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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS2020

Lower-Stratospheric Tracer Trends and Variability from Reanalyses

Previous studies have robustly identified a decrease since 1998 in lower stratospheric ozone in the Northern Hemisphere (NH). While this ozone decrease is qualitatively explained as resulting from changes in the large-scale circulation, there is not yet a quantitative mechanistic explanation of these changes. Here we explore the drivers of recent ozone changes using two different configurations of the Goddard Earth Observing System (GEOS) general circulation model. The first configuration of GEOS includes a full chemistry module and is constrained with meteorological fields from the MERRA-2 reanalysis. This configuration (M2GMI) is used to analyze an idealized tracer that covaries closely with ozone on interannual and decadal timescales, revealing that recent ozone decreases in the NH subtropics are associated with a poleward expansion of upwelling in the NH LS, with reduced (enhanced) downwelling over northern subtropics (midlatitudes). The second configuration of GEOS is a free-running version of the GEOS Chemistry-Climate Model (CCM) that is used to perform a ten-member ensemble of free-running simulations. Comparisons of the two configurations reveal that, while the free-running model can produce negative ozone changes in the NH LS, the magnitude of these changes is significantly weaker, relative to both M2GMI and MERRA-2; moreover, these weaker ozone decreases are consistent with weaker simulated changes in the residual circulation. Finally, we examine the GEOS model results in the broader context of the hindcast simulations performed as part of Phase 1 of the Chemistry Climate Modeling Initiative. We show that the majority of the free-running simulations considered here also exhibit weaker long-term residual circulation changes, compared to reanalyses.

Wargan, Kris↗
NASA NTRS2020

Mechanisms Linked to Recent Ozone Decreases in the Northern Hemisphere Lower Stratosphere

Previous studies have robustly identified a decrease since 1998 in lower stratospheric (LS) ozone in the Northern Hemisphere (NH). While this ozone decrease is qualitatively explained as resulting from changes in the large‐scale circulation, there is not yet a quantitative mechanistic explanation of these changes. Here we explore the drivers of recent ozone changes using two different configurations of the Goddard Earth Observing System (GEOS) general circulation model. The first configuration of GEOS includes a full chemistry module and is constrained with meteorological fields from the Modern‐Era Retrospective analysis for Research and Applications, Version 2 (MERRA‐2). This configuration (M2GMI) is used to analyze an idealized tracer that covaries closely with ozone on interannual and decadal timescales, revealing that recent ozone decreases in the NH subtropics are associated with a poleward expansion of upwelling in the NH LS, with reduced (enhanced) downwelling over northern subtropics (midlatitudes). The second configuration of GEOS is a free‐running version of the GEOS Chemistry‐Climate Model (CCM) that is used to perform a ten‐member ensemble of free‐running simulations. Comparisons of the two configurations reveal that, while the free‐running model can produce negative ozone changes in the NH LS, the magnitude of these changes is significantly weaker, relative to both M2GMI and MERRA‐2; moreover, these weaker ozone decreases are consistent with weaker simulated changes in the residual circulation. Finally, we examine the GEOS model results in the broader context of the hindcast simulations performed as part of Phase 1 of the Chemistry Climate Modeling Initiative. We show that the majority of the free‐running simulations considered here also exhibit weaker long‐term residual circulation changes, compared to reanalyses.

Ozone↗
NASA NTRS2022

Optimized Umkehr Profile Algorithm for Ozone Trend Analyses

The long-term record of Umkehr measurements from four NOAA Dobson spectrophotometers was reprocessed after updates to the instrument calibration procedures. In addition, a new data quality-control tool was developed for the Dobson automation software (WinDobson). This paper presents a comparison of Dobson Umkehr ozone profiles from NOAA ozone network stations (Boulder, OHP, MLO, Lauder) against several satellite records, including Aura Microwave Limb Sounder (MLS; ver. 4.2), and combined SBUV and OMPS records (NASA AGG and NOAA COH). A subset of satellite data is selected to match Dobson Umkehr observations at each station spatially (distance less than 200 km) and temporally (within 24 hours). Umkehr Averaging Kernels (AKs) are applied to vertically smooth all overpass satellite profiles prior to comparisons. The station Umkehr record consists of several instrumental records, which have different optical characterizations, and thus instrument-specific stray light contributes to the data processing errors and creates step changes in the record. This work evaluates the overall quality of Umkehr long-term measurements at NOAA ground-based stations and assesses the impact of the instrumental changes on the stability of the Umkehr ozone profile record. This paper describes a method designed to correct biases and discontinuities in the retrieved Umkehr profile that originate from the Dobson calibration process, repair, or optical realignment of the instrument. The M2GMI and GMI CTM ozone profile model output matched to station location and date of observation is used to evaluate instrumental step changes in the Umkehr record. Homogenization of the Umkehr record and discussion of the apparent stray light error in retrieved ozone profiles are the focus of this paper. Homogenization of ground-based records is of great importance for studies of long-term ozone trends and climate change.

Umkehr↗
NASA NTRS2019

Optimizing Umkehr Ozone Profile Retrievals

NOAA Dobson Umkehr ozone profile records have been collected since the 1970s. Umkehr ozone profiles are used to monitor stratospheric ozone recovery predicted to occur by the 2050s. Current operational Dobson Umkehr profile algorithms produce data that have uncertainty on the order of ~ 5 % in the stratosphere. However, when large volcanic eruptions inject aerosols into the stratosphere, the errors can be as large as 70 %. In order to evaluate Umkehr records for aerosol-related and instrumental artifacts, we compare observations with a Hindcast simulation of the NASA Merra-2 Global Modeling Initiative (GMI) Replay (M2GMI, Orbe et al, 2017; Wargan et al, 2018) and Chemistry Transport Model (GMI CTM, Strahan et al, 2013, Strahan et al, 2016). The biases found between the models and observations are summarized for each Dobson calibration and volcanic eruption period, thus providing a reference tool for homogenization of the Umkehr time series and removal of volcanic aerosol errors.

Petropavlovskikh, I.↗