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Results for “Optical transient phenomena”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Attosecond Optical Orientation

Circularly polarized light offers opportunities to probe symmetry-dependent properties of matter such as chirality and spin. Circular-dichroic measurements typically require further intrinsic or extrinsic breaking of symmetry by, e.g., enantiomeric excess, orientation, magnetic fields, or direction-sensitive detectors. Here we introduce circular-dichroic attosecond transient absorption spectroscopy by leveraging the angular momentum of two circularly polarized pulses, both pump and probe, in an isotropic medium, optically orienting the angular momentum of excited states on an attosecond timescale. We investigate a circular-dichroic measurement of the attosecond transient absorption of He Rydberg states. By limiting the allowed pathways via dipole selection rules for co- and counterrotating circularly polarized near-infrared and extreme ultraviolet (XUV) pulses, different spectral reshapings of the XUV transient absorption due to the AC Stark effect are observed. Furthermore, paired with time-dependent Schrödinger equation calculations, the results show the role of selection and propensity rules and open up new opportunities to study coupling pathways of excited states as well as spin-dependent dynamics in atoms and beyond via attosecond optical orientation.

Angular momentum of light↗
DOE OSTI2025

Probing coherent electronic superpositions of singly and doubly excited states of krypton with extreme-ultraviolet four-wave-mixing spectroscopy

Radiative nonlinear four-wave mixing can monitor the evolution of electronic wave packets, providing access to lifetimes and quantifying the light-induced couplings between excited states. In this article, we report the observation of quantum beats in an autoionizing electronic wave packet in krypton, probed using this technique. Analysis of the signal reveals that these beats originate from the contribution of previously unassigned, doubly excited states interacting with singly excited ones. We introduce a minimal theoretical model, based on multichannel quantum-defect theory, which quantitatively reproduces both the wave-packet dynamics and the static spectrum. This work combines a versatile, noncommensurate XUV-IR-based experimental scheme with a tractable model, establishing a powerful approach for the metrology and control of complex, correlated electronic states.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2024

Autoionizing polaritons with the Jaynes-Cummings model

Intense laser pulses have the capability to couple resonances in the continuum, leading to the formation of a split pair of autoionizing polaritons. These polaritons can exhibit extended lifetimes due to interference between radiative and Auger decay channels. In this work we show how an extension of the Jaynes-Cummings model to autoionizing states quantitatively reproduces the observed phenomenology. Furthermore, this extended model allows us to study how the dressing laser parameters can be tuned to control the ionization rate of the polariton multiplet.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS1977

Critical velocity phenomena and the LTP

When the relative velocity between magnetized plasma and neutral gas exceeds a critical value, the gas-plasma interaction is dominated by collective phenomena which rapidly excite and ionize the neutrals. The interaction of the solar wind with a large cloud (between 10 to the 24th and 10 to the 28th power neutrals) vented from the moon should be of this type. Line radiation from such an interaction can yield an apparent lunar surface brightness rivaling reflected sunlight levels over small areas, if the kinetic-energy flow density of the gas is sufficiently high. The aberrated solar-wind flow past the moon would enhance the visibility of such interactions near the lunar sunrise terminator, supporting the statistical studies which indicate that the 'Lunar Transient Phenomena' (anomalous optical phenomena on the moon) are significantly correlated with the position of the terminator on the lunar surface.

Srnka, L. J.↗
NASA NTRS1976

The Corralitos Observatory program for the detection of lunar transient phenomena

This is a final report on the establishment, observing procedures, and observational results of a survey program for the detection of lunar transient phenomena (LTP's) by electro-optical image conversion means. For survey, a unique detection system with an image orthicon was used as the primary element in conjunction with a 24-in. f/20 Cassegrainian telescope. Observations in three spectral ranges, with 6,466 man-hours of observing, were actually performed during the period from October 27, 1965, to April 26, 1972. Within this entire period, no color or feature change within the detection capabilities of the instrumentation was observed, either independently or in follow up of amateur LTP reports, with the exception of one general bluing and several localized bluings (probably ascribable to the effects of the terrestrial atmosphere) that were observed solely by the Corralitos system. A table is presented indicating amateur and professional reports of LTP's and the results of efforts to confirm these reports through the Corralitos system.

