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At least 19 records

Radon Isotopes and Stable Water Isotopes from Coal Creek Watershed, Colorado (2021)

The radon isotope and stable water isotope data for Coal Creek Watershed, Colorado, consists of d2H, d18O, and 222Rn values from samples collected at 8 stream location along Coal Creek, samples from 7 groundwater springs within the watershed, and precipitation isotope samples collected by Next Generation Water Observing System (NGWOS) from a collector within the watershed. All stream and spring samples were collected between June and October, 2021, and precipitation isotope samples were collected between November 2020 and September 2021. These data were collected to evaluate how groundwater contributions to Coal Creek originating from a fractured hillslope and alluvial fan respond to summer monsoon rains and seasonal drying. Understanding of groundwater-surface water interactions in montane systems in critical for the future of water availability in the Western US as groundwater contributions are expected to become more important for sustaining summer stream flows. This data package contains: (1) a csv of all radon samples; (2) a csv of all stream and spring isotope samples; (3) a csv of precipitation isotope samples; and (4) a csv of locations for each sampling site. The dataset additionally includes a file-level metadata (flmd.csv) file that lists each file contained in the dataset with associated metadata; and a data dictionary (dd.csv) file that contains column/row headers used throughout the files along with a definition, units, and data type.

54 ENVIRONMENTAL SCIENCES↗

An age- and sex-specific biokinetic model for radon *

Publication 137 of the International Commission on Radiological Protection (ICRP) describes a biokinetic model for radon used to derive dose coefficients for occupational intake of radon isotopes. The model depicts transfer of inhaled or ingested radon to blood, exchange of radon between blood and tissues, and gradual loss of radon from the body based on physical laws governing transfer of a non-reactive and soluble gas between materials. Here, this paper describes an age- and sex-specific variation of that model developed for use in an upcoming ICRP series of reports on environmental intake of radionuclides by members of the public titled ‘Dose Coefficients for Intakes of Radionuclides by Members of the Public’. The proposed model modifies the model structure and transfer coefficients presented in Publication 137 to allow more realistic dosimetric treatment of bone marrow and breast and expands the model to address pre-adult ages, based on the physical principles used in the development of the model of Publication 137 together with anatomical and physiological changes occurring during human development.

61 RADIATION PROTECTION AND DOSIMETRY↗

Alpha-particle spectrometer experiment

Mapping the radon emanation of the moon was studied to find potential areas of high activity by detection of radon isotopes and their daughter products. It was felt that based on observation of regions overflown by Apollo spacecraft and within the field of view of the alpha-particle spectrometer, a radon map could be constructed, identifying and locating lunar areas of outgassing. The basic theory of radon migration from natural concentrations of uranium and thorium is discussed in terms of radon decay and the production of alpha particles. The preliminary analysis of the results indicates no significant alpha emission.

Gorenstein, P.↗

Simulation of background from low-level tritium and radon emanation in the KATRIN spectrometers

The KArlsruhe TRItium Neutrino (KATRIN) experiment is a large-scale experiment for the model independent determination of the mass of electron anti-neutrinos with a sensitivity of 200 meV/c{sup 2}. It investigates the kinematics of electrons from tritium beta decay close to the endpoint of the energy spectrum at 18.6 keV. To achieve a good signal to background ratio at the endpoint, a low background rate below 10{sup −2} counts per second is required. The KATRIN setup thus consists of a high luminosity windowless gaseous tritium source (WGTS), a magnetic electron transport system with differential and cryogenic pumping for tritium retention, and electro-static retarding spectrometers (pre-spectrometer and main spectrometer) for energy analysis, followed by a segmented detector system for counting transmitted beta-electrons. A major source of background comes from magnetically trapped electrons in the main spectrometer (vacuum vessel: 1240 m{sup 3}, 10{sup −11} mbar) produced by nuclear decays in the magnetic flux tube of the spectrometer. Major contributions are expected from short-lived radon isotopes and tritium. Primary electrons, originating from these decays, can be trapped for hours, until having lost almost all their energy through inelastic scattering on residual gas particles. Depending on the initial energy of the primary electron, up to hundreds of low energetic secondary electrons can be produced. Leaving the spectrometer, these electrons will contribute to the background rate. This contribution describes results from simulations for the various background sources. Decays of {sup 219}Rn, emanating from the main vacuum pump, and tritium from the WGTS that reaches the spectrometers are expected to account for most of the background. As a result of the radon alpha decay, electrons are emitted through various processes, such as shake-off, internal conversion and the Auger deexcitations. The corresponding simulations were done using the KASSIOPEIA framework, which has been developed for the KATRIN experiment for low-energy electron tracking, field calculation and detector simulation. The results of the simulations have been used to optimize the design parameters of the vacuum system with regard to radon emanation and tritium pumping, in order to reach the stringent requirements of the neutrino mass measurement.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Discovery of the astatine, radon, francium, and radium isotopes

