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At least 19 records

Anthropogenic sulfate-climate interactions suppress dust activity over East Asia

Observational evidences indicate a significant decline in dust storm frequencies over the East Asian arid-semiarid region during recent decades, which creates a strong contrast with a great increase in sulfate emissions over monsoonal Asia. However, the causes for decline of dust activities are still controversial. Through conducting a set of idealized sensitivity experiments of regional aerosol perturbations, here we show that anthropogenic sulfate aerosols over monsoonal Asia remarkably suppress the regional dust activities over East Asia. Southward shift of Asian westerly jet stream induced by sulfate aerosols results in increasing precipitation and weakening surface wind speeds over the arid-semiarid region, thereby suppressing local dust emission fluxes. Further, the latest Sixth Coupled Model Intercomparison Project simulations indicate that anthropogenic aerosols partly drive the recent weakening in regional dust activities and that future change of regional dust activities will likely depend on emissions scenarios of Asian anthropogenic aerosols and greenhouse gases.

54 ENVIRONMENTAL SCIENCES↗

Anthropogenic sulfate aerosol pollution in South and East Asia induces increased summer precipitation over arid Central Asia

Precipitation has increased across the arid Central Asia region over recent decades. However, the underlying mechanisms of this trend are poorly understood. Here, we analyze multi-model simulations from the Precipitation Driver and Response Model Intercomparison Project (PDRMIP) to investigate potential drivers of the observed precipitation trend. We find that anthropogenic sulfate aerosols over remote polluted regions in South and East Asia lead to increased summer precipitation, especially convective and extreme precipitation, in arid Central Asia. Elevated concentrations of sulfate aerosols over remote polluted Asia cause an equatorward shift of the Asian Westerly Jet Stream through a fast response to cooling of the local atmosphere at mid-latitudes. This shift favours moisture supply from low-latitudes and moisture flux convergence over arid Central Asia, which is confirmed by a moisture budget analysis. High levels of absorbing black carbon lead to opposing changes in the Asian Westerly Jet Stream and reduced local precipitation, which can mask the impact of sulfate aerosols. This teleconnection between arid Central Asia precipitation and anthropogenic aerosols in remote Asian polluted regions highlights long-range impacts of anthropogenic aerosols on atmospheric circulations and the hydrological cycle.

54 ENVIRONMENTAL SCIENCES↗

Isolating the effect of biomass burning aerosol emissions on 20th century hydroclimate in South America and Southeast Asia

Abstract Biomass burning is a significant source of aerosol emissions in some regions and has a considerable impact on regional climate. Earth system model simulations indicate that increased biomass burning aerosol emissions contributed to statistically significant decreases in tropical precipitation over the 20th century. In this study, we use the Community Earth System Model version 1 Large Ensemble (CESM1-LENS) experiment to evaluate the mechanisms by which biomass burning aerosol contributed to decreased tropical precipitation, with a focus on South America and Southeast Asia. We analyze the all-but-one forcing simulations in which biomass burning aerosol emissions are held constant while other forcings (e.g., greenhouse gas concentrations) vary throughout the 20th century. This allows us to isolate the influence of biomass burning aerosol on processes that contribute to decreasing precipitation, including cloud microphysics, the radiative effects of absorbing aerosol particles, and alterations in regional circulation. We also show that the 20th century reduction in precipitation identified in the CESM1-LENS historical and biomass burning experiments is consistent across Coupled Model Intercomparison Project Phase 5 models with interactive aerosol schemes and the CESM2 single-forcing experiment. Our results demonstrate that higher concentrations of biomass burning aerosol increases the quantity of cloud condensation nuclei and cloud droplets, limiting cloud droplet size and precipitation formation. Additionally, absorbing aerosols (e.g., black carbon) contribute to a warmer cloud layer, which promotes cloud evaporation, increases atmospheric stability, and alters regional circulation patterns. Corresponding convectively coupled circulation responses, particularly over the tropical Andes, contribute to further reducing the flow of moisture and moisture convergence over tropical land. These results elucidate the processes that affect the water cycle in regions prone to biomass burning and inform our understanding of how future changes in aerosol emissions may impact tropical precipitation over the 21st century.

