPa, 14% at 10 hPa, and 26% at 50 hPa. Profile segments within about 2 km of the tropopause are often affected by emissions from clouds that appear in the finite field-of-view of the detector for the LIMS H2O channel. Zonally-averaged distributions of the LIMS V6 H2O are compared with those from the more recent Microwave Limb Sounder (MLS) satellite experiment for November, February, and May of 2004/2005. The patterns and values of their respective distributions are similar in many respects. Effects of a strengthened Brewer-Dobson circulation are indicated in the MLS distributions of the recent decade versus those of LIMS from 1978/79. A tropical tape recorder signal is present in the 7-month time series of LIMS V6 H2O with lowest values in February 1979, and the estimated, annually-averaged "entry-level" H2O is 3.5 to 3.8 ppmv. It is judged that this historic LIMS water vapor dataset is of good quality for studies of the near global-scale chemistry and transport for pressure levels from 3 hPa to about 70 to 100 hPa.

Remsberg, E. E.↗
NASA NTRS1981

The validation of LIMS ozone profiles using correlative rocket, ECC, and Dobson data sets

The Limb Infrared Monitor of the Stratosphere (LIMS) experiment is a limb scanning infrared sounder designed to measure vertical temperature profiles and the concentrations of key chemical compounds which are important in the stratospheric ozone-nitrogen photochemistry. Preliminary ozone profiles are being intercompared with correlative rocket and balloonsonde ozone data sets as part of the Nimbus 7 LIMS data validation activity. The LIMS ozone retrievals extend from the lower mesosphere to the tropopause (or cloud-top altitudes). In this paper, preliminary statistics of comparisons of ECC (electrochemical concentration cell) ozonesonde and rocket ozone profiles with LIMS ozone profiles are presented. ECC ozonesonde data taken at times of LIMS overpasses are also used to extend the LIMS retrieval down to ground level. Each combined profile is then integrated to obtain total column ozone. These integrated results are compared to Dobson data obtained at approximately the same time and location.

Remsberg, E. E.↗
NASA NTRS1985

LIMS HNO3 data above 5 mbar - Corrections based on simultaneous observations of other species

The Limb Infrared Monitor of the Stratosphere (LIMS) instrument monitored four trace gases (O3, H2O, HNO3, and NO2) and the temperature in the stratosphere and mesosphere. Recently, the seven months LIMS data, including the time from Oct. 25, 1978 to May 29, 1979, have become available to the scientific community. It is pointed out that the measurements are of great use in studying the dynamics and chemistry of the stratosphere. The LIMS HNO3 data appear to show a realistic behavior below 5 mbar, but above 5 mbar, the data appear to be too high. In the present paper, the LIMS HNO3 behavior is discussed, taking into account the reason for the unrealistic appearance of the data. Other LIMS data are used to derive HNO3 above 5 mbar through the intermediate species OH.

Jackman, C. H.↗
NASA NTRS1987

Comparison of Southern Hemisphere radiosonde and LIMS temperatures at 100 mb

Radiosonde (RS)and satellite-derived (Nimbus-7 LIMS) 100-mb temperatures over New Zealand at 12 GMT are compared for the 1978-79 summer. The colocated LIMS temperature information consists of synoptically mapped values (for 12 GMT), as well as the primary nighttime orbital retrievals valid at about 1030 GMT. The RS time series of temperature is dominated by temporal fluctuations associated mainly with the eastward passage of waves which have characteristic periods of 4-5 and 11-12 days and peak-to-peak amplitudes of 10-15 K. The LIMS temperatures and the corresponding temperature time series are also found to exhibit quite close agreement (in terms of temporal phase for the latter) with the RS data. However, the LIMS-mapped temperature fluctuations suffer from a noticeable attenuation in amplitude (approaching 50 percent for higher-frequency fluctuations), which will affect the accuracy of LIMS-derived estimates of dynamical quantities such as wind velocity and relative vorticity in the lower stratosphere.

Miles, T.↗
NASA NTRS1984

A comparison of U.S. and USSR rocketsondes using LIMS satellite temperature sounding as a transfer standard

In connection with the reduction of the number of sounding rockets launched per year, there is a general need to make the most effective use of each sounding. In particular, it is often necessary to combine the results from different types of instruments to obtain a meaningful and complete picture of the atmosphere. For this reason, data from different rockets must be compatible. The present investigation is concerned with the utilization of the temperature soundings of the Limb Infrared Monitor of the Stratosphere (LIMS) as the uniform comparison standard. Gille et al. (1984) have compared the LIMS temperatures to a set of 122 U.S. datasonde rockets. In the current study, a comparison between soundings by rocketborne instruments of the USSR and LIMS is combined with the results of the previous LIMS-U.S. rocketsonde comparison in the same latitude bands to provide an updated estimate of the differences between U.S. and USSR rocketborne temperature measurements.

