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At least 19 records

Modeling and Design of Micro Flux Monitors for Neutron Fluence Measurements

Measuring neutron flux is critical to understanding the characteristics of nuclear reactors and can provide information on the energy spectrum, total neutron fluence, and operational history of a facility. Such measurements are typically performed by irradiating high-purity materials in an operating reactor for a known length of time. By measuring and identifying activation products in the irradiated materials and referencing the energy-dependent cross section of each isotope, the neutron energy spectrum and total fluence can be determined. Historical techniques use a variety of small, individually pressed foils or wires for dosimeter devices, which can result in excessively high levels of radioactivity and complications in handling after irradiation. The present work describes a new neutron dosimetry concept, named the micro flux monitor, that uses semiconductor device fabrication processes to deposit thin films of flux monitoring materials in precise geometries onto a SiC wafer. This approach allows multiple dosimetry materials to be located on a single device, simplifying irradiation and subsequent analysis. The geometry, and therefore mass, of each material can be custom-tailored for a specific application—considering the expected neutron flux, duration of irradiation, and device retrieval time of a facility. Additionally, hundreds of identical dosimetry monitors can be produced simultaneously, reducing fabrication costs. Finally, the extremely thin metal dimensions of these devices could improve the fidelity of neutron fluence measurements by reducing neutron self-shielding and gamma self-attenuation effects.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Measured Thermal and Fast Neutrons Fluence Rates for ATF-1 Holders During ATR Cycle 166B

This report contains the thermal (2200 m/s) and fast (E>lMeV) neutron fluence rate data for the ATF-1 holders located in core for ATR Cycle 166B which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains measurements of the fluence rates corresponding to the particular elevations relative to the 80-ft. core elevation. The data in this report consist of (1) a table of the ATR power history and distribution, (2) a hard copy listing of all thermal and fast neutron fluence rates, and (3) plots of both the thermal and fast neutron fluence rates. All "BR" holder monitor wires for this cycle are 56.375 inches long. This length allows measurements from 31.17 inches above core midplane to 19.81 inches below core midplane. The distance from the end of the wires to the first count position was 4.25 inches for all wires counted from this cycle. The monitors were located in an outward small I-holes,1-22 and 1-23. Thermal neutron fluence was determined based on the activation of the CoAl wires and resonance corrections determined in the irradiation of Cycle 152A when the RML measured cadmium-covered as well as bare neutron monitors in the Southwest, Southeast, and H positions at the Center lobe to determine the division in neutron energy between epithermal and thermal neutrons. For more information please refer to letter “Radiation Measurements Laboratory measurements of in core ATR physics testing during cycle 152A. The measured values documented in RML procedure, “ACMM-3600, Flux Monitoring,” will be used indefinitely until further measurements supersede the current values. Fast neutron fluence was determined using the activation of nickel wires. Typically, a fission spectrum averaged cross section (E>1 MeV) is used as determined in detailed measurements described in “ATR Neutron Spectral Characterization,” which gives an effective cross section of 97 mb for the small I-holes. However, those measurements were performed with unfueled experiments. The fast fluence values reported here use a perturbed 114 mb effective>1 MeV spectrum averaged cross section for the small I-holes based on MCNP simulations for a previous fueled experiment in the1-24 position. Refer to “LWR- ATR Irradiation Measured Thermal and Fast Neutron Fluence Rates ATR CYCLE 133A 04/19/04 thru 05/17/04” for more information.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Measured Thermal And Fast Neutron Fluence Rates ATR Cycle 169A

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 169A which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains fluence rate values corresponding to the particular elevations (relative to the 80-ft. core elevation) where the measurements were taken. The data in this report consists of ( 1) a table of the ATR power history and distribution, (2) a hard copy listing of all thermal and fast neutron fluence rates, (3) plots of both the thermal and fast neutron fluence rates, and (4) an optical record (compact disk) containing a listing of the thermal and the fast neutron fluence rates, their assigned elevations and proper header identification of all monitor positions contained herein. The fluence rates reported are for the average power levels given in the table of power history and distribution. No neutron monitors were located in the N-2 position during this cycle. All "SR" holder monitor wires for this cycle are 55 inches long. This length allows measurements from 24.73 inches above core midplane to 25.25 inches below core midplane. The distance from the end of the wires to the first count position was 4.25 inches for all wires counted from this cycle.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measured Thermal And Fast Neutron Fluence Rates ATR Cycle 166B