Environmental Sciences & Ecology↗

Impact of solar geoengineering on temperatures over the Indonesian Maritime Continent

Climate change has been projected to increase the intensity and magnitude of extreme temperature in Indonesia. Solar radiation management (SRM) has been proposed as a strategy to temporarily combat global warming, buying time for negative emissions. Though the global impacts of SRM have been extensively studied in recent years, regional impacts, especially in the tropics, have received much less attention. This paper investigates the potential stratospheric sulfate aerosol geoengineering to modify mean and extreme temperature, as well as the relative humidity and wet bulb temperature (WBT) change over Indonesian Maritime Continent (IMC) based on simulations from three different earth system models. We applied statistical downscaling and corrected the bias of model output to reproduce historical temperatures and relative humidity over IMC. We compared SRM as specified by the Geoengineering Model Intercomparison Project (GeoMIP) G4 experiment – 5 Tg of SO 2 into the lower stratosphere between 2020 and 2069 – concurrent with the RCP4.5 emissions scenario. SRM is able to significantly reduce the temperature means and extremes, and although differences in magnitude of response and spatial pattern occur, there is a generally consistent response. Additionally, the spatial response of changes forced by RCP4.5 scenario and SRM impact is notably heterogeneous in the archipelago, highlighting uncertainties that would be critical in assessing socio-economic consequences of both doing, and not doing SRM. In general, SRM has bigger impacts in reducing temperatures over land than oceans, and the southern monsoon region shows more variability. SRM is also effective at reducing the likelihood of WBT > 27OC events compared to RCP4.5 after some years of SRM deployment as well as during the post-termination period of SRM. Regional downscaling may be an effective tool in obtaining policy-relevant information about local effects of different future scenarios involving SRM.

54 ENVIRONMENTAL SCIENCES↗

The Observed and Projected Changes of Global Monsoons: Current Status and Future Perspectives

The global monsoon system, encompassing the Asian-Australian, African, and American monsoons, sustains two-thirds of the world’s population by regulating water resources and agriculture. Monsoon anomalies pose severe risks, including floods and droughts. Recent research associated with the implementation of the Global Monsoons Model Intercomparison Project under the umbrella of CMIP6 has advanced our understanding of its historical variability and driving mechanisms. Observational data reveal a 20th-century shift: increased rainfall pre-1950s, followed by aridification and partial recovery post-1980s, driven by both internal variability (e.g., Atlantic Multidecadal Oscillation) and external forcings (greenhouse gases, aerosols), while ENSO drives interannual variability through ocean-atmosphere interactions. Future projections under greenhouse forcing suggest long-term monsoon intensification, though regional disparities and model uncertainties persist. Models indicate robust trends but struggle to quantify extremes, where thermodynamic effects (warming-induced moisture rise) uniformly boost heavy rainfall, while dynamical shifts (circulation changes) create spatial heterogeneity. Volcanic eruptions and proposed solar radiation modification (SRM) further complicate predictions: tropical eruptions suppress monsoons, whereas high-latitude events alter cross-equatorial flows, highlighting unresolved feedbacks. The emergent constraint approach is booming in terms of correcting future projections and reducing uncertainty with respect to the global monsoons. Critical challenges remain. Model biases and sparse 20th-century observational data hinder accurate attribution. The interplay between natural variability and anthropogenic forcings, along with nonlinear extreme precipitation risks under warming, demands deeper mechanistic insights. Additionally, SRM’s regional impacts and hemispheric monsoon interactions require systematic evaluation. Addressing these gaps necessitates enhanced observational networks, refined climate models, and interdisciplinary efforts to disentangle multiscale drivers, ultimately improving resilience strategies for monsoon-dependent regions.

climate extreme events↗

Examining the Impacts of Microphysical-Dynamical Feedbacks on Convective Clouds in Different Aerosol Environments Using Enhanced Observational and Modeling Strategies

