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Nuclear Data Sheets for A=218

The evaluated data are presented for 11 known A=218 nulcides (Pb, Bi, Po, At, Rn, Fr, Ra, Ac, Th, Pa and U). For {sup 218}Pb, {sup 218}Bi, {sup 218}At and {sup 218}Pa, data are available only for the ground states. For {sup 218}U, only the g.s. and a high-spin isomer are known, with no data on γ-ray transitions available. For {sup 218}Po, ten excited states are known from {sup 218}Bi decay, with no knowledge on the multipolarities of gamma-ray transitions. For {sup 218}Th, five excited states in the g.s. band are known from an in-beam γ-ray study. Data on level half-lives, multipolarities and mixing ratios of gamma transitions is generally lacking for A=218 nuclei. The static magnetic dipole moment has been measured for only an isomer in {sup 218}Fr. With the exception of a new nuclide, {sup 218}Pb, and measurements of half-lives of ground states of a few nuclides of A=218 and A=222, no substantial structure information has become available since the previous evaluation in 2006. Q values are adopted from 2017Wa10 (AME-2016). The present evaluation supersedes the previous A=218 ENSDF evaluations, 2006Ja03, 1995El08, 1987El12 and 1977To13. This evaluation was carried out as part of a joint IAEA-ICTP workshop for Nuclear Structure and Decay Data, organized and hosted by the IAEA, Vienna, and ICTP, Trieste, October 15–26, 2018.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Challenges and Practical Solutions for Conducting Structural MARSSIM Surveys in Elevated Radon Environments - 20413

The Multi-Agency Radiation Survey and Site Investigation Manual (MARSSIM) [1] provides comprehensive guidance for the development and implementation of radiological surveys conducted to demonstrate compliance with a dose- or risk-based cleanup goal during final status survey. The MARSSIM methodology follows an integrated strategy combining direct measurements and sampling to assess uniform residual contamination, and scanning surveys to identify localized areas of elevated activity. Building surveys assessing residual surface contamination present unique challenges from reliance on field measurements that may be subject to less than ideal environmental conditions. Additionally, limited characterization and excessive conservatism incorporated into the conceptual site model may result in derived concentration guideline levels (DCGL) and, as a consequence of relatively inefficient field instrumentation, corresponding attributable count rates generally comparable to background. The presence of elevated ambient radon concentrations and associated progeny deposition both exacerbate these intrinsic survey challenges and introduce a series of technical, logistic, and administrative obstacles that can wreak havoc on the statistical legitimacy of each component of the MARSSIM process. Short-lived radon progeny including polonium-218, lead-214, bismuth-214, and polonium-214 produce excessive alpha and beta radiation that may decrease instrument sensitivity through an increase in background count rates, and, at worst, may result in incorrect survey unit failure through the simulation of residual surface activity. Aside from the obvious solution of exhaustive radon mitigation, the primary objectives are to distinguish between radon progeny deposition and actual surface activity, and collect sufficient defensible data. The following is a technical discussion of the consequences of performing building MARSSIM surveys in the presence of elevated ambient radon atmospheres, conceptual examples, and an overview of practical strategies to minimize the effects of radon interference while collecting sufficient defensible data to complete the survey. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Measurement of the ion fraction and mobility of 218Po produced in 222Rn decays in liquid argon

We report measurements of the charged daughter fraction of 218Po as a result of the 222Rn alpha decay, and the mobility of 218Po+ ions, using radon-polonium coincidences from the 238U chain identified in 532 live-days of DarkSide-50 WIMP-search data. The fraction of 218Po that is charged is found to be 0.37 ± 0.03 and the mobility of 218Po+ is (8.6 ± 0.1) × 10-4 cm2/Vs.

Agnes, P↗

Flow-dependent tagging of 214 Pb decays in the LZ dark matter detector

The LUX-ZEPLIN (LZ) experiment is searching for dark matter interactions in a liquid xenon time projection chamber (LXe-TPC). This article demonstrates how control of the flow state in the LXe-TPC enables the identification of pairs of sequential alpha-decays, which are used to map fluid flow and ion drift in the liquid target. The resulting transport model is used to tag 214 Pb~ beta-decays, a leading background to dark matter signals in LZ. Temporally evolving volume selections, at a cost of 9.0% of exposure, target the decay of each 214 Pb~ atom up to 81 minutes after production, resulting in (63±6 (s⁢t⁢a⁢t) ±7 (s⁢y⁢s) )% identification of 214 Pb~decays to ground state. We also demonstrate how flow-based tagging techniques enable a novel calibration side band that is concurrent with science data. Lastly we report updated estimates of radon-chain charge branching fractions in liquid xenon, finding branching to 218 Po + at 0.49±0.01, 214 Pb + at 0.48±0.12, and 214 Bi + at 0.74±0.05, with a mean charged ion lifetime in the LZ TPC of 49±4 min.

Lorenzon, Wolfgang [University of Michigan, Ann Ar↗