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At least 19 records

Nanowire terahertz quantum cascade lasers

Quantum cascade lasers made of nanowire axial heterostructures are proposed. The dissipative quantum dynamics of their carriers is theoretically investigated using non-equilibrium Green functions. Their transport and gain properties are calculated for varying nanowire thickness, from the classical-wire regime to the quantum-wire regime. Our calculation shows that the lateral quantum confinement provided by the nanowires allows an increase of the maximum operation temperature and a strong reduction of the current density threshold compared to conventional terahertz quantum cascade lasers.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Frequency combs in optically injected terahertz ring quantum cascade lasers

Quantum cascade lasers (QCLs) have emerged as promising candidates for generating chip-scale frequency combs in mid-infrared and terahertz wavelengths. In this work, we demonstrate frequency comb formation in ring terahertz QCLs using the injection of light from a distributed feedback (DFB) laser. The DFB design frequency is chosen to match the modes of the ring cavity (near 3.3 THz), and light from the DFB is injected into the ring QCL via a bus waveguide. By controlling the power and frequency of the optical injection, we show that combs can be selectively formed and controlled in the ring cavity. Numerical modeling suggests that this comb is primarily frequency-modulated in character, with the injection serving to trigger comb formation. We also show that the ring can be used as a filter to control the output of the DFB QCL, potentially being of interest in terahertz photonic integrated circuits. Our work demonstrates that waveguide couplers are a compelling approach for injecting and extracting radiation from ring terahertz combs and offer exciting possibilities for the generation of new comb states in terahertz, such as frequency-modulated waves, solitons, and more.

47 OTHER INSTRUMENTATION↗

High-temperature operation of broadband bidirectional terahertz quantum-cascade lasers

Terahertz quantum cascade lasers (QCLs) with a broadband gain medium could play an important role for sensing and spectroscopy since then distributed-feedback schemes could be utilized to produce laser arrays on a single semiconductor chip with wide spectral coverage. QCLs can be designed to emit at two different frequencies when biased with opposing electrical polarities. Here, we develop terahertz QCLs with bidirectional operation to achieve broadband lasing from the same semiconductor chip. A three-well design scheme with shallow-well GaAs/Al 0.10 Ga 0.90 As superlattices is developed to achieve high-temperature operation for bidirectional QCLs. It is shown that shallow-well heterostructures lead to optimal quantum-transport in the superlattice for bidirectional operation compared to the prevalent GaAs/Al 0.15 Ga 0.85 As material system. Furthermore, broadband lasing in the frequency range of 3.1–3.7 THz is demonstrated for one QCL design, which achieves maximum operating temperatures of 147 K and 128 K respectively in opposing polarities. Dual-color lasing with large frequency separation is demonstrated for a second QCL, that emits at ~3.7 THz and operates up to 121 K in one polarity, and at ~2.7 THz up to 105 K in the opposing polarity. Finally, these are the highest operating temperatures achieved for broadband terahertz QCLs at the respective emission frequencies, and could lead to commercial development of broadband terahertz laser arrays.

42 ENGINEERING↗

High brightness angled cavity quantum cascade lasers

A quantum cascade laser (QCL) with an output power of 203 W is demonstrated in pulsed mode at 283 K with an angled cavity. The device has a ridge width of 300 μm, a cavity length of 5.8 mm, and a tilt angle of 12°. The back facet is high reflection coated, and the front facet is anti-reflection coated. The emitting wavelength is around 4.8 μm. In distinct contrast to a straight cavity broad area QCL, the lateral far field is single lobed with a divergence angle of only 3°. An ultrahigh brightness value of 156 MW cm{sup −2 }sr{sup −1} is obtained, which marks the brightest QCL to date.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Room temperature negative differential resistance in terahertz quantum cascade laser structures

The mechanisms that limit the temperature performance of GaAs/Al 0.15 GaAs-based terahertz quantum cascade lasers (THz-QCLs) have been identified as thermally activated LO-phonon scattering and leakage of charge carriers into the continuum. Consequently, the combination of highly diagonal optical transition and higher barriers should significantly reduce the adverse effects of both mechanisms and lead to improved temperature performance. Here, we study the temperature performance of highly diagonal THz-QCLs with high barriers. Our analysis uncovers an additional leakage channel which is the thermal excitation of carriers into bounded higher energy levels, rather than the escape into the continuum. Based on this understanding, we have designed a structure with an increased intersubband spacing between the upper lasing level and excited states in a highly diagonal THz-QCL, which exhibits negative differential resistance even at room temperature. Furthermore, this result is a strong evidence for the effective suppression of the aforementioned leakage channel.

