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NSUF CoMET Project, Implementation Plan FY2019

The Combined Materials and Experiment Toolkit (CoMET) is an NSUF information management resource designed to give users access to the information and tools necessary for designing meaningful experiments and writing clear, structured proposals. NSUF has a milestone to deploy an experiment design expert system to the NSUF website to support applications for the FY2020 CINR, due on August 30, 2019. To meet this milestone, the CoMET project work for FY2019 focuses on three main objectives: 1.) Integrate the three NSUF web applications by linking data fields in one application with the data found in the others. The NSUF web applications are: The Rapid Turnaround Experiment (RTE) Proposal Solicitation system, the Nuclear Fuels and Materials Library (NFML) and the Nuclear Energy Infrastructure Database (NEID) and the researcher and technical staff account and profile management systems. 2.) Build an Experiment Design Wizard (expert system) that will guide users through the process of writing a statement of work for a CINR or RTE experiment. 3.) Build an Irradiation Effects Calculator to help a PI choose the best neutron irradiation facility for their needs, estimate the time needed to achieve their goals, and estimate the resulting radioactivity of their samples, post-irradiation. These objectives are designed to support the mission of the NSUF and optimize the experiment design portion of the proposal processes. The new researcher database will make finding collaborators easier. The wizard will provide the PI with early NSUF expertise so that their proposed experiments, at the “Letter of Intent” and “Pre-Application” stages are better designed to work within the available NSUF facilities. Utilization of these tools should reduce the proportion of proposals that are judged to be infeasible or “not ready” for NSUF access. It should also improve the efficiency of the NSUF technical leads since the PI will be starting with a better statement of work for the project. The tools will also provide resources for NSUF staff to more efficiently screen and score incoming proposals. This implementation plan will layout the work breakdown structure, activities, resources required, and plan for completion of the activities for CoMET in FY2019.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

NSUF 2016 Annual Report

The Nuclear Science User Facilities (NSUF) and its partner facilities represent a prototype laboratory that utilizes a distributed partnership, with each facility bringing exceptional capabilities to the relationship including reactors, beamlines, state-of-the-art instruments, hot cells, and equally important, expertise. These capabilities and people together create a nationwide infrastructure that allows the best ideas to be tested using the most advanced capabilities. Through the NSUF, researchers and their collaborators are building on current knowledge to better understand the complex behavior of materials and fuels in a nuclear reactor. The NSUF’s partnership program in 2016 included eight universities, one research and education consortium, three national laboratories, and one industry partner. The avenues opened through these partnerships facilitate cooperative research across the country, matching people with capabilities and students with mentors. The NSUF in 2016 included Idaho National Laboratory (INL) and the following institutions: • Argonne National Laboratory • Center for Advanced Energy Studies (a research and education consortium between Boise State University, INL, Idaho State University, University of Idaho, and University of Wyoming) • Illinois Institute of Technology • Massachusetts Institute of Technology • North Carolina State University • Oak Ridge National Laboratory • Pacific Northwest National Laboratory • Purdue University • University of California, Berkeley • University of Michigan • University of Nevada, Las Vegas • University of Wisconsin • Westinghouse Materials Center of Excellence. This report contains details on new capabilities brought into the NSUF in 2016, the evidence of the increasing research facilitated by the NSUF, and new tools and activities to propel nuclear research and development forward to meet energy reliability and security needs. Learn about the NSUF Nuclear Fuels and Materials Library and the Nuclear Energy Infrastructure Database, and how the robust NSUF website continues to evolve to support new tools. Read about how the NSUF supports Department of Energy (DOE) missions through efforts like the 2016 NSUF Ion Beam Options Workshop, which led to a prioritiza-tion of ion beam facilities according to their ability to support Department of Energy Office of Nuclear Energy (DOE-NE) missions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Application of the FaMUS Methodology to the NSUF Research Outputs Through End of 2019