Gille, J. C.↗
NASA NTRS1986

The accuracy of Nimbus 7 LIMS temperatures in the mesosphere

Zonal-mean temperatures from the Nimbus 7 Limb Infrared Monitor of the Stratosphere (LIMS) experiment are compared with a temperature 'climatology' derived from 4 years of Rayleigh backscatter lidar measurements at 44 N and for the months of March, April, and May, when wave activity and thus atmospheric variability is very weak. The mean difference between the two data sets is less than 3.5 K between 37 and 64 km and is consistent with the theoretical estimates of accuracy reported for the LIMS data. The effects of longitudinal and year-to-year variaiations in this comparison were considered, but they do not change the conclusions significantly. These validation results extend the altitude range of accurate LIMS temperatures in the mesosphere some 10 km higher than previously reported. It also means the LIMS ozone and NO2 retrievals in the lower mesosphere should be free of any major temperature bias error effects.

Remsberg, E. E.↗
NASA NTRS1985

LIMS data - Inferred stratospheric distribution of NOx and HOx trace constituents and the calculated odd nitrogen budget

LIMS, SAMS, SBUV and in-situ data have been used to infer species not measured but which are of photochemical interest, e.g., O(3P), O(1D), NO, N2O5, OH, HO2, ClO and HCl. (LIMS = limb infrared monitor of the stratosphere; SAMS = stratospheric and mesospheric sounder; and SBUV = solar backscattered ultraviolet instrument.) Production and loss of odd nitrogen have been calculated and estimates have been made of the odd nitrogen transport due to adiabatically driven circulation derived from LIMS data. Data used from LIMS include O3, NO2, HNO3, H2O and T. CH4 and N2O were taken from SAMS and the UV solar flux from the SBUV instrument. Species were inferred for periods in October, December, March and May. Results for December are discussed. Results indicate: (1) maximum stratospheric odd nitrogen levels of 25 ppbv; (2) evidence of odd nitrogen transport from the mesosphere appearing at 25 km in the wintertime polar latitudes; (3) the polar night build-up of high levels of N2O5 beginning after the autumnal equinox; and (4) the possibility of large downward fluxes of odd nitrogen into the troposphere during the winter at latitudes poleward of 60 degrees.

Callis, L. B.↗
NASA NTRS2016

Effects of Polar Stratospheric Clouds in the Nimbus 7 LIMS Version 6 Data Set

The historic Limb Infrared Monitor of the Stratosphere (LIMS) measurements of 1978-1979 from the Nimbus 7 satellite were re-processed with Version 6 (V6) algorithms and archived in 2002. The V6 data set employs updated radiance registration methods, improved spectroscopic line parameters, and a common vertical resolution for all retrieved parameters. Retrieved profiles are spaced about every 1.6 of latitude along orbits and include the additional parameter of geopotential height. Profiles of O3 are sensitive to perturbations from emissions of polar stratospheric clouds (PSCs). This work presents results of implementing a first-order screening for effects of PSCs using simple algorithms based on vertical gradients of the O3 mixing ratio. Their occurrences are compared with the co-located, retrieved temperatures and related to the temperature thresholds needed for saturation of H2O and/or HNO3 vapor onto PSC particles. Observed daily locations where the major PSC screening criteria are satisfied are validated against PSCs observed with the Stratospheric Aerosol Monitor (SAM) II experiment also on Nimbus 7. Remnants of emissions from PSCs are characterized for O3 and HNO3 following the screening. PSCs may also impart a warm bias in the co-located LIMS temperatures, but by no more than 1-2K at the altitudes of where effects of PSCs are a maximum in the ozone; thus, no PSC screening was applied to the V6 temperatures. Minimum temperatures vary between 187 and 194K and often occur 1 to 2 km above where PSC effects are first identified in the ozone (most often between about 21 and 28 hPa). Those temperature-pressure values are consistent with conditions for the existence of nitric acid trihydrate (NAT) mixtures and to a lesser extent of super-cooled ternary solution (STS) droplets. A local, temporary uptake of HNO3 vapor of order 1-3 ppbv is indicated during mid-January for the 550K surface. Seven-month time series of the distributions of LIMS O3 and HNO3 are shown based on their gridded Level 3 data following the PSC screening. Zonal coefficients of both species are essentially free of effects from PSCs on the 550K surface, based on their average values along PV contours and in terms of equivalent latitude. Remnants of PSCs are still present in O3 on the 450K surface during mid- January. It is judged that the LIMS Level 3 data are of good quality for analyzing the larger-scale, stratospheric chemistry and transport processes during the Arctic winter of 1978- 1979.