This project investigated how microphysical–dynamical feedbacks influence deep convective clouds across a range of aerosol conditions, storm lifecycles, and meteorological regimes, and how these sensitivities depend on the modeling framework used to represent convection and microphysics. Using the Aerosol, Cloud, Precipitation, and Climate (ACPC) Working Group model intercomparison simulations of isolated deep convection in the Houston region, we found a robust warm-phase aerosol response in most cloud-resolving models. Increased aerosol loading tended to suppress warm-rain production, increase cloud water, and reduce surface rainfall and near-surface evaporation. These impacts were typically strongest early in the convective lifecycle, with the largest aerosol-driven differences occurring during the first half of storm evolution. The ice-phase response, on the other hand, varied widely across modeling frameworks, and differed in sign, timing, and vertical structure. Ice microphysical pathways and parameterizations are therefore leading sources of uncertainty in aerosol–deep convection interactions. Theoretical analyses further suggested that aerosol-driven invigoration through cold-phase processes was much weaker than previously hypothesized for cold-based storms, and in warm-based storms could even reduce updraft strength. These results imply that any invigoration signal is more likely linked to warm-phase processes and peaks early in storm development.

54 ENVIRONMENTAL SCIENCES↗

Climate change penalty and benefit on surface ozone: a global perspective based on CMIP6 earth system models

Abstract This work presents an analysis of the effect of climate change on surface ozone discussing the related penalties and benefits around the globe from the global modelling perspective based on simulations with five CMIP6 (Coupled Model Intercomparison Project Phase 6) Earth System Models. As part of AerChemMIP (Aerosol Chemistry Model Intercomparison Project) all models conducted simulation experiments considering future climate (ssp370SST) and present-day climate (ssp370pdSST) under the same future emissions trajectory (SSP3-7.0). A multi-model global average climate change benefit on surface ozone of −0.96 ± 0.07 ppbv °C −1 is calculated which is mainly linked to the dominating role of enhanced ozone destruction with higher water vapour abundances under a warmer climate. Over regions remote from pollution sources, there is a robust decline in mean surface ozone concentration on an annual basis as well as for boreal winter and summer varying spatially from −0.2 to −2 ppbv °C −1 , with strongest decline over tropical oceanic regions. The implication is that over regions remote from pollution sources (except over the Arctic) there is a consistent climate change benefit for baseline ozone due to global warming. However, ozone increases over regions close to anthropogenic pollution sources or close to enhanced natural biogenic volatile organic compounds emission sources with a rate ranging regionally from 0.2 to 2 ppbv C −1 , implying a regional surface ozone penalty due to global warming. Overall, the future climate change enhances the efficiency of precursor emissions to generate surface ozone in polluted regions and thus the magnitude of this effect depends on the regional emission changes considered in this study within the SSP3_7.0 scenario. The comparison of the climate change impact effect on surface ozone versus the combined effect of climate and emission changes indicates the dominant role of precursor emission changes in projecting surface ozone concentrations under future climate change scenarios.

Zanis, Prodromos↗

Distinct drivers of recent seasonal precipitation increase over Central Asia: roles of anthropogenic aerosols and greenhouse gases

Observational evidence reveals a pronounced wetting trend over Central Asia in recent decades, with the most substantial increases occurring during winter and summer. Yet the extent to which the drivers of these changes differ seasonally remains unknown. Here, we use single-forcing experiments from the Precipitation Driver and Response Model Intercomparison Project (PDRMIP) to examine the effects of various external forcings on winter and summer precipitation across Central Asia and to explore the physical mechanisms underlying seasonal precipitation changes. We find that greenhouse gas (GHG) forcing mainly increases winter precipitation by enhancing atmospheric moisture content through warming. In contrast, in summer, Asian sulfate aerosols enhance precipitation by modulating the westerly jet, which strengthens atmospheric moisture transport into the region. Asian black carbon exerts an opposing influence that partially offsets the sulfate-induced effect. Further attribution analysis based on CMIP6 simulations reinforces these sensitivity results and shows that GHG forcing is the primary driver of winter precipitation increases whereas anthropogenic aerosols dominate summer trends. Future CMIP6 projections suggest that under moderate- to high-emission scenarios, winter precipitation will continue to rise due to increasing GHG concentrations, while summer precipitation may decline across much of Central Asia as a result of reduced aerosol emissions following Asian clean air policies. These findings highlight a distinct seasonality in the drivers of recent precipitation increase and suggest a plausible divergence in future winter and summer precipitation trends.