The Nuclear Science User Facilities (NSUF) is one of a diverse group of DOE user facilities. It is focused on advancing the understanding of radiation effects in nuclear fuels and materials in support of nuclear energy applications. The NSUF has been operating since 2007 and has developed a significant portfolio of supported research. Therefore, it is appropriate to consider its achievements and to determine its successes and shortfalls. As part of this analysis of the NSUF research program, the NSUF has developed a novel and elegant formalism for assessing the current level of understanding of nuclear fuels and materials for use in nuclear environments: the NSUF Fuels and Materials Understanding Scale (FaMUS). The FaMUS methodology is being applied to the NSUF portfolio on an ongoing basis to quantify the progress made. This report summarizes the status of the assessment exercise and highlights general lessons learned. This examination will facilitate capability balancing of future research by identifying gaps in knowledge, understanding, testing, and demonstration allowing the NSUF program office in conjunction with DOE-NE to direct resources to important aspects of the DOE-NE mission using “emphasize & enhance”, “maintain”, and “encourage excellence” classifications as well as providing increased transparency to researchers.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NSUF Industry Engagement Meeting Summary

NSUF held its FY23 industry engagement committee (NIEC) meeting at EPRI in Charlotte, NC during September 26-27, 2023. Over 50 participants from 25 organizations joined the meeting in person or virtually. The Objectives of the meeting were to inform the industry about the NSUF program, to collect industry feedback, and to strengthen industry collaboration and partnerships. Invitees were encouraged to come prepared with questions for NSUF and to consider ways NSUF can be leveraged for the advancement of nuclear energy. The NIEC is one of the NSUF stakeholder communities that can provide input to NSUF and inform program decisions. For this meeting, NSUF partnered with EPRI, USNRC, GAIN, and the US nuclear energy industry to exchange information and provide feedback on topics within irradiation effects on nuclear fuels and materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of the FaMUS Methodology for Quantify Materials Understanding and its Application to the NSUF Research Portfolio.

The NSUF has been operating since 2007 and has developed a significant portfolio of supported science and engineering research. Therefore, it is appropriate to consider its achievements and to determine its successes and shortfalls. As part of this analysis of the NSUF research program, the NSUF has developed a new, novel and elegant formalism for assessing the current level of understanding of nuclear fuels and of (advanced) materials for use in nuclear environments, especially in reactor: the NSUF Fuels and Materials Understanding Scale (FaMUS). The NSUF’s FaMUS methodology is being applied to the NSUF portfolio to quantify the progress made in the understanding of radiation effects in nuclear fuels and materials. This presentation will describe the status of the assessment exercise, and present a summary of any notable outcomes found as well as preliminary conclusions.

36 MATERIALS SCIENCE↗

Opportunities with NSUF for Nuclear Energy R&D

The Nuclear Science User Facilities (NSUF) is one of a diverse number of U.S. Department of Energy (DOE) user facilities established to provide researchers with the most advanced tools of modern science. The idea of a user facility has been around since the Manhattan Project, when the first of the large government-owned R&D facilities was built. Currently there are over 50 such facilities in the US, but only one devoted to nuclear energy R&D. The NSUF was established in 2007 to open INL capabilities to outside users through a competitive process. The intent was to provide access to these capabilities to a broader range of researchers that represented significant intellectual capital. The combined nuclear energy community would then be able to address the important issues relevant to the mission of the DOE-NE with respect to irradiation effects in nuclear fuels and materials. The NSUF is fairly unique in that it is no longer composed of a single self-contained facility but represents a consortium of facilities distributed across the U.S. at a number of institutions. The NSUF is centered at and managed from the Idaho National Laboratory (INL), where it was originally founded, but it also coordinates activities at more than twelve NSUF partner facilities that include eight universities, plus the three Idaho universities that are part of the Center for Advanced Energy Studies (CAES), four national laboratories, and one nuclear industry vendor. The NSUF goal is to produce the highest quality research results to increase understanding of advanced nuclear energy technologies important to DOE-NE and support national priorities by adapting to the needs of DOE-NE programs, industry, and new innovative concepts.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

2017 Year End Nuclear Science User Facilities (NSUF) Post-Irradiation Examination Summary Report

The Nuclear Science User Facilities (NSUF) are part of a growing number of Department of Energy (DOE) user facilities in the U.S., and is the only national designated nuclear energy user facility. Through a peer-reviewed proposal process, NSUF provides external research teams cost-free access to reactor, post-irradiation examination (PIE) and beamline capabilities at INL and a diverse mix of affiliated partner institutions at universities, national laboratories and industry facilities located across the country. In Fiscal Year 2017 (FY17), the NSUF sponsored planning, management and execution of PIE activities at Idaho National Laboratory (INL), the Center for Advanced Energy Studies (CAES), and other NSUF partner facilities. The individual projects associated with these PIE activities are a result from DOE awards under the following mechanisms: Consolidated Innovative Nuclear Research (CINR) awards that include full sample irradiation and PIE, PIE only (using samples from the NSUF Fuel and Materials Library) awards, or Rapid Turn-Around Experiments (RTE). An accounting of FY17 activities for each project is provided in this report.

