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At least 19 records

ZPR/ZPPR Critical Experiment Facilities and As-Built ZPR/ZPPR Models

Argonne National Laboratory (ANL) operated four split-table critical experiment facilities, ZPR 3, ZPR-6, ZPR-9 and ZPPR, between 1955 and 1990. ZPR is the abbreviation for Zero Power Reactor, and ZPPR was the abbreviation for Zero Power Plutonium Reactor which was changed to Zero Power Physics Reactor in the 1980s due to negative views on Plutonium breeding and proliferation concerns. ZPR-3, ZPR-6, ZPR-9 and ZPPR were four reactors in a series of zero power (or lower power reactors) designed at Argonne in the 1950s and 1960s.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Advanced Lithium Ion Venus Explorer (ALIVE)

The COncurrent Multidisciplinary Preliminary Assessment of Space Systems (COMPASS) Team partnered with the Applied Research Laboratory to perform a NASA Innovative Advanced Concepts (NIAC) Program study to evaluate chemical based power systems for keeping a Venus lander alive (power and cooling) and functional for a period of days. The mission class targeted was either a Discovery ($500M) or New Frontiers ($750M to $780M) class mission. Historic Soviet Venus landers have only lasted on the order of 2 hours in the extreme Venus environment:temperatures of 460 degrees Centigrade and pressures of 93 bar. Longer duration missions have been studied using plutonium powered systems to operate and cool landers for up to a year. However, the plutonium load is very large. This NIAC study sought to still provide power and cooling but without the plutonium. Batteries are far too heavy but a system which uses the atmosphere (primarily carbon dioxide) and on on-board fuel to power a power generation and cooling system was sought. The resuling design was the Advanced Long-Life Lander Investigating the Venus Environment (ALIVE) Spacecraft (S/C) which burns lithium (Li) with the CO2 atmosphere to heat a Duplex Stirling to power and cool the lander for a 5-day duration (until the Li is exhausted). While it does not last years a chemical powered system surviving days eliminates the cost associated with utilizing a flyby relay S/C and allows a continuous low data rate direct to earth (DTE) link in this instance from the Ovda Regio of Venus. The five-day collection time provided by the chemical power systems also enables science personnel on earth to interact and retarget science - something not possible with an approximately 2-hour spacecraft lifetime. It also allows for contingency operations directed by the ground (reduced risk). The science package was based on that envisioned by the Venus Intrepid Tessera Lander (VITaL) Decadal Survey Study. The Li Burner within the long duration power system creates approximately 14000 W of heat. This 1300 degree Centigrade heat using Li in the bottom "ballast" tank is melted to liquid by the Venus temperature, drawn into a furnace by a wick and burned with atmospheric CO2. The Li carbonate exhaust is liquid at 1300 degrees Centigrade and being denser than Li drains into the the Li tank and solidifies. Since the exhaust product is a dense liquid no "chimney" is required which conserves the heat for the stirling power convertor. The Duplex Stirling provides about 300 W of power and removes about 300 W of heat from the avionics and heat that leaks into the 1-bar-insulated payload pressure vessel kept at 25 degrees Centigrade. The Na K radiator is run to the top of the drag flap.The ALIVE vehicle is carried to Venus via an Atlas 411 launch vehicle (LV) with a C3 of 7 km2/s2. An Aeroshell, derived from the Genesis mission, enables a direct entry into the atmosphere of Venus (-10 degrees Centigrade, 40 g max) and 6 m/s for landing (44 g) using a drag ring. For surface science and communication, a 100 WRF (WebEx Recording Format), X-Band 0.6-meter pointable DTE (Direct-to-Earth) antenna provides 2 kbps (kilobits per second) to DSN (Deep-Space Network) 34-meter antenna clusters.Table 1.1 summarizes the top-level details of each subsystem that was incorporated into the design. Cost estimates of the ALIVE mission show it at approximately $760M which puts it into the New Frontiers class.The ALIVE landed duration is only limited by the amount of Li which can be carried by the lander. Further studies are needed to investigate how additional mass can be carried, perhaps by a larger launcher and larger aeroshell.

