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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
NASA NTRS2006

Assessment of MODIS-Derived Visible and Near-IR Aerosol Optical Properties and their Spatial Variability in the Presence of Mineral Dust

Mineral dust aerosol is among the most difficult aerosol species to measure quantitatively from space. In this paper, we evaluate MODIS retrievals of spectral aerosol optical depth (AOD) from the visible to the near-IR off the US West Coast using measurements taken by the NASA Ames Airborne Tracking Sunphotometer, AATS-14, during the EVE (Extended-MODIS-lambda Validation Experiment, 2004) campaign in April of 2004. In EVE, a total of 35 and 49 coincident over-ocean suborbital measurements at the nominal level-2 retrieval scale of 10 km x 10 km were collected for Terra and Aqua, respectively. For MODIS-Terra about 80% of the AOD retrievals are within the estimated uncertainty, DELTA tau = plus or minus 0.03 plus or minus 0.05 tau; this is true for both the visible (here defined to include 466-855 nm) and near-IR (here defined to include 1243-2119 nm) retrievals. For MODIS-Aqua about 45% of the AOD retrievals are within DELTA tau = plus or minus 0.03 plus or minus 0.05 tau; the fraction of near-IR retrievals that fall within this uncertainty range is about 27%. We found an rms difference of 0.71 between the sunphotometer snd MODIS-Aqua estimates of the visible (553-855 nm) Angstrom exponent, while the MODIS-Terra visible Angstrom exponents show an rms difference of only 0.29 when compared to AATS. The cause of the differences in performance between MODIS-Terra and MODIS-Aqua could be instrument calibration and needs to be explored further. The spatial variability of AOD between retrieval boxes as derived by MODIS is generally larger than that indicated by the sunphotometer data.

Redemann, J.↗
NASA NTRS2020

Optical Design of the Earth Surface Mineral Dust Source Investigation (EMIT) Imaging Spectrometer

The Earth Surface Mineral Dust Source Investigation (EMIT) instrument is a high fidelity imaging spectrometer developed to characterize surface mineralogy of the Earth’s dust source regions over the spectral range of 380- 2500 nm and spectral sampling of 7.4 nm. EMIT will close the current knowledge gap in dust source mineral composition by collecting over 1 billion high signal-to-noise ratio spectra in this region of our planet. These new measurements will be used in conjunction with state-of-the-art Earth System Models to understand and reduce the uncertainty in the radiative forcing effect of mineral dust aerosols. EMIT will be deployed on the International Space Station that has an orbit that is well suited for measuring the arid land regions of the Earth. The optical design utilizes a Dyson spectrometer to reduce volume and mass for a fast (F/1.8) and wide swath (1240 samples) optical system. An overview of the EMIT optical design, development, and current status are discussed.

Green, Robert O.↗
NASA NTRS2020

The Earth Surface Mineral Dust Source Investigation: An Earth Science Imaging Spectroscopy Mission

The Earth Surface Mineral Dust Source Investigation, EMIT, is planned to operate from the International Space Station starting no earlier than the fall of 2021. EMIT will use visible to short wavelength infrared imaging spectroscopy to determine the mineral composition of the arid land dust source regions of the Earth to advance our knowledge of the radiative forcing effect of these aerosols. Mineral dust emitted into the atmosphere under high wind conditions is an element of the Earth system with many impacts to the Earth’s energy balance, atmosphere, surface, and oceans. The Earth’s mineral dust cycle with source, transport, and deposition phases are studied with advanced Earth System Models. Because the chemical composition, optical and surface properties of soil particles vary strongly with the mineral composition of the source, these models require knowledge of surface soil mineral dust source composition knowledge to accurately understand dust impacts on the Earth system now and in the future. At present, compositional knowledge of the Earth’s mineral dust source regions from existing data sets is uncertain as a result of limited measurements. EMIT will use spectroscopically derived surface mineral composition to update the prescribe boundary conditions for state-of-the-art Earth System Models. The EMIT-initialized models will be used to investigate the impact of direct radiative forcing in the Earth system that depends strongly on the composition of the mineral dust aerosols emitted into the atmosphere. These new measurements and related products will be used to address the EMIT science objectives and made available to the science community for additional investigations. An overview of the EMIT science, development, and mission is presented in this paper.

