Investigations into attachment properties of radioactive aerosols
Attachment of radioactive small ions and of neutral radioactive substances to aerosols, based on solution of diffusion equation
DIFFUSION↗
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Evaluation of Observed and Modelled Aerosol Lifetimes Using Radioactive Tracers of Opportunity and an Ensemble of 19 Global Models
Aerosols have important impacts on air quality and climate, but the processes affecting their removal from the atmosphere are not fully understood and are poorly constrained by observations. This makes modelled aerosol lifetimes uncertain. In this study, we make use of an observational constraint on aerosol lifetimes provided by radionuclide measurements and investigate the causes of differences within a set of global models. During the Fukushima Dai-Ichi nuclear power plant accident of March 2011, the radioactive isotopes cesium-137 (Cs-137) and xenon-133 (Xe-133) were released in large quantities. Cesium attached to particles in the ambient air, approximately according to their available aerosol surface area. Cs-137 size distribution measurements taken close to the power plant suggested that accumulation mode (AM) sulfate aerosols were the main carriers of cesium. Hence, Cs-137 can be used as a proxy tracer for the AM sulfate aerosol's fate in the atmosphere. In contrast, the noble gas Xe-133 behaves almost like a passive transport tracer. Global surface measurements of the two radioactive isotopes taken over several months after the release allow the derivation of a lifetime of the carrier aerosol. We compare this to the lifetimes simulated by 19 different atmospheric transport models initialized with identical emissions of Cs-137that were assigned to an aerosol tracer with each model's default properties of AM sulfate, and Xe-133 emissions that were assigned to a passive tracer. We investigate to what extent the modelled sulfate tracer can reproduce the measurements, especially with respect to the observed loss of aerosol mass with time. Modelled Cs-137and Xe-133 concentrations sampled at the same location and times as station measurements allow a direct comparison between measured and modelled aerosol lifetime. The e-folding lifetime e, calculated from station measurement data taken between 2 and 9 weeks after the start of the emissions, is 14.3 days (95% confidence interval 13.1-15.7 days). The equivalent modelled e lifetimes have a large spread, varying between 4.8 and 26.7 days with a model median of 9.42.3 days, indicating too fast a removal in most models. Because sufficient measurement data were only available from about 2 weeks after the release, the estimated lifetimes apply to aerosols that have undergone long-range transport, i.e. not for freshly emitted aerosol. However, modelled instantaneous lifetimes show that the initial removal in the first 2 weeks was quicker (lifetimes between 1 and 5 days) due to the emissions occurring at low altitudes and co-location of the fresh plume with strong precipitation. Deviations between measured and modelled aerosol lifetimes are largest for the northernmost stations and at later time periods, suggesting that models do not transport enough of the aerosol towards the Arctic. The models underestimate passive tracer (Xe-133) concentrations in the Arctic as well but to a smaller extent than for the aerosol (Cs-137) tracer. This indicates that in addition to too fast an aerosol removal in the models, errors in simulated atmospheric transport towards the Arctic in most models also contribute to the underestimation of the Arctic aerosol concentrations.
Radioactive isotopes↗
Advanced Filter Technology For Nuclear Thermal Propulsion
The Scrubber System focuses on using HEPA filters and carbon filtration to purify the exhaust of a Nuclear Thermal Propulsion engine of its aerosols and radioactive particles; however, new technology may lend itself to alternate filtration options, which may lead to reduction in cost while at the same time have the same filtering, if not greater, filtering capabilities, as its predecessors. Extensive research on various types of filtration methods was conducted with only four showing real promise: ionization, cyclonic separation, classic filtration, and host molecules. With the four methods defined, more research was needed to find the devices suitable for each method. Each filtration option was matched with a device: cyclonic separators for the method of the same name, electrostatic separators for ionization, HEGA filters, and carcerands for the host molecule method. Through many hours of research, the best alternative for aerosol filtration was determined to be the electrostatic precipitator because of its high durability against flow rate and its ability to cleanse up to 99.99% of contaminants as small as 0.001 micron. Carcerands, which are the only alternative to filtering radioactive particles, were found to be non-existent commercially because of their status as a "work in progress" at research institutions. Nevertheless, the conclusions after the research were that HEPA filters is recommended as the best option for filtering aerosols and carbon filtration is best for filtering radioactive particles.
