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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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Three Way Comparison between Two OMI/Aura and One POLDER/PARASOL Cloud Pressure Products

The cloud pressures determined by three different algorithms, operating on reflectances measured by two space-borne instruments in the "A" train, are compared with each other. The retrieval algorithms are based on absorption in the oxygen A-band near 760 nm, absorption by a collision induced absorption in oxygen near 477nm, and the filling in of Fraunhofer lines by rotational Raman scattering. The first algorithm operates on data collected by the POLDER instrument on board PARASOL, while the latter two operate on data from the OMI instrument on board Aura. The satellites sample the same air mass within about 15 minutes. Using one month of data, the cloud pressures from the three algorithms are found to show a similar behavior, with correlation coefficients larger than 0.85 between the data sets for thick clouds. The average differences in the cloud pressure are also small, between 2 and 45 hPa, for the whole data set. For optically thin to medium thick clouds, the cloud pressure the distribution found by POLDER is very similar to that found by OMI using the O2 - O2 absorption. Somewhat larger differences are found for very thick clouds, and we hypothesise that the strong absorption in the oxygen A-band causes the POLDER instrument to retrieve lower pressures for those scenes.

Sneep, M.↗

Remote Sensing of Aerosol in the Terrestrial Atmosphere from Space: New Missions

The distribution and properties of atmospheric aerosols on a global scale are not well known in terms of determination of their effects on climate. This mostly is due to extreme variability of aerosol concentrations, properties, sources, and types. Aerosol climate impact is comparable to the effect of greenhouse gases, but its influence is more difficult to measure, especially with respect to aerosol microphysical properties and the evaluation of anthropogenic aerosol effect. There are many satellite missions studying aerosol distribution in the terrestrial atmosphere, such as MISR/Terra, OMI/Aura, AVHHR, MODIS/Terra and Aqua, CALIOP/CALIPSO. To improve the quality of data and climate models, and to reduce aerosol climate forcing uncertainties, several new missions are planned. The gap in orbital instruments for studying aerosol microphysics has arisen after the Glory mission failed during launch in 2011. In this review paper, we describe several planned aerosol space missions, including the Ukrainian project Aerosol-UA that obtains data using a multi-channel scanning polarimeter and wide-angle polarimetric camera. The project is designed for remote sensing of the aerosol microphysics and cloud properties on a global scale.

Aerosol↗

Anthropogenic Sulphur Dioxide Load over China as Observed from Different Satellite Sensors

China, with its rapid economic growth and immense exporting power, has been the focus of many studies during this previous decade quantifying its increasing emissions contribution to the Earth's atmosphere. With a population slowly shifting towards enlarged power and purchasing needs, the ceaseless inauguration of new power plants, smelters, refineries and industrial parks leads infallibly to increases in sulphur dioxide, SO2, emissions. The recent capability of next generation algorithms as well as new space-borne instruments to detect anthropogenic SO2 loads has enabled a fast advancement in this field. In the following work, algorithms providing total SO2 columns over China based on SCIAMACHY/Envisat, OMI/Aura and GOME2/MetopA observations are presented. The need for post-processing and gridding of the SO2 fields is further revealed in this work, following the path of previous publications. Further, it is demonstrated that the usage of appropriate statistical tools permits studying parts of the datasets typically excluded, such as the winter months loads. Focusing on actual point sources, such as megacities and known power plant locations, instead of entire provinces, monthly mean time series have been examined in detail. The sharp decline in SO2 emissions in more than 90% - 95% of the locations studied confirms the recent implementation of government desulphurisation legislation; however, locations with increases, even for the previous five years, are also identified. These belong to provinces with emerging economies which are in haste to install power plants and are possibly viewed leniently by the authorities, in favour of growth. The SO2 load seasonality has also been examined in detail with a novel mathematical tool, with 70% of the point sources having a statistically significant annual cycle with highs in winter and lows in summer, following the heating requirements of the Chinese population.

