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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Column separation of tetravalent cerium fission products from trivalent rare earth radio-isotopes

Rapid and efficient isolation of individual rare earth element (REE) radioisotopes from complex mixtures is necessary to support the fields of nuclear forensics, medical isotope production and nuclear physics measurements. The separations must be robust and generate sufficiently high purity samples for subsequent radiological analysis. Current methodologies utilize a laborious two step Ce(IV)-iodate precipitation followed by Ce(IV)-nitrate di-(2-ethylhexyl)phosphoric acid/n-heptane extraction. This work reports an alternative method to isolate Ce fission product isotopes equilibrated with milligrams of cold carrier, from the remaining REE’s using a Ce(IV)/LN-resin (Eichrom Technologies) based separation. Optimization of Ce(IV) loading, REE(III) elution volume and subsequent Ce(III) stripping step utilized 166m Ho tracer. Mixed fission product experiments provided a further test of this LN-resin method, with analysis of purified 141/144 Ce, 147 Nd and 91 Y. Overall, while decontamination factors were lower for the LN-resin method, (vs. the combined precipitation/extraction) the simplicity of the technique and the satisfactory fission product analysis results point to the efficacy of this method.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2019

A Comparison of Adaptive and Template Matching Techniques for Radio-Isotope Identification

We compare and contrast the effectiveness of a set of adaptive and non-adaptive algorithms for isotope identi cation based on gamma-ray spectra. One dimensional energy spectra are simulated for a variety of dwell-times and source to detector distances in order to reflect conditions typically encountered in radiological emergency response and environmental monitoring applications. We nd that adaptive methods are more accurate and computationally efficient than non-adaptive in cases of operational interest.

97 MATHEMATICS AND COMPUTING↗
NASA NTRS2020

Nano-ALSEP: Use of Nano-Sat Technology to Advance Lunar Exploration Science/Engineering

During the Apollo program, unique ALSEP (Apollo Lunar Surface Experiments Package) stations were deployed and left on the surface for long term data collection. Powered by a SNAP-27 electrical power source, the packages continued to transmit useful data until September 30, 1977 (the end of the Fiscal year and termination of the budget). The instruments were varied but included an active seismic experiment (ASE), charged particle experiments, magnetometer experiment, micro-meteoroide/bolide detection experiments. Only only one, the Laser Ranging Retro-Reflector (LRRR) was continued to be used to the present day due to the passive nature of the device. After a dearth of data during an absence of 50 years, is it possible to restart similar packages using the advances in nano-sat technologies? An innovation effort is proposed that would first look at a 2U nano-sat package evolving to an eventual radio-isotope powered system that could be either part of a lunar lander or as an independent package. In the first phase, the packages would only survive during the Lunar day. In a second phase, the later radio-isotope options would place the surface packages in a semi-dormant mode during the Lunar night cycle. Communication capability developed in the TechEdSat-n flight series (UHF, S, X and optical bands) would help to independently close the link and potentially explore IoT devices that were powered only in the sunlight. In addition, limited mobility in the form factor of a nano-rover might also greatly extend the utility of such packages while adding evolutionary capability - and finally continue where the Apollo program was forced to leave off.

M Murbach↗
NASA NTRS2003

Mantle Metasomatism in Mars: Evidence from Bulk Chemical Compositions of Martian Basalts

Bulk compositions of martian meteorite basalts suggest that they formed from a highly depleted mantle that was variably metasomatised and enriched in incompatible elements. These results are consistent with radio-isotope results. Bulk chemical compositions of basaltic rocks retain clues and tracers to their origins and histories. Interpretations of bulk compositions are not so straight-forward as once envisioned, because real-world magmatic processes can be far from theoretical simple models like one-stage partial melting or closed-system fractional crystallization. Yet, bulk chemistry can shed a broad (if dim) light on Martian basalt petrogenesis that complements the sharply focussed illumination of radio-isotope systematics.