Green, Robert O.↗
NASA NTRS1996

Laboratory Measurements of Mineral Dust Scatterring Phase Function and Linear Polarization

With the goal of improving our understanding of how small mineral dust particles scatter light at visible and near-infrared wafelengths we measured the scattering phase function and linear polarization of small mineral dust particles over the scattering angle range 15 to 170 at three wavelengths (0.47, 0.652,and 0.937 m).

minerals dust dust particles SEM scanning electron↗
NASA NTRS2000

What we Hope to Learn about Global Mineral Dust Aerosols from EOS Multi-Angle Imaging SpectroRadiometer (MISR)

On global scales, just a few broad atmospheric aerosol compositional groups are commonly observed. Of these, "mineral dust" is the only group which both contains non-spherical particles, and typically has size distributions with enough large particles for particle shape to affect its visible-light-scattering properties. The MISR instrument is scheduled for launch into a 10:30 AM sun-synchronous, polar orbit aboard the EOS Terra satellite in 1999. MISR will measure the upwelling visible radiance from Earth in 4 spectral bands centered at 446, 558, 672, and 866 nm, at each of 9 emission angles spread out in the forward and aft directions along the flight path at +/-70.5 deg, +/-60.0 deg, +/-45.6 deg, +/-26.1deg, and nadir. Over a period of 7 minutes, as the spacecraft flies along, a 360 km wide swath of Earth will successively be viewed by each of the cameras, allowing MISR to sample a very large range of scattering angles; in mid latitudes, the instrument will observe scattering angles between about 60 deg and 160 deg. Global coverage will be acquired about once in 9 days at the equator; the nominal mission lifetime is 6 years. The distinction in single scattering phase function between natural distributions of spherical and randomly oriented, non-spherical particles, with a broad range of aspect ratios, shows up strongly for scattering angles ranging from about 90 deg to near 180 deg. For non-spherical particle distributions, single scattering phase functions tend to be much flatter in this region than for spherical particles. Since MISR samples the relevant range of scattering angles very well, we expect to be able to make critical distinctions between natural distributions of spherical and randomly oriented, non-spherical particles with MISR data. We anticipate that the new multiangle, multispectral data from MISR will also contain other information about particle properties, a major step beyond current spacecraft remote sensing retrievals, which obtain aerosol optical depth based on entirely assumed particle microphysical properties. According to simulations over cloud-free, calm ocean, for pure particles with natural ranges of optical depth, particle size, and indices of refraction, MISR should retrieve column optical depth for all but the darkest particles, to an uncertainty of at most 0.05 or 20%, whichever is larger, even if the particle properties are poorly known. For one common particle type, soot, constraints on the optical depth over dark ocean are very poor. The simulated measurements also should allow us to separate two to four compositional groups based on indices of refraction, and to identify three to four distinct size groups between 0.1 and 2.0 microns characteristic radius at most latitudes. The technique is most sensitive to particle microphysical properties in the "accumulation mode" sizes. where particle scattering undergoes the transition from Rayleigh to large-particle regimes for the MISR wavelengths. Based on these results, we expect to distinguish air masses containing different aerosol types, routinely and globally, with multiangle remote sensing data. Such data complements in situ and field data, which can provide details about aerosol size and composition locally that are needed to assess the radiative effects of aerosols quantitatively. Both field data and correlations in space and time with likely source and sink regions will also be helpful in developing a global picture of mineral dust aerosol budgets. Further work on the expected sensitivity of MISR to natural mixtures of pure particles, including climatologically likely mineral dust components, is currently underway.