42 ENGINEERING↗

High temperature, single mode, long infrared (λ = 17.8 μm) InAs-based quantum cascade lasers

We demonstrate quantum cascade lasers in the InAs/AlSb material system which operate up to 333 K (in pulsed regime) at λ = 17.8 μm. They employ metal-metal optical waveguides and the threshold current density is 1.6 kA/cm{sup 2} at 78 K. We also report distributed-feedback devices obtained using the same laser material via a 1{sup st}-order Bragg grating inscribed in the sole top metallic contact. Spectral single mode operation with more than 20 dB side mode suppression ratio is achieved at a temperature of 300 K. Large wavelength tuning rates, of the order of 1.5 nm/K, are demonstrated. A wavelength coverage of 0.38 μm is achieved in single-mode regime over a temperature range of 255 K.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

10-W 4.6-μm quantum cascade lasers

Ridge quantum-cascade lasers emitting near 4.6 μm are fabricated and their power and spectral characteristics are studied. Stable pulsed lasing with an output optical power exceeding 10 W (more than 5 W from one facet) at room temperature is demonstrated. (paper)

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Demonstration of a rapidly-swept external cavity quantum cascade laser for rapid and sensitive quantification of chemical mixtures

A rapidly-swept external cavity quantum cascade laser (ECQCL) system for fast open-path quantification of multiple chemicals and mixtures is presented. The ECQCL system is swept over its entire tuning range (>100 cm-1) at frequencies up to 200 Hz. At 200 Hz the wavelength tuning rate and spectral resolution are 2x104 cm-1/sec and < 0.2 cm-1, respectively. The capability of the current system to quantify changes in chemical concentrations on millesecond timescales is demonstrated at atmospheric pressure using an open-path multi-pass cell. The detection limits for chemicals ranged from ppb to ppm levels depending on the absorption cross-section.

Brumfield, Brian E.↗

Real-time standoff detection of nitrogen isotopes in ammonia plumes using a swept external cavity quantum cascade laser

A swept-wavelength external cavity quantum cascade laser is used to measure time-resolved 15NH3 and 14NH3 concentrations and isotope ratios in a turbulent plume source located at 10 m standoff distance. Measurements show excellent agreement with expected values of isotope ratios for samples with natural and enriched 15N abundance. Detection sensitivity of 150 ppb*m is demonstrated for a 50 ms measurement interval, improving to 10 ppb*m with 10 s averaging, with isotopic precision as good as 0.8%.

Phillips, Mark C.↗

High Temperature Laser Generation of Quantum-Cascade Lasers in the Spectral Region of 8 μm

Abstract—In this paper, we present studies of the characteristics of quantum-cascade lasers with a generation wavelength in the region of 8 μm at high temperatures of up to + 65°C. The characteristic temperatures of the temperature dependences of the threshold current and the differential efficiency are determined. Spectral studies showed the presence of two generation lines with a short wavelength of ~7800 nm and a long-wave wavelength of ~8100 nm. The observed competition between the short-wave and long-wave generation lines leads to a nonmonotonic character of the dependence of the radiation intensity on the pump current.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Long term reliability study and life time model of quantum cascade lasers

Here, we present results of quantum cascade laser lifetime tests under various aging conditions including an accelerated life test. The total accumulated life time exceeds 1.5 × 106 device hours. The longest single device aging time was 46 500 hours without failure in the room temperature aging test. Four failures were found in a group of 19 devices subjected to the accelerated life test with a heat-sink temperature of 60 °C and a continuous-wave current of 1 A. Failure mode analyses revealed that thermally induced oxidation of InP in the semi-insulating layer is the cause of failure. An activation energy of 1.2 eV is derived from the dependence of the failure rate on laser core temperature. The mean time to failure of the quantum cascade lasers operating at a typical condition with the current density of 5 kA/cm2 and heat-sink temperature of 25 °C is expected to be 809 000 hours.