Sulphur dioxide; China; Satellite remote sensing; ↗

Optimal Estimation-Based Algorithm to Retrieve Aerosol Optical Properties for GEMS Measurements Over Asia

The Geostationary Environment Monitoring Spectrometer (GEMS) is scheduled to be in orbit in 2019 onboard the GEO-KOMPSAT 2B satellite and will continuously monitor air quality over Asia. The GEMS will make measurements in the UV spectrum (300-500 nm) with 0.6 nm resolution. In this study, an algorithm is developed to retrieve aerosol optical properties from UV-visible measurements for the future satellite instrument and is tested using 3 years of existing OMI L1B data. This algorithm provides aerosol optical depth (AOD), single scattering albedo (SSA) and aerosol layer height (ALH) using an optimized estimation method. The retrieved AOD shows good correlation with Aerosol Robotic Network (AERONET) AOD with correlation coefficients of 0.83, 0.73 and 0.80 for heavy-absorbing fine (HAF) particles, dust and non-absorbing (NA) particles, respectively. However, regression tests indicate underestimation and overestimation of HAF and NA AOD, respectively. In comparison with AOD from the OMI/Aura Near-UV Aerosol Optical Depth and Single Scattering Albedo 1-orbit L2 Swath 13 km x 24 km V003 (OMAERUV) algorithm, the retrieved AOD has a correlation coefficient of 0.86 and linear regression equation, AOD(sub GEMS) = 1.18AOD(sub OMAERUV) + 0.09. An uncertainty test based on a reference method, which estimates retrieval error by applying the algorithm to simulated radiance data, revealed that assumptions in the spectral dependency of aerosol absorptivity in the UV cause significant errors in aerosol property retrieval, particularly the SSA retrieval. Consequently, retrieved SSAs did not show good correlation with AERONET values. The ALH results were qualitatively compared with the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) products and were found to be well correlated for highly absorbing aerosols. The difference between the attenuated-backscatter-weighted height from CALIOP and retrieved ALH were mostly closed to zero when the retrieved AOD is higher than 0.8 and SSA is lower than 0.93. Although retrieval accuracy was not significantly improved, the simultaneous consistent retrieval of AOD, SSA and ALH alone demonstrates the value of this stand-alone algorithm, given their nature for error using other methods. The use of these properties as input parameters for the air mass factor calculation is expected to improve the retrieval of other trace gases over Asia.

Geostationary Environment Monitoring Spectrometer ↗

Monitoring Volcanic Eruptions by OMI/OMPS, ASTER, and MERRA-2

Volcanic lava flows and/or the gas eruptions are the most common characteristics that can be remotely monitored with satellite technology in the global perspective and on different timescales. Atmospheric Sulfur Dioxide (SO2), one of the most abundant gases from volcanic eruptions apart from atmospheric common gases Carbon Dioxide and water vapor, can be directly detected by space-based sensors on satellites. The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) is one of the 12 Distributed Active Archive Centers (DAACs) within NASA's Earth Observing System Data and Information System (EOSDIS), which archives SO2 data sets from the Nimbus-7 Total Ozone Mapping Spectrometer (TOMS) in 1978, till the ongoing Ozone Monitoring Instrument (OMI) on NASA's EOS-Aura satellite, the Ozone Mapping Profiler Suite (OMPS) Nadir Mapper (NM) on both the Suomi National Polar-Orbiting Partnership (Suomi-NPP or SNPP) and the Joint Polar-orbiting Satellite System-1 (JPSS-1) satellites, into the future JPSS missions. In addition to the standard OMI/Aura and OMPS/S-NPP SO2 products, SO2 products created under the charter of the Making Earth System Data Records for Use in Research Environments (MEaSUREs) project, are also archived at GES DISC, through which NASA enacts to expand understanding the Earth system using consistent data records. The Land Processes Distributed Active Archive Center (LP DAAC) is another EOSDIS's DAAC that provides land data products and operates as a partnership with the U.S. Geological Survey (USGS). The LP DAAC has been archiving the satellite imagery from the Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) aboard NASA's EOS-Terra satellite, a high spatial resolution (15 meters) and 14 band multispectral instrument. The ASTER imagery is one of the land products contributing to the application for monitoring hot spots and land terrain changes caused by volcanic eruption events. The data potential in GES DISC and LP DAAC to monitor volcanic sources of SO2 and the influence of wind fields on the gas plume spread will be demonstrated with the most recent 2018 May-July Kilauea Volcano eruption.

