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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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A Predictive Transient Model of the TREAT-SIRIUS Experiments

To support experiments modeling and transient analysis of the NASA-sponsored SIRIUS experiments in the Transient Reactor Test Facility (TREAT), an innovative predictive transient model has been developed to simulate various transient experiments. The developed model is based on a new approach that utilizes steady-state Monte Carlo calculations along with a surrogate model based on polynomial regression to determine the core reactivity. The reactivity is supplied to an exact point kinetics model that determines the reactor power, and it is coupled to an adiabatic feedback model to determine the fuel average temperature. In this work, the newly developed model is introduced along with validation test results considering SIRIUS-1 experiments at different power levels. The initial test results show a very good agreement with experimental data at different power levels, which indicates that the model can be used to predict the power of other transient tests.

42 ENGINEERING↗

Data Compilation and Analysis from the Sirius-1 Experiment at TREAT for Transient Simulation Validation

This report assembles comprehensive data from the Sirius-1 experiment conducted by Idaho National Laboratory in collaboration with the National Aeronautics and Space Administration. The primary goal is to provide a robust data set that external users can utilize for the validation of computational methods for transient multiphysics simulations. By compiling all relevant data, including experiment design calculations, detailed engineering drawings for the experiment and data from reactor and fuel specimen measurement, this report is intended to serves as a reference for researchers and engineers working on the development and validation of computational models for transient nuclear behavior.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Sirius Irradiation Experiments and Post-Irradiation Examinations for Nuclear Thermal Propulsion

Nuclear Thermal Propulsion (NTP) systems hold promise in reducing transit times for exploration of the solar system by both crewed and uncrewed missions. NTP systems currently under investigation include a once-through high temperature gas-cooled fission reactor to provide thermal energy to heat the coolant which also serves as the propellant. The fuel systems of angular UN fuel particles dispersed in a matrix of W/Re, creating a ceramic and metallic composite or cermet, has been irradiated in Idaho National Laboratory’s (INL) Transient Reactor Test Facility (TREAT) enabling evaluation of these materials under representative nuclear heating rates (~95 K/s) and peak temperatures (~2527 K). These tests named Sirius-1 (UN-W/Re), have been irradiated and this paper will present post-irradiation examination results. The Sirius-1 test produced cracks in the fuel specimen and spalling of surface material. Uranium soot was found on the inner wall of the irradiation capsule indicating loss of some fissile material from the fuel specimen. Spalling from the surfaces was also noted upon visual inspection. Uranium diffusion from the fuel particles resulted in the formation of U/Re phases and edge features producing a laminar microstructure.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Multiphysics Simulation of the NASA SIRIUS-CAL Fuel Experiment in the Transient Test Reactor Using Griffin

After approximately 50 years, NASA is restarting efforts to develop nuclear thermal propulsion (NTP) for interplanetary missions. Building upon nuclear engine tests performed from the late 1950s to the early 1970s, the present research and testing focuses on advanced materials and fabrication methods. A number of transient tests have been performed to evaluate materials performance under high-temperature, high-flux conditions, with several more experiments in the pipeline for future testing. The measured data obtained from those tests are being used to validate the Griffin reactor multiphysics code for this particular type of application. Griffin was developed at Idaho National Laboratory (INL) using the MOOSE framework. This article describes the simulation results of the SIRIUS-CAL calibration experiment in the Transient Reactor Test Facility (TREAT). SIRIUS-CAL was the first transient test conducted on NASA fuels, and although the test was performed with a relatively low core peak power, the test specimen survived a temperature exceeding 900 K. Griffin simulations of the experiment successfully matched the reactor’s power transient after calibrating the initial control rod position to match the initial reactor period. The thermal-hydraulics model largely matches the time-dependent response of a thermocouple located within the experiment specimen to within the uncertainty estimate. However, the uncertainty range is significant and must be reduced in the future.

