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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Characterization of a silicon photo-multiplier array with summing board as a photo-multiplier tube replacement in organic scintillator assemblies

In this work, we report on the energy, timing, and pulse-shape discrimination performance of cylindrical 5.08 cm diameter x 5.08 cm thick and 7.62 cm diameter x 7.62 cm thick trans-stilbene crystals read out with the passively summed output of three different commercial silicon photo-multiplier arrays. Our results indicate that using the summed output of an 8 x 8 array of SiPMs provides performance competitive with photo-multiplier tubes for many neutron imaging and correlated particle measurements. For a 5.08 cm diameter x 5.08 cm thick crystal read out with SensL’s ArrayJ-60035_64P-PCB, which had the best overall properties, we measure the energy resolution as 17.8 ± 0.8% at 341 keVee (σ/E), the timing resolution in the 180–400 keVee range as 236 ± 61 ps (σ), and the pulse-shape discrimination figure-of-merit as 2.21 ± 0.03 in the 230–260 keVee energy range. For a 7.62 cm diameter x 7.62 cm thick crystal read out with SensL’s ArrayJ-60035_64P-PCB, we measure the energy resolution as 21.9 ± 2.3% at 341 keVee, the timing resolution in the 180–400 keVee range as 518 ± 42 ps, and the pulse-shape discrimination figure-of-merit as 1.49 ± 0.01 in the 230–260 keVee energy range. Our findings enable many scintillator-based instruments to enjoy the size, robustness, and power benefits of silicon photo-multiplier arrays as replacement for the photo-multiplier tubes that are predominantly used today.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Core–shell PdPb@Pd aerogels with multiply-twinned intermetallic nanostructures: facile synthesis with accelerated gelation kinetics and their enhanced electrocatalytic properties

Delicately engineering well-defined noble metal aerogels with favorable structural and compositional features is of vital importance for wide applications. Here, we reported a one-pot and facile method for synthesizing core–shell PdPb@Pd hydrogels/aerogels with multiply-twinned grains and an ordered intermetallic phase using sodium hypophosphite as a multifunctional reducing agent. Due to the accelerated gelation kinetics induced by increased reaction temperature and the specific function of sodium hypophosphite, the formation of hydrogels can be completed within 4 h. As a result, owing to their unique porous structure and favorable geometric and electronic effects, the optimized PdPb@Pd aerogels exhibit enhanced electrochemical performance towards ethylene glycol oxidation with a mass activity of 5.8 times higher than Pd black.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Perspective: Electrospray photoelectron spectroscopy: From multiply-charged anions to ultracold anions

Electrospray ionization (ESI) has become an essential tool in chemical physics and physical chemistry for the production of novel molecular ions from solution samples for a variety of spectroscopic experiments. ESI was used to produce free multiply-charged anions (MCAs) for photoelectron spectroscopy (PES) in the late 1990 s, allowing many interesting properties of this class of exotic species to be investigated. Free MCAs are characterized by strong intramolecular Coulomb repulsions, which create a repulsive Coulomb barrier (RCB) for electron emission. The RCB endows many fascinating properties to MCAs, giving rise to meta-stable anions with negative electron binding energies. Recent development in the PES of MCAs includes photoelectron imaging to examine the influence of the RCB on the electron emission dynamics, pump-probe experiments to examine electron tunneling through the RCB, and isomer-specific experiments by coupling PES with ion mobility for biological MCAs. The development of a cryogenically cooled Paul trap has led to much better resolved PE spectra for MCAs by creating vibrationally cold anions from the room temperature ESI source. Recent advances in coupling the cryogenic Paul trap with PE imaging have allowed high-resolution PE spectra to be obtained for singly charged anions produced by ESI. In particular, the observation of dipole-bound excited states has made it possible to conduct vibrational autodetachment spectroscopy and resonant PES, which yield much richer vibrational spectroscopic information for dipolar free radicals than traditional PES.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2017

The Tynode: A new vacuum electron multiplier

By placing, in vacuum, a stack of transmission dynodes (tynodes) on top of a CMOS pixel chip, a single free electron detector could be made with outstanding performance in terms of spatial and time resolution. The essential object is the tynode: an ultra thin membrane, which emits, at the impact of an energetic electron on one side, a multiple of electrons at the other side. The electron yields of tynodes have been calculated by means of GEANT-4 Monte Carlo simulations, applying special low-energy extensions. The results are in line with another simulation based on a continuous charge-diffusion model. By means of Micro Electro Mechanical System (MEMS) technology, tynodes and test samples have been realized. The secondary electron yield of several samples has been measured in three different setups. Finally, several possibilities to improve the yield are presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2019