Exploration↗

COMPASS Final Report: Advanced Long-Life Lander Investigating the Venus Environment (ALIVE)

The COncurrent Multi-disciplinary Preliminary Assessment of Space Systems (COMPASS) Team partnered with the Applied Research Laboratory to perform a NASA Innovative Advanced Concepts (NIAC) Program study to evaluate chemical based power systems for keeping a Venus lander alive(power and cooling) and functional for a period of days. The mission class targeted was either a Discovery ($500M) or New Frontiers ($750M to $780M) class mission. Historic Soviet Venus landers have only lasted on the order of 2 hours in the extreme Venus environment: temperatures of 460 C and pressures of 93 bar. Longer duration missions have been studied using plutonium powered systems to operate and cool landers for up to a year. However, the plutonium load is very large. This NIAC study sought to still provide power and cooling but without the plutonium.

COMPASS↗

Gamma Dose Measurements in ZPPR-15

Gamma doses were measured in the Zero Power Plutonium Reactor (ZPPR) to provide data for validation of calculations of gamma heating in important reactor components. Stainless steel-encapsulated LiF thermoluminescent dosimeters (TLDs) were irradiated in two configurations in ZPPR-15B and one configuration in ZPPR-15D to provide gamma heating data for the Integral Fast Reactor design in the mid-1980s. The ZPPR-15 experimental records were used to develop detailed as-built Monte Carlo models for the gamma dose measurements in ZPPR-15B and ZPPR-15D. These Monte Carlo models can be converted to deterministic models for calculations with deterministic codes. The reported uncertainty in the published gamma dose measurements is just the statistical uncertainty in the TLD readout. In addition to this statistical uncertainty in the TLD readout, several corrections and other factors contribute to the total uncertainty for the gamma dose measurements. The total uncertainty for the gamma dose measurements can be significantly larger than the published statistical uncertainty for the TLD readout. All known contributions to the total uncertainty were analyzed, and a total uncertainty was derived for the ZPPR-15 gamma dose measurements.

36 MATERIALS SCIENCE↗

Some neutron and gamma radiation characteristics of plutonium cermet fuel for isotopic power sources

Gamma and neutron measurements on various types of plutonium sources are presented in order to show the effects of O-17, O-18 F-19, Pu-236, age of the fuel, and size of the source on the gamma and neutron spectra. Analysis of the radiation measurements shows that fluorine is the main contributor to the neutron yields from present plutonium-molybdenum cermet fuel, while both fluorine and Pu-236 daughters contribute significantly to the gamma ray intensities.

Neff, R. A.↗

Integral Experiment Execution of Thermal or Epithermal eXperiments using Plutonium with Polyethylene and Iron, IER 519, TEX-Hanford (-Iron), CED-3b

This report documents the execution of experiments and measurements for IER 519, Thermal/Epithermal eXperiments (TEX) for Hanford applications, using plutonium Zero Power Physics Reactor (ZPPR) plates moderated by interstitial polyethylene and iron (Fe) absorber plates. Initial hand stack, mass, and dimensional measurements were performed in July 2025. The experiments were completed over three weeks from December 2025 to January 2026 at the National Criticality Experiments Research Center (NCERC) at the Nevada National Security Sites (NNSS). All photos and critical data were provided by NCERC and experimenters in LANL’s NEN-2.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Data Testing of Polyethylene Thermal Scattering Law with New Thermal Epithermal eXperiments (TEX) Plutonium Baseline Benchmark, PU-MET-MIXED-002

Five plutonium baseline experiments completed in September of 2018 from the Thermal Epithermal eXperiments (TEX) program have been accepted by the International Criticality Safety Benchmark Evaluation Project as PU-MET-MIXED-002 and will be included in the 2020 version of the handbook. The experiments were made up of stacked layers of plutonium Zero Power Physics Reactor (ZPPR) plates moderated by polyethylene (PE, chemical formula C2H4) to varying degrees to create configurations with five different neutron spectra, including one fast configuration, one thermal configuration, and three mixed configurations. Calculations of the benchmark show overprediction of k eff when using the most recent release of the Evaluated Nuclear Data File Version B (ENDF/B) library release (VIII.0) cross sections, particularly when compared to the previous ENDF/B-VII.1 results. One potential source of overprediction was hypothesized to be the new Molecular Dynamics (MD) generated PE Thermal Scattering Law (TSL). The overprediction was shown via calculation to not be caused by the new ENDF/B-VIII.0 thermal scattering law, and in fact the overprediction was mitigated by the new PE TSL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

