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An R-matrix analysis of the old high energy resolution experimental data [4, 5] in the excitation region of 11.7–13.78 MeV of 22 Ne was performed.
An established use of R-Matrix codes is being implemented at LANSCE. There are unique features accessible with detectors at LANSCE that can be used to perform more complete R-Matrix analysis. Further, Spin separation is a powerful technique that can be applied in DANCE measurements. Additionally, a unique method to measure transmission with DICER is being undertaken. Transmission and capture data were analyzed in this work. The study can be extended to other channels. The results of the 143 Nd data are presented in this work. New resonances found in this work: 21 compared to ENDF/B-VIII.0 and JEFF-3.3, and 24 compared to JENDL-5. Wrong spin assignment in 23 resonances in ENDF/B-VIII.0, 25 in JEFF-3.3 and 26 in JENDL-5. The 143 Nd and 147,149 Sm have been analyzed. Exciting future for new measurements and analysis!
This presentation covers how an established used of R-Matrix codes is being implemented at LANSCE. This presentation displays how there are unique features accessible with detectors at LANSCE that can be used to perform more complete R-Matrix analysis. Additionally discussed is how spin separation is a powerful technique that can be applied in DANCE measurements. Unique method to measure transmission with DICER are discussed. Finally, transmission and capture data are being analyzed in this work. The study can be extended to other channels. The ongoing analysis of the 143 Nd data is presented in this work. The same method is being applied to analyze the 147,149 Sm data. The 143 Nd and 147,149 Sm work started in FY-23 funded by NCSP.
This presentation covers motivation and Introduction, experimental Data Considered in the Analysis, R-Matrix Analysis and Model Details and Selection of Critical Benchmark Experiments.
This presentation highlights how capture and transmission measurements were performed with the DANCE (Detector for Advanced Neutron Capture Experiments) instrument with capture data from 8 eV – 1 keV, and DICER (Device for Indirect Capture Experiments on Radionuclides) instruments with transmission data from 1meV – 1 keV. There were additional measurements of 147 Sm which had contaminant in the samples, 3.4 eV strong resonance, interesting abnormalities. The data analysis is complete and the R-Matrix analysis almost (90%) complete.
This presentation includes a R-Matrix Analysis of 15N system with SAMMY, Discussion of Boundary Conditions in R-Matrix Analyses and a discussion of Analyses with Multiple Incident Channels [Slides]
Performed with support from the U.S. Nuclear Criticality Safety Program in an effort to provide improved chlorine cross section and corresponding covariance data, the R-matrix analysis of neutron induced reactions for two stable chlorine isotopes, 35,37 Cl, was performed in the energy range of thermal up to 1.2 MeV. Starting from the repository of the ENDF/B-VIII.0 library and following recent measurement campaigns, this work represents a significant improvement in the evaluation of the ( η , p ) reaction channel. The evaluation methodology uses the $\mathcal{R}$ -matrix code SAMMY to generate a set of Reich-Moore resonance parameters. As predicted by recently measured 35 Cl( η , p ) data, the presented evaluation features a dramatic increase in the magnitude of the ( η , p ) reaction channel over the ENDF/B-VIII.0 and previous nuclear data ENDF/B released libraries. Together with details of the evaluation procedure, the impact of the updates in the outgoing proton emissions on reactivity coefficients for different molten-salt reactor designs is presented and discussed.
Spectroscopy of the exotic, neutron-unbound beryllium isotope, 13 Be, is still a puzzle despite significant experimental efforts. To observe T = 5/2 states in 13 B, establish spin parities and spectroscopic factors, and use isospin symmetry to inform spectroscopy of 13 Be, excitation functions for resonance elastic scattering of 12 Be on protons were measured in the c.m. energy range from 1 MeV to 5 MeV. Two T = 5/2 states in 13 B at excitation energies 18.25 MeV and 19.95 MeV were observed. Unambiguous 1/2 + and 5/2 + spin-parity assignments were made, and spectroscopic factors were established using R-matrix analysis of the measured 12 Be + p excitation functions. Here, we provide the first direct and unambiguous spin-parity assignments and spectroscopic factor measurements for the resonances in the A = 13, T = 5/2 isobaric multiplet. This puts us on a solid footing to identify the 2.3 MeV state in 13 Be as 5/2 + and infer the existence of an s-wave (1/2 + ) resonance at around 0.6 MeV with a relatively small spectroscopic factor.
Oak Ridge National Laboratory completed the resolved resonance region (RRR) evaluation of the two most abundant cerium isotopes, 140 Ce (88.45%) and 142 Ce (11.11%), as requested by the US Nuclear Criticality Safety Program. These evaluations are based on recent high-resolution transmission and capture measurements performed on nat Ce and highly enriched 142 Ce samples at the JRC-Geel Linear Accelerator facility, as well as measured thermal constants available from the EXFOR database. Starting from the resonance parameters of the ENDF/B-VIII.0 library followed by a preliminary R-matrix analysis, an updated set of resonance parameters and corresponding covariance information were derived by fitting these measured data using the Reich–Moore approximation of the R -matrix theory, as implemented in the SAMMY code system. The 140 Ce RRR upper energy limit was kept at 200 keV, whereas the 142 Ce resonance region was extended from 13 to 26 keV. Updated statistical properties were obtained for the new evaluations and compared to those derived from the ENDF/B-VIII.0 nuclear data library. The new evaluation work improved some of the discrepancies found in previous work, such as the capture resonance integral and stellar Maxwellian-averaged cross sections. These integral quantities were mainly derived from the fit of the latest measured data, especially the neutron capture yield data for 142 Ce isotope.