54 ENVIRONMENTAL SCIENCES↗

Impacts of Suppressing Excessive Light Rain on Aerosol Radiative Effects and Health Risks

Global climate models (GCMs) have been used widely to study radiative forcing and health risks of aerosols. A recent study using two GCMs found that light rain plays a dominant role in controlling aerosol loading. However, “too much light rain and too little heavy rain” is a longstanding bias in GCMs. It is unclear how much light rain affects aerosol-cloud-radiation interactions and health risks from air pollution. Here, in this work, we show that, with the correction of the rainfall intensity spectrum in the National Center for Atmospheric Research Community Atmosphere Model version 5.3 by introducing a stochastic deep convection scheme, the reduced frequency of light rain (1–20 mm d -1 ) results in changes of aerosol direct radiative effects (DRE) of up to -0.5 ± 0.03 W/m 2 and aerosol cloud radiative effects (CRE) of up to -0.9 ± 0.03 W/m 2 . The total (CRE + DRE) radiative effects of light rain-mediated aerosol changes exceed the present-day anthropogenic forcing of aerosols relative to preindustrial levels from the Coupled Model Intercomparison Project (CMIP5&6) models. However, the correction of the rainfall intensity spectrum has little effect on anthropogenic aerosol forcing (defined as the radiative perturbation due to changes in aerosol concentrations between the industrial era and preindustrial levels). Due to increased exposure to fine particulates (PM 2.5 ), the estimated global total premature mortality is much higher than previously estimated, by 300,000 ± 60,000 deaths per year, and is more severe in populous regions such as India and China. The findings in this study highlight the need to understand uncertainties in radiative effects and health risks of aerosols due to simulation biases of precipitation in GCMs.

54 ENVIRONMENTAL SCIENCES↗

North Atlantic Oscillation response in GeoMIP experiments G6solar and G6sulfur: why detailed modelling is needed for understanding regional implications of solar radiation management

The realization of the difficulty of limiting global-mean temperatures to within 1.5 or 2.0°C above pre-industrial levels stipulated by the 21st Conference of Parties in Paris has led to increased interest in solar radiation management (SRM) techniques. Proposed SRM schemes aim to increase planetary albedo to reflect more sunlight back to space and induce a cooling that acts to partially offset global warming. Under the auspices of the Geoengineering Model Intercomparison Project, we have performed model experiments whereby global temperature under the high-forcing SSP5-8.5 scenario is reduced to follow that of the medium-forcing SSP2-4.5 scenario. Two different mechanisms to achieve this are employed: the first via a reduction in the solar constant (experiment G6solar) and the second via modelling injections of sulfur dioxide (experiment G6sulfur) which forms sulfate aerosol in the stratosphere. Results from two state-of-the-art coupled Earth system models (UKESM1 and CESM2-WACCM6) both show an impact on the North Atlantic Oscillation (NAO) in G6sulfur but not in G6solar. Both models show a persistent positive anomaly in the NAO during the Northern Hemisphere winter season in G6sulfur, suggesting an increase in zonal flow and an increase in North Atlantic storm track activity impacting the Eurasian continent and leading to high-latitude warming over Europe and Asia. These results are broadly consistent with previous findings which show similar impacts from stratospheric volcanic aerosol on the NAO and emphasize that detailed modelling of geoengineering processes is required if accurate impacts of SRM effects are to be simulated. Differences remain between the two models in predicting regional changes over the continental USA and Africa, suggesting that more models need to perform such simulations before attempting to draw any conclusions regarding potential continental-scale climate change under SRM.