IER 519 Experiment Execution Report: TEX Hanford

The TEX-Hanford experiments were performed at the National Criticality Experiments Research Center (NCERC) at the Device Assembly Facility (DAF) at the Nevada Nuclear Security Site (NNSS). Three configurations were measured, with the measurements occurring in December 2025 and January 2026. The Fe-14 configuration was executed in December 2025; the Fe-11 configuration began its handstack on the Planet critical assembly machine in December 2025, but was taken critical in January 2026; the Fe-16 configuration was executed entirely in January 2026. The TEX-Hanford experiments were performed on the Planet critical assembly machine utilizing using PANN (Plutonium Aluminum No Nickel) ZPPR (Zero Power Physics Reactor) plutonium plates as fuel. The configurations were moderated with varying thicknesses of HDPE and iron absorber. This document details the configurations that were measured, preliminary reactivity measurements of the measured configurations, data files from the neutron detection systems, and results from the coordinate-measuring machine (CMM) measurements of the final stack height measurements each configuration.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Benchmark of the Chlorine Worth Study Experiments in Support of Chlorine Nuclear Data Validation for Nuclear Criticality Safety

The Chlorine Worth Study (CWS) was a critical experiment to address an urgent need for thermal chlorine nuclear data validation in plutonium systems. This urgent need is tied directly to plutonium recycle and recovery operations in the plutonium facility at Los Alamos National Laboratory, where exceptionally conservative criticality safety limits are used because no credit is taken for the neutron capture by chlorine. The experiment used weapons-grade plutonium metal plates clad in stainless steel, known as the PANN (plutonium aluminum no nickel) ZPPR (zero power physics reactor) plates. The plutonium was reflected and moderated by high-density polyethylene and included combinations of polyvinyl chloride (PVC) and chlorinated polyvinyl chloride (CPVC) as absorbers. The experiment and benchmark included three configurations mimicking 30 g 239 Pu/L plutonium, 300 g 239 Pu/L plutonium, and 600 g 239 Pu/L plutonium in an aqueous chloride solution. Uncertainties in the benchmark included five broad categories: (1) criticality measurement, (2) mass and density, (3) dimensions, (4) material compositions, and (5) positioning. The largest contribution to the overall uncertainties for all three cases came from the material compositions, in particular the PVC and CPVC absorber compositions. A detailed model was created to be a near match (that is within expectations of transport code users) and a simplified model was created to minimize offset dimensions and expedite modeling for code validation. Sample calculations were completed in MCNP6.3 with ENDF/B-VIII.0 and ENDF/B-VII.1 nuclear data. For the detailed and simplified models, the average difference between the computed and experimental k eff was 951 pcm. CWS will serve as the key validation experiment for nuclear criticality safety in support of aqueous chloride operations. The sensitivity to the chlorine capture cross section is orders of magnitude greater than other existing benchmarks. The current limits, as defined by nuclear criticality safety, are 520 g Pu per batch, i.e. the minimum critical mass of the Pu solution infinitely reflected by water [Criticality Handbook: Volume II, (1969)]. This extremely conservative critical mass limit does not credit any neutron capture by chlorine (in particular neutron capture by 35 Cl) and greatly impedes the throughput required for current and future operations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Reactivity Coefficient Measurements to Aid in Reducing Compensating Errors in Plutonium Nuclear Data