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 166B which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains fluence rate values corresponding to the particular elevations (relative to the 80-ft. core elevation) where the measurements were taken. The data in this report consists of (1) a table of the ATR power history and distribution, (2) a hard copy listing of all thermal and fast neutron fluence rates, (3) plots of both the thermal and fast neutron fluence rates, and (4) an optical record (compact disk) containing a listing of the thermal and the fast neutron fluence rates, their assigned elevations and proper header identification of all monitor positions contained herein. The fluence rates reported are for the average power levels given in the table of power history and distribution. No neutron monitors were located in the N-2 position during this cycle.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Measured Thermal and Fact Neutron Fluence Rates for AFC Holders During Cycle 169A

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for the AFC holders located in core for ATR Cycle 169A which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains measurements of the fluence rates corresponding to the particular elevations relative to the 80-ft. core elevation. The data in this report consist of (1) a table of the ATR power history and distribution, (2) a hard copy listing of all thermal and fast neutron fluence rates, and (3) plots of both the thermal and fast neutron fluence rates. All "BR" holder monitor wires for this cycle are 56.375 inches long. This length allows measurements from 31.17 inches above core midplane to 19.81 inches below core midplane. The distance from the end of the wires to the first count position was 4.25 inches for all wires counted from this cycle.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Measured Thermal and Fast Neutron Fluence Rates for aLEU Holders During Cycle 169A

This report contains the thermal (2200 mis) and fast (E> IMeV) neutron fluence rate data for the aLEU holders located in core for ATR Cycle 169A which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains measurements of the fluence rates corresponding to the particular elevations relative to the 80-ft. core elevation. The data in this report consist of (1) a table of the ATR power history and distribution, (2) a hard copy listing of all thermal and fast neutron fluence rates, and (3) plots of both the thermal and fast neutron fluence rates. All "BR" holder monitor wires for this cycle are 56.375 inches long. This length allows measurements from 31.17 inches above core midplane to 19.81 inches below core midplane. The distance from the end of the wires to the first count position was 4.25 inches for all wires counted from this cycle.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of HELIOS/BIPR/PARCS/MCNP6 Computation Route for WWER RPV Neutron Fluence Analysis and Validation Against Ex-Vessel Detector Measurement Data

Here, a computational route was developed for precise calculation of fast neutron fluence on a WWER-type reactor pressure vessel (RPV). The method is based on the transfer of neutronics data from HELIOS-2 lattice calculations and nodal diffusion neutronics data (power, density, and temperature) from BIPR7.1 and PARCS 3.36/PATHS core calculations into a three-dimensional (pinwise axially distributed) fixed neutron source for modeling of transport of fast neutrons from the reactor core to the outer surface of the RPV using MCNP6.2. Validation of the proposed computational method was carried out based on comparative analysis of MCNP6.2-predicted and neutron dosimetry–measured reaction rates [ 54 Fe(n,p) 54 Мn, 93 Nb(n,n') 93 mNb, and 58 Ni(n,р) 58 Со] on the outer surface of the Armenian Nuclear Power Plant (ANPP) Unit 2 RPV. Validation revealed that the MCNP6.2-predicted fast neutron fluence results are very sensitive to the ENDF-B neutron data. Particularly, MCNP6.2 with ENDF/B-VIII.0 significantly underpredicts (20% to 30%) fast neutron fluence while using ENDF/B-VII.1 data overpredicts it. Adding revised beta-released evaluations of 54 Fe, 56 Fe, 57 Fe, and 16 O from the International Nuclear Data Evaluation Network (INDEN) to ENDF/B-VIII.0 allows one to obtain reasonable agreement with measurement results for all types of measured reaction rates.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measured Thermal and Fast Neutron Fluence Rates ATR Cycles 167A

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 167A which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. The report contains fluence rate values corresponding to the particular elevations (relative to the 80-ft. core elevation) where the measurements were taken. The data in this report consists of (1) a table of the ATR power history and distribution, (2) a hard copy listing of all thermal and fast neutron fluence rates, (3) plots of both the thermal and fast neutron fluence rates.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measured Thermal and Fast Neutron Fluence Rates ATR Cycles 171A ATF (Rev. 1)

