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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Schottky contact formation on polar and non-polar AlN

The interfaces of m- and c-plane AlN with metals of different work functions and electro-negativities were characterized and the Schottky barrier heights were measured. The Schottky barrier height was determined by measuring the valence band maximum (VBM) with respect to the Fermi level at the surface (interface) before (after) metallization. VBM determination included accurate modeling and curve fitting of density of states at the valence band edge with the XPS data. The experimental behavior of the barrier heights could not be explained by the Schottky-Mott model and was modeled using InterFace-Induced Gap States (IFIGS). A slope parameter (S{sub X}) was used to incorporate the density of surface states and is a measure of Fermi level pinning. The experimental barriers followed theoretical predictions with a barrier height at the surface Fermi level (Charge neutrality level (CNL)) of ∼2.1 eV (∼2.7 eV) on m-plane (c-plane) and S{sub X} ∼ 0.36 eV/Miedema unit. Slope parameter much lower than 0.86 implied a surface/interface states dominated behavior with significant Fermi level pinning and the measured barrier heights were close to the CNL. Titanium and zirconium provided the lowest barriers (1.6 eV) with gold providing the highest (2.3 eV) among the metals analyzed on m-plane. It was consistently found that barrier heights decreased from metal polar to non-polar surfaces, in general, due to an increasing CNL. The data indicated that charged IFIGS compensate spontaneous polarization charge. These barrier height and slope parameter measurements provided essential information for designing Schottky diodes and other contact-based devices on AlN.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Generalized adsorption isotherms for molecular and dissociative adsorption of a polar molecular species on two polar surface geometries: Perovskite (100) (Pm-3m) and fluorite (111) (Fm-3m)

Lattice based kinetic Monte Carlo simulations have been used to determine a functional form for the second order adsorption isotherms on two commonly investigated crystal surfaces: the (111) fluorite surface and the (100) perovskite surface which has the same geometric symmetry as the NaCl (100) surface. The functional form is generalized to be applicable to all values of the equilibrium constant by a shift along the pressure axis. Functions have been determined for estimating the pressure at which a desired coverage would be achieved and, conversely, for estimating the coverage at a certain pressure. The generalized form has been calculated by investigating the surface adsorbate coverage across a range of thermodynamic equilibrium constants that span the range 10{sup −26} to 10{sup 13}. The equations have been shown to be general for any value of the adsorption equilibrium constant.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Measurements of E-mode polarization and temperature-E-MODE correlation in the cosmic microwave background from 100 square degrees of SPTPOL data

We present measurements of E-mode polarization and temperature-E-mode correlation in the cosmic microwave background using data from the first season of observations with SPTpol, the polarization-sensitive receiver currently installed on the South Pole Telescope (SPT). The observations used in this work cover 100 deg{sup 2} of sky with arcminute resolution at 150 GHz. We report the E-mode angular auto-power spectrum (EE) and the temperature-E-mode angular cross-power spectrum (TE) over the multipole range 500 < ℓ ≤ 5000. These power spectra improve on previous measurements in the high-ℓ (small-scale) regime. We fit the combination of the SPTpol power spectra, data from Planck, and previous SPT measurements with a six-parameter ΛCDM cosmological model. We find that the best-fit parameters are consistent with previous results. The improvement in high-ℓ sensitivity over previous measurements leads to a significant improvement in the limit on polarized point-source power: after masking sources brighter than 50 mJy in unpolarized flux at 150 GHz, we find a 95% confidence upper limit on unclustered point-source power in the EE spectrum of D{sub ℓ}=ℓ(ℓ+1)C{sub ℓ}/2π<0.40 μK{sup 2} at ℓ=3000, indicating that future EE measurements will not be limited by power from unclustered point sources in the multipole range ℓ<3600, and possibly much higher in ℓ.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Helicity-Selective Enhancement and Polarization Control of Attosecond High Harmonic Waveforms Driven by Bichromatic Circularly Polarized Laser Fields