Hynek, J. A.↗
NASA NTRS1983

The Rapidly Moving Telescope: an Instrument for the Precise Study of Optical Transients

The development of a small telescope with a very rapid pointing capability is described whose purpose is to search for and study fast optical transients that may be associated with gamma-ray bursts and other phenomena. The primary motivation for this search is the discovery of the existence of a transient optical event from the known location of a gamma-ray bursts. The telescope has the capability of rapidly acquiring any target in the night sky within 0.7 second and locating the object's position with + or - 1 arcsec accuracy. The initial detection of the event is accomplished by the MIT explosive transient camera or ETC. This provides rough pointing coordinates to the RMT on the average within approximately 1 second after the detection of the event.

Teegarden, B. J.↗
NASA NTRS1981

Solar radio bursts of spectral type II, coronal shocks, and optical coronal transients

An examination is presented of the association of solar radio bursts of spectral type II and coronal shocks with solar flare ejecta observed in H-alpha, the green coronal line, and white-light coronagraphs. It is suggested that fast-moving optical coronal transients should for the most part be identified with piston-type phenomena well behind the outward-traveling shock waves that generate type II radio bursts. A general model is presented which relates type II radio bursts and coronal shocks to optically observed ejecta and consists of three main velocity regimes: (1) a quasi-hemispherical shock wave moving outward from the flare at speeds of 1000-2000 km/sec and Alfven Mach number of about 1.5; (2) the velocity of the piston driving the shock, on the order of 0.8 that of the shock; and (3) the regime of the slower-moving H-alpha ejecta, with velocities of 300-500 km/sec.

Maxwell, A.↗
DOE OSTI2025

All hard X-ray transient grating spectroscopy

Optical-domain transient grating (TG) spectroscopy is the ideal tool to investigate transport phenomena in gases, liquids and solids, but it is limited to typically micron-size grating periods. Extreme-Ultraviolet TG has represented a major leap forward to access the mesoscopic scales. Hard X-ray TGs open access in principle to the nanoscale. Hard X-ray TGs were recently generated using the Talbot effect and probed by optical pulses, but these hinder exploiting the advantages of the nanoscale gratings. Here, we present an all-X-ray TG study, in which few-femtosecond hard X-ray pulses are used both for excitation and probing. Our experiment was performed on an amorphous film of an FeGd alloy and on a thin silicon single crystal. The results show a manifestation of the TG induced by the X-ray pump and probe pulses in the form of Talbot carpets, as well as temporal evolution of the grating in crystalline silicon showing coherent optical phonons. Ultrafast all-X-ray TG spectroscopy has the potential to study fundamental excitations with femtosecond time resolution and nanometer spatial sensitivity.

Ferrari, Eugenio [Deutsches Elektronen-Synchrotron↗
DOE OSTI2025

Spatio-spectral optical fission in time-varying subwavelength layers

Transparent conducting oxides are highly doped semiconductors that exhibit favourable optical features compared with metals, including reduced material losses, tuneable electronic and optical properties, and enhanced damage thresholds. Recently, the photonic community has renewed its attention towards these materials, recognizing their remarkable nonlinear optical properties in the near-infrared spectrum. The exceptionally large and ultrafast change in the refractive index, which can be optically induced in these compounds, extends beyond the boundaries of conventional perturbative analysis and makes this class of materials the closest approximation to a time-varying system. Here we report the spatio-spectral fission of an ultrafast pulse trespassing a thin film of aluminium zinc oxide with a non-stationary refractive index. By applying phase conservation to this time-varying layer, our model can account for both space and time refraction and explain, in quantitative terms, the spatial separation of both spectrum and energy. Our findings represent an example of extreme nonlinear phenomena on subwavelength propagation distances, which provides new insights into transparent conducting oxides’ transient optical properties. This can be critical for the ongoing research on photonic time crystals, on-chip generation of non-classical states of light, integrated optical neural networks, ultrafast beam steering and frequency-division multiplexing.

integrated optics↗
NASA NTRS1974

Active mode-coupling phenomena in pulsed and continuous lasers

An optical modulator inside a laser cavity, if driven at the cavity c/2L frequency or a harmonic, will produce a variety of mode-coupled short-pulse and FM-laser phenomena. This paper reviews the kinds of CW and transient mode-coupling phenomena that can occur in CW lasers and in selected lower-power pulsed lasers using either an active optical modulator or in some cases passive saturable absorbers.

