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Development of Technology for Detachment of Calandria Tube Rolled Joint of Pressurised Heavy Water Reactors

Coolant channel assembly of PHWRs consisting mainly of pressure tube and calandria tube undergoes sag due to irradiation enhanced creep during its life time. Typical service life of the pressure tube is limited to about 15 full power years due to such ageing related degradation. On account of the degradation the pressure tube needs replacement more than twice during the licensed period of reactor operation. As the sag in the calandria tube is also excessive, it has to be replaced to facilitate installation of new and straight pressure tube during retubing and to avoid interference of sagged calandria tube with horizontal reactivity devices. The calandria tube and the tube sheet are joined by sandwich type rolled joints. For detaching the joint an improved technique has been developed that helps to detach the joint without affecting the groove geometry and integrity of the tube sheet. The system works on the principle of fast thermal cycle of heating and cooling of the insert and calandria tube in the rolled joint region while applying axial load to the calandria tube. Though rolled joint detachment by induction heating technique has been in use in CANDU reactors for removal of pressure tubes and calandria tubes, the present design incorporates a liquid nitrogen for faster cooling and simultaneous application of load with a gripping module for detachment and removal of calandria tube and the insert from the tube sheet of end shield in shorter time. This paper describes the methodology of rolled joint detachment, challenges involved in the design, features of the detachment system, findings of experimental trials and observations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

The Use of Thorium within the Nuclear Power Industry - 13472

Thorium is 3 to 4 times more abundant than uranium and is widely distributed in nature as an easily exploitable resource in many countries. Unlike natural uranium, which contains ∼0.7% fissile {sup 235}U isotope, natural thorium does not contain any fissile material and is made up of the fertile {sup 232}Th isotope only. Therefore thorium and thorium-based fuel as metal, oxide or carbide, has been utilized in combination with fissile {sup 235}U or {sup 239}Pu in nuclear research and power reactors for conversion to fissile {sup 233}U, thereby enlarging fissile material resources. During the pioneering years of nuclear energy, from the mid 1950's to mid 1970's, there was considerable interest worldwide to develop thorium fuels and fuel cycles in order to supplement uranium reserves. Thorium fuels and fuel cycles are particularly relevant to countries having large thorium deposits but very limited uranium reserves for their long term nuclear power programme. The feasibility of thorium utilization in high temperature gas cooled reactors (HTGR), light water reactors (LWR), pressurized heavy water reactors (PHWRs), liquid metal cooled fast breeder reactors (LMFBR) and molten salt breeder reactors (MSBR) were demonstrated. The initial enthusiasm for thorium fuels and fuel cycles was not sustained among the developing countries later, due to new discovery of uranium deposits and their improved availability. However, in recent times, the need for proliferation-resistance, longer fuel cycles, higher burnup, and improved waste form characteristics, reduction of plutonium inventories and in situ use of bred-in fissile material has led to renewed interest in thorium-based fuels and fuel cycles. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Application of SPH Factors to PHWR Lattice Homogenization