36 MATERIALS SCIENCE↗

2024 NSUF User Development Workshop on Irradiation Testing

Monday, May 20 – Thursday, May 23, 2024 at Center for Advanced Energy Studies at Idaho National Laboratory, Idaho Falls, Idaho. This pilot workshop was hosted to expand the NSUF user community and introduce irradiation testing of nuclear fuel and materials to new researchers, and to build long-term relationships between the NSUF program office, NSUF partner facilities, and NSUF university-affiliated users to provide better utilization of NSUF resources in addressing United States energy challenges.

Starks, Alexis↗

NSUF FY24 Program Overview and Updates

The Nuclear Science User Facilities (NSUF) is one of a diverse number of U.S. Department of Energy (DOE) user facilities established to provide researchers with the most advanced tools of modern science. The NSUF was established to provide access to unique capabilities to a broad range of researchers to address the important issues relevant to irradiation effects in nuclear fuels and materials. The NSUF represents a consortium of capabilities distributed across the U.S. at twenty institutions. The NSUF is centered at the Idaho National Laboratory, but it coordinates activities at nineteen “partner” institutions. These institutions have capabilities that include neutron, ion, and gamma irradiation, hot cells, advanced material characterization, and high-performance computing. The NSUF goal is to provide access these capabilities at no cost to nuclear energy researchers to produce the highest quality research results to increase understanding of advanced nuclear energy technologies important to DOE-NE.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Role of Nuclear Science User Facilities (NSUF) in Nuclear Energy Materials Research

The Nuclear Science User Facilities (NSUF) is one of a diverse number of U.S. Department of Energy (DOE) user facilities established to provide researchers with the most advanced tools of modern science. The NSUF is unique and represents a consortium of capabilities distributed across the U.S. at twenty-one institutions. The NSUF is centered at and managed from the Idaho National Laboratory (INL), where it was originally founded, but it coordinates activities at twenty “partner” institutions that include universities, the Center for Advanced Energy Studies (CAES), national laboratories, and a nuclear industry vendor. These institutions have capabilities that include neutron, ion, and gamma irradiation, hot cells, advanced materials characterization equipment, and high-performance computing resources. Many of these capabilities were beyond reach for most researchers before NSUF. The NSUF provides researchers to access these capabilities at no cost to nuclear energy researchers to produce the highest quality research results to increase understanding of advanced nuclear energy technologies important to DOE-NE and support national priorities by adapting to the needs of DOE-NE programs, industry, and new innovative concepts for sustainable nuclear future.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

NSUF FY 2024 Annual Report: Microscopy and Characterization Suite (MaCS) and National Synchrotron Light Source-II (NSLS-II)

The Microscopy and Characterization Suite (MaCS) laboratory at the Center for Advanced Energy Studies (CAES) and the National Synchrotron Light Source-II (NSLS-II) at Brookhaven National Laboratory (BNL) partner with the Nuclear Science User Facilities (NSUF). This partnership provides funding that allows researchers to access these facilities at no cost for studying irradiation effects on nuclear fuels and materials. Through NSUF, both MaCS and NSLS-II support post-irradiation examination (PIE) and irradiation activities for NSUF Rapid Turnaround Experiments (RTE) and NSUF Consolidated Innovative Nuclear Research (CINR) awards. This report details the work completed at these facilities for NSUF competitively selected awards during fiscal year 2024.