Siegman, A. E.↗
DOE OSTI2025

Symmetry-protected electronic metastability in an optically driven cuprate ladder

Optically excited quantum materials exhibit non-equilibrium states with remarkable emergent properties, but these phenomena are usually transient, decaying on picosecond timescales and limiting practical applications. Advancing the design and control of non-equilibrium phases requires the development of targeted strategies to achieve long-lived, metastable phases. Here, in this study, we report the discovery of symmetry-protected electronic metastability in the model cuprate ladder Sr 14 Cu 24 O 41 . Using femtosecond resonant X-ray scattering and spectroscopy, we show that this metastability is driven by a transfer of holes from chain-like charge reservoirs into the ladders. This ultrafast charge redistribution arises from the optical dressing and activation of a hopping pathway that is forbidden by symmetry at equilibrium. Relaxation back to the ground state is, hence, suppressed after the pump coherence dissipates. Our findings highlight how dressing materials with electromagnetic fields can dynamically activate terms in the electronic Hamiltonian, and provide a rational design strategy for non-equilibrium phases of matter.

36 MATERIALS SCIENCE↗
NASA NTRS1982

Optical studies of shock generated transient supersonic base flows

A shock tube employing interferometric and schlieren techniques is used to study transient base flow phenomena following shock wave passage over two plane bluff bodies: a hemicircular cylinder and a cylinder with the Galileo Jovian probe profile. An attempt is made to understand the physics of transition from transient to steady state flow, and to provide code verification for a study employing the Illiac IV computer. Transient base flow interactions include a series of shock diffraction, regular, and Mach reflections, coupled with boundary layer development, separation, and recompression. Vorticity generation and transport underlie these features. The quantitative verification of the computer code includes comparisons of transient pressure and density fields, near wake geometries, and bow shock standoff distances.

Liang, P.-Y.↗
NASA NTRS1979

X-ray observations of the 5 March 1979 gamma-burst field

An extremely intense burst of hard X-rays and gamma-rays that was recorded by the nine interplanetary spacecraft of the burst sensor network and localized by time-of-flight determinations to a position coincident with the supernova remnant N49 in the Large Magellanic Cloud is analyzed. The region of the sky was observed both before and after the gamma-ray event with the soft X-ray imaging instruments aboard the Einstein Observatory. Coupled with the optical plate material, the soft X-ray data is used to place severe constraints on models for the origin of the transient phenomena.

Helfand, D. J.↗
DOE OSTI2026

Bound Exciton Complexes in Near-Infrared Emitting Quantum Shells

Near-infrared (NIR) light sources based on colloidal semiconductor nanocrystals (NCs) represent a scalable, low-cost alternative to epitaxial semiconductor platforms. However, their performance remains hindered by rapid Auger recombination, a problem that is particularly pronounced in narrow-bandgap materials. Here, we report on CdS/HgS/CdS and CdS/HgCdSe/ ZnS quantum shells (QSs), a class of spherical quantum wells specifically engineered for a suppression of nonradiative Auger processes. Fabricated QSs exhibit tunable NIR emission with photoluminescence quantum yields reaching ∼60% below 1000 nm and up to 30% near 1300 nm. Optical gain and stimulated emission were observed in CdS/HgS/CdS QSs. In contrast, CdS/HgCdSe/ZnS QSs displayed a photoinduced absorption in lieu of optical gain despite demonstrating a comparatively stronger Auger suppression. Transient absorption spectroscopy revealed that this phenomenon arises from the formation of bound multiexciton complexes that induce long-lived sub-bandgap multiexciton states. The observation of such bound excitonic clusters at room temperature offers a pathway toward nonlinear NIR photonic phenomena, including biexciton−exciton cascade emission, optical modulation, and singleexciton gain.