Treiman, A. H.↗
NASA NTRS1993

Solid-state Isotopic Power Source for Computer Memory Chips

Recent developments in materials technology now make it possible to fabricate nonthermal thin-film radioisotopic energy converters (REC) with a specific power of 24 W/kg and a 10 year working life at 5 to 10 watts. This creates applications never before possible, such as placing the power supply directly on integrated circuit chips. The efficiency of the REC is about 25 percent which is two to three times greater than the 6 to 8 percent capabilities of current thermoelectric systems. Radio isotopic energy converters have the potential to meet many future space power requirements for a wide variety of applications with less mass, better efficiency, and less total area than other power conversion options. These benefits result in significant dollar savings over the projected mission lifetime.

Brown, Paul M.↗
DOE OSTI2022

Improvements to the 115g/115m Cd Nuclear Data

Repeated measurements of the isotope 115m Cd by Los Alamos National Laboratory (LANL), Pacific Northwest National Laboratory (PNNL), and Atomic Weapons Establishment (AWE) have revealed a consistent discrepancy between beta and gamma counting. This suggests that a significant disparity exists between the true value of the isotope’s gamma-ray branching ratios and the values reported by the National Nuclear Data Center (NNDC). Enriched 114 Cd was irradiated using thermal neutrons to produce a high-purity 115m/g Cd source for counting and analysis using traditional singles gamma-ray spectroscopy, liquid scintillation counting, gas-proportional counting, and analysis using the new Gamma-Alpha-Beta-Gamma (GABγ) and Gamma-Alpha-Beta Radio-Isotope EvaLuator (GABRIEL) coincidence detection systems. Using the D-T fusion generated neutrons, reduces the wait time required to let the short-lived 115Cd ground state decay away by leveraging the 1:1 production ratio of the ground and metastable state of 115 Cd from the 115 In (n,p) reaction relative to the 10:1 production ratio of the ground and metastable isotopes of 115 Cd by thermal neutron capture on 114 Cd. However, the much higher flux in from the Washington State University TRIGA reactor is a more rapid method of production of 115m/gCd but requires access to enriched 114 Cd. High purity 115m/g Cd samples were analyzed on regular intervals over a period of 140-days. The activity of 115m Cd measured by beta and gamma show a clear discrepancy using the current best known gamma-ray decay branching ratios. Based on these observations and measurements, a set of new branching ratio recommendations have been produced using conventional counting techniques and the advanced GAB? and GABRIEL instruments.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2021

Development of High-efficiency and Cost-effective Forged Ingot Niobium Technology for Science Frontiers and Accelerator Applications