Kahn, Ralph↗
NASA NTRS2008

Evidence of Mineral Dust Altering Cloud Microphysics and Precipitation

Multi-platform and multi-sensor observations are employed to investigate the impact of mineral dust on cloud microphysical and precipitation processes in mesoscale convective systems. It is clearly evident that for a given convection strength,small hydrometeors were more prevalent in the stratiform rain regions with dust than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust sector, particularly at altitudes where heterogeneous nucleation process of mineral dust prevails, further supports the observed changes of precipitation. The consequences of the microphysical effects of the dust aerosols were to shift the precipitation size spectrum from heavy precipitation to light precipitation and ultimately suppressing precipitation.

Min, Qilong↗
NASA NTRS2011

Global Distributions of Mineral Dust Properties from SeaWiFS and MODIS: From Sources to Sinks

The impact of natural and anthropogenic sources of mineral dust has gained increasing attention from scientific communities in recent years. Indeed, these airborne dust particles, once lifted over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across the oceans resulting in important biogeochemical impacts on the ecosystem. Due to the relatively short lifetime (a few hours to about a week), the distributions of these mineral dust particles vary extensively in both space and time. Consequently, satellite observations are needed over both source and sink regions for continuous temporal and spatial sampling of aerosol properties. With the launch of SeaWiFS in 1997, Terra/MODIS in 1999, and Aqua/MODIS in 2002, high quality comprehensive aerosol climatology is becoming feasible for the first time. As a result of these unprecedented satellite data records, studies of the radiative and biogeochemical effects due to dust aerosols are now possible. In this study, we will show the comparisons of satellite retrieved aerosol optical thickness using Deep Blue algorithm with data from AERONET sunphotometers over desert and semi-desert regions as well as vegetated areas. Our results indicate reasonable agreements between these two. These new satellite products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from Sea WiFS and MODIS-like instruments. The multiyear satellite measurements since 1997 from Sea WiFS will be compared with those retrieved from MODIS and MISR, and will be utilized to investigate the interannual variability of source, pathway, and dust loading associated with the dust outbreaks over the entire globe. Finally, the trends observed over the last decade based upon the SeaWiFS time series in the amounts of tropospheric aerosols due to natural and anthropogenic sources (such as changes in the frequency of dust storms) will be discussed.

Hsu, N. Christina↗
NASA NTRS2022

Dominant role of mineral dust in cirrus cloud formation revealed by global-scale measurements

Airborne mineral dust particles can act as natural seeds for cirrus clouds in the upper troposphere. However, the atmospheric abundance of dust is unconstrained in cirrus-forming regions, hampering our ability to predict these radiatively important clouds. Here we present global-scale measurements of dust aerosol abundance in the upper troposphere and incorporate these into a detailed cirrus-formation model. We show that dust aerosol initiates cirrus clouds throughout the extra-tropics in all seasons and dominates cirrus formation in the Northern Hemisphere (75–93% of clouds seasonally). Using a global transport model with improved dust treatment, we also explore which of Earth’s deserts are the largest contributors of dust aerosol to cirrus-forming regions. We find that the meteorological environment downstream of each emission region modulates dust atmospheric lifetime and transport efficiency to the upper troposphere so that source contributions are disproportionate to emissions. Our findings establish the critical role of dust in Earth’s climate system through the formation of cirrus clouds.

Airborne mineral dust particles↗
NASA NTRS2021

Mineral Dust Cycle in the Multiscale Online Nonhydrostatic AtmospheRe CHemistry Model (Monarch) Version 2.0