Compensating errors between several nuclear data observables in a nuclear data library can adversely impact application simulations. The primary goal of the EUCLID project (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) is to reduce compensating errors between fast (0.1–5 MeV) 239Pu nuclear data for prompt fission neutron spectra (PFNS), average prompt fission neutron multiplicities, and neutron induced fission, capture, elastic, and inelastic cross sections. This work will focus on the design and execution of void reactivity coefficient measurements in the EUCLID experiment, performed on the Planet vertical lift critical assembly machine at the National Criticality Experiments Research Center (NCERC). Two different base configurations were designed and measured, one with high neutron leakage, and one with low neutron leakage. Both were primarily made up of plutonium metal (Zero Power Physics Reactor plates) without interstitial moderators and reflected by half-inch aluminum. Design optimization showed that void reactivity coefficient measurements in three locations per configuration was most impactful to reduce nuclear data uncertainties due to the varying impacts from elastic and inelastic scattering, as well as fission and capture. The locations for measurements were chosen based on preliminary studies which balanced measurement uncertainty and measurement practicality. The measurements were also selected to have sensitivities maximally complementary to previous arrangements. Comparisons across nuclear data libraries highlight the potential impact.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Integral Experiment Final Design for Thermal/Epithermal eXperiments (TEX) using Highly Enriched Uranium with Polyethylene at Low Temperature (IER-479 CED-2 Report)

The goal of IER-479 is to design uranium critical experiments that can be used to validate low temperature cross sections and criticality safety analyses over multiple neutron energy regimes. Currently, there are no benchmarks in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook at temperatures lower than room temperature (International Criticality Safety Benchmark Evaluation Project Handbook, 2019). However, there are many needs for validation of criticality safety analysis at lower temperatures, including meeting transportation requirements and operations conducted outside or in unheated facilities. Additionally, NCSP has funded North Carolina State (NCSU) to generate new thermal scattering laws, including at lower temperatures, and the lack of integral benchmarks impedes data testing of these new cross sections. To address these needs, this report will present a critical experiment design covering various fission energy regimes with a goal temperature of -40°C (-40°F), which is based on the lower bound of expected non-cryogenic operational temperatures. The goal of the U.S. Nuclear Criticality Safety Program’s (NCSP) Thermal/Epithermal eXperiments (TEX) is to design and conduct new critical experiments to address high priority nuclear data needs from the nuclear criticality safety and nuclear data communities. The TEX program includes two series of baseline experimental configurations, one based on plutonium fuel (plutonium-aluminum Zero Power Physics Reactor (ZPPR) plates) and the other based on uranium fuel (highly enriched uranium (HEU) plates), that are moderated with varying thickness of polyethylene to create assemblies which span the thermal, intermediate, and fast fission energy regimes. The configurations are designed to be easily modified (for example, to add diluent materials of interest) to allow for efficient generation of additional benchmark configurations and allow for added nuclear data testing utility when comparing modified configurations to baseline configurations. The goal of IER-479 is to use the TEX-HEU concept (stack of HEU plates and polyethylene moderators) to design a critical experiment that can be used to validate low temperature cross sections and criticality safety analyses.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Microsphere Plutonium-238 Oxide Fuel to Revolutionize New Radioisotope Power Systems and Heat Sources for Planetary Exploration

Microsphere 238PuO2 fuels have potential to provide performance and safety enhancements for future radioisotope heat and power systems (RPS) as well as enable more flexible and compact RPS designs. Improvements in RPS specific power and more flexible geometries were recently investigated by JPL and PNNL as part of a study on cryobot devices for exploring Ocean Worlds. Missions to penetrate ice and explore oceans, such as on Europa, will require RPS with high specific power within the vehicle to provide both heat and power. Such missions will be mass-constrained, and the energy required to penetrate the ice is highly dependent on cryobot size. Therefore, compact RPS geometries are needed to maximize heat and power while minimizing 238Pu inventory. Microsphere-based heat sources are an attractive way to obtain flexible geometries and high volumetric power loadings because they can fill a region of any size and shape provided fuel temperatures are kept below a threshold and launch/re-entry safety are not compromised. The sol-gel technique to produce 238PuO2 microsphere particles for heat sources has the benefit of preventing dust generation, as opposed to the current 238PuO2 powder/pellet processing method, reducing hazards in the fuel fabrication line. Microspheres can also be individually coated to enhance thermal conductivity, and/or reduce the likelihood of 238PuO2 fuel dispersal in an accident. Although PNNL has produced 238PuO2 microspheres using the sol-gel method, the application of coatings and their integrity over time has yet to be investigated. Continued R&D could demonstrate the feasibility of advanced, microspherebased heat sources and provide baseline data for planning future missions requiring new RPS with different heat source configurations.