Development of Forged Ingot Niobium Technology: Worlds science frontier programs and SRF accelerator applications demand high performance and cost-effective SRF accelerator technology [1-8]. Fine-grain (FG) and Large-grain (LG) ingot niobium technologies have been very well developed and implemented in all the present-day accelerator projects. However, forged ingot niobium technology which is the focus of this development proposal will be much more cost-effective and expected to have several technical advantages. FG niobium sheet production is very complex involving more than ten processing steps making them prone to contamination. As a result, they are very expensive to produce and require stringent QA procedure to be ready for SRF cavity production. The accelerating cavity process steps are also numerous and require strict procedures in order to achieve high accelerating gradients and quality factors needed for science frontier programs. LG niobium disc production, directly sliced from the ingot, is relatively simple and straight forward to keep surface cleanness. The disc production cost is significantly low compared to FG niobium sheet production. However, there are (some) draw backs due to non-homogeneity of the grain boundary distribution, resulting in non-uniform mechanical properties and complex cavity fabrication, although the LG cavities achieve the expected high-gradient performance goals with lower cost. Medium-grain (MG) niobium disk production may be realized with a new approach/process, the disc directly sliced from the forged ingot, involves a simpler process steps contributing major production cost reduction [9]. These discs are expected to be superior as they tend to be homogenous with uniform sub millimeter grains and mechanical properties. We are eagerly looking forward to developing the forged ingot niobium SRF accelerator technology for the benefit of the world-wide science frontier programs, green energy subcritical nuclear energy systems and a wide variety of industrial applications including the production of radio isotopes and nuclear transmutation applications. Measurement of thermal characteristics of the forged ingot niobium: Measurement of the thermal diffusivity, D, of superconducting MG niobium is important to be understood in comparison with FG sheet and LG disc, as well as that of advanced composite material of Nb3Sn film sputtered on forged ingot Nb, which will be determined using transient pump-probe thermo-modulation [10,11]. Transient thermo-modulation is based on using an ultrafast laser pulse to heat the superconducting materials by a few K, then a synchronized laser pulse probes the reflectance of the heated material. For thin films on a substrate (e.g, 100-nm Nb3Sn on Nb), it takes <100 ps for the heat to reach the substrate by diffusion. Therefore, an ultrafast method is needed to probe D of the studied material. D will be measured from room temperature to liquid helium temperatures. Fundamental Research: The increase of rf loss in SRF cavities is related to trapping of residual magnetic field during the cavity cool-down. The study suggested that the micro structure plays the role in flux trapping sensitivity. The research includes the flux trapping and expulsion study as forged ingot niobium goes through several mechanical deformations, crystallization leading to the optimal SRF cavity performance. Furthermore, the cavity made from FG, MG, and LG sheet/disc will be compared to understand the optimal re-crystallization temperature that cavity needed to be heat treated which minimize the flux trapping and increase SRF cavity performance. References: 1. S. Belomestnykh, Overview of recent SRF developments for ERLs, presented at the SRF 2015, Whistler, BC, Canada (2015). 2. A. Yamamoto, M. Yamanaka and G. Myneni, Ingot Nb based SRF Technology for the International Linear Collider, in Science and Technology of Ingot Niobium for Superconducting Radio Frequency Applications, AIP Conf. Proc. 1687, 030005-1 ? 03005-6, 2015 3. Report of the Workshop on Energy and Environmental Applications of Accelerators, DOE Workshop Report. https://science.osti.gov/-/media/hep/pdf/Reports/2020/CASM_WorkshopReport.pdf? la=en&hash=AEB0B318ED0436B1C5FF4EE0FDD6DEB84C2F15B2 4. G. Ciovati, et al., Design of a cw, low-energy, high-power superconducting linac for environmental applications, Phys. Rev. Accel. Beams 21, 091601 (2018). 5. P. Dhakal, et al., Effect of high temperature heat treatments on the quality factor of a large-grain superconducting radio-frequency niobium cavity, Phys. Rev. ST Accel. Beams 16, 042001 (2013). 6. P. Kneisel et al., Review of ingot niobium as a material for superconducting radio frequency accelerating cavities, Nuclear Instruments and Methods in Physics Research A 774, 133 (2015). 7. G. Ciovati, P. Dhakal, and G. R, Myneni, Superconducting radio-frequency cavities made from medium and low-purity niobium ingots, Supercond. Sci. Technol. 29, 064002 (2016). 8. M. Drury et al., commissioning of the prototype C75 cavities in a CEBAF cryomodule, in Proc. of IPAC 2018, Vancouver, BC, Canada (2018) 9. Feasibility of forged-ingot niobium disc and SRF cavity fabrication technology recently demonstrated in cooperation of ATI, BSCE, and KEK (2020). 10. Hani E. Elsayed-Ali, ?Measurements of heat transport in thin films by ultrafast laser-based techniques,? 3rd International Conference on Thermal Issues in Emerging Technologies Theory and Applications, Cairo, Egypt, pp. 347 ? 350 (2010). DOI: 10.1109/ThETA17616.2010 11. W. M. G. Ibrahim, H. E. Elsayed-Ali, M. Schinn, and C. A. Bonner, Jr., ?Ultrafast investigation of electron dynamics in multilayer metals,? Int. J. Heat and Mass Transfer, 47(10?11), 2261?2268 (2004).

