Population inversion and giant bandgap renormalization in atomically thin WS2 layers
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Chernikov, Alexey↗
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Pumping Wavelength Related Population Inversion in Nd:doped Laser
Pumping wavelength related population inversion in Nd:doped laser has been investigated, where the laser is regarded as two thermodynamic equilibrium systems, upper state one and lower state one. The population inversion limits at various pumping wavelengths and temperatures are compared. The effective metastable life time has been derived, where both pump and laser fields within Nd:doped laser medium reduce the lifetime. The saturation of lifetime is discussed. As a result, in-band pumping of Nd: doped laser is good for improving the efficiency and achieving narrow-linewidth of laser wavelength due to less population inversion; off-band pumping is benefit for extracting high pulse energy thanks of large population inversion.
optical Parametric Oscillator↗
Intersubband Auger recombination and population inversion in quantum-well subbands
The intersubband-Auger-recombination time of electrons under population-inversion conditions in a single quantum well is calculated by taking into account momentum- and energy-conservation rules, and by employing Fermi-Dirac statistics. The screened matrix element of the electron-electron interaction and the overlap integral are calculated for an infinitely deep quantum well. The results are in a good agreement with published experimental data. As a major nonradiative process, the Auger recombination is related to threshold current of infrared lasers based on intersubband transitions in quantum-well structures. The realization of these devices and other limitations to achieving population inversion are discussed. In view of the results, development of these lasers for emission wavelengths corresponding to energies below the LO-phonon energy seems feasible.
Borenstain, S.↗
Population inversions in ions of astrophysical interest
Atomic configurations population inversions of astrophysical interest, assuming excitation by electron collisions, solving rate equations for level populations by computer
Smith, H. A.↗
Theoretical population inversion in a decaying nitrogen plasma column.
Theoretical population inversion in decaying nitrogen plasma column free from external fields and confined motionless in circular cylinder
Park, C.↗
Population inversion by chirped pulses
In this paper, we analyze the condition for complete population inversion by a chirped pulse over a finite duration. The nonadiabatic transition probability is mapped in the two-dimensional parameter space of coupling strength and detuning amplitude. Asymptotic forms of the probability are derived by the interference of nonadiabatic transitions for sinusoidal and triangular pulses. The qualitative difference between the maps for the two types of pulses is accounted for. The map is used for the design of stable inversion pulses under specific accuracy thresholds.
74 ATOMIC AND MOLECULAR PHYSICS↗
On the propagation of a light pulse in the “transparency window” of a medium with population inversion
The propagation of a light pulse through a layer of a substance with population inversion and, correspondingly, with an anomalous dispersion in the transparency range is considered. It is shown that, when the wave packet approaches the layer of the substance with a strong anomalous dispersion, two additional wave packets arise at the rear boundary of the layer. One of these packets has a negative energy and moves in the layer from its rear to the front boundary, while the other packet moves away from the rear boundary of the layer into a vacuum. As the initial wave packet comes into contact with the front boundary of the layer of the substance, it meets the packet of the negative energy. As a result, the two packets annihilate one another, after which only one packet remains, which moves away from the layer.
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
GaAs-laser-induced population inversion in the ground-state hyperfine levels of Cs133
Population inversion in Cs133 ground state hyperfine levels, using CW GaAs laser at 77 K for optical pumping
Alley, C. O.↗
Negative terahertz conductivity in disordered graphene bilayers with population inversion
The gapless energy band spectra make the structures based on graphene and graphene bilayer with the population inversion to be promising media for the interband terahertz (THz) lasing. However, a strong intraband absorption at THz frequencies still poses a challenge for efficient THz lasing. In this paper, we show that in the pumped graphene bilayer, the indirect interband radiative transitions accompanied by scattering of carriers by disorder can provide a substantial negative contribution to the THz conductivity (together with the direct interband transitions). In the graphene bilayer on high-κ substrates with point charged defects, these transitions substantially compensate the losses due to the intraband (Drude) absorption. We also demonstrate that the indirect interband contribution to the THz conductivity in a graphene bilayer with the extended defects (such as the charged impurity clusters) can surpass by several times the fundamental limit associated with the direct interband transitions, and the Drude conductivity as well. These predictions can affect the strategy of the graphene-based THz laser implementation.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Supersonically expanded sodium metal-dilute halogen gas interactions. The importance of reaction populated and energy storing reservoir states and population inversion created amplification in Na2
The reactions of Cl, Br, and I with Nan=2,3 produced in a supersonic expansion form Na2* and Na* excited states extending across the visible and ultraviolet regions. Emission in the region extending from 410 to 600 nm indicates selectively formed excited state Na2 emission features. Experimental evidence suggests that this emission is associated with Na3 + X reactions. Broadband (0.5 cm−1) laser measurements demonstrate gain (population inversion) for select features at∼524–528(1%), ∼492(0.3%), and ∼458.7–461(0.8%) nm. Single mode (0.007 cm−1) measurements extending from 528.03 to 527.63 nm demonstrate amplification involving five to six individual rovibronic levels with a maximum gain close to 3% recorded at 527.9 nm. The observed gain is associated with select transitions from levels of the Na2 11Πu state populated, via identified curve crossings, through collision induced transfer from long-lived Na2 21Σg+ and 11Πg reservoir states. Collision induced population buildup in the lowest vibrational levels of these reservoir states and collision induced transfer to the Na2 11Πu state create a population inversion in transitions to the X 1Σg+ state of Na2. The observed amplification is aided by rapid vibrational and rotational relaxation in both the Na2 ground and excited reservoir states producing amplifiers in the visible region like the HF amplifier in the infrared. This study suggests the importance of reaction populated and energy storing long-lived reservoir states in small sodium molecule combustion processes and indicates the potential for providing new short wavelength visible and ultraviolet amplifiers for future laser-based chemical propulsion concepts.