This presentation covers newly developed SAMMY module for inverse channel transformation. Additionally covered is the R-matrix analysis of 7 Be compound nucleus and the R-matrix analysis of 17 O compound nucleus. Further touched on is the evaluated Nuclear Data File generation and processing with the AMPX code. The presentation concludes with talks on future evaluation work and tests on light nuclei.
Oral presentation detailing recent results of measurements aimed to better determine the 14O(alpha,p)17F reaction rate of interest to Type I X-ray bursts. An aggregate R-matrix analysis of new and existing data along with a new recommended reaction rate is presented.
This presentation covers recent light-element standards-related work at Los Alamos. Points include sections on the updated R-Matrix Analyses/Evaluations. Includes charts on cross sections and system analysis and elastic scattering.
The pronounced threshold peaks found in cross sections for electron-impact excitation of the vibrational levels of HF have been studied using an R-matrix method, in which electron exchange, correlation effects and polarization are included. Vibration is modelled inside the R-matrix sphere using the energy-modified adiabatic phase matrix method (EMAP). Rotation of the target molecule is treated outside the R-matrix sphere, using the frame transformation method. The external rovibronic close-coupling equations are solved by analytic methods. Analysis of the multichannel threshold structures indicates that the peaks found for rovibrational excitation of nu = 1 can be interpreted as virtual states while those for nu = 2 correspond to nuclear-excited Feshbach resonances. These two different results correspond simply to a change of sign of a small parameter that is determined by the threshold analysis. Whereas the overall shapes of the excitation peaks agree with earlier theoretical results, we have found detailed rotational fine structures for scattering energies on the order of the rotational constant above and below the opening of the vibrational channels. The partial and total cross sections for rovibrational state-to-state transitions in the energy region of the peaks are analysed. Characteristic cusp structures and excitation peaks are found at the rovibrational thresholds for transitions with small angular momentum transfer (Delta)j =0, 1 and 2. Differential cross sections are similar to recent measurements. These experimental data do not show the relatively sharp rise at the vibrational thresholds indicated by theory. Theory and experiment are in good agreement for the shape and magnitude of the angular dependence of cross sections for rovibrational state-to-state transitions, especially at larger energies.
In this article, we use the Halfium R-matrix method to investigate the Rydberg states of the H 2 molecule up to n = 20, filling the gap above the low-lying bound states already calculated with configuration interaction packages. Moreover, we show that the use of Quantum Defect Theory scaling laws, allows for a comprehensive analysis of the regular patterns resulting from the coupling between Rydberg series and doubly excited states. The results should open the door for more efficient quasi-diabatization of the potential energy curves which is required for calculating cross sections and rate coefficients of the (e + H 2 + ) collisional processes, involved in the plasma modeling for fusion devices.
In support of the Nuclear Criticality Safety Program, a set of evaluated resonance parameters was generated for seven dysprosium isotopes in the neutron energy range from thermal up to a few keV. The evaluation methodology used the Reich-Moore approximation to fit, with the R-matrix code SAMMY, the high-resolution capture and transmission measurements on natural and enriched samples recently performed at the Rensselaer Polytechnic Institute Gaerttner LINear ACcelerator facility. Additional transmission data measured on enriched samples by Liou at the Columbia University Nevis synchrocyclotron in the mid-seventies were used to gauge the neutron widths above 15 eV. Thermal constants such as absorption and (in)coherent scattering cross sections and corresponding scattering lengths were calibrated to the National Institute of Standards and Technology’s compilation except for 161,164 Dy isotopes.
Here we present a method for measurement analyses based on probabilistic deep neural networks that provide several advantages over conventional analyses with phenomenological models. These include predicting physical quantities directly from data, the rapid generation of statistically robust uncertainties, and the ability to bypass some parameters that may induce ambiguities and complications in data analysis. As deep learning methods make predictions through “black boxes,” the uncertainty quantification is typically challenging. We use a probabilistic framework that provides thorough uncertainty quantification and is straightforward to follow in practice. With the network architecture based on the Transformer, we demonstrate the current method for predicting nuclear resonance parameters from scattering data using the phenomenological R-matrix model.
We examine the relationship between the asymptotic normalization coefficient (ANC) of 6 Li and other low-energy observables in the α–deuteron system. Our analysis uses a set of calculations carried out within the ab initio no core shell model with continuum (NCSMC) using a variety of inter-nucleon interactions and basis sizes, and yielding 6 Li deuteron separation energies between 1.3 and 1.8 MeV (Hebborn et al 2022 Phys. Rev. Lett. 129 042503). These NCSMC calculations show that the square of the ANC is strongly correlated with the separation energy over this range. In this work, we investigate the origin of this correlation using the phenomenological R-matrix, a single-channel potential and a perturbative approach. We show that this correlation occurs because the depth of the α–deuteron central potential changes by only a small relative amount as the separation energy varies. We then investigate if the ANC can be accurately extracted from α–deuteron phase shifts in an ideal case in which low-energy data are available and there are no experimental errors. We find that both R-matrix and Coulomb-modified effective-range theory (CM-ERE) yield extracted ANCs close to, although not exactly equal to, the NCSMC value, provided the extrapolation is constrained by the known position of the bound-state pole and at least three terms are included in the fit function. The R-matrix approach converges faster than the CM-ERE as the number of parameters increases and is also more robust against the inclusion of low-energy and high-energy phase shift data. Finally, our study also shows that a naive quantification of uncertainties by comparing different truncations used in both theories is not accurate, and suggests the accuracy of ANCs extracted from phase shift data needs further investigation.