Myneni, G.↗
DOE OSTI2018

Evaluation of Repurposing Archetypal Preventive Radiological/Nuclear Detectors to the Consequence Management Mission

In the first hours or days after an unplanned release of radioactive material to the environment, the radiation detection instruments most widely available to local first responders may be those currently fielded for interdiction missions. This study investigated how such preventative radiological / nuclear detection instruments could perform if repurposed to consequence management missions. A representative sample of three archetypes (body-worn, human carried, and other/large detection volume) encompassed six categories: personal radiation detector, extended range personal radiation detector, personal emergency radiation detector, radio-isotope identification device, human portable detector/backpack, and vehicle mounted large detection volume. Overall 19 models of equipment were included in the study. Laboratory evaluations were designed to assess the capabilities of the instruments in four consequence management missions: exposure rate, integrated exposure, radiation survey, and contamination screening. As applicable, the evaluations included measurement of exposure rate, integrated exposure, overrange response, and angular response. The results were compared to benchmarks from the American National Standards Institute ANSI N42.49A. The performance of the instruments for initial screening for contamination was assessed by an automated radioactive source moving past the detectors at various speeds and distances. The results demonstrate that if the equipment is used in accordance with the mission analysis and categories, and within the original equipment manufacturer specifications, it is possible to achieve sufficient accuracy to estimate and document doses to responders, plan entries into contaminated areas, detect contamination, and protect the public, until such time as outside resources arrive with sufficient numbers of standard health physics instruments and personnel dosimetry to replace the preventative radiological / nuclear detection instruments. Finally, this evaluation campaign was conducted to complement the National Council on Radiation Protection and Measurements Report-179 on Guidance for Emergency Response Dosimetry.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

The ARGUS Solution Reactor and Molybdenum Production: A Summary Report Based on Open Literature

The (Aqueous Homogeneous Reactor) AHR was conceptualized at Los Alamos for work in advancing weapon design with initial experiments completed at Los Alamos National Laboratory (LANL) and Oak Ridge National Laboratory (ORNL) in the early 1940s and 1950s. The reactor design was discovered to be an efficient mean of production for medical radio isotopes (e.g. molybdenum-99 and other fission products) due to its streamlined process of extracting target radioactive sources from the fissile solution via a separation system. As the demand for medical radioisotopes has increased so has the need for a safe and low cost isotope source, the most commonly used of which is technetium-99m (99m Tc), daughter product from molybdenum decay. Studies indicate solution reactors pose a significantly lower hazard to the workers, public and environment, compared to other modern reactors (International Atomic Energy Agency 2008). The inherent safety and ability to selectively extract radionuclides from its fuel solution make AHRs particularly well suited for medical isotope production. This discussion narrows its focus to one of the longest running aqueous homogeneous reactor systems, ARGUS. A study of the conversion of ARGUS to a low-enriched uranyl (LEU) sulfate fuel solution was part of the Global Threat Reduction Initiative (GTRI) program. The goal of this paper is to provide a summary of the ARGUS reactor system based on open literature available.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2024

The Evolution of Radioisotope Thermal Generators (RTG)

Introduction The advancement of space exploration owes a lot to the development of nuclear power in space. The Radio Isotopic thermal generator (RTG) was first invented in 1954 and earned its place in the inventor’s hall of fame in 2015. The RTG was and still it the key to our success in the exploration of deep space

Belian, Olivian↗
DOE OSTI2020

The Nucleosynthetic Yields of Core-collapse Supernovae: Prospects for the Next Generation of Gamma-Ray Astronomy

Though the neutrino-driven convection model for the core-collapse explosion mechanism has received strong support in recent years, there are still many uncertainties in the explosion parameters—such as explosion energy, remnant mass, and end-of-life stellar abundances as initial conditions. Using a broad set of spherically symmetric core-collapse simulations we examine the effects of these key parameters on explosive nucleosynthesis and final explosion yields. The post-bounce temperature and density evolution of zero-age main-sequence 15, 20, and 25 solar mass progenitors are post-processed through the Nucleosynthesis Grid nuclear network to obtain detailed explosive yields. In particular, this study focuses on radio isotopes that are of particular interest to the next generation of gamma-ray astronomical observations: 43 K, 47 Ca, 44 Sc, 47 Sc, 48 V, 48 Cr, 51 Cr, 52 Mn, 59 Fe, 56 Co, 57 Co, and 57 Ni. Furthermore, these nuclides may be key in advancing our understanding of the inner workings of core-collapse supernovae by probing the parameters of the explosion engine. We find that the isotopes that are strong indicators of explosion energy are 43 K, 47 Ca, 44 Sc, 47 Sc, and 59 Fe, those that are dependent on the progenitor structure are 48 V, 51 Cr, and 57 Co, and those that probe neither are 48 Cr, 52 Mn, 57 Ni, and 56 Co. We discuss the prospects of observing these radionuclides in supernova remnants.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1974