99 GENERAL AND MISCELLANEOUS↗

Infrastructure Investments in LAMDA: SEM Mill and Vault (NSUF 2019 Milestone Report)

This document summarizes the procurement, installation, and commissioning of a scanning electron microscope (SEM) mill produced by Fischione Instruments and a lead-shielded vault for specimen storage in support of Nuclear Science User Facility (NSUF) awards for use in Oak Ridge National Laboratory’s (ORNL) Low Activation Materials Development and Analysis (LAMDA) laboratory. The Model 1061 SEM mill is a tabletop ion milling system for advanced sample preparation of high-quality SEM samples. This device was chosen for its broad range of ion energies allowing for both rapid milling and final polishing of the sample surface. The purchase order with Fischione Instruments was released and awarded by ORNL procurement on September 11, 2018. The instrument was shipped in December of 2018 and was installed in the LAMDA laboratory in March of 2019. During the commissioning of this equipment, electron backscatter diffraction (EBSD) was performed on specimens before and after milling to show the enhanced surface quality. With the purchase of a lead vault dedicated to NSUF library materials co-located in the LAMDA laboratory, the NSUF program will be able to maintain a significant sample library in LAMDA. These specimens will be easily accessible for rapid turnaround experiment (RTE) awards and will reduce the overall cost of year-over-year storage and shipments to and from ORNL hot cell facilities. The contract to fabricate a fourth lead vault dedicated to NSUF specimen storage was awarded by ORNL procurement on August 10, 2018. Installation of the new vault was completed in January of 2019.

47 OTHER INSTRUMENTATION↗

The effect of neutron irradiation on conventional and nanocrystalline nickel: NSUF Work Package UA-22PN080501 Milestone M3UA-22PN0805012 (Final Report)

Even though nanocrystalline materials (20-100 nm) present an unprecedented potential, scientific knowledge related to the effect of neutron irradiation on the mechanical properties and microstructure is still scarce. Most of the past studies were conducted using ion irradiation which may not have the same effect as neutron irradiation because of the smaller irradiation volume and the higher dose rate. To reach a firm conclusion on the potential of nanocrystalline materials for nuclear reactor applications, extensive study of model metals with different stacking fault energy (SFE) is required to elucidate their behavior in radiation environments. Nanocrystalline copper and nickel are typically chosen because they are commonly used as model FCC metals in studies of radiation effects. Nickel is an FCC metal with a high stacking-fault energy (~125 mJ/m 2 ) compared to copper (~45 mJ/m 2 ). Hence, microcrystalline and nanocrystalline nickel samples were irradiated in the INL’s Advanced Test Reactor (ATR), as a part of FY08 North Carolina State University NSUF Irradiation Experiment# 96 to evaluate the irradiation behavior of these materials. The objective of this FY20 NSUF project# 19122 is to perform PIE (at PNNL NSUF facility) on previously ATR-neutron irradiated (1.2 and 2.6 dpa; 80-89°C) nanocrystalline and microcrystalline nickel samples to investigate the changes in mechanical properties and microstructures and evaluate whether nanocrystalline nickel is relatively more radiation resistant compared to conventional microcrystalline nickel. To perform PIE at PNNL, sixteen neutron irradiated specimens (microcrystalline and nanocrystalline) were transferred from the NSUF Nuclear Fuels and Materials Library at INL. Experimental techniques such as SEM/EBSD, XRD, TEM, Vickers microhardness and tensile testing were employed to characterize the effect of neutron irradiation on the microstructure and mechanical properties of nanocrystalline nickel and compared them with corresponding characteristics of microcrystalline nickel.

36 MATERIALS SCIENCE↗

2024 NSUF Annual Program Review

The Department of Energy - Office of Nuclear Energy’s (DOE-NE) Nuclear Science User Facilities (NSUF) program held its annual review on Monday, April 15 through Thursday, April 18, 2024. The meeting involved in-person participation at Idaho National Laboratory as well as a virtual component. The NSUF program review included overview presentations by the NSUF program office and select partner facilities, as well as technical highlights from NSUF supported research projects and the user community. For questions regarding this event, please contact our program office at nsuf@inl.gov.

