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Nuclear Data Sheets for A=136☆

Spectroscopic data for all nuclei with mass number A=136 have been evaluated and the corresponding level schemes from radioactive decay and reaction studies are presented. No excited states are known in {sup 136}In, {sup 136}Eu, or {sup 136}Gd and {sup 136}Tb remains unidentified. Discrepancies between experiments on isomeric decays in {sup 136}Sb and {sup 136}La suggest the need for futher experimental investigation. The decay of {sup 136}Eu has only been observed in a mixed source. The energy of the 17.5 s isomer in {sup 136}Cs was determined since the last evaluation, however, the branching ratio remains unknown. This work supersedes the earlier full evaluation of A=136 by A.A. Sonzogni (2002So05), and benefited tremendously from all previous evaluations of A=136.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Miniature motorized inspection tool for DOE Hanford site tank bottoms - 15700

Recently, small amounts of waste have been found in the annulus of tank AY-102, prompting the need for developing inspection tools that can identify the cause and location of the leak. Three separate access paths can be used to obtain information regarding the tank bottom condition. The inspection may be conducted via: 1) Refractory air slots through the annulus; 2) 4'' annulus air supply pipe to central air slots; 3) 6'' leak detection pit drain from the central sump. There are various environmental and physical constraints which the tool will have to adhere to. In order for the tool to be successful, it must be capable of the following: Travel through small cooling channels with dimensions as small as 1.5'' x 1.5''; Provide live video feedback; Produce enough torque to overcome the tether drag force; Inverted travel to avoid obstacles such as tank corrosion; Navigate up to 38 feet to the tank center, while maneuvering through four 90 deg. turns. A model of the inspection tool has been designed, assembled and reported. Areas of potential performance improvement were observed; these areas are the basis of the following design, as seen above. The changes include: The addition of an additional 4 wheels; Body modification to house the camera; A loft on the bottom from the tools edge to the magnets lowest edge; Shaving the hubs of the current wheels; Control method changed to a joystick. The tank configuration through which the tool will have to maneuver are the following: 72 outer ring slots (1.5'' x 1.5'' x 17'); 36 ring slots (2'' x 1.5'' x 12'); 18 inner slots (3'' x 1.5'' x 7'). The components used for this design iteration are not radiation hardened nor are they designed to withstand elevated temperatures. However, this prototype has been constructed with the final goal of being radiation hardened and able to withstand elevated temperatures in mind. The components that make up this design iteration are the following: Arduino Uno board with ATMega328 micro-controller; Joystick shield kit for the Arduino Uno; Eggsnow USB Borescope Endoscope 5.5 mm inspection camera; 136:1 Sub-micro Plastic Planetary Gearmotor; 14 x 4.5 mm wheels; 3D-printed body; 3D-printed free rolling shafts; Neodymium magnet - 1 h x 3/8 h x 1/16 h; 4.53 lb pull force. In the time to come, there are a few goals that are to be completed. The first group of tasks is associated with the testing and recording of data of the current prototype. This data will be analyzed and appropriate action will be taken based on the results of the testing. The testing will include simulating the challenges that the tool will face in the AY-102 tank. Working with the Hanford DOE site, a bag of Kaolin 2200 will be acquired to be used for the test bed to simulate tank conditions. Further modification will then be made to enable the tool to be able to maneuver through a 90 deg. turn. Completion of this task will be a major milestone, as this tool will be readily usable in the other tanks containing HLW; as other tanks will be easier to maneuver through.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Barium and neodymium isotopic anomalies in the Allende meteorite

The discovery of Ba and Nd isotopic anomalies in two inclusions from the Allende meteorite is reported. The inclusions are Ca-Al-rich objects typical of the type considered as high-temperature condensation products in the solar nebula and contain distinctive Mg and O isotopic anomalies of the FUN (mass Fractionation, Unknown Nuclear processes) type. Mass-spectrometry results are discussed which show that inclusion C1 has anomalies in Ba at masses 134 and 136, while inclusion EK1-4-1 exhibits large marked negative anomalies at 130, 132, 134, and 136, as well as a positive anomaly at 137. It is also found that inclusion EK1-4-1 shows marked negative anomalies in Nd at masses 142, 146, 148, and 150, in addition to a positive anomaly at 145. These isotopic shifts are attributed to addition of r-process nuclei rather than mass fractionation. It is suggested that an onion-shell supernova explosion followed by injection into the solar nebula is the most likely generic model that may explain the observations.

Mcculloch, M. T.↗

Magnetic Transition and Magnetocaloric Effect of Gd{sub 1−x}Nd{sub x}Mn{sub 2}Ge{sub 2} (x = 0.3 and 0.4) Compounds

Gd{sub 1−x}Nd{sub x}Mn{sub 2}Ge{sub 2} compounds with x = 0.3 and 0.4 were prepared by arc melting and crystallized in the ThCr{sub 2}Si{sub 2}-type structure with the space group I4/mmm based on X-ray powder diffraction (XRD) results. Magnetic transition and magnetocaloric effect (MCE) of the Gd{sub 1−x}Nd{sub x}Mn{sub 2}Ge{sub 2} compounds were investigated by magnetic measurements on a physical property measurement system (PPMS). Gd{sub 0.7}Nd{sub 0.3}Mn{sub 2}Ge{sub 2} compound exhibits complicated magnetic transitions at around 63 K (T{sub comp}), 86 K (T{sub 1}), 136 K (T{sub C}), 260 K (T{sub N}{sup inter}), and 347 K (T{sub C}{sup inter}), respectively, while Gd{sub 0.6}Nd{sub 0.4}Mn{sub 2}Ge{sub 2} compound shows a spin re-orientation transition at about 52 K. Combined with isothermal magnetization curves and the Maxwell relation, the maximum magnetic entropy changes of Gd{sub 0.7}Nd{sub 0.3}Mn{sub 2}Ge{sub 2} and Gd{sub 0.6}Nd{sub 0.4}Mn{sub 2}Ge{sub 2} were calculated to be 4.31 and 5.15 J kg{sup − 1} K{sup − 1} under the applied magnetic field changing from 0 to 5 T, respectively.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The Study of (n, 2n) Reaction Cross Sections for Ce and Nd Isotopes up to 20 MeV

Neutron cross section calculations for {sup 136}Ce(n, 2n){sup 135}Ce, {sup 138}Ce(n, 2n){sup 137}Ce, {sup 140}Ce(n, 2n){sup 139}Ce, {sup 142}Ce(n, 2n){sup 141}Ce, {sup 142}Nd(n, 2n){sup 141}Nd, {sup 144}Nd(n, 2n){sup 143}Nd, {sup 146}Nd(n, 2n){sup 145}Nd, {sup 148}Nd(n, 2n){sup 147}Nd, and {sup 150}Nd(n, 2n){sup 149}Nd were done in the incident energy range from 10 to 20 MeV. The calculations were performed using three codes TALYS-1.6 for two-component Exciton model, EMPIRE-3.2 Malta for Exciton model, and ALICE/ASH for the Geometry-Dependent Hybrid (GDH) model. The results of model calculations were compared with the available experimental data and also with the evaluated data in the TENDL-2015 (based on the modified TALYS code), ENDF/B-VII.1 libraries. The calculated cross section data were compared with the available experimental data obtained from EXFOR and also compared with semiempirical formulas around 14–15 MeV. The results of model calculation were found to be in good agreement with the experimental data given in literature and semiempirical data around 14–15MeV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