We present the dust module in the Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) version 2.0, a chemical weather prediction system that can be used for regional and global modeling at a range of resolutions. The representations of dust processes in MONARCH were upgraded with a focus on dust emission (emission parameterizations, entrainment thresholds, considerations of soil moisture and surface cover), lower boundary conditions (roughness, potential dust sources), and dust–radiation interactions. MONARCH now allows modeling of global and regional mineral dust cycles using fundamentally different paradigms, ranging from strongly simplified to physics-based parameterizations. We present a detailed description of these updates along with four global benchmark simulations, which use conceptually different dust emission parameterizations, and we evaluate the simulations against observations of dust optical depth. We determine key dust parameters, such as global annual emission/deposition flux, dust loading, dust optical depth, mass-extinction efficiency, single-scattering albedo, and direct radiative effects. For dust-particle diameters up to 20 µm, the total annual dust emission and deposition fluxes obtained with our four experiments range between about 3500 and 6000 Tg, which largely depend upon differences in the emitted size distribution. Considering ellipsoidal particle shapes and dust refractive indices that account for size-resolved mineralogy, we estimate the global total (longwave and shortwave) dust direct radiative effect (DRE) at the surface to range between about −0.90 and −0.63 W m−2 and at the top of the atmosphere between −0.20 and −0.28 W m−2. Our evaluation demonstrates that MONARCH is able to reproduce key features of the spatiotemporal variability of the global dust cycle with important and insightful differences between the different configurations.

Dust cycle↗
NASA NTRS2003

Effects of Non-Sphericity on Mineral Dust Modeling

The dependency of non-sphericity on gravitational settling of mineral dust particles is parameterized for prolate ellipsoids and Reynolds number lower than 2. The settling speed is numerically solved from the momentum equation as a function of particle diameter and aspect ratio. The reduction of settling speed due to non-sphericity is included in the GO-CART model to simulate dust size distribution for April 2001. Two numerical schemes for solving sedimentation are compared. For particles of diameter greater than 5 micron the simulated size distribution is sensitive to the numerical sedimentation scheme. Changing the particle shape from spherical to non-spherical with lambda=2, makes little difference to the simulated surface concentration and size distribution except at the periphery of the dust sources. However, when very elongated particles (lambda=5) are simulated the differences between non-spherical and spherical particles are significant. With limited in-situ measurements reporting most frequent lambda around 1.5, the overall effects on global modeling is rather negligible and the essential benefit is to relax the CFL condition of Eulerian settling schemes.

Ginoux, Paul↗
NASA NTRS2013

Impact of Surface Roughness and Soil Texture on Mineral Dust Emission Fluxes Modeling

Dust production models (DPM) used to estimate vertical fluxes of mineral dust aerosols over arid regions need accurate data on soil and surface properties. The Laboratoire Inter-Universitaire des Systemes Atmospheriques (LISA) data set was developed for Northern Africa, the Middle East, and East Asia. This regional data set was built through dedicated field campaigns and include, among others, the aerodynamic roughness length, the smooth roughness length of the erodible fraction of the surface, and the dry (undisturbed) soil size distribution. Recently, satellite-derived roughness length and high-resolution soil texture data sets at the global scale have emerged and provide the opportunity for the use of advanced schemes in global models. This paper analyzes the behavior of the ERS satellite-derived global roughness length and the State Soil Geographic data base-Food and Agriculture Organization of the United Nations (STATSGO-FAO) soil texture data set (based on wet techniques) using an advanced DPM in comparison to the LISA data set over Northern Africa and the Middle East. We explore the sensitivity of the drag partition scheme (a critical component of the DPM) and of the dust vertical fluxes (intensity and spatial patterns) to the roughness length and soil texture data sets. We also compare the use of the drag partition scheme to a widely used preferential source approach in global models. Idealized experiments with prescribed wind speeds show that the ERS and STATSGO-FAO data sets provide realistic spatial patterns of dust emission and friction velocity thresholds in the region. Finally, we evaluate a dust transport model for the period of March to July 2011 with observed aerosol optical depths from Aerosol Robotic Network sites. Results show that ERS and STATSGO-FAO provide realistic simulations in the region.

textures↗
NASA NTRS2021

The Thermal Infrared Optical Depth of Mineral Dust Retrieved from Integrated CALIOP and IIR Observations

