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At least 19 records

Unveiling field-transverse spin anisotropy in the spin liquid candidate α-RuCl3 via spin Hall magnetoresistance

α-RuCl3 has emerged as a possible candidate for a quantum spin liquid (QSL) that promises exotic quasiparticles relevant for fault-tolerant quantum computation. Here, we report spin-sensitive transport measurements using a proximal spin Hall metal, platinum (Pt), to probe magnetic moments in the insulator α-RuCl3. We observe spin Hall magnetoresistance (SMR), where both the transverse and longitudinal resistivities exhibit angular oscillations between the in-plane magnetic field and the current, driven by the interplay between the spin Hall effect in Pt and local magnetic moments in α-RuCl3. These oscillations occur from 1.5 to 18 T, covering the zigzag antiferromagnetic, putative QSL, and supposedly partially field-polarized phases. The phase of the SMR oscillations suggests that the local moments, whether static or fluctuating, develop spin anisotropy with a quantization axis in-plane and largely transverse to the magnetic field across all fields from 1.5 to 18 T. Temperature dependence indicates that the spin anisotropy operates at an energy scale similar to that of the reported QSL signatures in α-RuCl3.

Idzuchi, Hiroshi [Tohoku University, Japan]

Spinning Characteristics of the XN2Y-1 Airplane Obtained from the Spinning Balance and Compared with Results from the Spinning Tunnel and from Flight Tests

Report presents the results of tests of a 1/10-scale model of the XN2Y-1 airplane tested in the NACA 5-foot vertical wind tunnel in which the six components of forces and moments were measured. The model was tested in 17 attitudes in which the full-scale airplane had been observed to spin, in order to determine the effects of scale, tunnel, and interference. In addition, a series of tests was made to cover the range of angles of attack, angles of sideslip, rates of rotation, and control setting likely to be encountered by a spinning airplane. The data were used to estimate the probable attitudes in steady spins of an airplane in flight and of a model in the free-spinning tunnel. The estimated attitudes of steady spin were compared with attitudes measured in flight and in the spinning tunnel. The results indicate that corrections for certain scale and tunnel effects are necessary to estimate full-scale spinning attitudes from model results.

Bamber, M J

Spin-tunnel investigation of the spinning characteristics of typical single-engine general aviation airplane designs. 2: Low-wing model A; tail parachute diameter and canopy distance for emergency spin recovery

A spin tunnel study is reported on a scale model of a research airplane typical of low-wing, single-engine, light general aviation airplanes to determine the tail parachute diameter and canopy distance (riser length plus suspension-line length) required for energency spin recovery. Nine tail configurations were tested, resulting in a wide range of developed spin conditions, including steep spins and flat spins. The results indicate that the full-scale parachute diameter required for satisfactory recovery from the most critical conditions investigated is about 3.2 m and that the canopy distance, which was found to be critical for flat spins, should be between 4.6 and 6.1 m.

Burk, S. M., Jr.

Mechanistic implications of excited high-spin states, spin–spin coupling, and differential [2Fe–2S] + cluster temperature relaxations in the electron-bifurcating NfnABC from Thermococcus sibiricus

Electron bifurcation (EB) is a mechanism of biological energy transduction in which multiple oxidation–reduction (redox) reactions are thermodynamically coupled within a single enzyme, enabling the enzyme to harness the excess free energy from an exergonic process to drive an endergonic process. Because of this unprecedented chemistry, there is interest to translate EB principles to artificial and bioengineered systems, but a hurdle is that knowledge pertaining to the fundamental design principles of EB enzymes remains scarce. Here, we investigated the fundamental physical and electronic properties of electron transfer sites in a spectroscopically uncharacterized member of the BfuABC family of EB enzymes, the NADH-dependent reduced-ferredoxin:NADP + oxidoreductase from Thermococcus sibiricus (Tsi NfnABC). Cryo-EM structures of Tsi NfnABC previously demonstrated that it contains twelve redox cofactors: two flavins (one FAD and one FMN), eight [4Fe–4S] clusters, and two [2Fe–2S] clusters. The FMN, one [4Fe–4S] cluster, and one [2Fe–2S] cluster comprise the bifurcating active site termed the electron-bifurcating flavobicluster (BF-FBC), which is found in all BfuABC family members. By using electron paramagnetic resonance spectroscopy, we identified spectral signatures originating from interactions between the FMN radical and [4Fe–4S] + cluster in the BF-FBC and observed temperature dependent behavior of the BF-FBC's [2Fe–2S] + cluster indicative of moderately slow spin–lattice relaxation. Additionally, we uncovered numerous spectral features corresponding to half-integer, S > ½ spin states of [4Fe–4S] + clusters, including one attributable to the consequences of lysine-ligation of a [4Fe–4S] cluster unique to NfnABC. We contextualize these findings to electron transfer theory and NfnABC's structure. Our insights further the understanding of how enzymes are designed to exert control over electron transfer to conduct thermodynamically challenging reactions.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI

Spin squeezing of macroscopic nuclear spin ensembles

Spin squeezing has been explored in atomic systems as a tool for quantum sensing, improving experimental sensitivity beyond the spin standard quantum limit for certain measurements. To optimize absolute metrological sensitivity, it is beneficial to consider macroscopic spin ensembles, such as nuclear spins in solids and liquids. Coupling a macroscopic spin ensemble to a parametrically-modulated resonant circuit can create collective spin squeezing by generating spin correlations mediated by the circuit. We analyze the squeezing dynamics in the presence of decoherence and finite spin polarization, showing that achieving 7 dB spin squeezing is feasible in several nuclear spin systems. The metrological benefit of squeezing a macroscopic spin ensemble lies in the suppression of technical noise sources in the spin detection system relative to the spin projection noise. This expands the experimental sensitivity bandwidth when searching for signals of unknown frequency and can improve the resonant signal-to-noise ratio. Squeezing macroscopic spin ensembles may prove to be a useful technique for fundamental physics experiments aimed at detecting spin interactions with oscillating background fields, such as ultralight dark matter. Published by the American Physical Society 2025

Boyers, Eric

Hidden Spin-Valley Locking Stabilizes Nanosecond Spin Polarization in 2D Perovskites

Room-temperature spin control in semiconductors is fundamental to spin-optoelectronics. Although inversion symmetry breaking offers one path for spin control in semiconductors, strong spin dephasing at elevated temperatures remains a persistent limitation. Hidden spin polarization without global symmetry breaking provides another promising material design strategy, but robust spin stabilization from this effect has yet to be experimentally realized. Here we show spin stabilization at room temperature in two-dimensional hybrid organic-inorganic perovskites through hidden spin-valley locking. We use functional non-primary ammonium cations to induce symmetry-breaking distortions in the metal-halide layers, producing giant local spin splitting while preserving global inversion symmetry. Time-resolved circular dichroism measurements reveal optically generated spin-polarized carriers that persist for 686 ps in (AzOH)2PbI4 and 4.7 ns in the lead-free analogue (AzOH)2SnI4 at room temperature, without an external magnetic field. First-principles calculations suggest that these long lifetimes arise from hidden spin valleys, enhanced dielectric screening and reduced spin-orbit-induced scattering in the Sn-based compound. Our design paradigm unlocks inversion-symmetric semiconductors with ultralong spin lifetimes, broadening the materials options for light-driven spin control.

14 SOLAR ENERGY

High-throughput spin-bath characterization of spin defects in semiconductors

Detailed knowledge of the local environments of spin defects in semiconductors, such as nitrogenvacancy (NV) centers in diamond or divacancies in silicon carbide, is crucial for optimizing control and entanglement protocols in quantum sensing and information applications. However, at present a direct experimental characterization of individual defect environments is not scalable, as conventional spin-bath measurements are time consuming and difficult to automate. Achieving high-throughput characterization requires short experiments to probe the spin bath. However, with fewer and noisier measurements, the inverse problem of recovering spin-bath properties from measured data becomes ill posed, with multiple spin baths having a high likelihood of yielding the same data. In this work, we present a set of computational tools to resolve the ill-posed inverse problem of recovering the atomic positions and hyperfine couplings of random nuclei surrounding spin defects from sparse, noisy experimental coherence data, which can be obtained in hours. Here, we use a trans-dimensional Bayesian approach that incorporates ab initio data to yield full posterior distributions over nuclear spin environments, enabling robust recovery from limited data. We also provide practical tools and guidelines to determine the limits of detectability for hyperfine couplings under specific dynamical decoupling sequences and sampling conditions. In addition, we demonstrate how the tools developed here, in combination with ab initio simulations of spin baths, can guide the design of efficient experimental protocols for application-specific high-throughput screening. To showcase the utility of our approach, we apply it to design fast dynamical decoupling experiments to characterize the spin baths often individual NV centers in diamond. While the primary focus is on accelerating spin-bath characterization of spin defects, this Bayesian approach also lays the foundation for digital-twin studies of spin defects, where a virtual model of the spin-defect system evolves in real time with ongoing experimental measurements. Together, the set of tools we designed and applied paves the way for scalable deployment of spin defects in semiconductors for quantum sensing and information applications.