Chemistry↗
On the Intracenter Relaxation of Shallow Arsenic Donors in Stressed Germanium. Population Inversion under Optical Excitation
The relaxation rates of lower excited states 1s(T), 2p{sub 0}, 2s, 3p{sub 0}, and 2p{sub ±} of arsenic donors in a germanium crystal are calculated upon the interaction with long-wavelength acoustic phonons depending on the uniaxial stress in the crystallographic direction [111]. The populations of states under optical excitation are estimated for calculated times. It is shown theoretically that optical excitation of the medium forms an inverse population of arsenic donor levels and leads to the possibility of the implementation of a four-level laser scheme with the radiative transition between 2p states and the 1s triplet state at zero strain. The estimated value of the expected gain in the medium under optical excitation conditions by CO{sub 2} laser radiation in the medium at a donor concentration of 2 × 10{sup 15} cm{sup –3} is ~0.35 cm{sup –1} at a frequency of 1.98 THz if the laser transition is 2p{sub ±} → 1s(T) and 1.25 THz if the laser transition is 2p{sub 0} → 1s(T).
36 MATERIALS SCIENCE↗
Mid-infrared pump-related electric-field domains in GaAs/(Al,Ga)As quantum-cascade structures for terahertz lasing without population inversion
We investigate the effect of mid-infrared (MIR) pumping on the transport properties of GaAs/(Al,Ga)As terahertz (THz) quantum lasers (TQLs), which rely on quantum coherence effects of intersubband transitions. Aiming at THz lasing at elevated temperatures, we extend the concept of THz gain with and without population inversion of a single, MIR-pumped, electrically driven THz stage proposed by Waldmueller et al.[Phys. Rev. Lett. 99, 117401 (2007)] to an entire TQL. However, experiments using a CO{sub 2} as well as a free-electron laser and numerical simulations show that this resonant MIR pumping causes a negative differential conductivity (NDC) in addition to the NDC caused by sequential tunneling. Lasing of these TQLs is prevented by the formation of electric-field domains below the resonance field strength for gain of each single THz stage.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Population inversion of A. U. V. atomic line in recombining plasma nozzle flow
Arc heated plasma expansion through nozzle, observing population inversion of neutral carbon self-absorption UV atomic line
Bowen, S. W.↗
Functional possibilities for forming different inverse population distributions in diode-side-pumped laser heads
The functional possibilities of diode-side-pumped laser heads of solid-state lasers for forming inverse population distributions of different types are analysed. The invariants determining the relationship between the laser head parameters upon scaling are found. The results of comparative experimental studies are presented. (lasers)
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Population inversion calculations using near resonant charge exchange as a pumping mechanism
Near resonance charge exchange between ions of a large ionization potential gas such as helium or neon and vapors of metals such as zinc, cadmium, selenium, or tellurium has produced laser action in the metal ion gas. The possibility of obtaining population inversions in near resonant charge exchange systems (Xe-Ca, Xe-Mg, Xe-Sr, Xe-Ba, Ar-Mg, N-Ca) was investigated. The analysis is an initial value problem that utilizes rate equations for the densities of relevant levels of the laser gas (Ca, Ba, Mg, or Sr) and an electron energy equation. Electron excitation rates are calculated using the Bohr-Thomson approximation for the cross section. Approximations to experimental values of the electron ionization cross section and the ion-atom charge exchange cross section are used. Preliminary results have been obtained for the Ca-Xe system and show that it is possible to obtain gains greater than 10 to the 14th power/m with inversion times up to 8x10 to the minus 7th power second. A possible charge exchange laser system using a MPD arc plasma accelerator is also described.
Chubb, D. L.↗
Long-Lived Population Inversion in Resonantly Driven Excitonic Antiferromagnet
Van der Waals magnets are an emerging material family for investigating light-matter interactions and spin-correlated excitations. Here, we report the discovery of a photo-induced state with a lifetime of 17 ps in the van der Waals antiferromagnet NiPS 3 , which appears exclusively with resonant pumping at 1.476 eV in the antiferromagnetic state. Furthermore, the long-lived state comes with a negative photoconductivity, a characteristic optical response of population inversion. Our findings demonstrate a promising pathway to potentially achieve long-lived lasing at terahertz frequencies in reduced dimensions.
36 MATERIALS SCIENCE↗
Quantum mechanical calculations of vibrational population inversion in chemical reactions - Numerically exact L-squared-amplitude-density study of the H2Br reactive system
Numerically exact, fully three-dimensional quantum mechanicl reactive scattering calculations are reported for the H2Br system. Both the exchange (H + H-prime Br to H-prime + HBr) and abstraction (H + HBR to H2 + Br) reaction channels are included in the calculations. The present results are the first completely converged three-dimensional quantum calculations for a system involving a highly exoergic reaction channel (the abstraction process). It is found that the production of vibrationally hot H2 in the abstraction reaction, and hence the extent of population inversion in the products, is a sensitive function of initial HBr rotational state and collision energy.
Zhang, Y. C.↗