Author, Unknown↗

Evaluation of the NSUF Reactor Activation and Damage (RAD) Calculator damage component

The Nuclear Science User Facilities (NSUF) provide researchers access to nuclear research facilities and expertise all over the United States and at the Belgian Center for Nuclear Research (SCK/CEN). One special capability of the NSUF is providing access to nuclear research and test reactors often used for conducting material testing experiments. These services are provided at no cost to the researcher through a competitive, peer-reviewed process. With so many proposals being submitted simultaneously, an NSUF information management resource called the Combined Materials Experiment Toolkit (CoMET) was implemented to speed up the review process and give users access to the information and tools necessary for designing meaningful experiments and writing the best proposals possible. One of CoMET’s tools is the Reactor Activation and Damage (RAD) Calculator. For those with little or no background in it, neutron irradiation in research and test reactors can be a challenging subject to include in a proposal. That is why the RAD Calculator was created to assist users with providing estimates of irradiation and post-irradiation conditions, enabling them to select the best neutron irradiation and post-irradiation examination facilities for reaching their experiment goals. The RAD Calculator is a general scoping tool that estimates radiation damage in terms of DPA, in addition to the resulting radioactivity of the material post-irradiation. This report evaluates the neutron damage component of the RAD Calculator. The evaluation of the activation component of the calculator is covered in report INL/EXT-20-58080.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Application of NSUF Capabilities Towards Understanding the Emulation of High Dose Neutron Irradiations with Ion Beams

Development of new materials for current nuclear power plants (NPPs) or materials for new NPPs requires extensive research, development, and deployment programs. Central to these efforts, particularly for core internals, are studies on the microstructural and mechanical changes due to neutron irradiation. These radiation effects studies are typically completed using materials test reactors followed by expensive and time-consuming post-irradiation examinations (PIE). This sluggish approach has severely limited the nuclear materials field to develop new materials or verify materials for new reactor design use. It is also very difficult to achieve the high levels of damage proposed for future reactors. A logical approach to accelerating the field is the application of ion beams to simulate neutron damage, especially for high dose applications. Ion beams have been used for decades to study radiation effects but not to emulate high dose reactor irradiations. In this regard, new (or renewed) methods for ion beam irradiations, new developments in materials characterization, and greater understanding on the governing mechanisms controlling observed radiation effects have led to a need for further studies to refine the technique. A primary challenge is the ability to determine the ion irradiation conditions that produce microstructures and mechanical properties relevant to in-core neutron irradiation conditions. A large, multi-disciplinary, multi-laboratory program deemed the High Fidelity Ion Beam Simulation of High Dose Neutron Irradiation has been formed to assess and overcome the challenges associated with emulating high dose neutron irradiations using ion beams. Central to this program is the use of dual-beam ion irradiations and corresponding neutron irradiations within the BOR-60 fast reactor. These irradiations have produced hundreds of specimens for microstructural and mechanical characterization. A significant issue regarding the samples is the radioactivity of the neutron irradiated specimens as well as the need to characterize both irradiation types using the same equipment to maintain consistency and repeatability. The use of the Nuclear Science User Facilities (NSUF) has been central towards overcoming the mentioned issues and thereby enabling robust PIE in both the ion and neutron irradiated specimens of interest. In particular, the electron microscopes housed within the Low Activation Materials Development and Analysis (LAMDA) facility at Oak Ridge National Laboratory (ORNL) - an NSUF partner facility - has been instrumental in gathering high quality data for analysis. This paper will briefly highlight the PIE efforts using the NSUF capabilities within LAMDA.

36 MATERIALS SCIENCE↗

Advanced Characterization Capabilities for Nuclear Materials via Nuclear Science User Facilities (NSUF)

Advanced post-irradiation examination (PIE) techniques are required to design new or improved nuclear materials, characterize, and understand in-core behavior of fuel and materials, and support the qualification of new reactor materials. The Nuclear Science User Facilities (NSUF) is the U.S. Department of Energy Office of Nuclear Energy's only designated nuclear science user facility. NSUF provides researchers access to PIE capabilities at Idaho National Laboratory and at a diverse mix of university, national laboratory and industrial partner institutions. The PIE capabilities include novel destructive and non-destructive techniques for radiation damage characterization, such as advanced diffraction techniques (X-ray, electron, or neutron) coupled to extreme environments; in-situ observation of microstructural evolution under irradiation; in-situ irradiation to monitor corrosive attack in coolant environments; in-situ irradiation and mechanical testing; and test methods for synergistic effects of superimposed extreme environments (temperature, irradiation, stress, corrosion) on materials behaviors. This talk will provide an overview of NSUF PIE capabilities.

36 MATERIALS SCIENCE↗