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 171A ATF which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains fluence rate values corresponding to the particular elevations (relative to the 80-ft. core elevation) where the measurements were taken. The data in this report consists of (1) a table of the ATR power history and distribution, (2) a listing of the calculated thermal and fast neutron fluence rates, and (3) plots of calculated both the thermal and fast neutron fluence rates. The fluence rates reported are for the average power levels given in the table of power history and distribution. During the irradiation of Cycle 152A, the RML performed additional flux measurements to assess core reconfiguration issues. Measurements using cadmium covered as well as bare neutron monitors in the Southwest, Southeast, and H positions of the Center lobe were performed to determine the division in neutron energy between epithermal and thermal neutrons. This is defined as the resonance correction defined in this report. It is used to quantify both thermal and fast neutron flux. For more information please refer to letter, “RADIATION MEASUREMENTS LABORATORY MEASUREMENTS OF IN CORE ATR PHYSICS TESTING DURING CYCLE 152A” dated January 24, 2013, to Casey Stengel from C. C. Jensen. The measured values documented in RML Procedure, “ACMM-3600, Flux Monitoring,” will be used indefinitely until further measurements supersede the current values.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Measured Thermal and Fast Neutron Fluence Rates ATR Cycles 171A IR TMIST 3B

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 171A which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains fluence rate values corresponding to the particular elevations (relative to the 80-ft. core elevation) where the measurements were taken. The data in this report consists of (1) a table of the ATR power history and distribution, (2) a listing of the calculated thermal and fast neutron fluence rates, and (3) plots of calculated both the thermal and fast neutron fluence rates. The fluence rates reported are for the average power levels given in the table of power history and distribution. During the irradiation of Cycle 152A, the RML performed additional flux measurements to assess core reconfiguration issues. Measurements using cadmium covered as well as bare neutron monitors in the Southwest, Southeast, and H positions of the Center lobe were performed to determine the division in neutron energy between epithermal and thermal neutrons. This is defined as the resonance correction defined in this report. It is used to quantify both thermal and fast neutron flux. For more information please refer to letter, “RADIATION MEASUREMENTS LABORATORY MEASUREMENTS OF IN CORE ATR PHYSICS TESTING DURING CYCLE 152A” dated January 24, 2013, to Casey Stengel from C. C. Jensen. The measured values documented in RML Procedure, “ACMM-3600, Flux Monitoring,” will be used indefinitely until further measurements supersede the current values.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Measured Thermal and Fast Neutron Fluence Rates ATR Cycles 171A AFC (Rev. 1)

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 171A AFC which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order. This report contains fluence rate values corresponding to the particular elevations (relative to the 80-ft. core elevation) where the measurements were taken. The data in this report consists of (1) a table of the ATR power history and distribution, (2) a listing of the calculated thermal and fast neutron fluence rates, and (3) plots of calculated both the thermal and fast neutron fluence rates.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Revealing the chemical environment of Cr, Fe, and Ni in high temperature-ultrafine precipitate strengthened steel subjected to low fluence neutron irradiation

High-temperature ultrafine-precipitate-strengthened (HT-UPS) steel has potential applications in advanced nuclear reactors as a structural material. However, little is currently known about its response to neutron irradiation. This research provides insight into the neutron irradiation-induced physicochemical changes of the major constituents in HT-UPS steels, including Fe, Cr, and Ni, using synchrotron X-ray absorption near edge structure (XANES) and diffraction. This study is the first known investigation using XANES to characterize HT-UPS steel to analyze the evolution of the atomic level chemistry. It was found that following irradiation, nucleation, ballistic dispersion, and/or coarsening of Cr 23 C 6 precipitates occurred at very low neutron irradiation fluences, from 0.003 displacements per atom (dpa) up to 0.3 dpa, at ~600°C, which were at least an order of magnitude lower than previous studies. Calculations of the angular momentum projections, partial density of states, and the XANES spectra confirmed the experimental findings of the Cr 23 C 6 precipitate evolution. In contrast, the local atomic structure around Fe and Ni atoms demonstrated irradiation resistance.