High harmonics driven by two-color counter-rotating circularly-polarized laser fields are a unique source of bright, circularly-polarized, extreme ultraviolet and soft x-ray beams, where the individual harmonics themselves are completely circularly polarized. Here, we demonstrate the ability to preferentially select either the right or left circularly polarized harmonics simply by adjusting the relative intensity ratio of the bichromatic circularly polarized driving laser field. In the frequency domain, this significantly enhances the harmonic orders that rotate in the same direction as the higher intensity driving laser. In the time domain, this helicity-dependent enhancement corresponds to control over the polarization of the resulting attosecond waveforms. Here, this helicity control enables the generation of circularly-polarized high harmonics with a user-defined polarization of the underlying attosecond bursts. In the future, this technique should allow for the production of bright highly elliptical harmonic supercontinua as well as the generation of isolated elliptically polarized attosecond pulses.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2016

Intrinsic polarization control in rectangular GaN nanowire lasers

In this study, we demonstrate intrinsic, linearly polarized lasing from single GaN nanowires using cross-sectional shape control. A two-step top-down fabrication approach was employed to create straight nanowires with controllable rectangular cross-sections. A clear lasing threshold of 444kW/cm 2 and a narrow spectral line width of 0.16 nm were observed under optical pumping at room temperature, indicating the onset of lasing. The polarization was along the short dimension (y-direction) of the nanowire due to the higher transverse confinement factors for y-polarized transverse modes resulting from the rectangular nanowire cross-section. The results show that cross-sectioned shape control can enable inherent control over the polarization of nanowire lasers without additional environment requirements, such as placement onto lossy substrates.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2023

Universal Polarization Transformations: Spatial Programming of Polarization Scattering Matrices Using a Deep Learning‐Designed Diffractive Polarization Transformer

Abstract Controlled synthesis of optical fields having nonuniform polarization distributions presents a challenging task. Here, a universal polarization transformer is demonstrated that can synthesize a large set of arbitrarily‐selected, complex‐valued polarization scattering matrices between the polarization states at different positions within its input and output field‐of‐views (FOVs). This framework comprises 2D arrays of linear polarizers positioned between isotropic diffractive layers, each containing tens of thousands of diffractive features with optimizable transmission coefficients. After its deep learning‐based training, this diffractive polarization transformer can successfully implement N i N o = 10 000 different spatially‐encoded polarization scattering matrices with negligible error, where N i and N o represent the number of pixels in the input and output FOVs, respectively. This universal polarization transformation framework is experimentally validated in the terahertz spectrum by fabricating wire‐grid polarizers and integrating them with 3D‐printed diffractive layers to form a physical polarization transformer. Through this set‐up, an all‐optical polarization permutation operation of spatially‐varying polarization fields is demonstrated, and distinct spatially‐encoded polarization scattering matrices are simultaneously implemented between the input and output FOVs of a compact diffractive processor. This framework opens up new avenues for developing novel devices for universal polarization control and may find applications in, e.g., remote sensing, medical imaging, security, material inspection, and machine vision.

Optical neural networks↗
DOE OSTI2014

Studies of basic limitations on production, transport and acceleration of the high intensity polarized H{sup −} beam in the RHIC polarized ion source

Basic limitations on the high-intensity polarized H{sup −} ion beam production and transport were experimentally studied in charge-exchange collisions of the neutral atomic hydrogen beam in the Na-vaporjet ionizer cell. The energy dependence of space-charge effects on the beam instabilities and losses were studied and described in the model of synthetic H{sup +} — H{sup −} beam transport. A xenon gas admixture to the H{sup −} ion production cell and beam transport line greatly improves the space-charge compensation, which is also successfully described in the simulations. These studies are the part of the polarized source upgrade project for RHIC.

43 PARTICLE ACCELERATORS↗
DOE OSTI2019

Dual Polarity Ion Confinement and Mobility Separations

Structures for Lossless Ion Manipulations (SLIM) have been rapidly gaining prominence for applications where ultra-high resolution Ion Mobility (IM) separations are desired to provide performance features and information unattainable using the currently available IM platforms. Although most routine analyses are done in either positive or negative polarity modes, there are significant benefits to both, potentially making them highly complementary if performed simultaneously. In the effort to develop a robust dual polarity IM platform, we explored an evaluation of a novel SLIM platform developed to perform simultaneous cationic and anionic IM separations (i.e. without requiring polarity switching).

