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Nuclear Data Sheets for A = 129

The experimental nuclear spectroscopic data for known nuclides of mass number 129 (Ag, Cd, In, Sn, Sb, Te, I, Xe, Cs, Ba, La, Ce, Pr, Nd, Pm, Sm) have been evaluated and presented together with adopted properties for levels and γ rays. This evaluation represents a revision of the previous one 18 years ago by Y. Tendow (1996Te01). Extensive new data have become available for many nuclides in the intervening years, although, no data are available for excited states in {sup 129}Pm and {sup 129}Sm, and for {sup 129}Ag and {sup 129}Cd, only limited information is available for the g.s. and isomers. The decay schemes of {sup 129}Ag, {sup 129}Pm and {sup 129}Sm are unknown, and those for {sup 129}Cd, {sup 129}In, {sup 129}Ce, {sup 129}Pr and {sup 129}Nd are incomplete. Many γ rays and extended level schemes have been reported for the ground state and isomer decays of {sup 129}Ba to {sup 129}Cs, yet the adopted set of intensities in this evaluation originate from a brief paper in an annual laboratory report. There remain several unplaced gamma rays, coupled with ambiguity about division of intensities amongst the two activities of {sup 129}Ba with nearly the same half-lives. Isomerism is expected in {sup 129}Pr, but there is no confirmed identification. Low-lying level structure in {sup 129}Nd, including identification of a possible third long-lived isomer in this nuclide, remains uncertain. The spin-parity assignments of (5/2+) for the ground state and (7/2−) for an isomer at 107.6 keV in {sup 129}Ce are assigned based on strong support from systematics and band configurations, yet this result is in contradiction with the quadrupole interaction hyperfine structure measurement which favors 9/2− over 7/2− for the isomer, consequently 7/2+ for the ground state. Direct measurements of spins of ground state and isomer of {sup 129}Ce are needed to settle this issue. Confirmed spins and parities of the ground state and isomer of {sup 129}La are also lacking. Assignments in this work are mainly based on systematics of h{sub 11/2} decoupled structures. A direct measurement of ground state spin of {sup 129}La will also be desirable. Recommended data presented in this work supersede those in previous NDS evaluations of A=129 nuclides published by 1996Te01, 1983Ha46 and 1972Ho55.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Structure and magnetic properties of the REAuBi{sub 2} (RE=La–Nd, Sm) phases

We present the crystal structures and basic magnetic properties of the REAuBi{sub 2} (RE=La–Nd, Sm) compounds. This isostructural family crystallizes in the tetragonal P4/nmm (no. 129) HfCuSi{sub 2}-type, as determined by single crystal X-ray diffraction. Three distinct substructures are present: an RE layer, a tetrahedral AuBi layer, and a Bi square net layer. Electronic structure calculations indicate that these compounds display bands which cross the Fermi level, derived from both the Bi square net and the covalent AuBi layer. The small size of LaAuBi{sub 2} crystals precluded detailed physical property measurements, whereas large single crystals could be grown for all other phases investigated here. Single crystal measurements of CeAuBi{sub 2}, PrAuBi{sub 2}, and NdAuBi{sub 2} show overall antiferromagnetic ordering and decreasing magnetic anisotropy with decreasing rare earth size. SmAuBi{sub 2} also shows signatures of magnetic ordering. - Graphical abstract: The crystal structures and basic electronic and magnetic properties of the five REAuBi{sub 2} (RE=La–Nd, Sm) phases are presented. These tetragonal structures have alternating layers of AuBi{sub 4} tetrahedra and a Bi square net balanced by RE cations. Measurements performed on single crystals show strong magnetic anisotropy for CeAuBi{sub 2} and PrAuBi{sub 2} and weak anisotropy for NdAuBi{sub 2}. SmAuBi{sub 2} is weakly magnetic. - Highlights: • We present the structures and basic properties of single crystals of the new, tetragonal REAuBi{sub 2} (RE=La–Nd, Sm) phases. • CeAuBi{sub 2}, PrAuBi{sub 2}, NdAuBi{sub 2}, and SmAuBi{sub 2} order magnetically. • CeAuBi{sub 2} and PrAuBi{sub 2} display magnetic anisotropy. • CeAuBi{sub 2} appears analogous to CeAuSb{sub 2} and may be worthy of further study as a potential system for quantum criticality.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