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Fuel Performance Evaluation of THOR-C Experiments

The Temperature Heatsink Overpower Response Commissioning (THOR-C) and THOR-Metal (THOR-M) experiments will be performed as part of an ongoing project for testing sodium fast reactor fuels with the Japan Atomic Energy Agency (JAEA). The THOR-C experiments consist of fresh metallic fuel pins and have been analyzed using the ABAQUS, Ansys codes and the BISON fuel performance code. THOR-M-Loss of Flow-1 (THOR-M-LOF-1) is designed to test an EBR-II irradiated fuel pin under LOF conditions. Simulation of the THOR-MLOF-1 experiment required first simulating the base irradiation of the fuel pin in EBR-II. MFUEL module of SAS4A/SASSYS-1 [1] is a physics-based metallic fuel performance model applicable to the normal operation, transient scenarios and fuel failure modeling including scenarios with bulk fuel melting. The model has been validated using EBR-II normal operation, separate effect transient tests as well as TREAT M-Series transient tests [2]. In this study, MFUEL models has been utilized together with a new capsule heat transfer model developed in this project. The new heat transfer model was necessary due to (1) significant amount of heat losses that required 2D heat transfer, (2) the presence of a titanium heat sink, rejecting a significant amount of heat, and (3) stagnant coolant conditions, which are inconsistent with SAS4A/SASSYS-1 (SAS) heat transfer model. Updates to SAS4A/SASSYS-1 and MFUEL has been described below, followed by a preliminary validation effort using the results from THOR-C-2 fresh fuel capsule experiment. A previous study for THOR-C-2 analysis using BISON code is also utilized in this study to model this test [3]. [1] D. O’Grady, A. J. Brunett, L. Ibarra, A. Karahan, T. Kim, T. S. Sumner, R. Thomas, T. H. Fanning, “The SAS4A/SASSYS-2 Version 5.7 Safety Analysis Code System,” Argonne National Laboratory,ANL/NSE-SAS/5.7, (2023). [2] A. Karahan, T. Kim, T. Fanning, D. O’Grady, “Validation of MFUEL Metal Fuel Performance Models of SAS4A/SASSYS-1,” Argonne National Laboratory, ANL/NSE-23/11, (2023). [3] M. Mihelish, A. Zabriskie, K. Paaren, P. Medvedev, C. Jensen, “Fuel Performance Predictions for the TREAT THOR-C Experiments,” Idaho National Laboratory, INL/RPT-23-73397, Revision 0, (2023)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

thor

The THOR Project (Tensors for High-dimensional Object Representations)

Korobkin, Oleg

Terrestrial Gamma‐Ray Flash Following Intense Negative Return Stroke Observed With BIMAP‐3D

We report ground-based observations of a terrestrial gamma-ray flash (TGF) associated with a strong negative cloud-to-ground lightning strike (-CG) which occurred near Los Alamos National Laboratory (LANL) in New Mexico, USA. Gamma photons were detected by the Terrestrial High-energy Observations of Radiation (THOR) instrument, developed at the University of California, Santa Cruz, which has been hosted at LANL since 2022. Simultaneous measurements were also made with the 3-Dimensional Broadband Interferometric Mapping and Polarization (BIMAP-3D) system, which includes 3D lightning mapping, two fast antennas, and an additional plastic scintillator. Additional field change waveforms were obtained from the Earth Networks Total Lightning Network (ENTLN). The lightning initiated about 1 km above the ground, leading to a powerful -CG with an ENTLN peak current of −237 kA and bipolar field change matching the recently described “energetic compact stroke” (ECS) shape. The TGF was then observed ∼35 µs after the start of the return stroke. We also observe an electric field pulse likely produced by the TGF either in isolation or by coupling to the lightning channel. Based on modeling of the radiated electric field and photon propagation through the atmosphere we infer that the TGF source was on the order of 1⁢0 17 photons. This TGF and associated lightning are extremely similar to some recently reported ECS TGFs in coastal Japan in winter, but we report the first observation of this phenomenon outside of Japan in a different climate, terrain, and season.