Fleurial, Jean-Pierre↗

Comparative Analysis of Thermal Conversion Technologies for Deep Space Missions

Radioisotope power systems (RPS) utilizing Plutonium-238 as a heat source for thermal-to-electric energy conversion have been used as a reliable power source for NASA’s deep space missions for sixty years. Recent innovations and improvements to thermal energy technologies show potential increases to radioisotope system efficiencies from current measurements of ~5-7% to efficiencies upwards of 20%. This report surveys and ranks recent, innovative thermal-to-electric energy conversion research technologies. Technologies being developed at universities and industry are compared with respect to thermal conversion method and relevant key performance parameters. Key performance parameters are identified as system specific power per kg, efficiency, power output, technology readiness level, and system mass. Analytical Hierarchy Process (AHP) was utilized to create weighted values for each evaluation criterion. The AHP tables combined with decision matrices create table scores for past, present, and potential future systems. The table score was combined with a conversion method score in an adjustable system to add value to flight-proven or well-tested thermal conversion technologies such as thermoelectrics. While the three highest-ranking systems reviewed are currently being developed by NASA’s RPS Program, the additional highest-ranking systems not under-development by RPS could warrant further research.

Radioisotope Power System↗

Power source considerations for Grand Tour missions.

At the present time, there exists no known power source that will satisfy the power, weight, lifetime, and other stringent requirements of an extended outer-planet mission. Exploratory studies indicate the need for a solar-independent power source capable of supplying approximately 500 W of power over mission lifetimes of up to 12 years. The only known power source which can possibly meet these requirements, in the 1975 to 1979 time period, is a radioisotope thermoelectric generator (RTG). In 1969 a program began to develop a long-life, plutonium-fueled radioisotope thermoelectric power system. Aspects of spacecraft configuration are discussed together with power source requirements, RTG/spacecraft integration, operational details, and problems of safety.

Merrill, O. S.↗

Environmental Impact Statement for the Cassini Mission

This Final Supplemental Environmental Impact Statement (FSEIS) to the 1995 Cassini mission Environmental Impact Statement (EIS) focuses on information recently made available from updated mission safety analyses. This information is pertinent to the consequence and risk analyses of potential accidents during the launch and cruise phases of the mission that were addressed in the EIS. The type of accidents evaluated are those which could potentially result in a release of plutonium dioxide from the three Radioisotope Thermoelectric Generators (RTGS) and the up to 129 Radioisotope Heater Units (RHUS) onboard the Cassini spacecraft. The RTGs use the heat of decay of plutonium dioxide to generate electric power for the spacecraft and instruments. The RHUs, each of which contains a small amount of plutonium dioxide, provide heat for controlling the thermal environment of the spacecraft and several of its instruments. The planned Cassini mission is an international cooperative effort of the National Aeronautics and Space Administration (NASA), the European Space Agency (ESA), and the Italian Space Agency (ASI) to conduct a 4-year scientific exploration of the planet Saturn, its atmosphere, moons, rings, and magnetosphere.

Source record↗

Economical Production of Pu-238: NIAC Phase I Final Report

All space exploration missions traveling beyond Jupiter must use radioisotopic power sources for electrical power. The best isotope to power these sources is plutonium-238 (Pu-238). The US supply of Pu-238 is almost exhausted and will be gone within the next decade. The Department of Energy has initiated a production program with a $10M allocation from NASA but the cost is estimated at over $100M to get to production levels. The Center for Space Nuclear Research (CSNR) has conceived of a potentially better process to produce Pu-238 earlier and for significantly less cost. Potentially, the front end capital costs could be provided by private industry such that the government only had to pay for the product produced. In the Phase I NIAC (NASA Innovative Advanced Concepts) grant, the CSNR has evaluated the feasibility of using a low power, commercially available nuclear reactor to produce 1.5 kg of Pu-238 per year. The impact on the neutronics of the reactor have been assessed, the amount of Neptunium target material estimated, and the production rates calculated. In addition, the size of the post-irradiation processing facility has been established. Finally, as the study progressed, a new method for fabricating the Pu-238 product into the form used for power sources has been identified to reduce the cost of the final product. In short, the concept appears to be viable, can produce the amount of Pu-238 needed to support the NASA missions, can be available within a few years, and will cost significantly less than the current DOE program.

Plutonium↗