Xie, Feng↗

Spectral modification of the laser emission of a terahertz quantum cascade laser induced by broad-band double pulse injection seeding

We demonstrate by injection seeding that the spectral emission of a terahertz (THz) quantum cascade laser (QCL) can be modified with broad-band THz pulses whose bandwidths are greater than the QCL bandwidth. Two broad-band THz pulses delayed in time imprint a modulation on the single THz pulse spectrum. The resulting spectrum is used to injection seed the THz QCL. By varying the time delay between the THz pulses, the amplitude distribution of the QCL longitudinal modes is modified. By applying this approach, the QCL emission is reversibly switched from multi-mode to single mode emission.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Continuous wave room temperature external ring cavity quantum cascade laser

An external ring cavity quantum cascade laser operating at ∼5.2 μm wavelength in a continuous-wave regime at the temperature of 15 °C is demonstrated. Out-coupled continuous-wave optical powers of up to 23 mW are observed for light of one propagation direction with an estimated total intra-cavity optical power flux in excess of 340 mW. The uni-directional regime characterized by the intensity ratio of more than 60 for the light propagating in the opposite directions was achieved. A single emission peak wavelength tuning range of 90 cm{sup −1} is realized by the incorporation of a diffraction grating into the cavity.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Achieving comb formation over the entire lasing range of quantum cascade lasers

Frequency combs based on quantum cascade laser (QCL) are finding promising applications in highspeed broadband spectroscopy in the terahertz regime, where many molecules have their "fingerprints". To form stable combs in QCLs, an effective control of group velocity dispersion plays a critical role. The dispersion of the QCL cavity has two main parts: a static part from the material and a dynamic part from the intersubband transitions. Unlike the gain, which is clamped to a fixed value above the lasing threshold, dispersion associated with the intersubband transitions changes with bias even above the threshold, and this reduces the dynamic range of comb formation. Here, by incorporating tunability into the dispersion compensator, we demonstrate a QCL device exhibiting comb operation from I th to I max , which greatly expands the operation range of the frequency combs.

47 OTHER INSTRUMENTATION↗

A hybrid plasmonic waveguide terahertz quantum cascade laser

We present the realization of a quantum cascade laser emitting at around 2.85 THz, based on a hybrid plasmonic waveguide with a low refractive index dielectric cladding. This hybrid waveguide design allows the performance of a double-metal waveguide to be retained, while improving the emission far-field. A set of lasers based on the same active region material were fabricated with different metal layer thicknesses. A detailed characterization of the performance of these lasers revealed that there is an optimal trade-off that yields the best far-field emission and the maximum temperature of operation. By exploiting the pure plasmonic mode of these waveguides, the standard operation conditions of a double-metal quantum cascade laser were retrieved, such that the maximum operating temperature of these devices is not affected by the process. These results pave the way to realizing a class of integrated devices working in the terahertz range which could be further exploited to fabricate terahertz on-chip circuitry.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Frequency locking and monitoring based on Bi-directional terahertz radiation of a 3 rd -order distributed feedback quantum cascade laser

In this study, we have performed frequency locking of a dual, forward reverse emitting third-order distributed feedback quantum cascade laser (QCL) at 3.5 THz. By using both directions of THz emission in combination with two gas cells and two power detectors, we can for the first time perform frequency stabilization, while monitor the frequency locking quality independently. We also characterize how the use of a less sensitive pyroelectric detector can influence the quality of frequency locking, illustrating experimentally that the sensitivity of the detectors is crucial. Using both directions of terahertz (THz) radiation has a particular advantage for the application of a QCL as a local oscillator, where radiation from one side can be used for frequency/phase stabilization, leaving the other side to be fully utilized as a local oscillator to pump a mixer.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Terahertz GaAs/AlAs quantum-cascade lasers

We have realized GaAs/AlAs quantum-cascade lasers operating at 4.75 THz exhibiting more than three times higher wall plug efficiencies than GaAs/Al{sub 0.25}Ga{sub 0.75}As lasers with an almost identical design. At the same time, the threshold current density at 10 K is reduced from about 350 A/cm{sup 2} for the GaAs/Al{sub 0.25}Ga{sub 0.75}As laser to about 120 A/cm{sup 2} for the GaAs/AlAs laser. Substituting AlAs for Al{sub 0.25}Ga{sub 0.75}As barriers leads to a larger energy separation between the subbands reducing the probability for leakage currents through parasitic states and for reabsorption of the laser light. The higher barriers allow for a shift of the quasi-continuum of states to much higher energies. The use of a binary barrier material may also reduce detrimental effects due to the expected composition fluctuations in ternary alloys.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