Recent studies reveal that a higher fraction of coarse mineral dust particles than that estimated by climate model simulations has been observed in the atmosphere, leading to a more significant positive (i.e., warming) longwave (LW) thermal infrared (TIR) direct radiative effect (DRE). However, the magnitude of this DRE remains highly uncertain because our understanding of the radiative properties, quantitatively represented by the optical depth of dust, especially information on the TIR, remains limited. This study presents a simple approach to retrieve the thermal infrared dust aerosol optical depth (DAODTIR) over oceans during nighttime using the observations from the Infrared Imaging Radiometer (IIR) and the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard CALIPSO. For each cloud-free dust-laden profile identified by the IIR-CALIOP observation, a Lookup-Table (LUT) of the 10.6 μm IIR band brightness temperatures difference (dBT) under different DAODTIR with respect to their dust-free BTs is constructed based on the CALIOP retrieved dust vertical profile and pre-assumed dust scattering properties using a fast radiative transfer model. Then the DAODTIR is retrieved by projecting the IIR-observed dBT on the LUT. Sensitivity studies show that the DAODTIR retrieval at 10.6 μm is more susceptible to the dust particle size distribution (PSD) assumption than dust refractive indices. To estimate the uncertainty caused by PSD assumption, two DAODTIR retrieval products, one based on the dust PSD from the AERONET at Cape Verde and the other on an in situ measured PSD from the recent Fennec campaign, are provided. The retrieval uncertainty is mainly contributed by the BT difference between the observation and simulation using auxiliary atmospheric data. The climatology of the retrieval from 2013 to 2019 shows confident spatiotemporal variations of DAODTIR with the global-averaged value of 0.006 and 0.008 based on different pre-assumed dust PSDs. Climatological results agree reasonably well with two independent DAODTIR retrieval products based on the Infrared Atmospheric Sounding Interferometer (IASI) over the active dust transport regions, such as North and Tropical Atlantic (r = 0.904 and 0.819) and Indian Ocean (r = 0.832). The seasonal and interannual variation is also well-compared (r = 0.758) with AERONET coarse-mode AOD at 97 selected sites. The synergic CALIOP observation allows the retrieved DAODTIR to directly compare with the extrapolated DAODTIR from DAOD in visible (i.e., 532 nm), which helps evaluate the observational constraints on DAODTIR. This study offers a unique prospect of collocating active lidar and passive IR observations for retrieving dust DAODTIR.

aerosol↗
NASA NTRS1994

Modeling of mineral dust in the atmosphere: Sources, transport, and optical thickness

A global three-dimensional model of the atmospheric mineral dust cycle is developed for the study of its impact on the radiative balance of the atmosphere. The model includes four size classes of minearl dust, whose source distributions are based on the distributions of vegetation, soil texture and soil moisture. Uplift and deposition are parameterized using analyzed winds and rainfall statistics that resolve high-frequency events. Dust transport in the atmosphere is simulated with the tracer transport model of the Goddard Institute for Space Studies. The simulated seasonal variations of dust concentrations show general reasonable agreement with the observed distributions, as do the size distributions at several observing sites. The discrepancies between the simulated and the observed dust concentrations point to regions of significant land surface modification. Monthly distribution of aerosol optical depths are calculated from the distribution of dust particle sizes. The maximum optical depth due to dust is 0.4-0.5 in the seasonal mean. The main uncertainties, about a factor of 3-5, in calculating optical thicknesses arise from the crude resolution of soil particle sizes, from insufficient constraint by the total dust loading in the atmosphere, and from our ignorance about adhesion, agglomeration, uplift, and size distributions of fine dust particles (less than 1 micrometer).