Bayesian methods

Free-Spinning-Tunnel Investigation to Determine the Effect of Spin-Recovery Rockets and Thrust Simulation on the Recovery Characteristics of a 1/21-Scale Model of the Chance Vought F7U-3 Airplane, TED No. NACA AD 3103

An investigation of a l/21-scale model of the Chance Vought F7U-3 airplane in the co&at-load- condition has been conducted in the Langley 20-foot free-spinning tunnel, The recovery characteristics of the model were determined by use of spin-recovery rockets for the erect and inverted spinning condition. The rockets were so placed as to provide either a yawing or rolling moment about the model center of gravity. Also included in the investigation were tests to determine the effect of simulated engine thrust on the recovery characteristics of the model. On the basis of model tests, recoveries from erect and inverted spins were satisfactory when a yawing moment of 22,200 foot-pounds (full scale) was provided against the spin by rockets attached to the wing tips; the anti-spin yawing moment was applied for approximately 9 seconds, (full scale). Satisfactory recoveries were obtained from erect spins when a rolling moment of 22,200 foot-pounds (full scale) was provided with the spin (rolls right wing down in right spin). Although the inverted spin was satisfactorily terminated when a rolling moment of equal magnitude was provided, a roll rocket was not considered to be an optimum spin-recovery device to effect recoveries from inverted spins for this airplane because of resulting gyrations during spin recovery. Simulation of engine thrust had no apparent effect on the spin recovery characteristics.

Burk, Sanger H., Jr.

Floquet Spin Splitting and Spin Generation in Antiferromagnets

In antiferromagnetic spintronics, accessing the spin degrees of freedom is essential for generating spin currents and manipulating magnetic order, which generally requires lifting spin degeneracy. This is typically achieved through relativistic spin-orbit coupling or nonrelativistic spin splitting in altermagnets. Here, we propose an alternative approach: a dynamical spin splitting induced by an optical field in antiferromagnets. By coupling the driven system to a thermal bath, we demonstrate the emergence of steady-state pure spin currents as well as linear-response longitudinal and transverse spin currents. Crucially, thermal bath engineering enables a nonrelativistic Edelstein effect—the generation of a net spin accumulation—without relying on spin-orbit coupling. Furthermore, our results provide a broadly applicable and experimentally tunable route to control spins in antiferromagnets, offering new opportunities for spin generation and manipulation in antiferromagnetic spintronics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND

Investigation of Spinning and Tumbling Characteristics of a 1/20-Scale Model of the Consolidated Vultee XFY-1 Airplane in the Free-Spinning Tunnel, TED No. NACA DE 370

An investigation has been conducted in the Langley 20-foot free-spinning tunnel on a l/20-scale model of the Consolidated Vultee XFY-1 airplane with a windmilling propeller simulated to determine the effects of control setting and movements upon the erect spin and recovery characteristics for a range of airplane-loading conditions. The effects on the model's spin-recovery characteristics of removing the lower vertical tail, removing the gun pods, and fixing the rudders at neutral were also investigated briefly. The investigation included determination of the size parachute required for emergency recovery from demonstration spins. The tumbling tendencies of the model were also investigated. Brief static force tests were made to determine the aerodynamic characteristics in pitch at high angles of attack. The investigation indicated that the spin and recovery characteristics of the airplane with propeller windmilling will be satisfactory for all loading conditions if recovery is attempted by full rudder reversal accompanied by simultaneous movement of the stick laterally to full with the spin (stick right in a right spin) and longitudinally to neutral. Inverted spins should be satisfactorily terminated by fully reversing the rudder followed immediately by moving the stick laterally towards the forward rudder pedal and longitudinally to neutral. Removal of the gun pods or fixing the rudders at neutral will not adversely affect the airplane's spin-recovery characteristics, but removal of the lower vertical tail will result in unsatisfactory spin-recovery characteristics. The model-test results showed that a 13.3-foot wing-tip conventional parachute (drag coefficient approximately 0.7) should be effective as an emergency spin-recovery device during demonstration spins of the airplane. It was indicated that the airplane should not tumble and that no unusual longitudinal-trim characteristics should be obtained for the center-of-gravity positions investigated.