Pressurized Heavy-Water Reactors (PHWRs) are heavy-water moderated and cooled. They consist of a horizontal, cylindrical, non-pressurized calandria vessel which contains the heavy-water moderator and is penetrated axially by fuel channels. Fuel channels consist of two concentric tubes separated by a gas gap: an inner tube called the pressure tube, and an outer tube called the calandria tube. The pressure tubes hold the fuel bundles, which are cooled by the flow of coolant at high temperature and pressure. The coolant flows in opposite directions in adjacent channels. The gap between the pressure and calandria tubes ensures that the temperature of the moderator remains relatively low, below 80 deg. C. For a CANDU 6 reactor, there are 380 fuel channels, each holding 12 37-element fuel bundles, approximately 10-cm in diameter and 50-cm long each. The fuel pins are arranged in three concentric rings (consisting of 6, 12 and 18 pins respectively), plus a central pin. The distance between channels (lattice pitch) is approximately 28.6 cm. Production core-level neutronics calculations are usually performed in a Cartesian geometry using few group diffusion and a simplified core model, whereby neutronics properties are homogenized over large regions called nodes. For Light Water reactors (LWRs), the two-dimensional axial (x-y) projection of a node corresponds to one fuel assembly. For PHWRs, a node usually consists of one fuel bundle and its associated moderator. For LWRs, advanced core-level calculations based on advanced node-level homogenization methods, such as Generalized Equivalence Theory (GET) or Super-homogenisation (SPH), improve the accuracy of full-core calculations compared to - standard homogenization. For rectangular fuel-pin arrangements, SPH can be used to perform pin-cell level homogenization which allows subsequent core-level diffusion calculations to be performed using fine Cartesian meshes. For PHWRs, the distribution of fuel pins in concentric rings makes the use of Cartesian mesh refinement impractical. However, SPH can still be applied, albeit using a coarser node subdivision, by dividing the heterogeneous node into 3x3 sub-regions in such a way that the central sub-region includes the entire fuel channel. This work investigates the use of SPH homogenization using a 3x3 subdivision of the PHWR node. Preliminary results show that the use of SPH factors does not yield more accurate results than standard homogenization when applied to PHWR nodes using a 3x3 subdivision. The explanation appears to lie in the fact that SPH factors are dependent on node-boundary leakage. Future investigations to confirm the leakage-dependence of SPH factors are recommended. Accuracy improvements may also be achievable by using smaller SPH regions at the periphery of the PHWR node, in an attempt to reduce the SPH factors' dependence on node-boundary leakage. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Methodology and Software for Gross Defect Detection of Spent Nuclear Fuel at the Atucha-I Reactor [Novel Methodology and Software for Spent Fuel Gross Defect Detection at the Atucha-I Reactor]

Here, fuel assemblies in the spent fuel pool are stored by suspending them in two vertically stacked layers at the Atucha Unit 1 nuclear power plant (Atucha-I). This introduces the unique problem of verifying the presence of fuel in either layer without physically moving the fuel assemblies. Given that the facility uses both natural uranium and slightly enriched uranium at 0.85 wt% 235 U and has been in operation since 1974, a wide range of burnups and cooling times can exist in any given pool. A gross defect detection tool, the spent fuel neutron counter (SFNC), has been used at the site to verify the presence of fuel up to burnups of 8000 MWd/t. At higher discharge burnups, the existing signal processing software of the tool was found to fail due to nonlinearity of the source term with burnup.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Solidification technology for organic liquid waste combined with solid materials from Cernavoda NPP, Romania - 16453

Canadian Deuterium Uranium (CANDU{sup R}) reactor designs were initially developed in the late 1950's and 1960's by the Atomic Energy of Canada Limited (AECL) in partnership with Ontario Power Generation. CANDU{sup R} 6 reactors are Pressurized Heavy Water Reactors (PHWRs), with an integrated containment system and are designed as either multi or single unit systems. Two single CANDU 6 systems are currently operating at Cernavoda with an additional two units expected to be brought online in the near future. The radioactive waste produced by the plant is currently stored in a waste interim storage facility located on-site. The main sources of radioactive waste in a CANDU plant are: - Primary Heat Transport (PHT) systems, - Moderator systems, - Other sources of radionuclides. The radioactive waste management system at Cernavoda Nuclear Power Plant (NPP) was designed to maintain acceptable levels of safety for workers and to protect human health and the environment from exposure to unacceptable levels of radiation. During the operation of the Cernavoda NPP, a series of waste streams have been generated for waste treatment purposes. One important waste stream is the combination of solid materials and liquid organic waste, creating flammable solids. Flammable solids represent solid materials, such as cloth, plastic, contaminated with oil containing gamma nuclides and H-3 from maintenance activities. This paper explores a method to solve the problem of liquid residues on solid materials by the application of absorbent materials. The existence of liquid residues on solid materials is a common problem at nuclear power stations globally. The primary issue centers on an effective method of eliminating the liquid to allow for the final acceptance and disposal of the solid waste by regulators. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Development of an internally cooled annular fuel bundle for pressurized heavy water reactors