Properties of perhalogenated {closo-B10} and {closo-B11} multiply charged anions and a critical comparison with {closo-B12} in the gas and the condensed phase

Anionic closo-borate anions [closo-BnXn]2- are part of the most famous textbook examples of polyhedral compounds. Substantial differences in their reactivity and interactions with other compounds depending on the substituent X and clustersize n have been recognized, which favors specific closo-borates for different applications in cancer treatment, chemical synthesis, and materials science. Surprisingly, a fundamental understanding of the molecular properties underlying these differences is lacking. Here, we report our study of electronic structure and reactivity of closo-borate anions [closo-BnXn]2- (X = Cl, Br, I, n = 10, 11, 12 in all combinations). We investigated the free dianions and the ion pairs [nBu4N]+[closo-BnXn]2- by gas phase anion photoelectron spectroscopy accompanied by theoretical investigations. Strong similarities in electronic structure for n = 10 and 11 were observed, while n = 12 clusters are different. A systematic picture of the development in electronic stability along the dimension X is derived. Collision induced dissociation shows that fragmentation of the free dianions is mainly dependent on the substituent X and gives access to a large variety of boron-rich molecular ions. Fragmentation of the ion pair depends strongly on n. The results reflect the high chemical stability of cluster with n = 10 and 12, while those with n = 11 are much easier prone to dissociation. We bridge our study to the condensed phase by performing comparative electrochemistry and reactivity studies on closo-borates in solution. The trends found at the molecular level are also reflected in the condensed-phase properties. We discuss how the gas phase values allow to evaluate the influence of the condensed phase on the electronic stability of closo-borates. A novel synthetic method via an oxidation/chlorination reaction yielding [closo-B10Cl10]2– from highly chlorinated {closo-B11} clusters is introduced, which underlines the intrinsically high reactivity of the {closo-B11} cage.

Warneke, Jonas↗
DOE OSTI2018

Characterization of a Silicon photo-multiplier summing breakout board for photo-multiplier tube replacement

We present the relative timing and pulse-shape discrimination performance of a H1949-50 photomultiplier tube to SensL ArrayX-B0B6_64S coupled to a SensL ArrayC-60035-64P- PCB Silicon Photomultiplier array. The goal of this work is to enable the replacement of photomultiplier readout of scintillators with Silicon Photomultiplier devices, which are more robust and have higher particle detection efficiency. The report quantifies the degradation of these performance parameters using commercial off the shelf summing circuits, and motivates the development of an improved summing circuit: the pulse-shape descrimination figure-of-merit drops from 1.7 at 500 keVee to 1.4, and the timing resolution (σ) is 288 ps for the photomultiplier readout and approximately 1 ns for the Silicon Photomultiplier readout. A degradation of this size will have a large negative impact on any device that relies on timing coincidence or pulse-shape discrimination to detect neutron interactions, such as neutron kinematic imaging or multiplicity measurements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1992

Frequency multipliers for millimeter and submillimeter wavelengths

All-solid-state local oscillators in the terahertz frequency range are especially needed for space-borne radio astronomy and remote sensing of the atmosphere. Because solid-state oscillators cannot yet produce the necessary local oscillator power at submillimeter wavelengths, frequency multipliers are needed. So far, submillimeter-wave frequency multipliers are mainly based on a whisker-contacted Schottky diode as the nonlinear element. This paper discusses the multiplier theory and tools for analysis and design of millimeter- and submillimeter-wave multipliers. Experimental work is reviewed. The Schottky diode model at submillimeter frequencies, use of Schottky multiplier chains versus direct higher-order multipliers, and the effect of cooling on Schottky diode multipliers are discussed. Alternative diodes such as the high electron mobility varactor, the barrier-intrinsic n(+) diode, the barrier-n-n(+) diode, the quantum well diode, and the single barrier varactor are discussed, with attention also given to their potential as submillimeter frequency multipliers.