58 GEOSCIENCES

Pre-Transient Characterization of MLOF-1 Test Pin

This study focuses on the pre-transient characterization of U-10Zr test and sibling fuel pins for the THOR-M-LOF test series. Using neutron radiography, element contact profilometry (ECP), precise gamma scan (PGS), and gas assay, sampling, and recharge (GASR) analysis, it was confirmed that the fuel pins were intact and suitable for testing. Key fuel behaviors quantified include axial elongation, diametral strain, fluff structure geometry, axial isotope distribution, and fission gas release. Any deviations from historically expected behaviors were investigated and attributed to factors other than the irradiation behavior of the fuel pin. These pre-transient measurements establish a baseline for future post-transient analysis, which will be used to inform fuel performance models and safety criteria for sodium-cooled fast reactors (SFRs). The results will enhance understanding of transient fuel behavior and expand limited data on LOF scenarios.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS

The forward physics facility: Physics opportunities and conceptual design

The Forward Physics Facility (FPF) is a proposed extension of the HL-LHC program designed to exploit the unique scientific opportunities offered by the intense flux of high energy neutrinos, and possibly new particles, in the far-forward direction. Located in a well-shielded cavern 627 m downstream of one of the LHC interaction points, the facility will support a broad and ambitious physics program that significantly expands the discovery potential of the HL-LHC. Equipped with four complementary detectors -- FLArE, FASER$ν$2, FASER2, and FORMOSA -- the FPF will enable breakthrough measurements that will advance our understanding of neutrino physics, quantum chromodynamics, and astroparticle physics, and will search for dark matter and other new particles. With this Letter of Intent, we propose the construction of the FPF cavern and the construction, integration, and installation of its experiments. We summarize the physics case, the facility design, the layout and components of the detectors, as well as the envisioned collaboration structure, cost estimate, and implementation timeline.

Astroparticle physics

Tuning the Conformations of an M4L4 Cage and Their Impact on Catalysis

Enzymes catalyze chemical reactions with remarkable rate enhancements and selectivity. Supramolecular catalysis seeks to understand and emulate these outcomes, leveraging noncovalent interactions, electric fields, and controlled active site microenvironments to enhance catalysis in an enzyme-like fashion. The effects of conformational dynamics on supramolecular catalysts and assemblies are, however, relatively unexplored, despite their crucial role in enzyme rate enhancement. Here, we elucidate the conformational landscape of a model M4L4 supramolecular host through a rational approach: stabilizing a high-energy conformer through distal ligand modification and a transient intermediate state through symmetry-matched guest encapsulation, as well as tuning the conformer distribution through same-charge metal exchange at the host vertices. Each of these structural modifications induces a substantial shift in the host's conformational landscape, offering insights into the rational design of conformationally dynamic cages and enzymes. Although the thermodynamic properties of the dynamic Ga4L412- cage can be influenced by temperature, solvent, and guest binding, we find that conformational change occurs on a time scale that renders it rate-limiting in a model catalytic reaction, precluding rate enhancement through conformational selection. This concept is illustrated by locking the catalytically inactive conformer to a high-energy conformer that is catalytically competent. These findings demonstrate that precise modulation of the conformational landscape of supramolecular hosts provides an effective strategy for controlling their catalytic activity and binding.

Catalysis

Serial-femtosecond crystallography reveals how a phytochrome variant couples chromophore and protein structural changes

The photoreaction and commensurate structural changes of a chromophore within biological photoreceptors elicit conformational transitions of the protein promoting the switch between deactivated and activated states. We investigated how this coupling is achieved in a bacterial phytochrome variant, Agp2-PAiRFP2. Contrary to classical protein crystallography, which only allows probing (cryo-trapped) stable states, we have used time-resolved serial femtosecond x-ray crystallography (tr-SFX) and pump-probe techniques with various illumination and delay times with respect to photoexcitation of the parent Pfr state. Thus, structural data for seven time frames were sorted into groups of molecular events along the reaction coordinate. They range from chromophore isomerization to the formation of Meta-F, the intermediate that precedes the functional relevant secondary structure transition of the tongue. Structural data for the early events were used to calculate the photoisomerization pathway to complement the experimental data. Late events allow identifying the molecular switch that is linked to the intramolecular proton transfer as a prerequisite for the following structural transitions.

59 BASIC BIOLOGICAL SCIENCES

Searching for Short-Lived Particles Using the FASER Neutrino Detector

Short-lived particles such as $\tau$ leptons and charm hadrons produced from high-energy neutrino interactions can provide key insights into the Standard Model and beyond. In this study, initial results of the performance of dedicated search tools developed for FASERν are presented. For charged charm searches, all daughter tracks are identified for ~3/4 of the events. Advanced yet reliable machine learning tools are used for D0 detection. For $\tau$ searches, a signal / background ratio of 3.8 is achieved. These results are a major step towards discovering the first charm hadrons and $\tau$ leptons produced from collider neutrinos.

Thor, Simon [CERN] (ORCID:000000029183526X)