Remsberg, Ellis↗
NASA NTRS1984

The validation of Nimbus 7 LIMS measurements of ozone

Approximately seven and one half months of stratospheric ozone profiles have been processed from the LIMS (Limb Infrared Monitor of the Stratosphere) experiment on the Nimbus 7 satellite. Data profiles cover the stratosphere and mesosphere from 100 to 0.1 mbar and from 84 degrees N to 64 degrees S latitude. Topics covered include the ozone channel characteristics, precision, systematic uncertainties, and comparisons with data from balloon and rocket underflights, Umkehr soundings, and Dobson measurements. Comparisons with Dobson total ozone are made by integrating combined LIMS plus balloon profiles. The estimated on-orbit precision is 0.02-0.16 ppmv. Simulations of the experiment indicate potential systematic uncertainties ranging from 15 percent in the 1-mbar region to an upper limit of 40 percent at 100 mbar and 0.1 mbar. Results are well within the uncertainties for the correlative sensors themselves. LIMS detects significant vertical structure in the ozone profile even below the ozone mixing ratio peak. Several other comparisons showing good agreement are noted.

Remsberg, E. E.↗
NASA NTRS1983

An intercomparison of ozone profile measurements from LIMS, SAGE, and SBUV

Ozone profile measurements by the Limb IR Monitor of Stratosphere (LIMS) and the Solar Backscatter UV (SBUV) aboard the Nimbus satellite, and the Stratospheric Aerosol and Gas Experiment (SAGE) aboard the AEM-2 satellite are intercompared in an effort to assess the quality of satellite ozone retrieval techniques. Good correlation between LIMS and SBUV observations is noted in the ozone layer bounded by pressures of 31.2-15.6 mb; absolute differences are generally less than 10 percent, with similar zonal variations. Above 35 km SAGE values are systematically larger than SBUV or LIMS. The differences generally increase with height and are largest in the tropics. Finally, excellent agreement is noted to exist among the three data sets between 10 and 35 km of altitude with respect to the latitude dependence of the ozone profiles.

Fleig, A. J.↗
NASA NTRS1987

An intercomparison of nitrogen-containing species in Nimbus 7 LIMS and SAMS data

Odd-nitrogen chemistry and transport are analyzed using a two-dimensional model and Nimbus 7 data. The Nimbus 7 data include: measurements of O3, NO2, HNO3, H2O, and temperature by the LIMS instrument; N2O, CH4, and temperature measurements by the SAMS instrument; and O3 data from the SBUV instrument. The characteristics of the two-dimensional model used in the study, a modified Guthrie et al. (1984) model, are described. NO2 and HNO3 are calculated using the two-dimensional model, and the computed data are compared with the LIMS NO2 and HNO3 measurements. The model uncertainties are computed based on the photochemical equilibrium assumption, and the role of stratospheric dynamics in determining NO2 and HNO3 is discussed. It is observed that there is good correlation between the LIMS and model data in the upper stratosphere; however, the data do not correspond in the lower stratosphere. The effect of nitrogen sources, such as lightning, on the stratospheric odd nitrogen distribution is examined.

Jackman, Charles H.↗
NASA NTRS1987

Laboratory Information Management System (LIMS): A case study

In the late 70's, a refurbishment of the analytical laboratories serving the Materials Division at NASA Lewis Research Center was undertaken. As part of the modernization efforts, a Laboratory Information Management System (LIMS) was to be included. Preliminary studies indicated a custom-designed system as the best choice in order to satisfy all of the requirements. A scaled down version of the original design has been in operation since 1984. The LIMS, a combination of computer hardware, provides the chemical characterization laboratory with an information data base, a report generator, a user interface, and networking capabilities. This paper is an account of the processes involved in designing and implementing that LIMS.

