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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records

Valley Hall Effect and Magnetic Moment in Magnetized Silicene

We investigate the physical properties of silicene with both staggered sublattice potential and magnetization by using Kubo formalism, the latter arises from the magnetic proximity effect by depositing Fe atoms to silicene or depositing silicene on an appropriate ferromagnetic insulator. Based on the low-energy continuum model of the system where inversion symmetry is broken, we show that the system exhibits spin half metal state when staggered sublattice potential is in the same magnitude with mean and staggered magnetization. Besides, Hall conductivity and magnetic moment are all valley dependent, so we investigate the valley Hall effect of the system further by considering magnetization exclusively. This means carriers in different valleys turning into opposite directions transverse to an in-plane electric field. At last, we prove these results by investigating Berry curvature that characterizing Hall transport, which is also valley dependent. These effects can be used to generate valley-polarized currents solely by magnetization, forming the basis for the valley-based electronics applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Induced versus intrinsic magnetic moments in ultrafast magnetization dynamics

Ferromagnetic metal alloys are today commonly used in spintronic and magnetic data storage devices. These multicompound structures consist of several magnetic sublattices exhibiting both intrinsic and induced magnetic moments. Here, we study the response of the element-specific magnetization dynamics for thin film systems based on purely intrinsic (CoFeB) and partially induced (FePt) magnetic moments using extreme ultraviolet pulses from high-harmonic generation (HHG) as an element-sensitive probe. In FePt, on the one hand, we observe an identical normalized transient magnetization for Fe and Pt throughout both the ultrafast demagnetization and the subsequent remagnetization. On the other hand, Co and Fe show a clear difference in the asymptotic limit of the remagnetization process in CoFeB, which is supported by calculations for the temperature-dependent behavior of the equilibrium magnetization using a dynamic spin model. Furthermore, in this work, we provide a vital step toward a comprehensive understanding of ultrafast light-induced magnetization dynamics in ferromagnetic alloys with sublattices of intrinsic and induced magnetic moments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic moment distribution of magnetic cataclysmic variables

A simulation study is made of the relative numbers of the AM Herculis binaries and the intermediate polars as a function of the orbital period using random variables subject to suitable constraints to describe the various parameters. It is shown that the observations can be matched by a single distribution in the magnetic moment equals 0.7 +/- 0.3. For such an ensemble, the intermediate polars are distributed in the log(Porb) - log(Ps) diagram about the critical disk line but with a larger scatter than observed.

Wu, Kinwah↗

Phonon Magnetic Moment from Electronic Topological Magnetization

The traditional theory of magnetic moments for chiral phonons is based on the picture of the circular motion of the Born effective charge, typically yielding a small fractional value of the nuclear magneton. Here we investigate the adiabatic evolution of electronic states induced by the lattice vibration of a chiral phonon and obtain an electronic orbital magnetization in the form of a topological second Chern form. We find that the traditional theory needs to be refined by introducing a k resolved Born effective charge, and identify another contribution from the phonon-modified electronic energy together with the momentum-space Berry curvature. The second Chern form can diverge when there is a Yang’s monopole near the parameter space of interest as illustrated by considering a phonon at the Brillouin zone corner in a gapped graphene model. We also find large magnetic moments for the optical phonon in bulk topological materials where nontopological contribution is also important. Our results agree with recent observations in experiments.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Canting of the Magnetic Moments on the Octahedral Site of an Iron Oxide Garnet in Response to Diamagnetic Cation Substitution

Using neutron powder diffraction and magnetic susceptibility measurements, we report on the preparation and characterization of the temperature- and field-dependent properties of CaY2ZrFe4O12, a composition closely related to the high-temperature ferrimagnet Y3Fe5O12. By diluting the concentration of paramagnetic ions on the octahedral sublattice of the garnet structure, we find temperature-dependent canting of the magnetic moments. This reflects the importance of the octahedral sublattice in mediating the magnetic interactions between the tetrahedral sites and offers insight into a large number of competing magnetic interactions in the garnet structure.

Milam-Guerrero, JoAnna↗

Neutron star kick velocity induced by neutrino chirality flip and a lower bound for the neutrino magnetic moment

We study the neutrino chirality flip during the birth of a neutron star, produced in a core made of strange quark matter. This mechanism is applied to the neutron star kick velocity problem and we show that it is efficient when the neutrino magnetic moment is not smaller than 4.7 × 10 −15 μ B , where μ B is the Bohr magneton. When this lower bound is combined with the most stringent upper bound, our results set a range for the neutrino magnetic moment given by 4.7 × 10 −15 ≤ μ ν / μ B ≤ (0.1 − 0.4) × 10 −11 . The obtained kick velocities for natal conditions are consistent with the observed ones and span the correct range of radii for typical magnetic field intensities.