Tegen, Ina↗
NASA NTRS2022

Inferring iron-oxide species content in atmospheric mineral dust from DSCOVR EPIC observations

The iron-oxide content of dust in the atmosphere and most notably its apportionment between hematite (α-Fe2O3) and goethite (α-FeOOH) are key determinants in quantifying dust’s light absorption, its top of atmosphere UV radiances used for dust monitoring, and ultimately shortwave dust direct radiative effects (DRE). Hematite and goethite column mass concentrations and iron-oxide mass fractions of total dust mass concentration were retrieved from the DeepSpace Climate Observatory (DSCOVR) Earth Polychromatic Imaging Camera (EPIC) measurements in the ultraviolet–visible (UV–Vis) channels. The retrievals were performed for dust-identified aerosol plumes over land using aerosol optical depth (AOD) and spectral imaginary refractive index provided by the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm over six continental regions (North America, North Africa, West Asia, Central Asia, EastAsia, and Australia). The dust particles are represented as an internal mixture of non-absorbing host and absorbing hematite and goethite. We use the Maxwell–Garnett effective medium approximation with carefully selected complex refractive indices of hematite and goethite that produce mass fractions of iron oxides species consistent with in situ values found in the literature to derive the hematite and goethite volumetric/mass concentrations from MAIAC EPIC products. We compared the retrieved hematite and goethite concentrations with in situ dust aerosol mineralogical content measurements, as well as with published data. Our data display variations within the published range of hematite, goethite, and iron-oxide mass fractions for pure mineral dust cases. A specific analysis is presented for 15 sites over the main dust source regions. Sites in the central Sahara, Sahel, and Middle East exhibit a greater temporal variability of iron oxides relative to other sites. Niger site(13.52°N, 2.63°E) is dominated by goethite over Harmattan season with median of ~2 weight percentage (wt.%) of iron-oxide. Saudi Arabia site (27.49°N, 41.98°E) over Middle East also exhibited surge of goethite content with the beginning of Shamal season. The Sahel dust is richer in iron-oxide than Saharan and northern China dust except in Summer. The Bodélé Depression area shows a distinctively lower iron-oxide concentration (~1 wt.%) throughout the year. Finally, we show that EPIC data allow to constrain the hematite refractive index. Specifically, we select 5 out of 13 different number of hematite refractive indices widely variable in published laboratory studies by constraining the iron-oxide mass ratio to the known measured values. Provided climatology of hematite and goethite mass fractions across main dust regions of the Earth will be useful for dust shortwave DRE studies and climate modeling.

Sujung Go↗
NASA NTRS2015

How the Assumed Size Distribution of Dust Minerals Affects the Predicted Ice Forming Nuclei

The formation of ice in clouds depends on the availability of ice forming nuclei (IFN). Dust aerosol particles are considered the most important source of IFN at a global scale. Recent laboratory studies have demonstrated that the mineral feldspar provides the most efficient dust IFN for immersion freezing and together with kaolinite for deposition ice nucleation, and that the phyllosilicates illite and montmorillonite (a member of the smectite group) are of secondary importance.A few studies have applied global models that simulate mineral specific dust to predict the number and geographical distribution of IFN. These studies have been based on the simple assumption that the mineral composition of soil as provided in data sets from the literature translates directly into the mineral composition of the dust aerosols. However, these tables are based on measurements of wet-sieved soil where dust aggregates are destroyed to a large degree. In consequence, the size distribution of dust is shifted to smaller sizes, and phyllosilicates like illite, kaolinite, and smectite are only found in the size range 2 m. In contrast, in measurements of the mineral composition of dust aerosols, the largest mass fraction of these phyllosilicates is found in the size range 2 m as part of dust aggregates. Conversely, the mass fraction of feldspar is smaller in this size range, varying with the geographical location. This may have a significant effect on the predicted IFN number and its geographical distribution.An improved mineral specific dust aerosol module has been recently implemented in the NASA GISS Earth System ModelE2. The dust module takes into consideration the disaggregated state of wet-sieved soil, on which the tables of soil mineral fractions are based. To simulate the atmospheric cycle of the minerals, the mass size distribution of each mineral in aggregates that are emitted from undispersed parent soil is reconstructed. In the current study, we test the null-hypothesis that simulating the presence of a large mass fraction of phyllosilicates in dust aerosols in the size range 2 m, in comparison to a simple model assumption where this is neglected, does not yield a significant effect on the magnitude and geographical distribution of the predicted IFN number. Results from sensitivity experiments are presented as well.

Dust↗