Castillon, Erick↗
Regional ventilation-perfusion distribution is more uniform in the prone position
The arterial blood PO(2) is increased in the prone position in animals and humans because of an improvement in ventilation (VA) and perfusion (Q) matching. However, the mechanism of improved VA/Q is unknown. This experiment measured regional VA/Q heterogeneity and the correlation between VA and Q in supine and prone positions in pigs. Eight ketamine-diazepam-anesthetized, mechanically ventilated pigs were studied in supine and prone positions in random order. Regional VA and Q were measured using fluorescent-labeled aerosols and radioactive-labeled microspheres, respectively. The lungs were dried at total lung capacity and cubed into 603-967 small ( approximately 1.7-cm(3)) pieces. In the prone position the homogeneity of the ventilation distribution increased (P = 0.030) and the correlation between VA and Q increased (correlation coefficient = 0.72 +/- 0.08 and 0.82 +/- 0.06 in supine and prone positions, respectively, P = 0.03). The homogeneity of the VA/Q distribution increased in the prone position (P = 0.028). We conclude that the improvement in VA/Q matching in the prone position is secondary to increased homogeneity of the VA distribution and increased correlation of regional VA and Q.
NASA Program Biomedical Research and Countermeasur↗
Implications of using MERRA-2 cloud water in aerosol wet scavenging for Pb-210 surface concentrations and vertical profiles in GEOS-Chem
Precipitation scavenging is the dominant loss process for a whole suite of aerosols but model parameterizations of this process are highly uncertain, substantially contributing to large uncertainties in the simulated loadings and radiative forcing of aerosols. Lead-210 (210Pb, radioactive half-life of 22.3 years) is produced by radioactive decay of soil-emitted gaseous 222Rn. It attaches to ambient submicron aerosols and is subject to precipitation scavenging processes. Liu et al. [2001] estimated the global mean lifetime of tropospheric 210Pb aerosols to be ~9 days using the GEOS-Chem model. Luo et al. [2019, 2020] provided an option to use MERRA-2 cloud water in the model aerosol scavenging scheme. In this study, we examine the impact of this revision on 210Pb simulations and compare results with climatological observations of 210Pb surface and UT/LS concentrations, as well as aircraft profile measurements from eleven NASA field missions.
Bo Zhang↗
Transport and residence times of tropospheric aerosols inferred from a global three-dimensional simulation of Pb-210
A global three-dimensional model is used to investigate the transport and tropospheric residence time of Pb-210, an aerosol tracer produced in the atmosphere by radioactive decay of Rn-222 emitted from soils. The model uses meteorological input with 4 deg x 5 deg horizontal resolution and 4-hour temporal resolution from the Goddard Institute for Space Studies general circulation model (GCM). It computes aerosol scavenging by convective precipitation as part of the wet convective mass transport operator in order to capture the coupling between vertical transport and rainout. Scavenging in convective precipitation accounts for 74% of the global Pb-210 sink in the model; scavenging in large-scale precipitation accounts for 12%, and scavenging in dry deposition accounts for 14%. The model captures 63% of the variance of yearly mean Pb-210 concentrations measured at 85 sites around the world with negligible mean bias, lending support to the computation of aerosol scavenging. There are, however, a number of regional and seasonal discrepancies that reflect in part anomalies in GCM precipitation. Computed residence times with respect to deposition for Pb-210 aerosol in the tropospheric column are about 5 days at southern midlatitudes and 10-15 days in the tropics; values at northern midlatitudes vary from about 5 days in winter to 10 days in summer. The residence time of Pb-210 produced in the lowest 0.5 km of atmosphere is on average four times shorter than that of Pb-210 produced in the upper atmosphere. Both model and observations indicate a weaker decrease of Pb-210 concentrations between the continental mixed layer and the free troposphere than is observed for total aerosol concentrations; an explanation is that Rn-222 is transported to high altitudes in wet convective updrafts, while aerosols and soluble precursors of aerosols are scavenged by precipitation in the updrafts. Thus Pb-210 is not simply a tracer of aerosols produced in the continental boundary layer, but also of aerosols derived from insoluble precursors emitted from the surface of continents. One may draw an analogy between Pb-210 and nitrate, whose precursor NO(sub x) is sparingly soluble, and explain in this manner the strong correlation observed between nitrate and Pb-210 concentrations over the oceans.