Raisanen, Antti V.↗
DOE OSTI2019

Low energy consumption mantissa multiplication for floating point multiply-add operations

A floating point multiply-add unit having inputs coupled to receive a floating point multiplier data element, a floating point multiplicand data element, and a floating point addend data element. The multiply-add unit including a mantissa multiplier to multiply a mantissa of the multiplier data element and a mantissa of the multiplicand data element to calculate a mantissa product. The mantissa multiplier including a most significant bit portion to calculate most significant bits of the mantissa product, and a least significant bit portion to calculate least significant bits of the mantissa product. The mantissa multiplier has a plurality of different possible sizes of the least significant bit portion. Energy consumption reduction logic to selectively reduce energy consumption of the least significant bit portion, but not the most significant bit portion, to cause the least significant bit portion to not calculate the least significant bits of the mantissa product.

Hasenplaugh, William C.↗
NASA NTRS1984

Systolic multipliers for finite fields GF(2 exp m)

Two systolic architectures are developed for performing the product-sum computation AB + C in the finite field GF(2 exp m) of 2 exp m elements, where A, B, and C are arbitrary elements of GF(2 exp m). The first multiplier is a serial-in, serial-out one-dimensional systolic array, while the second multiplier is a parallel-in, parallel-out two-dimensional systolic array. The first multiplier requires a smaller number of basic cells than the second multiplier. The second multiplier needs less average time per computation than the first multiplier, if a number of computations are performed consecutively. To perform single computations both multipliers require the same computational time. In both cases the architectures are simple and regular and possess the properties of concurrency and modularity. As a consequence, they are well suited for use in VLSI systems.

Yeh, C.-S.↗
NASA NTRS1987

Pipeline active filter utilizing a booth type multiplier

Multiplier units of the modified Booth decoder and carry-save adder/full adder combination are used to implement a pipeline active filter wherein pixel data is processed sequentially, and each pixel need only be accessed once and multiplied by a predetermined number of weights simultaneously, one multiplier unit for each weight. Each multiplier unit uses only one row of carry-save adders, and the results are shifted to less significant multiplier positions and one row of full adders to add the carry to the sum in order to provide the correct binary number for the product Wp. The full adder is also used to add this product Wp to the sum of products .SIGMA.Wp from preceding multiply units. If m.times.m multiplier units are pipelined, the system would be capable of processing a kernel array of m.times.m weighting factors.

Nathan, Robert↗
DOE OSTI2018

Prompt fission neutron anisotropy in low-multiplying subcritical plutonium metal assemblies

Fission neutron anisotropy, due to the kinematics of the fission process, has been studied for non-multiplying sources and highly multiplying subcritical plutonium metal assemblies (i.e. relatively long fission chains). The studies on highly multiplying assemblies show that the observed neutron-neutron angular distribution appear isotropic, while the studies on non-multiplying sources show that the neutron-neutron angular distribution appear anisotropic. No measured data exists, however, that investigates the dependence of neutron anisotropy on multiplication for low-multiplying assemblies. We have experimentally characterized the dependence of fission neutron anisotropy on multiplication for low-multiplying plutonium metal assemblies. Here, an array of 16 organic scintillators was used to measure plutonium metal assemblies (95% 239 Pu, by mass) exhibiting a leakage multiplication of 1.0722(3) to 1.6006(4). Full neutron-neutron angular distributions were measured, and the fission neutron anisotropy was quantified with the ratio of neutron-neutron coincidences observed at 180° and 90°. The results show that the neutron-neutron angular distribution becomes more isotropic as the multiplication increases. Additionally, energy-angle correlations were also characterized showing that the angular distributions are more anisotropic when observing neutrons of higher energy.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1993

Synthesis algorithm of VLSI multipliers for ASIC

Multipliers are critical sub-blocks in ASIC design, especially for digital signal processing and communications applications. A flexible multiplier synthesis tool is developed which is capable of generating multiplier blocks for word size in the range of 4 to 256 bits. A comparison of existing multiplier algorithms is made in terms of speed, silicon area, and suitability for automated synthesis and verification of its VLSI implementation. The algorithm divides the range of supported word sizes into sub-ranges and provides each sub-range with a specific multiplier architecture for optimal speed and area. The algorithm of the synthesis tool and the multiplier architectures are presented. Circuit implementation and the automated synthesis methodology are discussed.