36 MATERIALS SCIENCE↗

Description of historical and future projection simulations by the global coupled E3SMv1.0 model as used in CMIP6

Abstract. This paper documents the experimental setup and general features of the coupled historical and future climate simulations with the first version of the US Department of Energy (DOE) Energy Exascale Earth System Model (E3SMv1.0). The future projected climate characteristics of E3SMv1.0 at the highest emission scenario (SSP5-8.5) designed in the Scenario Model Intercomparison Project (ScenarioMIP) and the SSP5-8.5 greenhouse gas (GHG) only forcing experiment are analyzed with a focus on regional responses of atmosphere, ocean, sea ice, and land. Due to its high equilibrium climate sensitivity (ECS of 5.3 K), E3SMv1.0 is one of the Coupled Model Intercomparison Project phase 6 (CMIP6) models with the largest surface warming by the end of the 21st century under the high-emission SSP5-8.5 scenario. The global mean precipitation change is highly correlated with the global temperature change, while the spatial pattern of the change in runoff is consistent with the precipitation changes. The oceanic mixed layer generally shoals throughout the global ocean. The annual mean Atlantic meridional overturning circulation (AMOC) is overly weak with a slower change from ∼ 11 to ∼ 6 Sv (Sverdrup) relative to other CMIP6 models. The sea ice, especially in the Northern Hemisphere, decreases rapidly with large seasonal variability. We detect a significant polar amplification in E3SMv1.0 from the atmosphere, ocean, and sea ice. Comparing the SSP5-8.5 all-forcing experiment with the GHG-only experiment, we find that the unmasking of the aerosol effects due to the decline of the aerosol loading in the future projection period causes transient accelerated warming in the all-forcing experiment in the first half of the 21st century. While the oceanic climate response is mainly controlled by the GHG forcing, the land runoff response is impacted primarily by forcings other than GHG over certain regions, e.g., southern North America, southern Africa, central Africa, and eastern Asia. However, the importance of the GHG forcing on the land runoff changes grows in the future climate projection period compared to the historical period.

54 ENVIRONMENTAL SCIENCES↗

Comparison of Current and Future PM2.5 Air Quality in China Under CMIP6 and DPEC Emission Scenarios

The latest scenarios for the sixth Coupled Model Intercomparison Project (CMIP6) provide opportunities to explore future climate and air pollution mitigation pathways with socioeconomic features. However, to what extent inadequate consideration of region-specific policies in the CMIP6 scenarios would affect regional air quality projections is still not clear. Here, we simulated China’s future PM2.5 concentrations and compositions with local policy-based scenarios and the original CMIP6 datasets, for the first time estimating future air quality differences induced by the lack of local pollution control policies in the CMIP6 scenarios. We found that the CMIP6-driven projections overestimate major chemical aerosols by 10% – 70% in 2015 and fail to capture the rapid PM2.5 concentration decline during 2015–2019. Near-term differences further lead to 43% – 49% (5 – 9 µg/m3) PM2.5 overpredictions in 2050 in CMIP6 scenarios compared with policy-based mitigation scenarios. Our study demonstrates the indispensable influences of local policies on regional analyses and suggests that the research community should incorporate more region-specific information in future scenario designs.

Cheng, Jing↗

Interconnection of Aerosol‐Cloud Interactions and Cloud Feedback Through Warm Rain Process

Recent research has revealed a correlation within the Coupled Model Intercomparison Project Phase 6 (CMIP6) simulations: models exhibiting more pronounced warming due to positive cloud feedback simultaneously show enhanced cooling from aerosol‐cloud interactions (ACI). However, the interplay between ACI and cloud feedback is not well understood in these models. Our study addresses this gap by modifying the autoconversion rate in two Earth system models (ESMs), elucidating how ACI could connect with cloud feedback through the warm rain process. We find that higher autoconversion rates, which are associated with stronger ACI, suppress the increase in cloud liquid water path (LWP) and cloud optical depth with warming by enhancing the precipitation efficiency over the extratropical regions, leading to a larger positive cloud feedback. This study offers new insights into the compensatory mechanism between ACI and cloud feedback through the warm rain process and highlights the importance of constraining the autoconversion parameterization in models.