On thermal stress failure of the SNAP-19A RTG heat shield

Results of a study on thermal stress problems in an amorphous graphite heat shield that is part of the launch-abort protect system for the SNAP-19A radio-isotope thermoelectric generators (RTG) that will be used on the Viking Mars Lander are presended. The first result is from a thermal stress analysis of a full-scale RTG heat source that failed to survive a suborbital entry flight test, possibly due to thermal stress failure. It was calculated that the maximum stress in the heat shield was only 50 percent of the ultimate strength of the material. To provide information on the stress failure criterion used for this calculation, some heat shield specimens were fractured under abort entry conditions in a plasma arc facility. It was found that in regions free of stress concentrations the POCO graphite heat shield material did fracture when the local stress reached the ultimate uniaxial stress of the material.

Pitts, W. C.↗
NASA NTRS1974

Two-watt radioisotope power generators for underwater applications

Materials and design considerations are discussed for a low-cost, reliable radio-isotope-fueled thermoelectric generator for use in an undersea application. Plutonium has been selected as fuel, and the generator has to meet design goals of 2 watts after 20 years with a direct output voltage of 6-8 volts. The pressed and sintered form of Bi2Te3 appears to be the most appropriate thermoelectric material. Both fibrous and multilayer foil insulation could be used with proper processing and quality control, but there is less risk with fibrous type insulation. Min-K 1400 is recommended with a nitrogen cover gas. The heat source recommended is a three-layer capsule using T-111 for both the liner and strength member with an outer liner of Hastelloy-C.

Caputo, R. S.↗
NASA NTRS1979

Visual imaging control systems of the Mariner to Jupiter and Saturn spacecraft

Design and fabrication of optical systems for the Mariner Jupiter Saturn (Voyager) mission is described. Because of the long distances of these planets from the sun, the spacecraft was designed without solar panels with the electricity generated on-board by radio-isotope thermal generators (RTG). The presence of RTG's and Jupiter radiation environment required that the optical systems be fabricated out of radiation stabilized materials. A narrow angle and a wide angle camera are located on the spacecraft scan platform, with the narrow angle lens a modification of the Mariner 10 lens. The optical system is described, noting that the lens was modified by moving the aperture correctors forward and placing a spider mounted secondary mirror in the original back surface of the second aperture corrector. The wide angle lens was made out of cerium doped, radiation stabilized optical glass with greatest blue transmittance, which would be resistant to RTG and Jupiter radiation.

Larks, L.↗
NASA NTRS1981

The International Solar Polar Mission - United States and Europe plan for a new look at the sun

A three-dimensional polar orbit exploration of the sun and solar-related phenomena in the heliosphere through the International Solar Polar Mission (ISPM) is discussed. The characteristics of the out-of-the-ecliptic mission are mentioned and a detailed list of the scientific objectives is given: properties of the solar corona, the solar wind, the structure of the sun-wind interface, the heliospheric magnetic field, solar and non-solar cosmic rays, solar radio bursts and plasma waves, and the interstellar/interplanetary neutral gas and dust. Measurements of the Jovian magnetosphere during the Jupiter flyby phase and interplanetary physics investigations during the initial earth-Jupiter phase are pointed out as secondary objectives. The Nasa spacecraft with a sun-pointing despun platform on which the White Light Coronagraph/X-Ray and Extreme Ultraviolet Telescope (CXX), and the Mass Separating Ion Instrument are mounted, is detailed. The operational configuration of EASA, a spin stabilized spacecraft, is given and characteristics of special features such as the large paraboloidal high gain antenna, the radio-isotope thermoelectric generator, the radial boom and the central equipment compartment are described and shown in a diagram. The mission design and launch parameters block diagrams are given.

Purdy, W. I., Jr.↗