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The Status of Cross Section Measurements for Neutron-induced Reactions Needed for Cosmic Ray Studies

Cosmic ray interactions with lunar rocks and meteorites produce small amounts of radionuclides and stable isotopes. Advances in Accelerator Mass Spectrometry (AMS) allow production rates to be measured routinely in well-documented lunar rocks and meteorites. These measurements are analyzed using theoretical models to learn about the object itself and the history of the cosmic rays that fell on it. Good cross section measurements are essential input to the theoretical calculations. Most primary cosmic ray particles are protons so reliable cross sections for proton-induced reactions are essential. A cross section is deemed accurate if measurements made by different experimenters using different techniques result in consistent values. Most cross sections for proton induced reactions are now well measured. However, good cross section measurements for neutron-induced reactions are still needed. These cross sections are required to fully account for all galactic cosmic ray interactions at depth in an extraterrestrial object. When primary galactic cosmic ray (GCR) particles interact with an object many secondary neutrons are produced, which also initiate spallation reactions. Thus, the total GCR contribution to the overall cosmogenic nuclide archive has to include the contribution from the secondary neutron interactions. Few relevant cross section measurements have been reported for neutron-induced reactions at neutron energies greater than approximately 20 MeV. The status of the cross section measurements using quasi-monoenergetic neutron energies at iThemba LABS, South Africa and white neutron beams at Los Alamos Neutron Science Center (LANSCE), Los Alamos are reported here.

Sisterson, J. M.↗

Revised Production Rates for Na-22 and Mn-54 in Meteorites Using Cross Sections Measured for Neutron-induced Reactions

The interactions of galactic cosmic rays (GCR) with extraterrestrial bodies produce small amounts of radionuclides and stable isotopes. The production rates of many relatively short-lived radionuclides, including 2.6-year Na-22 and 312-day Mn-54, have been measured in several meteorites collected very soon after they fell. Theoretical models used to calculate production rates for comparison with the measured values rely on input data containing good cross section measurements for all relevant reactions. Most GCR particles are protons, but secondary neutrons make most cosmogenic nuclides. Calculated production rates using only cross sections for proton-induced reactions do not agree well with measurements. One possible explanation is that the contribution to the production rate from reactions initiated by secondary neutrons produced in primary GCR interactions should be included explicitly. This, however, is difficult to do because so few of the relevant cross sections for neutron-induced reactions have been measured.

Sisterson, J. M.↗

Barites - Anomalous xenon from spallation and neutron-induced reactions

Sedimentary barites from South Africa and Western Australia (about 3 billion years old) contain spallogenic Xe isotopes produced by reactions of Ba with nuclear-active particles in cosmic rays. 'Surface residence time' of these samples was calculated from the observed concentrations of spallogenic Xe-126. Comparison of spallogenic ratios of Xe-131/Xe-126 in the two samples provides evidence for the reaction Ba-130(n, gamma) yields Xe-131, which is characterized by a large number of resonances for neutron absorption in the epithermal region. This observation lends additional support to the conclusions already reached regarding the origin of anomalous Xe-131 in lunar samples.

Srinivasan, B.↗

Cosmogenic Cl-36 production rates in meteorites and the lunar surface

Activity vs. depth profiles of cosmic ray produced Cl-36 were measured in metal from two cores each in the St. Severin and Jilin chondrites and in lunar core 15008. Production of Cl-36 in these samples range from high-energy reactions with Fe and Ni to low-energy reactions with Ca and K and possibly neutron-capture reactions with Cl-36. The cross sections used in the Reedy-Arnold model for neutron-induced reactions were adjusted to get production rates that fit the measured Cl-36 activities in St. Severin metal and in the lunar soil of core 15008. The Cl-36 in metal from St. Severin has a fairly flat activity-vs-depth profile, unlike most other cosmogenic nuclides in bulk samples from St. Severin, which increase in concentration with depth. In metal from Jilin, a decrease in Cl-36 was observed near its center. The length of Jilin's most recent cosmic-ray exposure was approximately 0.5 My. Lunar core 15008 has an excess in Cl-36 of about 4 dpm/kg near its surface that was produced by solar-proton-induced reactions. The calculated production rates are consistent with these measured trends in 15008.

Nishiizumi, K.↗

Rare-gas analyses on neutron irradiated Apollo 12 samples.

Argon, krypton, and xenon from stepwise heating of five Apollo 12 rocks that had been irradiated to a neutron fluence of about 10 to the 19th neutrons/sq cm were analyzed mass-spectrometrically. The Ar40-Ar39 ages were determined and range from 3.18 plus or minus 0.06 x 10 to the 9th years to 3.32 plus or minus 0.06 x 10 to the 9th years. Trace elements Ba, Br, I, and U were measured via the neutron-induced reactions that produce isotopes of krypton and xenon. The following concentration ranges were observed: Ba, 46 to 70 ppm; Br, 48 to 146 ppb; I, 16 to 73 ppb; and U, 170 to 247 ppb.