A number of preliminary studies have been conducted at Atomic Energy of Canada Limited to explore the potential of using internally cooled annular fuel (ICAF) in CANDU reactors including finite element thermo-mechanical modelling, reactor physics, thermal hydraulics, fabrication and mechanical design. The most compelling argument for this design compared to the conventional solid-rod design is the significant reduction in maximum fuel temperature for equivalent LERs (linear element ratings). This feature presents the potential for power up-rating or higher burnup and a decreased defect probability due to in-core power increases. The thermal-mechanical evaluation confirmed the significant reduction in maximum fuel temperatures for ICAF fuel compared to solid-rod fuel for equivalent LER. The maximum fuel temperature increase as a function of LER increase is also significantly less for ICAF fuel. As a result, the sheath stress induced by an equivalent power increase is approximately six times less for ICAF fuel than solid-rod fuel. This suggests that the power-increase thresholds to failure (due to stress-corrosion cracking) for ICAF fuel should be well above those for solid-rod fuel, providing improvement in operation flexibility and safety.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Imminent: Irradiation Testing of (Th,Pu)O{sub 2} Fuel - 13560

Commercial-prototype thorium-plutonium oxide (Th-MOX) fuel pellets have been loaded into the material test reactor in Halden, Norway. The fuel is being operated at full power - with instrumentation - in simulated LWR / PHWR conditions and its behaviour is measured 'on-line' as it operates to high burn-up. This is a vital test on the commercialization pathway for this robust new thoria-based fuel. The performance data that is collected will support a fuel modeling effort to support its safety qualification. Several different samples of Th-MOX fuel will be tested, thereby collecting information on ceramic behaviours and their microstructure dependency. The fuel-cycle reasoning underpinning the test campaign is that commercial Th- MOX fuels are an achievable intermediate / near-term SNF management strategy that integrates well with a fast reactor future. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Economic Module Development for the Fuel Cycle Simulation Tool CLASS

An economical module to calculate the financial aspect of nuclear industry was developed based on CLASS, a library used for performing dynamic fuel cycle simulations. The tool will be introduced and a simple case of a PWR reactor will be presented to validate the module looking forward to evaluate a symbiotic scenario in the full paper involving UOX reactors, MOX reactors for recycling the plutonium and PHWR reactors for recycling the uranium.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Is spent nuclear fuel immune from delayed hydride cracking during dry storage? An IAEA coordinated research project - 2016-0048

Delayed hydride cracking (DHC) has been responsible for cracking in zirconium alloy pressure tubes and fuel cladding and is a concern for spent fuel storage. For cracking to start, sufficient hydrogen must be present for hydride to form at a flaw tip and the local tensile stress must be sufficiently large to crack the hydride (a crack will not extend if the threshold in the stress intensity factor, K{sub IH}, is not exceeded. A high-temperature limit exists when the yield stress of the cladding alloy becomes too low to crack the hydride. In this paper we describe measurements of K{sub IH} and the crack growth rate, V, in unirradiated Zircaloy-4 fuel cladding containing approximately 130 ppm hydrogen in the cold-worked stress-relieved condition representing pressurized water reactors (PWRs) and pressurized heavy-water (PHWR) reactors. Four methods are used to evaluate K{sub IH}. The test specimen and fixture used in these methods was the pin-loading tension configuration. The test temperature ranged from 227 to 315 deg. C. The mean value of K{sub IH} below 280 deg. C had little temperature dependence; it was about 5.5 MPa√m in the PWR cladding and slightly higher at 7 MPa√m in the PHWR material. At higher test temperatures, K{sub IH} increased dramatically to more than 12 MPa√m, whereas the crack growth rate declined toward zero. This behavior suggests that unirradiated Zircaloy-4 fuel cladding is immune from DHC above about 320 deg. C; this temperature may be increased to 360 deg. C by irradiation. The implications for spent fuel storage are that during early storage when the temperatures are high, any flaw will not extend by DHC, whereas at low temperatures, after many years of storage, flaws would have to be very large, approaching through wall, before being extended by DHC. To date, spent nuclear fuel is not known to have failed by DHC during storage, confirming the inference. (authors)