33 ADVANCED PROPULSION SYSTEMS↗

Thermal Analysis of the Sirius-3 Nuclear Propulsion Fuel Experiments

To support long space missions, NASA is designing and testing different fuels for nuclear thermal propulsion. These designs include a number ceramic metallic fuels which are to be irradiated in the Tranisent Test Reactor to test the fuel’s performance at protypical conditions. The irradiation campaign of these fuels is referred to as the Sirius experiments, and includes single and stacked experiment samples. In this paper we present the thermal analysis of the Sirius-3 experiment. For this analysis, temperatures from a Bison finite element model are compared to the temperatures obtained from an experiment thermocouple where good agreement between the two are found. Because agreement of the thermocouple and Bison finite element model, insight into the heat flow is provided to experimenters as they design future experiments. As an example of this insight, the rods through the fuel specimen as shown in Sirius A and B [1] were removed and replaced with hold down rings for the Sirius-2C

33 ADVANCED PROPULSION SYSTEMS↗

Thermal Analysis of the SIRIUS3 Nuclear Propulsion Fuel Calibration Experiment

NASA is considering Nuclear Thermal Propulsion (NTP) for long range extraterrestrial missions; these engines eject hot hydrogen gas heated by a nuclear reactor for rocket thrust. To economize the use of hydrogen to the greatest extent possible, the NTP engines will be expected to, in a very short time (i.e., on the order of a minute or less), go from warm$(\sim 300 K)$ zero power conditions to full operational power, with a coolant outlet temperature on the order of 2700–3000 K \cite{en15176181}. These conditions will introduce significant thermomechanical stresses on the NTP fuel. The objective of the SIRIUS series of experiments is to examine the performance of candidate NTP fuel materials when subjected to temperature ramp rates that are prototypical of NTP system startup and operation. The SIRIUS experiments are a series of experiments that will be irradiated in the TREAT reactor and are subjected to power ramps and cycles that are prototypical for NTP operation. The experiments will be accomplished by executing a series of shaped transients on the SIRIUS specimens while collecting in situ specimen temperature data. These tests will determine whether operational startup ramps and peak temperatures will result in detrimental fuel performance phenomena (i.e. fuel deformation, fragmentation and cracking) To this end, INL has been evaluating a number of SIRIUS experiments, and these evaluations include thermal analysis of the SIRIUS experiments. Thermal analysis were performed for the calibration irradiation of the SIRIUS-3 experiment, and the focus of this memo is to document the results from the calibration irradiation thermal analysis. The thermal analysis reveals that radiation heat emission of the outer fuel elements and conduction to different metal components such as the molybdenum element tubes remove significant quantities of heat from the fuel element specimen, and future experiment designs need to consider these heat transfer mechanics. This paper begins with a brief experiment overview with a discussion of the fuel sample and experiment configuration. The experiment and model description section is followed by a set of results with a brief discussion, and finally the memo concludes with suggestion for future work.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Prediction of The TREAT Facility Power and Temperature of Sirius-2c Nuclear Propulsion Fuel Experiment

This paper presents simulation results of the Sirius-2c full power experiment that was performed at the TREAT facility to support experiment modeling and transient analysis of the NASA-sponsored Sirius series of experiments for nuclear thermal propulsion applications. We presents a novel approach to predict the control rod motion and power of the reactor and the temperature of the specimen during transient experiments using the Griffin and Bison packages of the Multiphysics Object Oriented Simulation Environment (MOOSE). First, the model predicts the transient rod motion that results in the desired reactor power shape. Then, the temperature of the specimen is predicted based on the power deposited in the specimen. The prediction results are in good agreement with the measured reactor power and control rod position and over-predicted the specimen temperature which is mainly related to specimen surface emissivities. The reactor reaches a peak power of 80 MW and a specimen temperature of 2500 K and considering the right specimen emissivities the predicted temperature is in an excellent agreement with the measured values. This model can be utilized in helping and supporting the design and optimization a new experiments that are going to be irradiated in the TREAT facility.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Forward and inverse predictive transient models of TREAT using surrogate reactivity models