Thirty-nine astatine, thirty-nine radon, thirty-five francium, and thirty-four radium isotopes have so far been observed; the discovery of these isotopes is described. For each isotope a brief summary of the first refereed publication, including the production and identification method, is presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

US EPA superfund radon vapor intrusion preliminary remediation goal (RAD-VIPRG) electronic calculator - 15349

Currently, there is no U.S. EPA guidance on correlating soil or groundwater levels of radon with indoor radon concentrations at Superfund sites. EPA is developing the Radon Vapor Intrusion Preliminary Remediation Goal (RAD-VIPRG) Calculator which is a spreadsheet tool that (1) lists two radon isotopes (Rn-220 and Rn-222) known to pose a potential cancer risk through the inhalation pathway; (2) provides generally recommended risk and Applicable or Relevant and Appropriate Requirements (ARAR) based preliminary remediation goals (PRG) for groundwater, soil gas (exterior to buildings and sub-slab) and indoor air for default target risk and ARAR based levels and exposure scenarios; and (3) allows calculation of site-specific PRGs based on user-defined target risk and ARAR levels and exposure scenarios. EPA developed the RAD-VIPRG calculator to help risk assessors, remedial project managers, and others involved with risk assessment and decision making at radioactively contaminated sites.(authors)

61 RADIATION PROTECTION AND DOSIMETRY↗

US EPA Superfund Radon Vapor Intrusion Screening Level (RVISL) Electronic Calculator - 20340

Currently, there is no U.S. Environmental Protection Agency (EPA) guidance on correlating soil or groundwater levels of radon with indoor radon concentrations at Superfund sites. EPA is developing the Radon Vapor Intrusion Level Calculator (RVISL) Calculator which is an online tool. The RVISL calculator: (1) lists three radon isotopes (Rn-219, Rn-220 and Rn-222) known to pose a potential cancer risk through the inhalation pathway; (2) provides generally recommended risk and Applicable or Relevant and Appropriate Requirements (ARAR) based preliminary remediation goals (PRG) for groundwater, soil gas (exterior to buildings and sub-slab) and indoor air for default target risk and ARAR based levels and exposure scenarios; and (3) allows calculation of site-specific PRGs based on user-defined target risk and ARAR based levels and exposure scenarios. EPA developed the RVISL calculator to help risk assessors, remedial project managers, and others involved with risk assessment and decision making at radioactively contaminated sites. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Nuclear Data Sheets for A = 207

Evaluated nuclear structure and decay data for all nuclei within the A=207 mass chain are presented. The experimental data are evaluated and best values for level and gamma-ray energies, quantum numbers, lifetimes, gamma-ray intensities, and other nuclear properties are recommended. Inconsistencies and discrepancies that exist in the literature are noted. This work supersedes the earlier evaluation by M.J. Martin (1993Ma73), published in Nuclear Data Sheets70, 315 (1993).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Atomic electric dipole moment induced by the nuclear electric dipole moment: The magnetic moment effect

We have considered a mechanism for inducing a time-reversal violating electric dipole moment (EDM) in atoms through the interaction of a nuclear EDM d{sub N} with the hyperfine interaction, the ''magnetic moment effect''. We have derived the operator for this interaction and presented analytical formulas for the matrix elements between atomic states. Induced EDMs in the diamagnetic atoms {sup 129}Xe, {sup 171}Yb, {sup 199}Hg, {sup 211}Rn, and {sup 225}Ra have been calculated numerically. From the experimental limits on the atomic EDMs of {sup 129}Xe and {sup 199}Hg we have placed the following constraints on the nuclear EDMs, |d{sub N}({sup 129}Xe)|<1.1x10{sup -21}|e|cm and |d{sub N}({sup 199}Hg)|<2.8x10{sup -24}|e|cm.