36 MATERIALS SCIENCE↗

Condition-Based Maintenance of a Circulating Water System of a Canadian Nuclear Power Plant using Machine Learning and Statistical Tools

Canada Deuterium Uranium pressurized-heavy-water reactors (PHWR) are a type of nuclear power plant that generate clean and reliable energy. The scope of this work is to automate data analysis methodologies to inform a condition-based maintenance strategy of a circulating water system (CWS) of a PHWR. The multiunit CWS provides a continuous supply of water to cool steam condensers, even during transient scenarios, thereby improving the thermal efficiency. This work aims to develop a machine learning (ML) based approach to detect anomalies in heterogeneous data of a CWS in a PHWR to help inform a predictive maintenance strategy. The heterogeneous data include textual and numeric time series data for a PHWR. Natural-language-processing (NLP)-based models are used to analyze textual data contained in work orders and operator logs and an event-timeseries correlation detection method is applied to assist anomalies diagnoses for CWS. An ML model Robust Linear Model (RLM) is also used to remove the seasonal variations in the system variable distributions based on distributions of environmental variables. A machine learning model, Density-Based Spatial Clustering of Applications with Noise (DBSCAN), trained on both original data and data without any seasonal variations will then be used to detect if an anomaly exists. Thus, by moving to an automated methodology to detect, classify, and forecast anomalies, the maintenance strategy would be based on component condition instead of a time-based schedule.

97 - MATHEMATICS AND COMPUTING↗

Development of the computer code for multi-calculations of source term of spent fuel - 15351

Many PWR spent fuels have been transferred between the neighboring nuclear power plants at Kori, Hanbit, Hanwul site, and from nuclear power plant to the KAERI(Korea Atomic Energy Research Institute) for the research purpose in Korea. In case of the PHWR type spent fuels, these have been transferred from the spent fuel pool to an on-site dry storage facility. Total radioactivity of spent fuels has to be calculated before transport in advance by the regulation requirement. In case of PWR, KN-12 transport cask can transfer 12 spent fuel assemblies at one time and in case of PHWR, Hi-STAR 63 transport cask can transfer 120 spent fuel assemblies at one time. Therefore, total radioactivity of all transported spent fuel assemblies that are transported generally are calculated by using the ORIGEN-ARP to meet this regulatory requirement. Basically, ORIGEN-ARP calculates the one fuel assembly at one time. SCALE code including this code provides the batch mode to perform the multi-calculations of the source term. In this study, in order to use the batch mode of ORIGEN-ARP, ARP-auto program was developed to generate input files and batch file of ORIGEN-ARP automatically and to make the summary file extracting the result from output files of ORIGEN-ARP. This code enhances the efficiency at the field. The working time to complete the calculation of source terms of 120 spent fuel assemblies take only 20 minutes. In order to confirm the credibility of this code, total radioactivity of 12 spent fuel assemblies of 17x17 Westinghouse type were calculated and compared to the previous result. The initial enrichments of these spent fuels are 3.46 ∼ 3.50 w/o and burnups are 29 ∼ 43 GWD/MTU. As the results, the relative errors are about 0.9 ∼ 3.0%. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

ORIGEN-based Nuclear Fuel Inventory Module for Fuel Cycle Assessment: Final Project Report