Crandall, Karen S.↗
NASA NTRS1988

Comparison of LIMS temperatures and geostrophic winds with Berlin radiosonde temperature and wind measurements

The temperature and the derived winds obtained from the LIMS Map Archival Tape data for the period of October 25, 1978, to May 28, 1979, were compared with corresponding data from the Berin (Tempelhof) radiosonde station at several representative levels in the stratosphere, to assess the quality of the LIMS satellite data for use in dynamics and transport studies. It was found, on the basis of this single-station time series comparison, that the synoptically mapped LIMS temperature and wind analyses are of a sufficiently high quality for investigating large-scale dynamics in the stratosphere in conjunction with high-resolution radiosonde measurements.

Grose, W. L.↗
NASA NTRS1988

The Nimbus 7 LIMS (Limb Infrared Monitor of the Stratosphere) water vapor measurements

Earth orbital instruments, designed to measure the vertical and spatial distribution of atmospheric water vapor is discussed. Specifically, the operation of the Limb Infrared Monitor of the Stratosphere (LIMS) experiment is examined. The LIMS is a six channel limb scanning radiometer that was launched aboard Nimbus 7 in 1978. Profiles of stratospheric and mesospheric temperature, water vapor, and various other constituents were obtained by inverting the LIMS radiance measurements. This same technique was used in 1981 to analyze the data returned from another limb scanning radiometer aboard the Solar Mesosphere Explorer.

Remsberg, Ellis E.↗
NASA NTRS2010

LIMS Version 6 Level 3 Dataset

This report describes the Limb Infrared Monitor of the Stratosphere (LIMS) Version 6 (V6) Level 3 data products and the assumptions used for their generation. A sequential estimation algorithm was used to obtain daily, zonal Fourier coefficients of the several parameters of the LIMS dataset for 216 days of 1978-79. The coefficients are available at up to 28 pressure levels and at every two degrees of latitude from 64 S to 84 N and at the synoptic time of 12 UT. Example plots were prepared and archived from the data at 10 hPa of January 1, 1979, to illustrate the overall coherence of the features obtained with the LIMS-retrieved parameters.

Remsberg, Ellis E.↗
NASA NTRS2021

Residual Temperature Bias Effects in Stratospheric Species Distributions from LIMS

The Nimbus 7 Limb Infrared Monitor of theStratosphere (LIMS) instrument operated from 25 Octo-ber 1978 through 28 May 1979. Its version 6 (V6) profileswere processed and archived in 2002. We present severaldiagnostic examples of the quality of the V6 stratospheric species distributions based on their level 3 zonal Fourier co-efficient products. In particular, we show that there are smalldifferences in the ascending (A) minus descending (D) or-bital temperature–pressure orT(p) profiles (theirA−Dval-ues) that affect (A−D) species values. SystematicA−Dbi-ases inT(p) can arise from small radiance biases and/or fromviewing anomalies along orbits. There can also be (A−D)differences inT(p) due to not resolving and correcting forall of the atmospheric temperature gradient along LIMS tan-gent view-paths. An error inT(p) affects species retrievalsthrough (1) the Planck blackbody function in forward calcu-lations of limb radiance that are part of the iterative retrievalalgorithm of LIMS, and (2) the registration of the measuredLIMS species radiance profiles in pressure altitude, mainlyfor the lower stratosphere. There are clearA−Ddifferencesfor ozone, H2O, and HNO3but not for NO2. Percentage differences are larger in the lower stratosphere for ozone andH2O because those species are optically thick. We evaluateV6 ozone profile biases in the upper stratosphere with the aid of comparisons against a monthly climatology of UV–ozone soundings from rocketsondes. We also provide resultsof time series analyses of V6 ozone, H2O, and potential vor-ticity for the middle stratosphere to show that their average(A+D) V6 level 3 products provide a clear picture of the evolution of those tracers during Northern Hemisphere win-ter. We recommend that researchers use the average V6 level3 product for their science studies of stratospheric ozone andH2O, while keeping in mind that there are uncorrected non-local thermodynamic equilibrium effects in daytime ozone inthe lower mesosphere and in daytime H2O in the uppermoststratosphere. We also point out that the present-day Soundingof the Atmosphere using Broadband Emission Radiometry(SABER) experiment provides measurements and retrievalsof temperature and ozone that are nearly free of anomalousdiurnal variations and of effects from gradients at low and middle latitudes.

Ellis Remsberg↗