54 ENVIRONMENTAL SCIENCES↗

A Strong Anthropogenic Black Carbon Forcing Constrained by Pollution Trends Over China

Estimates of the effective radiative forcing from aerosol-radiation interaction (ERF ari ) of anthropogenic Black Carbon (BC) have been disputable and require better constraints. Here we find a substantial decline in atmospheric absorption of −5.79Wm −2 decade −1 over eastern central China (ECC) responding to recent anthropogenic BC emission reductions. By combining the observational finding with advances from Coupled Model Intercomparison Project phase6 (CMIP6), we identify an emergent constraint on the ERF ari of anthropogenic BC. We show that across CMIP6 models the simulated trends correlate well with simulated annual mean shortwave atmospheric absorption by anthropogenic BC over China. Making use of this emergent relationship allows us to constrain the aerosol absorption optical depth of anthropogenic BC and further provide a constrained range of 2.4–3.0 Wm −2 for its top-of-atmosphere ERF ari over China, higher than existing estimates. Furthermore, our work supports a strong warming effect of BC over China, and highlights the need to improve BC simulations over source regions.

CMIP6 models↗

ARM Data-Oriented Metrics and Diagnostics Package for Climate Model Evaluation

A Python-based metrics and diagnostics package is currently being developed by the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Infrastructure Team at Lawrence Livermore National Laboratory (LLNL) to facilitate the use of long-term, high-frequency measurements from the ARM Facility in evaluating the regional climate simulation of clouds, radiation, and precipitation. This metrics and diagnostics package computes climatological means of targeted climate model simulation and generates tables and plots for comparing the model simulation with ARM observational data. The Coupled Model Intercomparison Project (CMIP) model data sets are also included in the package to enable model intercomparison as demonstrated in Zhang et al. (2017). The mean of the CMIP model can serve as a reference for individual models. Basic performance metrics are computed to measure the accuracy of mean state and variability of climate models. The evaluated physical quantities include cloud fraction, temperature, relative humidity, cloud liquid water path, total column water vapor, precipitation, sensible and latent heat fluxes, and radiative fluxes, with plan to extend to more fields, such as aerosol and microphysics properties. Process-oriented diagnostics focusing on individual cloud- and precipitation-related phenomena are also being developed for the evaluation and development of specific model physical parameterizations. The version 1.0 package is designed based on data collected at ARM’s Southern Great Plains (SGP) Research Facility, with the plan to extend to other ARM sites. The metrics and diagnostics package is currently built upon standard Python libraries and additional Python packages developed by DOE (such as CDMS and CDAT). The ARM metrics and diagnostic package is available publicly with the hope that it can serve as an easy entry point for climate modelers to compare their models with ARM data. In this report, we first present the input data, which constitutes the core content of the metrics and diagnostics package in section 2, and a user's guide documenting the workflow/structure of the version 1.0 codes, and including step-by-step instruction for running the package in section 3.

54 ENVIRONMENTAL SCIENCES↗

RCEMIP‐ACI: Aerosol‐Cloud Interactions in a Multimodel Ensemble of Radiative‐Convective Equilibrium Simulations

Aerosol‐cloud interactions are a persistent source of uncertainty in climate research. This study presents findings from a model intercomparison project examining the impact of aerosols on clouds and climate in convection‐permitting radiative‐convective equilibrium (RCE) simulations. Specifically, 11 different modeling teams conducted RCE simulations under varying aerosol concentrations, domain configurations, and sea surface temperatures (SSTs). We analyze the response of domain‐mean cloud and radiative properties to imposed aerosol concentrations across different SSTs. Additionally, we explore the potential impact of aerosols on convective aggregation and large‐scale circulation in large‐domain simulations. The results reveal that the cloud and radiative responses to aerosols vary substantially across models. However, a common trend across models, SSTs, and domain configurations is that increased aerosol loading tends to suppress warm rain formation, enhance cloud water content in the mid‐troposphere, and consequently increase mid‐tropospheric humidity and upper‐tropospheric temperature, thereby impacting static stability. The warming of the upper troposphere can be attributed to reduced lateral entrainment effects due to the higher environmental humidity in the mid‐troposphere. However, models do not agree on aerosol impacts on convective updraft velocity based on the preliminary examination of high‐percentiles of vertical velocity at a single mid‐troposheric layer (500 hPa). In large‐domain simulations, where convection tends to self‐organize, aerosol loading does not consistently influence self‐organization but tends to reduce the intensity of large‐scale circulation forming between convective clusters and dry regions. This reduction in circulation intensity can be explained by the increase in static stability due to the upper tropospheric warming.