Auger recombination↗
NASA NTRS1978

Research in space physics at the University of Iowa

Specific fields of current investigation by satellite observation and ground-based radio-astronomical and optical techniques are discussed. Topics include: aspects of energetic particles trapped in the earth's magnetic field and transiently present in the outer magnetosphere and the solar, interplanetary, and terrestrial phenomena associated with them; plasma flows in the magnetosphere and the ionospheric effects of particle precipitation, with corresponding studies of the magnetosphere of Jupiter, Saturn, and possibly Uranus; the origin and propagation of very low frequency radio waves in the earth's magnetosphere and ionosphere; solar particle emissions and their interplanetary propagation and acceleration; solar modulation and the heliocentric radial dependence of the intensity of galactic cosmic rays; radio frequency emissions from the quintescent and flaring sun; shock waves in the interplanetary medium; radio emissions from Jupiter; and radio astronomy of pulsars, flare stars, and other stellar sources.

Vanallen, J. A.↗
DOE OSTI2026

How Does Metal Spin State Affect Electronic Communication in Mixed-Valence Dimers? Insights from Ultrafast Near-Infrared and Soft X-ray Transient Absorption Spectroscopy

Recent advancements in photocatalysis, photovoltaics, and quantum information science take advantage of electron spin, and determining how spin multiplicity affects electron transfer is key to understanding these phenomena. Here, in this study, we examine how metal spin state affects electronic communication in an organometallic mixed-valence dimer, ferrocenyl cobaltocenium ([Fe II Cp 2 Co III Cp 2 ] + ). This complex can be photoexcited from its low-spin singlet Fe II ground state to form intermediate-spin triplet Fe II and high-spin quintet Fe II excited states. Using femtosecond optical transient absorption (OTA) spectroscopy with visible (vis), near-infrared (NIR), and short-wave IR (SWIR) probes, supported by time-dependent density functional theory (TD-DFT) calculations, we measure Fe II Co III →Fe III Co II intervalence charge transfer (IVCT) bands in each of the Fe II spin states. Mulliken–Hush analysis of the excited-state IVCT bands was used to compute the electronic coupling between the metal centers in all three spin states, which increased as quintet < triplet < singlet. Meanwhile, the peak energy of the bands, and thus the ΔG of the IVCT transition, increased as triplet < quintet < singlet. Then, to directly probe the electronic structure at each metal center, we employed picosecond soft X-ray transient absorption (XTA) spectroscopy at the Fe and Co L 3 edges. Our results show that the low-spin and high-spin states of [Fe II Cp 2 Co III Cp 2 ] + are valence-localized, while the intermediate-spin state is partially delocalized. The differences in charge delocalization are attributed to differences in orbital occupation and geometry that affect the free energy and superexchange coupling.

Burke, John H. [Univ. of Illinois at Urbana-Champa↗
NASA NTRS1977

Dynamic modeling of coronal and interplanetary responses to solar events

Recent progress in the dynamic modeling of responses of the corona and interplanetary medium to solar events (such as surges, eruptive prominences, flares, etc.) is reviewed. In particular, coronal transients and wave phenomena are discussed in some detail including pertinent mathematical requirements. Within the context of hydrodynamics and magnetohydrodynamics, a summary of both one- and two-dimensional time-dependent models is presented. A comparison of theoretical results with ground-based optical, radio, ATM Skylab observations, Pioneer 9 and Pioneer 10 solar wind observations is also presented. It is illustrated that: (1) substantial progress has been made in the theoretical (i.e., numerical) modeling of coronal and interplanetary responses within the last few years; (2) two-dimensional, time-dependent modeling is needed to examine the details of nonlinear wave coupling; and (3) theoretical results of modeling appear to reproduce physical consequences successfully.

Wu, S. T.↗
NASA NTRS1974

An interdisciplinary study of the estuarine and coastal oceanography of Block Island Sound and adjacent New York coastal waters

The author has identified the following significant results. Photo-optical additive color quantitative measurements were made of ERTS-1 reprocessed positives of New York Bight and Block Island Sound. Regression of these data on almost simultaneous ship sample data of water's physical, chemical, biological, and optical properties showed that ERTS bands 5 and 6 can be used to predict the absolute value of the total number of particles and bands 4 and 5 to predict the relative extinction coefficient in New York Bight. Water masses and mixing patterns in Block Island Sound heretofore considered transient were found to be persistent phenomena requiring revision of existing mathematical and hydraulic models.

Yost, E. F.↗