74 ATOMIC AND MOLECULAR PHYSICS↗

Radioactive Thoron 220 Rn Exhalation From Unfired Mud Building Material Into Room Air of Earthen Dwellings

Thoron ( 220 Rn), an isotope of radon with a strong α-decay energy, and its short-lived metallic progeny can pose an elevated lung cancer hazard in room air when unfired-soil derived building materials are used in earthen dwellings. Changes in moisture content and density influencing the thoron exhalation rate from earthen materials into room air were studied in the laboratory with terra rossa from a village on the Ðòng Van Karst Plateau Geopark, Viêt Nam, where ethnic minorities construct traditional dwellings with unfired terra rossa walls and floors. Our results show that the thoron exhalation rate from mud surfaces depends on (i) the content of radioactive parental nuclides in mineral components; (ii) the moisture content of mud where ~5–10 weight % water maximizes the 220 Rn exhalation rate; and (iii) the density of dry mud as primarily controlled by internal macroscopic voids, fractures, and porosity. Additional time-series of 220 Rn exhalation data from an interior mud wall of a terra rossa-built house under different seasonal and weather conditions show that the temperature is influencing thoron exhalation via the water vapor pressure deficit (VPD) in air and the associated amount of atmospheric moisture adsorbed onto indoor mud surfaces. Our data suggest that occupants of “mud house” earthen dwellings in northern Viêt Nam are exposed to an increased thoron geohazard during cooler weather, low VPD, and high relative humidity in air. Detailed studies are needed to evaluate the thoron geohazard for inhabitants of mud-built dwellings in other climates and geological terrains.

58 GEOSCIENCES↗

The Apollo Alpha Spectrometer.

Located in the Science Instrument Module of Apollo 15 and 16, the Alpha Particle Spectrometer was designed to detect and measure the energy of alpha particles emitted by the radon isotopes and their daughter products. The spectrometer sensor consisted of an array of totally depleted silicon surface barrier detectors. Biased amplifier and linear gate techniques were utilized to reduce resolution degradation, thereby permitting the use of a single 512 channel PHA. Sensor identification and in-flight radioactive calibration were incorporated to enhance data reduction.

Jagoda, N.↗

Minimizing Backgrounds for the SuperCDMS SNOLAB Dark-Matter Experiment

Astronomical and cosmological observations indicate that large amounts of some slowly moving, unseen Dark Matter pervades the universe and outweighs normal matter by a factor of five. The Standard Model of Physics has no contender with the properties of this as-yet-undetected particle, so experimentalists build state-of-the-art radiation detectors to attempt to directly measure this Dark Matter. The Super Cryogenic Dark Matter Search (SuperCDMS) at Snolab is one such experiment, currently being constructed. This experiment uses ultra-cold, superconducting, high-purity silicon and germanium detectors to measure low-energy nuclear recoils from the elastic scattering of Dark Matter. I contributed to the calibration of the energy scale of low-energy nuclear recoils in CDMS II silicon detectors by computing an improved livetime correction for calibration data to verify the Monte Carlo rate normalization. Results indicate that the phonon collection efficiency of nuclear recoils relative to electron recoils is 95.2$^{+0.9}_{-0.7\%}$, and the ionization collection efficiency of low-energy nuclear recoils in silicon is lower than Lindhard prediction, consistent with other recent measurements. Backgrounds from the progeny decay of the abundant, naturally-occurring radioactive isotope radon-222 obstruct the sensitivity of essentially every dark-matter search. Radon concentrations in the Snolab cavern would contribute prohibitively large backgrounds if the volume surrounding the detectors were not purged with a low-flow low-radon gas. By measuring the radon diffusion and emanation, we identified acceptable gasket materials for sealing this radon purge, ensuring that the radon-induced backgrounds will be significantly lower than the other experimental backgrounds. A radon emanation system with a gas handling system and low-background radon detector was commissioned and used to measure the radon emanation of the proposed gaskets. A low-cost apparatus was constructed to measure the radon diffusion of gaskets with a commercial radon detector. The sensitivity of future generations of dark-matter detectors are expected to be dominated by long-lived low-energy beta- and alpha-emitting radon daughters such as 210 Pb on detector surfaces. I describe simulations indicating the detector could also be used to reduce background from material impurities plaguing rare-event searches, the commissioning of a prototype demonstration detector, and a gas handling system necessary to operate the detector. I demonstrated that the gas handling system reduces the otherwise dominant backgrounds by a factor of 62. This detector will therefore be able to detect 32 Si and 210 Pb 100 times better than currently available screeners.