Zeng, Jian↗

NO2 Anomalies - Economy Attribution and Rapid Climate Response

Using principal component (PC) analysis of 16 years of monthly series of NO2 from OMI/Aura, we show that it is the third PC (PC3) from the full hierarchy of principal modes that is best coupled with the economic indicators. This coupling is positive, i.e. PC3 and economic indicators manifest positive covariance. However, the economic variability can explain only 40% of the information in PC3. Furthermore, this mode by itself explains only 3% of the total deseasonalized NO2 variability. We thus conclude that, while having an unambiguous impact, the economy can be awarded at best third order of importance in driving the deseasonalized NO2 series, i.e. after seasonal variability is removed from the series. Once we identified PC3 as the NO2 mode that is coupled with economic variability, we use this mode as an indicator and look for rapid climate adjustments to that part of NO2 variability that we are confident is coupled with the economic variability. We focus on observational data from the Atmospheric Infrared Sounder (AIRS) on board of NASA Aqua satellite, decompose series of surface skin temperature and clear-sky outgoing longwave radiances (OLR) into principal components, and identify potential impacts of NO2 PC3 on these climate variables.

NO2↗

NO2 Anomalies - Economy Attribution and Rapid Climate Response

Using principal component (PC) analysis of 16 years of monthly series of NO2 from OMI/Aura, we show that it is the third PC (PC3) from the full hierarchy of principal modes that is best coupled with the economic indicators. This coupling is positive, i.e. PC3 and economic indicators manifest positive covariance. However, the economic variability can explain only 40%of the information in PC3. Furthermore, this mode by itself explains only 3% of the total deseasonalized NO2 variability. We thus conclude that, while having an unambiguous impact, the economy can be awarded at best third order of importance in driving the deseasonalized NO2 series, i.e. after seasonal variability is removed from the series. Once we identified PC3 as the NO2 mode that is coupled with economic variability, we use this mode as an indicator and look for rapid climate adjustments to that part of NO2 variability that we are confident is coupled with the economic variability. We focus on observational data from the Atmospheric Infrared Sounder (AIRS) on board of NASA Aqua satellite, decompose series of surface skin temperature and clear-sky outgoing longwave radiances (OLR) into principal components, and identify potential impacts of NO2 PC3 on these climate variables.

NO2↗

Evaluating Drought Responses of Surface Ozone Precursor Proxies: Variations With Land Cover Type, Precipitation, and Temperature

Prior work suggests drought exacerbates US air quality by increasing surface ozone concentrations. We analyze 2005–2015 tropospheric column concentrations of two trace gases that serve as proxies for surface ozone precursors retrieved from the OMI/Aura satellite: Nitrogen dioxide (ΩNO2; NOx proxy) and formaldehyde (ΩHCHO; VOC proxy). We find 3.5% and 7.7% summer drought enhancements (classified by SPEI) for ΩNO2 and ΩHCHO, respectively, corroborating signals previously extracted from ground‐level observations. When we subset by land cover type, the strongest ΩHCHO drought enhancement (10%) occurs in the woody savannas of the Southeast US. By isolating the influences of precipitation and temperature, we infer that enhanced biogenic VOC emissions in this region increase ΩHCHO independently with both high temperature and low precipitation during drought. The strongest ΩNO2 drought enhancement (6.0%) occurs over Midwest US croplands and grasslands, which we infer to reflect the sensitivity of soil NOx emissions to temperature.

drought↗

Global Fine Scale Changes in Ambient NO2 During COVID-19 Lockdowns

Nitrogen dioxide (NO2) is an important contributor to air pollution and can adversely affect human health(1–9) . A decrease in NO2 concentrations has been reported as a result of lockdown measures to reduce the spread of COVID-19(10–20). Questions remain, however, regarding the relationship of satellite-derived atmospheric column NO2 data with health-relevant ambient ground-level concentrations, and the representativeness of limited ground-based monitoring data for global assessment. Here we derive spatially resolved, global ground-level NO2 concentrations from NO2 column densities observed by the TROPOMI satellite instrument at sufficiently fine resolution (approximately one kilometre) to allow assessment of individual cities during COVID-19 lockdowns in 2020 compared to 2019. We apply these estimates to quantify NO2 changes in more than 200 cities, including 65 cities without available ground monitoring, largely in lower-income regions. Mean country-level population-weighted NO2 concentrations are 29% ± 3% lower in countries with strict lockdown conditions than in those without. Relative to long-term trends, NO2 decreases during COVID-19 lockdowns exceed recent Ozone Monitoring Instrument (OMI)-derived year-to-year decreases from emission controls, comparable to 15 ± 4 years of reductions globally. Our case studies indicate that the sensitivity of NO2 to lockdowns varies by country and emissions sector, demonstrating the critical need for spatially resolved observational information provided by these satellite-derived surface concentration estimates.

Ground level NO2↗