Lee, Henry A.

Supplementary Investigation in the Langley Free-Spinning Tunnel of a 1/20-Scale Model of the Douglas XF4D-1 Airplane Including Spin-Recovery Parachute Tests of the Model Loaded to Simulate the Douglas F5D-1 Airplane

A supplementary investigation has been conducted in the Langley 20-foot free-spinning tunnel of a l/20-scale model of the Douglas XF4D-1 airplane to determine the effect of only neutralizing the rudder for recovery from an inverted spin, and the effect of partial aileron deflection with the spin for recovery from an erect spin. An estimation of the size parachute required for satisfactory recovery from a spin with the model ballasted to represent the Douglas F5D-1 (formerly the Douglas XF4D-2) airplane was also made. Results of the original investigation on the XF4D-1 design are presented in NACA RM SL50K30a. The results indicated that satisfactory recoveries from inverted spins of the airplane should be obtained by rudder neutralization when the longitudinal stick position is neutral or forward. Recoveries from erect spins from the normal-spin control configuration should be satisfactory by full rudder reversal with simultaneous movement of the ailerons to two-thirds with the spin. For the parachute tests with the model loaded to represent the F5D-1 airplane, the tests indicated that a 16.7-foot-diameter hemispherical-tail parachute (drag coefficient of 1.082 based on the projected area) with a towline 20.0 feet long (full- scale values) should be satisfactory for an emergency spin-recovery device during demonstration spins of the airplane.

Klinar, Walter J.

Extraction of the non-spin- and spin-transfer isovector responses via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B reaction

The isovector response in 12 B was investigated via the 12 C ⁡( 10 Be, 10 B + 𝛾)⁢ 12 B* reaction at 100⁢𝐴MeV. By utilizing the 𝛾-decay properties of the 1.74 MeV 0 + and 0.718 MeV 1 + states in 10 B, the separate extraction of the non-spin-transfer (Δ⁢𝑆 = 0) and spin-transfer (Δ⁢𝑆 = 1) isovector responses up to an excitation energy of 50 MeV in 12 B in a single measurement is demonstrated. The experimental setup employed the S800 spectrometer to detect and analyze the 10 B ejectiles and the Gamma-Ray Energy Tracking In-beam Nuclear Array (GRETINA) for obtaining the Doppler-reconstructed spectrum for 𝛾 rays emitted in flight by 10 B. A 12 C foil was placed at the pivot point of the spectrograph. Here, the 12 B reaction product was not detected. Contributions from transitions associated with the transfer of different units of angular momentum in the non-spin- and spin-transfer responses were analyzed using a multipole decomposition analysis. The extracted non-spin-dipole (Δ⁢𝑆 = 0, Δ⁢𝐿 = 1) and spin-dipole (Δ⁢𝑆 = 1, Δ⁢𝐿 = 1) responses were found to be consistent with available data from other charge-exchange probes, validating the non-spin- and spin-transfer filters used. While statistical uncertainties and experimental resolutions were relatively large due to the modest intensity of the 10 Be secondary beam, the results show that, with the much higher intensities that will be available at new rare-isotope beam facilities, the ( 10 Be, 10 B + 𝛾) reaction and its Δ⁢𝑇 𝑧 = −1 partner, the ( 10 C, 10 B + 𝛾) reaction, are powerful tools for elucidating the isovector non-spin- and spin-transfer responses in nuclei.