Bowles, Michael A.↗

Shifting groundwater fluxes in bedrock fractures: Evidence from stream water radon and water isotopes

Geologic features (e.g., fractures and alluvial fans) can play an important role in the locations and volumes of groundwater discharge and degree of groundwater-surface water (GW-SW) interactions. However, the role of these features in controlling GW-SW dynamics and streamflow generation processes are not well constrained. GW-SW interactions and streamflow generation processes are further complicated by variability in precipitation inputs from summer and fall monsoon rains, as well as declines in snowpack and changing melt dynamics driven by warming temperatures. Using high spatial and temporal resolution radon and water stable isotope sampling and a 1D groundwater flux model, we evaluated how groundwater contributions and GW-SW interactions varied along a stream reach impacted by fractures (fractured-zone) and below the fractured hillslope (non-fractured zone) in Coal Creek, a Colorado River headwater stream affected by summer monsoons. During early summer, groundwater contributions from the fractured zone dominated, but declined throughout the summer. Groundwater contributions from the non-fractured zone were constant throughout the summer and became proportionally more important later in the summer. We hypothesize that groundwater in the non-fractured zone is dominantly sourced from a high-storage alluvial fan at the base of a tributary that is connected to Coal Creek throughout the summer and provides consistent groundwater influx. Water isotope data revealed that Coal Creek responds quickly to incoming precipitation early in the summer, and summer precipitation becomes more important for streamflow generation later in the summer. We quantified the change in catchment dynamic storage and found it negatively related to stream water isotope values, and positively related to modeled groundwater discharge and the ratio of fractured zone to non-fractured zone groundwater. Importantly, we interpret these relationships as declining hydrologic connectivity throughout the summer leading to late summer streamflow supported predominantly by shallow flow paths, with variable response to drying from geologic features based on their storage. As groundwater becomes more important for sustaining summer flows, quantifying local geologic controls on groundwater inputs and their response to variable moisture conditions may become critical for accurate predictions of streamflow.

54 ENVIRONMENTAL SCIENCES↗

β-decay and β-delayed Neutron Emission Measurements at GSI-FRS Beyond N=126, for r-process Nucleosynthesis

New measurements of very exotic nuclei in the neutron-rich region beyond N=126 have been performed at the GSI facility with the fragment separator (FRS). The aim of the experiment is to determine half-lives and β-delayed neutron emission branching ratios of isotopes of Hg, Tl and Pb in this region. This contribution summarizes final counting statistics for identification and for implantation, as well as the present status of the data analysis of the half-lives. In summary, isotopes of Pt, Au, Hg, Tl, Pb, Bi, Po, At, Rn and Fr were clearly identified and several of them ({sup 208-211}Hg, {sup 211-215}Tl, {sup 214-218}Pb) were implanted with enough statistics to determine their half-lives. About half of them are expected to be neutron emitters, in such cases it will become possible to obtain the neutron emission probabilities, Pn.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Radiological Monitoring of Waste Treatment Plant

Scheduled waste in West Malaysia is handled by Concession Company and is stored and then is incinerated. It is known that incineration process may result in naturally occurring radioactive materials (NORM) to be concentrated. In this study we have measured three samples consist of by-product from the operation process such as slag, filter cake and fly ash. Other various environmental media such as air, surface water, groundwater and soil within and around the plant have also been analysed for their radioactivity levels. The concentration of Ra-226, Ac-228 and K-40 in slag are 0.062 Bq/g, 0.016 Bq/g and 0.19 Bq/g respectively. The total activity (Ra{sub eq}) in slag is 99.5 Bq/kg. The concentration in fly ash is 0.032 Bq/g, 0.16 Bq/g and 0.34 Bq/g for Ra-226, Ac-228 and K-40 respectively resulting in Raeq of 287.0 Bq/kg. For filter cake, the concentration is 0.13 Bq/g, 0.031 Bq/g and 0.33 Bq/g for Ra-226, Ac-228 and K-40 respectively resulting in Raeq of 199.7 Bq/kg. The external radiation level ranges from 0.08 {mu}Sv/h (Administrative building) to 0.35 {mu}Sv/h (TENORM storage area). The concentration level of radon and thoron progeny varies from 0.0001 to 0.0016 WL and 0.0006 WL to 0.002 WL respectively. For soil samples, the activity ranges from 0.11 Bq/g to 0.29 Bq/g, 0.06 Bq/g to 0.18 Bq/g and 0.065 Bq/g to 0.38 Bq/g for Ra-226, Ac-228 and K-40 respectively. While activity in water, except for a trace of K-40, it is non-detectable.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