Chua, O. H.↗
NASA NTRS1987

A comparison of VLSI architecture of finite field multipliers using dual, normal or standard basis

Three different finite field multipliers are presented: (1) a dual basis multiplier due to Berlekamp; (2) a Massy-Omura normal basis multiplier; and (3) the Scott-Tavares-Peppard standard basis multiplier. These algorithms are chosen because each has its own distinct features which apply most suitably in different areas. Finally, they are implemented on silicon chips with nitride metal oxide semiconductor technology so that the multiplier most desirable for very large scale integration implementations can readily be ascertained.

Hsu, I. S.↗
NASA NTRS1988

A comparison of VLSI architecture of finite field multipliers using dual, normal, or standard bases

Three different finite-field multipliers are presented: (1) a dual-basis multiplier due to Berlekamp; the Massey-Omura normal basis multiplier; and (3) the Scott-Tavares-Peppard standard basis multiplier. These algorithms are chosen because each has its own distinct features that apply most suitably in different areas. Finally, they are implemented on silicon chips with nitride metal oxide semiconductor technology so that the multiplier most desirable for VLSI implementation can readily be ascertained.

Hsu, I. S.↗
NASA NTRS1997

Monte Carlo Simulation of THz Multipliers

Schottky Barrier diode frequency multipliers are critical components in submillimeter and Thz space based earth observation systems. As the operating frequency of these multipliers has increased, the agreement between design predictions and experimental results has become poorer. The multiplier design is usually based on a nonlinear model using a form of harmonic balance and a model for the Schottky barrier diode. Conventional voltage dependent lumped element models do a poor job of predicting THz frequency performance. This paper will describe a large signal Monte Carlo simulation of Schottky barrier multipliers. The simulation is a time dependent particle field Monte Carlo simulation with ohmic and Schottky barrier boundary conditions included that has been combined with a fixed point solution for the nonlinear circuit interaction. The results in the paper will point out some important time constants in varactor operation and will describe the effects of current saturation and nonlinear resistances on multiplier operation.

East, J.↗
NASA NTRS2010

Diamond Heat-Spreader for Submillimeter-Wave Frequency Multipliers

The planar GaAs Shottky diode frequency multiplier is a critical technology for the local oscillator (LO) for submillimeter- wave heterodyne receivers due to low mass, tenability, long lifetime, and room-temperature operation. The use of a W-band (75-100 GHz) power amplifier followed by a frequency multiplier is the most common for submillimeter-wave sources. Its greatest challenge is to provide enough input power to the LO for instruments onboard future planetary missions. Recently, JPL produced 800 mW at 92.5 GHz by combining four MMICs in parallel in a balanced configuration. As more power at W-band is available to the multipliers, their power-handling capability be comes more important. High operating temperatures can lead to degradation of conversion efficiency or catastrophic failure. The goal of this innovation is to reduce the thermal resistance by attaching diamond film as a heat-spreader on the backside of multipliers to improve their power-handling capability. Polycrystalline diamond is deposited by hot-filament chemical vapor deposition (CVD). This diamond film acts as a heat-spreader to both the existing 250- and 300-GHz triplers, and has a high thermal conductivity (1,000-1,200 W/mK). It is approximately 2.5 times greater than copper (401 W/mK) and 20 times greater than GaAs (46 W/mK). It is an electrical insulator (resistivity approx. equals 10(exp 15) Ohms-cm), and has a low relative dielectric constant of 5.7. Diamond heat-spreaders reduce by at least 200 C at 250 mW of input power, compared to the tripler without diamond, according to thermal simulation. This superior thermal management provides a 100-percent increase in power-handling capability. For example, with this innovation, 40-mW output power has been achieved from a 250-GHz tripler at 350-mW input power, while the previous triplers, without diamond, suffered catastrophic failures. This breakthrough provides a stepping-stone for frequency multipliers-based LO up to 3 THz. The future work for this design is to apply the high output power from both the 250 and 300 GHz to multiple chains in order to generate milliwatts at 2.3 THz. Using the first generation of results for this innovation, 40 mW of output power were produced from a 240-GHz tripler at 350-mW input power, and 27- mW output power was produced from a 300-GHz tripler at 408-mW input power. This is two times higher than the current state-of-the-art output power capability. A finite-element thermal simulation also shows that 30-microns thick diamond dropped the temperature of the anodes by at least 200 C.

Lin, Robert H.↗