The goal of this project, “ORIGEN-based Nuclear Fuel Depletion Module for Fuel Cycle Assessment" is to create a physics-based reactor depletion and decay module for the Cyclus nuclear fuel cycle simulator in order to assess nuclear fuel inventories over a broad space of reactor operating conditions. The overall goal of this approach is to facilitate evaluations of nuclear fuel inventories for a broad space of scenarios, including extended used nuclear fuel storage and cascading impacts on fuel cycle options such as actinide recovery in used nuclear fuel, particularly for multiple recycle scenarios. The advantages of a physics-based approach (compared to a recipe-based approach which has been typically employed for fuel cycle simulators) is in its inherent flexibility; such an approach can more readily accommodate the broad space of potential isotopic vectors that may be encountered under advanced fuel cycle options. In order to develop this flexible reactor analysis capability, we are leveraging the Origen nuclear fuel depletion and decay module from SCALE to produce a standalone “depletion engine” which will serve as the kernel of a Cyclus-based reactor analysis module. The ORIGEN depletion module is a rigorously benchmarked and extensively validated tool for nuclear fuel analysis and thus its incorporation into the Cyclus framework can bring these capabilities to bear on the problem of evaluating long-term impacts of fuel cycle option choices on relevant metrics of interest, including materials inventories and availability (for multiple recycle scenarios), long-term waste management and repository impacts, etc. Developing this Origen-based analysis capability for Cyclus requires the refinement of the Origen analysis sequence to the point where it can reasonably be compiled as a standalone sequence outside of SCALE; i.e., wherein all of the computational aspects of Origen (including reactor cross-section library processing and interpolation, input and output processing, and depletion/decay solvers) can be self-contained into a single executable sequence. Further, to embed this capability into other software environments (such as the Cyclus fuel cycle simulator) requires that Origen’s capabilities be encapsulated into a portable, self-contained library which other codes can then call directly through function calls, thereby directly accessing the solver and data processing capabilities of Origen. Additional components relevant to this work include modernization of the reactor data libraries used by Origen for conducting nuclear fuel depletion calculations. This work has included the development of new fuel assembly lattices not previously available (such as for CANDU heavy-water reactor assemblies) as well as validation of updated lattices for light-water reactors updated to employ modern nuclear data evaluations. The CyBORG reactor analysis module as-developed under this workscope is fully capable of dynamic calculation of depleted fuel compositions from all commercial U.S. reactor assembly types as well as a number of international fuel types, including MOX, VVER, MAGNOX, and PHWR CANDU fuel assemblies. In addition, the Origen-based depletion engine allows for CyBORG to evaluate novel fuel assembly and reactor design types via creation of Origen reactor data libraries via SCALE. The establishment of this new modeling capability affords fuel cycle modelers a substantially improved ability to model dynamically-changing fuel cycle and reactor conditions, including recycled fuel compositions from fuel cycle scenarios involving material recycle into thermal-spectrum systems.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advanced Fuel Cycle Cost Basis Report: Module D1-7 Contact-Handled Pelletized Pressurized Heavy Water (PHWR) UOX Fuel Fabrication (Rev.1)

In addition to literature-based pressurized heavy-water reactor (PHWR) fuel price information in the 2017 AFC-CBR, the what-it-takes (WIT) unit cost data in this update is informed by new analysis and escalation of the 1978 PHWR-UOX fuel life cycle cost (LCC) data from ORNL reports prepared for the 1977–1980 Nonproliferation Alternative Systems Assessment Program (NASAP). (These reports are referenced and summarized in detail in Module D1-PR.) The PHWR fuel fabrication LCC data in these reports is scaled from a bottom-up cost estimate for a reference technology pressurized-water reactor (PWR)—uranium oxide (UOX) fuel fabrication plant by using algorithms that consider the manufacturing process complexity, fuel design complexity, plant floor space requirements, and the radiation and health, safety, and environmental (HS&E) regulatory environment of PHWR-UOX fuel production vis-à-vis light-water reactor (LWR)-UOX production (PWR fuel in this case). The module name has been changed from “Canadian Deuterium Uranium (CANDU)” to the more generic PHWR fuel fabrication in recognition that not all power reactors that might use this fuel type are considered. Unfortunately, the detailed algorithms and their design bases were not archived at the end of the NASAP effort of the commercial CANDU concept specifically developed in the middle of the last century by Atomic Energy of Canada Limited (AECL).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