Ayala, Alejandro↗

Circumventing data imbalance in magnetic ground state data for magnetic moment predictions

Abstract Magnetic materials play a crucial role in the transition to more sustainable forms of energy and electric vehicles. There is an anticipated shortage in magnetic materials in the future, and as a result there is an urgent need to discover and design new magnetic materials. Computational magnetic material design using density functional theory is daunting because of the challenge in identifying magnetic ground states from a combinatorially large set of possibilities. Machine learning offers a path forward by enabling efficient surrogate models that can more readily enumerate these states, but there is a dearth of training data available, and what is available tends to be imbalanced with too much non-magnetic data. In this work we show that the discrete and previously tackled data imbalance that exists at the level of the magnetic ordering leads to an imbalanced continuous distribution with many zeros when the data is unraveled at the atomic magnetic moment level, which subsequently leads to models with low accuracy for magnetic properties. We mitigate this by using a two-part model framework. Our scheme is able to classify atoms into magnetic and non-magnetic with an F1 score and Matthew’s correlation coefficient (MCC) of ~91% and then to provide an implicit embedding representation that maps directly onto the magnitude of the magnetic moment with a mean absolute error of 0.1 μ B . Beyond screening for new magnetic materials, we demonstrate an additional practical use case of our scheme: the provision of good initial guesses for magnetic moments in first-principles electronic relaxations. Such initialization is shown to lead to faster convergence to configurations that lie closer to the ground state.

Computer Science↗

Spin-Selective Oxygen Evolution Reaction in Chiral Iron Oxide Nanoparticles: Synergistic Impact of Inherent Magnetic Moment and Chirality

Electron spin polarization is identified as a promising avenue for enhancing the oxygen evolution reaction (OER), which is the bottleneck that limits the energy efficiency of water-splitting. Here, in this work, we report that both ferrimagnetic (f-Fe 3 O 4 ) and superparamagnetic iron oxide (s-Fe 3 O 4 ) catalysts can exhibit external magnetic field (Hext)-induced OER enhancement, and the activity is proportional to their intrinsic magnetic moment. Additionally, the chirality-induced spin selectivity (CISS) effect was utilized in synergy with Hext to get a maximum enhancement of up to 89% improvement in current density (at 1.8 V vs RHE) with a low onset potential of 270 mV in s-Fe 3 O 4 catalysts. Spin polarization and the resultant spin selectivity suppress the production of H 2 O 2 and promote the formation of ground state triplet O 2 during the OER. Furthermore, the design of chiral s-Fe 3 O 4 with synergistic spin potential effect demonstrates a high spin polarization of ∼42%, as measured using conductive atomic force microscopy (c-AFM).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Influence of the Magnetic Moment of the Probe of a Magnetic Resonance Force Microscope on the Spin-Wave Resonance Spectra

Abstract—The ferromagnetic resonance in an array of permalloy microstrips 3000 × 500 × 30 nm{sup 3} in size, which are ordered on a rectangular 3.5 × 6 μm{sup 2} lattice, is studied using magnetic resonance force microscopy with strong probe–sample interaction. This interaction induces intricate modifications of the observed spectra, which are manifested both in line splitting and in changes in shape. The dependences of the observed spectra on the sample–probe distance and the orientation of the magnetic moment of the probe are analyzed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The Neutrino Magnetic Moment Portal

We discuss neutrino magnetic moments as a way of constraining physics beyond the Standard Model. In fact, new physics at the TeV scale can easily generate observable neutrino magnetic moments, and there exists a multitude of ways of probing them. We highlight in particular direct dark matter detection experiments (which are sensitive to neutrino magnetic moments because of the predicted modifications to the solar neutrino scattering rate), stellar cooling, and cosmological constraints.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Magnetic moments of charmed baryons. I, II

The magnetic moments of all charmed baryons belonging to the totally symmetric 20 (underlined) representation, the mixed symmetry 20 prime (underlined) and the totally antisymmetric 4 (underlined) representation have been compared under U(4) symmetry, assuming that the magnetic-moment operator is proportional to the charge operator. The magnetic moments of all charmed particles have been expressed in terms of the moments of proton, neutron and delta particles in the case of U(4) symmetry. Then assuming that the magnetic moment operator is a tensor transforming as the (15,3) members of a 63 (underlined) representation of U(8) or SU(8), the magnetic moments of all the baryons belonging to the 120 (underlined) representation are compared.

Choudhury, A. L.↗

Nonadiabatic behavior of the magnetic moment of a charged particle in a dipole magnetic field

This paper investigates the dynamic behavior of the magnetic moment of a particle confined in a magnetic dipole field in the presence of a low-frequency electrostatic wave. It is shown that there exist two kinds of resonances (the bounce-E x B drift resonance and the wave-drift resonance) by which the adiabaticity of the magnetic moment is broken. The unstable conditions obtained by theoretical considerations showed good agreement with the numerical results.

Murakami, Sadayoshi↗