Alexander, E. C., Jr.↗

Lunar and Planetary Science XXXV: Isotopes in Meteorites

The session"Isotopes in Meteorites" consisted of the following presentations:The Common Property of Isotopic Anomalies in Meteorites; Revised Production Rates for 22Na and 54Mn in Meteorites Using Cross Sections Measured for Neutron-induced Reactions; Modeling of 14C and 10Be Production Rates in Meteorites and Lunar Samples; Investigating Xenon Isotopic Fractionation During Rayleigh-type Distillation; The Mean Life Squared Relationship for Abundances of Extinct Radioactivities; and Magnesium Isotopic Fractionation of Forsterite During Evaporation from Different Crystallographic Surfaces.

Source record↗

Induced radioactivity of LDEF materials and structural components

We present an overview of the Long Duration Exposure Facility (LDEF) induced activation measurements. The LDEF, which was gravity-gradient stabilized, was exposed to the low Earth orbit (LEO) radiation environment over a 5.8 year period. Retrieved activation samples and structural components from the spacecraft were analyzed with low and ultra-low background HPGe gamma spectrometry at several national facilities. This allowed a very sensitive measurement of long-lived radionuclides produced by proton- and neutron-induced reactions in the time-dependent, non-isotropic LEO environment. A summary of major findings from this study is given that consists of directionally dependent activation, depth profiles, thermal neutron activation, and surface beryllium-7 deposition from the upper atmosphere. We also describe a database of these measurements that has been prepared for use in testing radiation environmental models and spacecraft design.

NASA Discipline Radiation Health↗

Neutron-induced 2.2 MeV background in gamma ray telescopes

Neutron-induced gamma ray production is an important source of background in Compton scatter gamma ray telescopes where organic scintillator material is used. Most important is deuteron formation when atmospheric albedo and locally produced neutrons are thermalized and subsequently absorbed in the hydrogenous material. The resulting 2.2 MeV gamma ray line radiation essentially represents a continuous isotropic source within the scintillator itself. Interestingly, using a scintillator material with a high hydrogen-to-carbon ratio to minimize the scintillator material with a high hydrogen-to-carbon ratio to minimize the neutron-induced 4.4 MeV carbon line favors the np reaction. The full problem of neutron-induced background in Compton scatter telescopes has been previously discussed. Results are presented of observations with the University of California balloon-borne Compton scatter telescope where the 2.2 MeV induced line emission is prominently seen.

Zanrosso, E. M.↗

Sulfur Isotopes in Gas-rich Impact-Melt Glasses in Shergottites

Large impact melt glasses in some shergottites contain huge amounts of Martian atmospheric gases and they are known as gas-rich impact-melt (GRIM) glasses. By studying the neutron-induced isotopic deficits and excesses in Sm-149 and Sm-150 isotopes resulting from Sm-149 (n,gamma) 150Sm reaction and 80Kr excesses produced by Br-79 (n,gamma) Kr-80 reaction in the GRIM glasses using mass-spectrometric techniques, it was shown that these glasses in shergottites EET79001 and Shergotty contain regolith materials irradiated by a thermal neutron fluence of approx.10(exp 15) n/sq cm near Martian surface. Also, it was shown that these glasses contain varying amounts of sulfates and sulfides based on the release patterns of SO2 (sulfate) and H2S (sulfide) using stepwise-heating mass-spectrometric techniques. Furthermore, EMPA and FE-SEM studies in basaltic-shergottite GRIM glasses EET79001, LithB (,507& ,69), Shergotty (DBS I &II), Zagami (,992 & ,994) showed positive correlation between FeO and "SO3" (sulfide + sulfate), whereas those belonging to olivine-phyric shergottites EET79001, LithA (,506, & ,77) showed positive correlation between CaO/Al2O3 and "SO3".

Rao, M. N.↗

Nuclear Propulsion for Space Applications

Basics of Nuclear Systems: Long history of use on Apollo and space science missions. 44 RTGs and hundreds of RHUs launched by U.S. during past 4 decades. Heat produced from natural alpha (a) particle decay of Plutonium (Pu-238). Used for both thermal management and electricity production. Used terrestrially for over 65 years. Fissioning 1 kg of uranium yields as much energy as burning 2,700,000 kg of coal. One US space reactor (SNAP-10A) flown (1965). Former U.S.S.R. flew 33 space reactors. Heat produced from neutron-induced splitting of a nucleus (e.g. U-235). At steady-state, 1 of the 2 to 3 neutrons released in the reaction causes a subsequent fission in a "chain reaction" process. Heat converted to electricity, or used directly to heat a propellant. Fission is highly versatile with many applications.

Houts, M. G.↗