Attah, Isaac K.↗
DOE OSTI2015

Measurements of sub-degree B-mode polarization in the cosmic microwave background from 100 square degrees of SPTPOL data

We present a measurement of the B-mode polarization power spectrum (the BB spectrum) from 100 deg{sup 2} of sky observed with SPTpol, a polarization-sensitive receiver currently installed on the South Pole Telescope. The observations used in this work were taken during 2012 and early 2013 and include data in spectral bands centered at 95 and 150 GHz. We report the BB spectrum in five bins in multipole space, spanning the range 300⩽ℓ⩽2300, and for three spectral combinations: 95 GHz × 95 GHz, 95 GHz × 150 GHz, and 150 GHz × 150 GHz. We subtract small (<0.5σ in units of statistical uncertainty) biases from these spectra and account for the uncertainty in those biases. The resulting power spectra are inconsistent with zero power but consistent with predictions for the BB spectrum arising from the gravitational lensing of E-mode polarization. If we assume no other source of BB power besides lensed B modes, we determine a preference for lensed B modes of 4.9σ. After marginalizing over tensor power and foregrounds, namely, polarized emission from galactic dust and extragalactic sources, this significance is 4.3σ. Fitting for a single parameter, A{sub lens}, that multiplies the predicted lensed B-mode spectrum, and marginalizing over tensor power and foregrounds, we find A{sub lens}=1.08±0.26, indicating that our measured spectra are consistent with the signal expected from gravitational lensing. The data presented here provide the best measurement to date of the B-mode power spectrum on these angular scales.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Measurement of the absolute neutron beam polarization from a supermirror polarizer and the absolute efficiency of a neutron spin rotator for the NPDGamma experiment using a polarized 3 He neutron spin-filter

Accurately measuring the neutron beam polarization of a high flux, large area neutron beam is necessary for many neutron physics experiments. The Fundamental Neutron Physics Beamline (FnPB) at the Spallation Neutron Source (SNS) is a pulsed neutron beam that was polarized with a supermirror polarizer for the NPDGamma experiment. The polarized neutron beam had a flux of ~10 9 neutrons per second per cm 2 and a cross sectional area of 10 x 12 cm 2 . The polarization of this neutron beam and the efficiency of a RF neutron spin rotator installed downstream on this beam were measured by neutron transmission through a polarized 3 He neutron spin-filter. The pulsed nature of the SNS enabled us to employ an absolute measurement technique for both quantities which does not depend on accurate knowledge of the phase space of the neutron beam or the 3 He polarization in the spin filter and is therefore of interest for any experiments on slow neutron beams from pulsed neutron sources which require knowledge of the absolute value of the neutron polarization. The polarization and spin-reversal efficiency measured were done for the NPDGamma experiment, which measures the parity violating γ-ray angular distribution asymmetry with respect to the neutron spin direction in the capture of polarized neutrons on protons. Finally, the experimental technique, results, systematic effects, and applications to neutron capture targets are discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2016

Measurement of polarization observables in vector meson photoproduction using a transversely-polarized frozen-spin target and polarized photons at CLAS, Jefferson Lab