In this work, we present two novel approaches for predicting the power evolution and control rod height of the Transient Reactor Test Facility (TREAT) to support experiment modeling; specifically, transient analysis of the NASA-sponsored Sirius series of experiments. These approaches utilize steady-state Monte Carlo model, point kinetics model, and surrogate models to predict power evolution and control rod axial position during transient experiments. Both approaches were tested and validated against several Sirius experiments that were performed in the TREAT facility at different power levels. The validation test results show very good agreement with the experimental data, and the models were able to accurately predict the power evolution and the axial control rod position with an average error within 3.0%. Finally, this indicates that these approaches will help the reactor engineering team of the TREAT facility in preparing and predicting the power and temperature of the experiment.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

New Grids of Pure-hydrogen White Dwarf NLTE Model Atmospheres and the HST/STIS Flux Calibration

Nonlocal thermodynamic equilibrium (NLTE) calculations of hot white dwarf (WD) model atmospheres are the cornerstone of modern flux calibrations for the Hubble Space Telescope and for the CALSPEC database. These theoretical spectral energy distributions (SEDs) provide the relative flux versus wavelength, and only the absolute flux level remains to be set by reconciling the measured absolute flux of Vega in the visible with the Midcourse Space Experiment values for Sirius in the mid-IR. The most recent SEDs calculated by the tlusty and tmap NLTE model atmosphere codes for the primary WDs G191-B2B, GD 153, and GD 71 show improved agreement to 1% from 1500 Å to 30 μm, in comparison to the previous 1% consistency only from 2000 Å to 5 μm. These new NLTE models of hot WDs now provide consistent flux standards from the far UV to the mid-IR.

79 ASTRONOMY AND ASTROPHYSICS↗

Post-irradiation examination of UN-Mo-W fuels for space nuclear propulsion

The National Aeronautics and Space Administration's return to space nuclear propulsion stems from the need for a more efficient method of space travel. Nuclear thermal propulsion systems have been shown to be two times more efficient than chemical propulsion. NASA's Sirius program was created to fabricate and test fuels for space nuclear propulsion, specifically to determine their performance under prototypical startup conditions. The Sirius project featured 4 test capsules, Sirius-1 featured uranium nitride fuel dispersed in a matrix of tungsten and rhenium, while Sirius-2A, -2B, and -3 featured uranium nitride-molybdenum-tungsten fuel (UN-Mo-W). This study discusses the Sirius-2A and -2B irradiation experiments at the Idaho National Laboratory, specifically their performance under irradiation at the Transient Reactor Test Facility. It was found that the fuel samples overall did not exhibit significant cracking, though the Sirius-2A fuel did have one large crack on the surface of the fuel. There was minimal hydrogen absorption in the samples, though it is unknown if the absorption occurred during irradiation or during fabrication. Mechanical testing indicated that the UN fuel demonstrated ceramic behavior as expected, and the Mo/W matrix demonstrated linear elastic behavior to failure.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sirius I: prototype of a prime-power source for future 1 - 10 GJ fusion-yield experiments

We have designed, assembled, and tested a prototype coaxial impedance-matched Marx generator (IMG). An IMG is a pulsed-power device that achieves electromagnetic-power amplification by triggered emission of radiation. Hence an IMG is a pulsed-power analog of a laser, with an energy efficiency of 90%. We have demonstrated that the prototype performs as predicted theoretically, thereby proving the IMG concept. We propose that a system of IMGs drive a next-generation pulsed-power accelerator that delivers 90 MA to a physics load. Such a machine would attain thermonuclear-fusion yields as high as 1 – 10 GJ, and revolutionize high energy-density-physics experiments in support of the national-security mission.