36 MATERIALS SCIENCE↗

Neutron Fluence and Kerma Responses to Bare, Steel-Reflected, and Lucite-Reflected Steady-State Operations of the ORNL Health Physics Research Reactor

The experiments evaluated in this report were conducted at the Health Physics Research Reactor (HPRR), also known as the Fast Burst Reactor. The reactor was designed and built at Oak Ridge National Laboratory (ORNL) in 1961. In this evaluation, a total of 12 experiments were evaluated (6 shield configurations and two responses). Six of them are considered acceptable as benchmark experiments and are thoroughly described: the measurands are bare, steel-shielded and Lucite-shielded neutron fluences and neutron KERMA responses to steady-state operations of the HPRR. It is important to mention that there is a general lack of information in the experimental methodology and neutron spectrum unfolding, and in some cases, unexpected and unexplained discrepancies between calculation and experiment. The HPRR’s unique characteristics were that it is a fast reactor, the use of a Lucite shield as the shielding material, and the use of the neutron fluence as the main benchmark measurand. There are no known, significant correlations between benchmarks in this evaluation and benchmarks in other evaluations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A neutron fluence map of the Los Alamos National Laboratory Godiva IV critical assembly

A neutron fluence map and a total ionizing dose map of the Los Alamos National Laboratory Godiva IV fast burst critical assembly was generated using passive reactor dosimetry, comprised of sulfur pellets and thermoluminescent dosimeters. Godiva IV is an unmoderated, fast burst, critical assembly constructed of approximately 65 kg of highly enriched uranium fuel alloyed with 1.5 % molybdenum for strength. The mapping was performed during a single 75.6 ºC temperature rise burst operation, with the top and sides of the cylindrical Godiva-IV Top Hat covered in passive dosimetry. Dosimetry was placed in a symmetric pattern around the Top Hat, with higher concentrations near the control rods and burst rod. A specific portion of the lower quadrant of the burst rod was mapped to confirm a testing region where the neutron fluence varied by no more than ± 5%. The results will be used to assess the neutron, gamma, and total ionizing dose environment in three-dimensional space around the assembly for higher fidelity experiment placement, active dosimetry positioning, and radiation field characterization.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

High-yield and high-angular-fluence neutron generation from deuterons accelerated by laser-driven collisionless shock

Since a bright collimated neutron source is an essential tool for global security missions and fundamental scientific research. In this paper, we study a compact high-yield and high-angular-fluence neutron source particularly suitable for high-energy neutron applications utilizing the breakup reaction of laser-driven deuterons in a 9 Be converter. The neutron generation scaling from such a reaction is used to guide the choice and optimization of the acceleration process for bulk ions in a low density CD 2 foam. In particular, the collisionless shock acceleration mechanism is exploited with proper choice in the laser and target parameter space to accelerate these ions toward energies above the temperature of the distribution. Particle-in-cell and Monte Carlo simulations are coupled here to investigate this concept and possible adverse effects as well as the contribution from the surface ions accelerated and the optimal converter design. The simulation results indicated that our design can be a practical approach to increase both the neutron yield and angular fluence of laser-driven neutron sources, reaching >10 11 neutron/pulse (or >10 8 neutron/J) and >10 11 neutron/sr (or >10 8 neutron/sr/J) with present-day kJ-class high-power lasers. Such developments will advance fundamental neutron science, high precision radiography, and other global security applications with laser-driven sources.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Measured Thermal and Fast Neutron Fluence Rates ATR Cycles 171A

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 171A SR which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Measured Thermal and Fast Neutron Fluence Rates ATR Cycles 171B.SR

This report contains the thermal (2200 m/s) and fast (E>1MeV) neutron fluence rate data for ATR Cycle 171B SR which were measured by the Radiation Measurements Laboratory (RML) as requested by the Power Reactor Programs (ATR Experiments) Radiation Measurements Work Order.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Survey of Neutron Flux Sensors for Monitoring Advanced Reactor Concepts Operating with Low Neutron Fluence Rate and Extended Uninterrupted Lifespans

The purpose of this report is to provide a survey of neutron sensors applicable to the low power levels (low neutron fluence rate) for reactor monitoring and controls. A survey of detectors for reactor power monitoring and controls from various commercial vendors—Reuter Stokes, Framatome, Exosens, and Mirion—is presented in the following sections based on application of reactor power ranges. Detector specifications are provided where available per each of the vendor’s catalogues and specification sheets found on their websites. While this is not an all encompassing list, it provides an example of detector options. Fission chambers and self powered neutron detectors (SPNDs) for in-core application with changes to the neutron-sensitive materials—fissile depots for fission chambers and emitters for SPNDs—for regenerative capabilities will be discussed in the latter sections.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