The study of baryon resonances provides a deeper understanding of the strong interaction because the dynamics and relevant degrees of freedom hidden within them are re ected by the properties of the excited states of baryons. Higher-lying excited states at and above 1.7 GeV/c 2 are generally predicted to have strong couplings to final states involving a heavier meson, e. g. one of the vector mesons, ρ, ω φ, as compared to a lighter pseudoscalar meson, e. g. π and η. Decays to the ππΝ final states via πΔ also become more important through the population of intermediate resonances. We observe that nature invests in mass rather than momentum. The excited states of the nucleon are usually found as broadly overlapping resonances which may decay into a multitude of final states involving mesons and baryons. Polarization observables make it possible to isolate single resonance contributions from other interference terms. The CLAS g9 (FROST) experiment, as part of the N* spectroscopy program at Jefferson Laboratory, accumulated photoproduction data using circularly- & linearly-polarized photons incident on a transversely-polarized butanol target (g9b experiment) in the photon energy range 0:3-2:4 GeV & 0:7-2:1 GeV, respectively. In this work, the analysis of reactions and polarization observables which involve two charged pions, either in the fully exclusive reaction γρ -> ρπ+π- or in the semi-exclusive reaction with a missing neutral pion, γρ -> ρπ + π - (π 0 ) will be presented. For the reaction ρπ + π - , eight polarization observables (I s , I c , P x , P y , $P^s_{x;y}$, $P^c_{x; y}$) have been extracted. The high statistics data rendered it possible to extract these observables in three dimensions. All of them are first-time measurements. The fairly good agreement of Is, Ic obtained from this analysis with the experimental results from a previous CLAS experiment provides support for the first-time measurements. For the reaction γρ -> ρω -> ρπ + π(π 0 , five polarization observables (T, Σ, F, H, P) have been extracted, four of which are first-time measurements at all energies. This analysis thus represents a comprehensive program on vector-meson photoproduction: The ω is observed and studied directly from the data and the polarization observables for the (broad) ω can be extracted from the double-pion reaction in a partial-wave analysis. The 13 polarization observables extracted in this analysis substantially augment the world database of polarization observables for these reactions and are expected to play a crucial role in identifying the contributing baryon resonances.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2015

A polarized Drell-Yan experiment to probe the dynamics of the nucleon sea

In QCD, nucleon spin comes from the sum of the quark spin, gluon spin, and the quark and gluon orbital angular momentum, but how these different components contribute and the interplay among them is not yet understood. For instance, sea quark orbital contribution remains largely unexplored. Measurements of the Sivers function for the sea quarks will provide a probe of the sea quark orbital contribution. The upcoming E1039 experiment at Fermilab will measure the Sivers asymmetry of the sea quarks via the Drell-Yan process using a 120 GeV unpolarized proton beam directed a transversely polarized ammonia target. We report on the status and plans of the E1039 polarized Drell-Yan experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2014

Polarization field engineering of GaN/AlN/AlGaN superlattices for enhanced thermoelectric properties

A novel polarization field engineering based strategy to simultaneously achieve high electrical conductivity and low thermal conductivity in thermoelectric materials is demonstrated. Polarization based electric fields are used to confine electrons into two-dimensional electron gases in GaN/AlN/Al{sub 0.2}Ga{sub 0.8}N superlattices, resulting in improved electron mobilities as high as 1176 cm{sup 2}/Vs and in-plane thermal conductivity as low as 8.9 W/mK. The resulting room temperature ZT values reach 0.08, a factor of four higher than InGaN and twelve higher than GaN, demonstrating the potential benefits of this polarization based engineering strategy for improving the ZT and efficiencies of thermoelectric materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Non-Gaussian structure of B-mode polarization after delensing

The B-mode polarization of the cosmic microwave background on large scales has been considered as a probe of gravitational waves from the cosmic inflation. Ongoing and future experiments will, however, suffer from contamination due to the B-modes of non-primordial origins, one of which is the lensing induced B-mode polarization. Subtraction of the lensing B-modes, usually referred to as delensing, will be required for further improvement of detection sensitivity of the gravitational waves. In such experiments, knowledge of statistical properties of the B-modes after delensing is indispensable to likelihood analysis particularly because the lensing B-modes are known to be non-Gaussian. In this paper, we study non-Gaussian structure of the delensed B-modes on large scales, comparing it with that of the lensing B-modes. In particular, we investigate the power spectrum correlation matrix and the probability distribution function (PDF) of the power spectrum amplitude. Assuming an experiment in which the quadratic delensing is an almost optimal method, we find that delensing reduces correlations of the lensing B-mode power spectra between different multipoles, and that the PDF of the power spectrum amplitude is well described as a normal distribution function with a variance larger than that in the case of a Gaussian field. These features are well captured by an analytic model based on the 4th order Edgeworth expansion. As a consequence of the non-Gaussianity, the constraint on the tensor-to-scalar ratio after delensing is degraded within approximately a few percent, which depends on the multipole range included in the analysis.

79 ASTRONOMY AND ASTROPHYSICS↗