54 ENVIRONMENTAL SCIENCES↗

The Misrepresentation of the Southern African Easterly Jet in Models and Its Implications for Aerosol, Clouds, and Precipitation Distributions

The southern African easterly jet (AEJ-S) is an important midtropospheric feature critical to understanding the tropical convective system over central Africa and the aerosol–cloud interactions over the southeast Atlantic Ocean. However, it remains unclear how well models represent the AEJ-S and its influence on aerosol transport, clouds, and precipitation distribution. Here, in this work, we use ground- and satellite-based observations and reanalysis datasets to assess the representation of AEJ-S in the Coupled Model Intercomparison Project phase 6 (CMIP6) models between September and October during the peak of midtropospheric winds, aerosol transport, clouds, and precipitation. We find that most CMIP6 models have difficulty accurately simulating the strength, position, and spatial distribution of the AEJ-S. Specifically, the AEJ-S is relatively weaker and at a slightly lower altitude in the ensemble of CMIP6 models than represented by observation and reanalysis datasets. To assess the influence of the misrepresented the AEJ-S on CMIP6-simulated aerosol, clouds, and precipitation distributions, we performed composite analyses using models with low and high biases based on the estimates of their midtropospheric easterly wind speed. We find that the misrepresentation of the AEJ-S in CMIP6 models is associated with the overestimation of clouds and precipitation over central Africa, the underestimation of clouds over the southeast Atlantic Ocean, and the limitation of aerosol transport over the continent or the deviation of its spatial distribution from the typical zonal transport over the Atlantic Ocean. Because aerosols, clouds, and precipitation are important components of the regional climate system, we conclude that accurate representation of the AEJ-S is essential over central Africa and the southeast Atlantic Ocean.

54 ENVIRONMENTAL SCIENCES↗

Distinct responses of Asian summer monsoon to black carbon aerosols and greenhouse gases

Black carbon (BC) aerosols emitted from natural and anthropogenic sources induce positive radiative forcing and global warming, which in turn significantly affect the Asian summer monsoon (ASM). However, many aspects of the BC effect on ASM remain elusive and largely inconsistent among previous studies, which is strongly dependent on different low-level thermal feedbacks over the Asian continent and the surrounding ocean. This study examines the response of ASM to BC forcing in comparison with the effect of doubled greenhouse gases (GHGs) by analyzing the Precipitation Driver Response Model Intercomparison Project (PDRMIP) simulations under an extreme high BC level (10 times modern global BC emissions or concentrations, labeled by BC $\times$ 10) from nine global climate models (GCMs). The results show that although BC and GHGs both enhance the ASM precipitation minus evaporation (P–E) (a 13.6 % increase for BC forcing and 12.1 % for GHGs from the nine-model ensemble, respectively), there exists a much larger uncertainty in changes in ASM P–E induced by BC than by GHGs. The summer P–E is increased by 7.7 % to 15.3 % due to these two forcings over three sub-regions including East Asian, South Asian, and western North Pacific monsoon regions. Further analysis of moisture budget reveals distinct mechanisms controlling the increases in ASM P–E induced by BC and GHGs. The change in ASM P–E by BC is dominated by the dynamic effect due to the enhanced large-scale monsoon circulation, whereas the GHG-induced change is dominated by the thermodynamic effect through increasing atmospheric water vapor. Radiative forcing of BC significantly increases the upper-level atmospheric temperature over the Asian region to enhance the upper-level meridional land-sea thermal gradient (MLOTG), resulting in a northward shift of the upper-level subtropical westerly jet and an enhancement of the low-level monsoon circulation; whereas radiative forcing of GHGs significantly increases the tropical upper-level temperature, which reduces the upper-level MLOTG and suppresses the low-level monsoonal circulation. Hence, our results indicate a different mechanism of BC climate effects under the extreme high BC level, that BC forcing significantly enhances the upper-level atmospheric temperature over the Asian region, determining ASM changes, instead of low-level thermal feedbacks as indicated by previous studies.

54 ENVIRONMENTAL SCIENCES↗