Charge-exchange reactions

Chemical Design of Spin Frustration to Realize Topological Spin Glasses

Patterning spins to generate collective behavior is at the core of condensed matter physics. Physicists develop techniques, including the fabrication of magnetic nanostructures and precision layering of materials specifically to engender frustrated lattices. As chemists, we can access such exotic materials through targeted chemical synthesis and create new lattice types by chemical design. Here, in this study, we introduce a new approach to induce magnetic frustration on a modified honeycomb lattice through a competition of alternating antiferromagnetic (AFM) and ferromagnetic (FM) nearest-neighbor interactions. By subtly modulating these two types of interactions through facile synthetic modifications, we created two systems: (1) a topological spin glass and (2) a frustrated spin-canted magnet with low-temperature exchange bias. To design this unconventional magnetic lattice, we used a metal–organic framework (MOF) platform, Ni 3 (pymca) 3 X 3 (NipymcaX where pymca = pyrimidine-2-carboxylato and X = Cl, Br). We isolated two MOFs, NipymcaCl and NipymcaBr, featuring canted Ni 2+ -based moments. Despite this similarity, differences in the single-ion anisotropies of the Ni 2+ spins result in distinct magnetic properties for each material. NipymcaCl is a topological spin glass, while NipymcaBr is a rare frustrated magnet with low-temperature exchange bias. Density functional theory calculations and Monte Carlo simulations on the NipymcaX lattice support the presence of magnetic frustration as a result of alternating AFM and FM interactions. Our calculations enabled us to determine the ground-state spin configuration and the distribution of spin–spin correlations relative to paradigmatic kagomé and triangular lattices. This modified honeycomb lattice is similar to the electronic Kekulé-O phase in graphene and provides a highly tunable platform to realize unconventional spin physics.

Exchange bias

Direct and indirect spin current generation and spin-orbit torques in ferromagnet/nonmagnet/ferromagnet trilayers

Spin-orbit torques in ferromagnet/nonmagnet/ferromagnet trilayers are studied using a combination of symmetry analysis, circuit theory, semiclassical simulations, and first-principles calculations using the nonequilibrium Green's function method with supercell disorder averaging. Here, we focus on unconventional processes involving the interplay between the two ferromagnetic layers, which are classified into direct and indirect mechanisms. The direct mechanism involves spin current generation by one ferromagnetic layer and its subsequent absorption by the other. In the indirect mechanism, the in-plane spin-polarized current from one ferromagnetic layer “leaks” into the other layer, where it is converted into an out-of-plane spin current and reabsorbed by the original layer. The direct mechanism results in a predominantly dampinglike torque, which damps the magnetization towards a certain direction 𝐬 𝑑 . The indirect mechanism results in a predominantly fieldlike torque with respect to a generally different direction 𝐬 𝑓 . Similarly to the current-in-plane giant magnetoresistance, the indirect mechanism is only active if the thickness of the nonmagnetic spacer is smaller than or comparable to the mean free path. Numerical calculations for a semiclassical model based on the Boltzmann equation confirm the presence of both direct and indirect mechanisms of spin current generation. First-principles calculations reveal sizable unconventional spin-orbit torques in Co/Cu/Co, Py/Cu/Py, and Co/Pt/Co trilayers and provide strong evidence of indirect spin current generation.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC

Optical and spin coherence of Er spin qubits in epitaxial cerium dioxide on silicon

Robust spin-photon interfaces with optical transitions in the telecommunication band are essential for quantum networking technologies. Erbium (Er) ions are the ideal candidate with environmentally protected transitions in telecom-C band. Finding the right technologically compatible host material to enable long-lived spins remains a major hurdle. We introduce a new platform based on Er ions in cerium dioxide (CeO 2 ) as a nearly-zero nuclear spin environment (0.04%) epitaxially grown on silicon, offering silicon compatibility for opto-electrical devices. Our studies focus on Er 3+ ions and show a narrow homogeneous linewidth of 440 kHz with an optical coherence time of 0.72 μs at 3.6 K. The reduced nuclear spin noise enables a slow spin-lattice relaxation with a spin relaxation time up to 2.5 ms and an electron spin coherence time of 0.66 μs (in the isolated ion limit) at 3.6 K. These findings highlight the potential of Er 3+ :CeO 2 platform for quantum networks applications.

Zhang, Jiefei

Spin Tests of a Low-lying Monoplane in Flight and in the Free-spinning Wind Tunnel

Comparative full-scale and model spin tests were made with a low-lying monoplane in order to extend the available information as to the utility of the free-spinning wind tunnel as an aid in predicting full-scale spin characteristics. For a given control disposition the model indicated steeper spins than were actually obtained with the airplane, the difference being most pronounced for spins with elevators up. Recovery characteristics for the model, on the whole, agreed with those for the airplane, but a disagreement was noted for the case of recovery with elevators held full up. Free-spinning wind-tunnel tests are a useful aid in estimating spin characteristics of airplanes, but it must be appreciated that model results can give only general indications of full-scale behavior.

Seidman, Oscar