42 ENGINEERING↗

Opportunities and new developments for the study of surfaces and interfaces in soft condensed matter at the SIRIUS beamline of Synchrotron SOLEIL

The SIRIUS beamline of Synchrotron SOLEIL is dedicated to X-ray scattering and spectroscopy of surfaces and interfaces, covering the tender to mid-hard X-ray range (1.1–13 keV). The beamline has hosted a wide range of experiments in the field of soft interfaces and beyond, providing various grazing-incidence techniques such as diffraction and wide-angle scattering (GIXD/GIWAXS), small-angle scattering (GISAXS) and X-ray fluorescence in total reflection (TXRF). SIRIUS also offers specific sample environments tailored for in situ complementary experiments on solid and liquid surfaces. Recently, the beamline has added compound refractive lenses associated with a transfocator, allowing for the X-ray beam to be focused down to 10 µm × 10 µm while maintaining a reasonable flux on the sample. This new feature opens up new possibilities for faster GIXD measurements at the liquid–air interface and for measurements on samples with narrow geometries.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

(Doublon) Benchmarking of Different Inverse Point Kinetics Implementations for an Autocorrected Reactimeter Algorithm

In November 2017, the Transient Reactor Test Facility returned to operation. Since that time, many transient test series have been completed, such as the Transient Heatsink Overpower Response capsule (THOR), the Transient Water Irradiation System for TREAT (TWIST), and Sirius. Each has provided valuable data for materials performance and reactor safety that can be applied in future designs. During each experimental series, detector count rates provided important information on the core behavior during transients. However, a limitation of these data is that variations in the neutron distribution during experiments can cause errors when attempting to infer reactivity evolution from detector signals. Neutron physics codes can be used to compute the flux shape variations. However, this is a poor solution when the experimental data is used for code verification, validation and uncertainty quantification. Indeed, if the output of the code is used both as a reference and to correct what the reference is compared to, the circular dependency limits the quality of the verification, validation and uncertainty quantification approach. To overcome this problem, the autocorrected reactimeter algorithm (ACRA) has been developed. This approach infers a time-dependent reactivity evolution by testing different spatial corrections and selecting the one that minimizes reactivity variations when the core is in a frozen configuration (i.e., when there is no variation in parameters affecting reactivity). However, the scope of this method was limited to transients where there were negligible thermal feedback. Indeed, the core is never in a frozen configuration when the fuel temperature varies during the whole transient. This is our motivation for developing an improved version of the ACRA that does not require frozen configurations. To develop this new algorithm, we need a precise and unbiased implementation of the inverse point kinetic equations (IPKEs) as any error in the reactivity evaluation will be propagated into the choice of the optimal spatial correction. Indeed, the previous reactimeter algorithm would use approximations, such as a negligible flux amplitude derivative, to focus on rapidity. For the numerical validation of ACRA, we aim at absolute error under for reactivity derived from signals similar to the one of this study. In this summary, we test eight different IPKE implementations. Each will process a mockup signal built for this study, similar to those that the future ACRA will process. Each reactivity output will be compared to the reference reactivity that has been used to generate the mockup signal. The implementation minimizing the difference with the reference reactivity will be used in the development of a new ACRA formulation.

73 - NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A versatile X-ray phase retarder for lock-in XMCD measurements

X-ray magnetic circular dichroism (XMCD) is a technique commonly used to probe magnetic properties of materials with element and orbital selectivity, which requires the use of circularly polarized (CP) X-rays. It is possible to accomplish XMCD experiments with fixed CP and alternating the magnetic field orientation, but most reliable data are obtained when alternating the magnetization orientation and the polarization between right and left helicities. A versatile strategy has been developed to perform XMCD experiments using a hard X-ray quarter-wave plate, at both polychromatic dispersive and conventional monochromatic optics, in combination with synchronous data acquisition. The switching frequency waveform is fed into a lock-in amplifier to detect and amplify the XMCD signal. The results on a reference sample demonstrate an improvement in data quality and acquisition time. The instrumentation successfully generated 98% of CP X-rays switching the beam helicity at 13 Hz, with the possibility of faster helicity switching once it is installed at the new Brazilian fourth-generation source, SIRIUS.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