Balkanski, Yves J.↗
Thunderstorm and Fair-weather Quasi-Static Electric Fields Over Land and Ocean
Natural lightning and the associated clouds are known to behave differently over land and ocean, but many questions remain. We expand the related observational datasets by obtaining simultaneous quasi-static electric field observations over coastal land, near-shore water, and deep ocean regions during both fair-weather and thunderstorm periods. Oceanic observations were obtained using two 3-m NOAA buoys that were instrumented with Campbell Scientific electric field mills to measure the quasi-static electric fields. These data were compared to selected electric field records from the existing on-shore electric field mill suite of 31 sensors at Kennedy Space Center (KSC). Lightning occurrence times, locations and peak current estimates for both onshore and ocean were provided by the U.S. National Lightning Detection Network. The buoy instruments were first evaluated on-shore at the Florida coast, and the first system was calibrated for field enhancements and to confirm proper behavior of the system in elevated-field environments. The buoys were then moored 20 mi and 120 mi off the coast of KSC in February (20 mi) and August (120 mi) 2014. Diurnal fair-weather fields at both ocean sites matched will with each other and with those found during the Carnegie cruise, but mean values were 33% smaller, due at least in-part to constraints on the calibration procedure. Diurnal fair-weather fields variations at coastal and inland sites were a poorer match than offshore, likely because the offshore environment is “cleaner” with limited variations in local space charge, lower surface aerosol densities, little surface heating to disturb the surface charge layer during fair weather, and fewer local radioactive sources to modulate the near-surface electrical conductivity. Storm-related static fields were 4-5× larger at both oceanic sites than over land, likely due to decreased screening by near-surface space charge produced by corona current. The time-evolution of the electric field and field changes during storm approach are sufficiently different over land and ocean to warrant further study. This work shows the quality, accuracy, and reliability of these data, and has demonstrated the practicality of off-shore electric field measurements for safety- and launch-related decision making at KSC.
Lightning↗
Global environmental effects of impact-generated aerosols: Results from a general circulation model
Cooling and darkening at Earth's surface are expected to result from the interception of sunlight by the high altitude worldwide dust cloud generated by impact of a large asteroid or comet, according to the one-dimensional radioactive-convective atmospheric model (RCM) of Pollack et al. An analogous three-dimensional general circulation model (GCM) simulation obtains the same basic result as the RCM but there are important differences in detail. In the GCM simulation the heat capacity of the oceans, not included in the RCM, substantially mitigates land surface cooling. On the other hand, the GCM's low heat capacity surface allows surface temperatures to drop much more rapidly than reported by Pollack et al. These two differences between RCM and GCM simulations were noted previously in studies of nuclear winter; GCM results for comet/asteroid winter, however, are much more severe than for nuclear winter because the assumed aerosol amount is large enough to intercept all sunlight falling on Earth. In the simulation the global average of land surface temperature drops to the freezing point in just 4.5 days, one-tenth the time required in the Pollack et al. simulation. In addition to the standard case of Pollack et al., which represents the collision of a 10-km diameter asteroid with Earth, additional scenarios are considered ranging from the statistically more frequent impacts of smaller asteroids to the collision of Halley's comet with Earth. In the latter case the kinetic energy of impact is extremely large due to the head-on collision resulting from Halley's retrograde orbit.
Covey, C.↗
Direct measurements of ozone and nitrogen dioxide photolysis rates in the troposphere
The photolysis frequencies of ozone and nitrogen dioxide were measured under a variety of conditions commonly found in the troposphere. Ozone photolysis frequencies show a strong dependence on solar zenith angle, overhead ozone column, and temperature, but only a weak dependence on altitude (when only downward radiation is detected). Nitrogen dioxide photolysis frequencies also show strong dependence on solar zenith angle, but show little dependence on temperature, pressure, or altitude. Both j values are strongly affected by cloud cover, but aerosol loading has much less effect. The disagreement of measured j(O3) and j(NO2) with many modeled values, especially disagreement over altitude dependence, shows that atmospheric UV radioactive processes are complicated and poorly understood, although experimental conditions may not always be applicable to conditions modeled.
Dickerson, R. R.↗